arXiv subjects

Frédéric Mila

Publications and source records attributed to Frédéric Mila.

At least 55 records · Page 3Linked to original sources

arXiv2022

Possibility to detect the bound state of the Heisenberg ferromagnetic chain at intermediate temperature

Motivated by the lack of direct evidence with inelastic neutron scattering of the well documented bound state of Heisenberg ferromagnets, we use the time-dependent Thermal Density Matrix Renormalization Group algorithm to study the temperature dependence of the dynamical spin structure factor of Heisenberg ferromagnetic spin chains. For spin-1/2, we show that the bound state appears as a well defined excitation with significant spectral weight in the temperature range $J/12 \lesssim T \lesssim J/3$, pointing to the possibility of detecting it with inelastic neutron scattering near $k=π$ provided the temperature is neither too low nor too high - at low temperature, the spectral weight only grows as $T^{3/2}$, and at high temperature the bound state peak merges with the two-magnon continuum. For spin-1, the situation is more subtle because the bound state with two neighboring spin flips competes with an anti-bound state with two spin-flips on the same site. As a consequence, the relative spectral weight of the bound state is smaller than for spin-1/2, and a weak resonance due to the anti-bound state appears in the continuum. A clearer signature of the bound state (resp. anti-bound state) can be obtained if a negative (resp. positive) biquadratic interaction is present.

cond-mat.str-el↗

arXiv2021

Quