arXiv subjects
Publications and source records attributed to Daniel J. Blumenthal.
We demonstrate dual-frequency stabilization of a hybrid-integrated multi-channel laser to an integrated high Q-factor silicon nitride (SiN) coil resonator with more than 40 dB frequency noise suppression. The frequency locked channels are utilized for a proof-of-concept fiber sensing experiment.
Integrating precise, stable, ultra-low noise visible light lasers into atomic systems is critical for advancing quantum information sciences and improving scalability and portability. Trapped ions are a leading approach for high-fidelity quantum computing, high-accuracy optical clocks, and precision quantum sensors. However, current ion-based systems rely on bulky, lab-scale precision lasers and optical stabilization cavities for optical clock and qubit operations, constraining the size, weight, scalability, and portability of atomic systems. Chip-scale integration of ultra-low noise lasers and reference cavities operating directly at optical clock transitions and capable of qubit and clock operations will represent a major transformation in atom and trapped ion-based quantum technologies. However, this goal has remained elusive. Here we report the first demonstration of chip-scale optical clock and qubit operations on a trapped ion using a photonic integrated direct-drive visible wavelength Brillouin laser stabilized to an integrated 3-meter coil-resonator reference cavity and the optical clock transition of a $^{88}$Sr$^+$ ion trapped on a surface electrode chip. We also demonstrate for the first time, to the best of our knowledge, trapped-ion spectroscopy and qubit operations such as Rabi oscillations and high fidelity (99%) qubit state preparation and measurement (SPAM) using direct drive integrated photonic technologies without bulk optic stabilization cavities or second harmonic generation. Our chip-scale stabilized Brillouin laser exhibits a 6 kHz linewidth with the 0.4 Hz quadrupole transition of $^{88}$Sr$^+$ and a self-consistent coherence time of 60 $μ$s via Ramsey interferometry on the trapped ion qubit. Furthermore, we demonstrate the stability of the locked Brillouin laser to 5$\times10^{-13}/ \sqrtτ$ at 1 second using dual optical clocks.
Optical frequency division (OFD) has revolutionized microwave and mmWave generation and set spectral purity records owing to its unique capability to transfer high fractional stability from optical to electronic frequencies. Recently, rapid developments in integrated optical reference cavities and microresonator-based optical frequency combs (microcombs) have created a path to transform OFD technology to chip scale. Here, we demonstrate an ultra-low phase noise mmWave oscillator by leveraging integrated photonic components and Kerr optical frequency division. The oscillator derives its stability from an integrated CMOS-compatible SiN coil cavity, and the optical frequency division is achieved spontaneously through Kerr interaction between the injected reference lasers and soliton microcombs in the integrated SiN microresonator. Besides achieving record-low phase noise for integrated mmWave oscillators, our demonstration greatly simplifies the implementation of integrated OFD oscillators and could be useful in applications of Radar, spectroscopy, and astronomy.
Heterogeneous and monolithic integration of the versatile low loss silicon nitride platform with low temperature materials such as silicon electronics and photonics, III-V compound semiconductors, lithium niobate, organics, and glasses, has been inhibited by the need for high temperature annealing as well as the need for different process flows for thin and thick waveguides. New techniques are needed to maintain the state-of-the-art losses, nonlinear properties, and CMOS compatible processes while enabling this next generation of 3D silicon nitride integration. We report a significant advance in silicon nitride integrated photonics, demonstrating the lowest losses to date for an anneal-free process at a maximum temperature of 250 C, with the same deuterated silane based fabrication flow, for nitride and oxide, for an order of magnitude range in nitride thickness without requiring stress mitigation or polishing. We report record low losses for anneal-free nitride core and oxide cladding, enabling 1.77 dB/m loss and 14.9 million Q for 80 nm nitride core waveguides, more than half an order magnitude lower loss than previously reported 270 C processes, and 8.66 dB/m loss and 4.03 million Q for 800 nm thick nitride. We demonstrate laser stabilization with over 4 orders of magnitude frequency noise reduction using a thin nitride reference cavity. And using a thick nitride micro-resonator, we demonstrate parametric gain and Optical Parametric Oscillation (OPO) with the lowest reported OPO threshold per unit resonator length for low temperature fabricated nitride, and supercontinuum generation over two octaves. These results represent a significant step towards a uniform ultra-low loss silicon nitride homogeneous and heterogeneous platform for both thin and thick waveguides capable of linear and nonlinear photonic circuits and integration with low temperature materials and processes.
Today's state of the art precision experiments in quantum, gravimetry, navigation, time keeping, and fundamental science have strict requirements on the level and spectral distribution of laser frequency noise. For example, the laser interaction with atoms and qubits requires ultra-low frequency noise at multiple offset frequencies due to hyperfine atomic transitions, motional sidebands, and fast pulse sequencing. Chip-scale integration of lasers that meet these requirements is essential for reliability, low-cost, and weight. Here, we demonstrate a significant advancement in atomic precision light sources by realizing a chip-scale, low-cost, 780 nm laser for rubidium atom applications with record-low 640 mHz (white noise floor at 0.2 Hz$^2$/Hz) fundamental and 732 Hz integral linewidths and a frequency noise that is multiple orders of magnitude lower than previous hybrid and heterogeneous self-injection locked 780 nm lasers and lower noise than bulk microresonator implementations. The laser is a Fabry-Pérot laser diode self-injection locked to an ultra-high Q photonic integrated silicon nitride resonator. This performance is enabled by a 145 million resonator Q with a 30 dB extinction ratio, the highest Q at 780 nm, to the best of our knowledge. We analyze the impact of our frequency noise on specific atomic applications including atomic frequency references, Rydberg quantum gates, and cold atom gravimeters. The photonic integrated resonator is fabricated using a CMOS foundry-compatible, wafer-scale process, with demonstrated integration of other components showing promise for a full system-on-a-chip. This performance is scalable to other visible atomic wavelengths, opening the door to a variety of transitions across many atomic species and enabling low-power, compact, ultra-low noise lasers impacting applications including quantum sensing, computing, clocks and more.
Cold atoms are important for precision atomic applications including timekeeping and sensing. The 3D magneto-optical trap (3D-MOT), used to produce cold atoms, will benefit from photonic integration to improve reliability and reduce size, weight, and cost. These traps require the delivery of multiple, large area, collimated laser beams to an atomic vacuum cell. Yet, to date, beam delivery using an integrated waveguide approach has remained elusive. We report the demonstration of a 87Rb 3D-MOT using a fiber-coupled photonic integrated circuit to deliver all beams to cool and trap > 1 x 10^6 atoms to near 200 μK. The silicon nitride photonic circuit transforms fiber-coupled 780 nm cooling and repump light via waveguides to three mm-width non-diverging free-space cooling and repump beams directly to the rubidium cell. This planar, CMOS foundry-compatible integrated beam delivery is compatible with other components, such as lasers and modulators, promising system-on-chip solutions for cold atom applications.
The silicon nitride integration platform has been successful at realizing extremely low waveguide losses across the visible to infrared and components including high performance lasers, filters, resonators, stabilization cavities, and optical frequency combs. Yet, progress towards implementing low loss, low power modulators in the silicon nitride platform, while maintaining the planar, wafer-scale process compatibility has been limited. Here we report a significant advance in integration of a piezo-electric (PZT) actuated micro-ring modulation in a fully-planar, wafer-scale silicon nitride platform, that maintains low optical loss (0.03 dB/cm in a 625 um resonator) at 1550 nm, with an order of magnitude increase in bandwidth (DC to 20 MHz 3-dB) and order of magnitude lower power consumption of 20 nW improvement over prior PZT modulators. The modulator provides a >14 dB ER and 7.1 million Q over the entire 4 GHz tuning range, a tuning efficiency of 200 MHz/V, and delivers the linearity required for control applications with 65.1 dBHz2/3 and 73.8 dBHz2/3 IMD3 SFDR at 1 MHz and 10 MHz respectively. We demonstrate two control applications, laser stabilization in a PDH lock loop, reducing laser frequency noise by 40 dB, and as a laser carrier tracking filter. This PZT modulator design can be extended to the visible in the ultra-low loss silicon nitride platform with minor waveguide design changes. This integration of PZT modulation in the ultra-low loss silicon nitride waveguide platform enables modulator control functions in a wide range of visible to IR applications such as atomic and molecular transition locking for cooling, controllable optical frequency combs, low-power external cavity tunable lasers, atomic clocks, and tunable ultra-low linewidth lasers and ultra-low phase noise microwave synthesizers.
A central requirement for photonic quantum information processing systems lies in the combination of nonclassical light sources and low-loss, phase-stable optical modes. While substantial progress has been made separately towards ultra-low loss, $\leq1$ dB/m, chip-scale photonic circuits and high brightness single-photon sources, integration of these technologies has remained elusive. Here, we report a significant advance towards this goal, in the hybrid integration of a quantum emitter single-photon source with a wafer-scale, ultra-low loss silicon nitride photonic integrated circuit. We demonstrate triggered and pure single-photon emission directly into a Si$_3$N$_4$ photonic circuit with $\approx1$ dB/m propagation loss at a wavelength of $\approx920$ nm. These losses are more than two orders of magnitude lower than reported to date for any photonic circuit with on-chip quantum emitter sources, and $>50$ % lower than for any prior foundry-compatible integrated quantum photonic circuit, to the best of our knowledge. Using these circuits we report the observation of resonance fluorescence in the strong drive regime, a milestone towards integrated coherent control of quantum emitters. These results constitute an important step forward towards the creation of scaled chip-integrated photonic quantum information systems.
Laser stabilization sits at the heart of many precision scientific experiments and applications, including quantum information science, metrology and atomic timekeeping. These systems narrow the laser linewidth and stabilize the carrier by use of Pound-Drever-Hall (PDH) locking to a table-scale, ultra-high quality factor (Q), vacuum spaced Fabry-Perot reference cavity. Integrating these cavities, to bring characteristics of PDH stabilization to the chip-scale, is critical to reduce their size, cost, and weight, and enable a wide range of portable and system-on-chip applications. We report a significant advance in integrated laser linewidth narrowing, stabilization and noise reduction, by use of a photonic integrated 4.0-meter-long coil resonator to stabilize a semiconductor laser. We achieve a 36 Hz 1/π-integral linewidth, an Allan deviation (ADEV) of 1.8x10^{-13} at 10 ms measurement time, and a 2.3 kHz/sec drift, to the best of our knowledge the lowest integral linewidth and highest stability demonstrated for an integrated reference cavity. Two coil designs, stabilizing lasers operating at 1550 nm and 1319 nm are demonstrated. The resonator is bus coupled to a 4.0-meter-long coil, with a 49 MHz free spectral range (FSR), a mode volume of 1.0x10^{10} μm^3 and a 142 million intrinsic Q, fabricated in a CMOS compatible, ultra-low loss silicon nitride waveguide platform. Our measurements and simulations show that the thermorefractive noise floor for this particular cavity is reached for frequencies down to 20 Hz in an ambient environment with simple passive vibration isolation and without vacuum or thermal isolation. The TRN limited performance is estimated to be an 8 Hz 1/π integral linewidth and ADEV of 5x10^{-14} at 10 ms, opening a stability regime that heretofore has only been available in fundamentally un-integrated systems.
Owing to their highly coherent emission and compact form factor, Brillouin lasers have been identified as a valuable asset for applications including portable atomic clocks, precision sensors, coherent microwave synthesis and energy-efficient approaches to coherent communications. While the fundamental emission linewidth of these lasers can be very narrow, noise within dielectric materials leads to drift in the carrier frequency, posing vexing challenges for applications requiring ultra-stable emission. A unified understanding of Brillouin laser performance may provide critical insights to reach new levels of frequency stability, however existing noise models focus on only one or a few key noise sources, and do not capture the thermo-optic drift in the laser frequency produced by thermal fluctuations or absorbed power. Here, we develop a coupled mode theory of Brillouin laser dynamics that accounts for dominant forms of noise in non-crystalline systems, capturing the salient features of the frequency and intensity noise for a variety of systems. As a result, theory and experiment can be directly compared to identify key sources of noise and the frequency bands they impact, revealing strategies to improve the performance of Brillouin lasers and pave the way for highly-coherent sources of light on a chip.
Integrated photonics is at the heart of many classical technologies, from optical communications to biosensors, LIDAR, and data center fiber interconnects. There is strong evidence that these integrated technologies will play a key role in quantum systems as they grow from few-qubit prototypes to tens of thousands of qubits. The underlying laser and optical quantum technologies, with the required functionality and performance, can only be realized through the integration of these components onto quantum photonic integrated circuits (QPICs) with accompanying electronics. In the last decade, remarkable advances in quantum photonic integration and a dramatic reduction in optical losses have enabled benchtop experiments to be scaled down to prototype chips with improvements in efficiency, robustness, and key performance metrics. The reduction in size, weight, power, and improvement in stability that will be enabled by QPICs will play a key role in increasing the degree of complexity and scale in quantum demonstrations. In the next decade, with sustained research, development, and investment in the quantum photonic ecosystem (i.e. PIC-based platforms, devices and circuits, fabrication and integration processes, packaging, and testing and benchmarking), we will witness the transition from single- and few-function prototypes to the large-scale integration of multi-functional and reconfigurable QPICs that will define how information is processed, stored, transmitted, and utilized for quantum computing, communications, metrology, and sensing. This roadmap highlights the current progress in the field of integrated quantum photonics, future challenges, and advances in science and technology needed to meet these challenges.
Laser-frequency stabilization with on-chip photonic integrated circuits will provide compact, low cost solutions to realize spectrally pure laser sources. Developing high-performance and scalable lasers is critical for applications including quantum photonics, precision navigation and timing, spectroscopy, and high-capacity fiber communications. We demonstrate a significant advance in compact, stabilized lasers to achieve a record low integral emission linewidth and precision carrier stabilization by combining integrated waveguide nonlinear Brillouin and ultra-low loss waveguide reference resonators. Using a pair of 56.4 Million quality factor (Q) Si$_3$N$_4$ waveguide ring-resonators, we reduce the free running Brillouin laser linewidth by over an order of magnitude to 330 Hz integral linewidth and stabilize the carrier to 6.5$\times$10$^{-13}$ fractional frequency at 8 ms, reaching the cavity-intrinsic thermorefractive noise limit for frequencies down to 80 Hz. This work demonstrates the lowest linewidth and highest carrier stability achieved to date using planar, CMOS compatible photonic integrated resonators, to the best of our knowledge. These results pave the way to transfer stabilized laser technology from the tabletop to the chip-scale. This advance makes possible scaling the number of stabilized lasers and complexity of atomic and molecular experiments as well as reduced sensitivity to environmental disturbances and portable precision atomic, molecular and optical (AMO) solutions.
Optical frequency stabilization is a critical component for precision scientific systems including quantum sensing, precision metrology, and atomic timekeeping. Ultra-high quality factor photonic integrated optical resonators are a prime candidate for reducing their size, weight and cost as well as moving these systems on chip. However, integrated resonators suffer from temperature-dependent resonance drift due to the large thermal response as well as sensitivity to external environmental perturbations. Suppression of the cavity resonance drift can be achieved using precision interrogation of the cavity temperature through the dual-mode optical thermometry. This approach enables measurement of the cavity temperature change by detecting the resonance difference shift between two polarization or optical frequency modes. Yet this approach has to date only been demonstrated in bulk-optic whispering gallery mode and fiber resonators. In this paper, we implement dual-mode optical thermometry using dual polarization modes in a silicon nitride waveguide resonator for the first time, to the best of our knowledge. The temperature responsivity and sensitivity of the dual-mode TE/TM resonance difference is 180.7$\pm$2.5 MHz/K and 82.56 $μ$K, respectively, in a silicon nitride resonator with a 179.9E6 intrinsic TM mode Q factor and a 26.6E6 intrinsic TE mode Q factor. Frequency stabilization is demonstrated by locking a laser to the TM mode cavity resonance and applying the dual-mode resonance difference to a feedforward laser frequency drift correction circuit with a drift rate improvement to 0.31 kHz/s over the uncompensated 10.03 kHz/s drift rate. Allan deviation measurements with dual-mode feedforward-correction engaged shows that a fractional frequency instability of 9.6E-11 over 77 s can be achieved.
Photonic molecules can be used to realize complex optical energy states and modes, analogous to those found in molecules, with properties useful for applications like spectral engineering and quantum optics. It is desirable to implement photonic molecules using high quality factor photonic integrated ring resonators due to their narrow atom-like spectral resonance, tunability, and the ability to scale the number of resonators on a photonic circuit. However, to take full advantage of molecule spectral complexity and tuning degree of freedom, resonator structures should have full symmetry in terms of inter-resonator coupling and resonator-waveguide coupling as well as independent resonance tuning, and low power dissipation operation, in a scalable integration platform. To date, photonic molecule symmetry has been limited to dual- and triple-cavity geometries coupled to single- or dual-busses, and resonance tuning limited to dual resonator molecules. In this paper, we demonstrate a three-resonator photonic molecule, consisting of symmetrically coupled 8.11 million intrinsic Q silicon nitride rings, where each ring is coupled to the other two rings. The resonance of each ring, and that of the collective molecule, is controlled using low power dissipation, monolithically integrated thin-film lead zirconate titanate (PZT) actuators that are integrated with the ultra-low loss silicon nitride resonators. This performance is achieved without undercut waveguides, yielding the highest Q to date for a PZT controlled resonator. This advance leads to full control of complex photonic molecule resonance spectra and splitting in a wafer-scale integration platform. The resulting six tunable supermodes can be fully controlled, including degeneracy, location and splitting as well as designed by a model that can accurately predict the energy modes and transmission spectrum and tunable resonance splitting.
Narrow linewidth visible light lasers are critical for atomic, molecular and optical (AMO) applications including atomic clocks, quantum computing, atomic and molecular spectroscopy, and sensing. Historically, such lasers are implemented at the tabletop scale, using semiconductor lasers stabilized to large optical reference cavities. Photonic integration of high spectral-purity visible light sources will enable experiments to increase in complexity and scale. Stimulated Brillouin scattering (SBS) is a promising approach to realize highly coherent on-chip visible light laser emission. While progress has been made on integrated SBS lasers at telecommunications wavelengths, barriers have existed to translate this performance to the visible, namely the realization of Brillouin-active waveguides in ultra-low optical loss photonics. We have overcome this barrier, demonstrating the first visible light photonic integrated SBS laser, which operates at 674 nm to address the 88Sr+ optical clock transition. To guide the laser design, we use a combination of multi-physics simulation and Brillouin spectroscopy in a 2 meter spiral waveguide to identify the 25.110 GHz first order Stokes frequency shift and 290 MHz gain bandwidth. The laser is implemented in an 8.9 mm radius silicon nitride all-waveguide resonator with 1.09 dB per meter loss and Q of 55.4 Million. Lasing is demonstrated, with an on-chip 14.7 mW threshold, a 45% slope efficiency, and linewidth narrowing as the pump is increased from below threshold to 269 Hz. To illustrate the wavelength flexibility of this design, we also demonstrate lasing at 698 nm, the wavelength for the optical clock transition in neutral strontium. This demonstration of a waveguide-based, photonic integrated SBS laser that operates in the visible, and the reduced size and sensitivity to environmental disturbances, shows promise for diverse AMO applications.
Precision frequency and phase synchronization between distinct fiber interconnected nodes is critical for a wide range of applications, including atomic timekeeping, quantum networking, database synchronization, ultra-high-capacity coherent optical communications and hyper-scale data centers. Today, many of these applications utilize precision, tabletop laser systems, and would benefit from integration in terms of reduced size, power, cost, and reliability. In this paper we report a record low 3x10^-4 rad^2 residual phase error variance for synchronization based on independent, spectrally pure, ultra-high mutual coherence, photonic integrated lasers. This performance is achieved with stimulated Brillouin scattering lasers that are stabilized to independent microcavity references, realizing sources with 30 Hz integral linewidth and a fractional frequency instability less than or equal to 2x10^-13 at 50 ms. This level of low phase noise and carrier stability enables a new type of optical-frequency-stabilized phase-locked loop (OFS-PLL) that operates with a less than 800 kHz loop bandwidth, eliminating traditional power consuming high bandwidth electronics and digital signal processors used to phase lock optical carriers. Additionally, we measure the residual phase error down to a received carrier power of -34 dBm, removing the need to transmit in-band or out-of-band synchronized carriers. These results highlight the promise for a path to spectrally pure, ultra-stable, integrated lasers for network synchronization, precision time distribution protocols, quantum-clock networks, and multiple-Terabit per second coherent DSP-free fiber-optic interconnects.
High Q optical resonators are a key component for ultra-narrow linewidth lasers, frequency stabilization, precision spectroscopy and quantum applications. Integration of these resonators in a photonic waveguide wafer-scale platform is key to reducing their cost, size and power as well as sensitivity to environmental disturbances. However, to date, the intrinsic Q of integrated all-waveguide resonators has been relegated to below 150 Million. Here, we report an all-waveguide Si3N4 resonator with an intrinsic Q of 422 Million and a 3.4 Billion absorption loss limited Q. The resonator has a 453 kHz intrinsic linewidth and 906 kHz loaded linewidth, with a finesse of 3005. The corresponding linear loss of 0.060 dB/m is the lowest reported to date for an all-waveguide design with deposited upper cladding oxide. These are the highest intrinsic and absorption loss limited Q factors and lowest linewidth reported to date for a photonic integrated all-waveguide resonator. This level of performance is achieved through a careful reduction of scattering and absorption loss components. We quantify, simulate and measure the various loss contributions including scattering and absorption including surface-state dangling bonds that we believe are responsible in part for absorption. In addition to the ultra-high Q and narrow linewidth, the resonator has a large optical mode area and volume, both critical for ultra-low laser linewidths and ultra-stable, ultra-low frequency noise reference cavities. These results demonstrate the performance of bulk optic and etched resonators can be realized in a photonic integrated solution, paving the way towards photonic integration compatible Billion Q cavities for precision scientific systems and applications such as nonlinear optics, atomic clocks, quantum photonics and high-capacity fiber communications systems on-chip.
The dynamics of cascaded-order Brillouin lasers make them ideal for applications such as rotation sensing, highly coherent optical communications, and low-noise microwave signal synthesis. Remark- ably, when implemented at the chip-scale, recent experimental studies have revealed that Brillouin lasers can operate in the fundamental linewidth regime where optomechanical and quantum noise sources dominate. To explore new opportunities for enhanced performance, we formulate a simple model to describe the physics of cascaded Brillouin lasers based on the coupled mode dynamics governed by electrostriction and the fluctuation-dissipation theorem. From this model, we obtain analytical formulas describing the steady state power evolution and accompanying noise properties, including expressions for phase noise, relative intensity noise and power spectra for beat notes of cascaded laser orders. Our analysis reveals that cascading modifies the dynamics of intermediate laser orders, yielding noise properties that differ from single-mode Brillouin lasers. These modifications lead to a Stokes order linewidth dependency on the coupled order dynamics and a broader linewidth than that predicted with previous single order theories. We also derive a simple analytical expression for the higher order beat notes that enables calculation of the Stokes linewidth based on only the relative measured powers between orders instead of absolute parameters, yielding a method to measure cascaded order linewidth as well as a prediction for sub-Hz operation. We validate our results using stochastic numerical simulations of the cascaded laser dynamics.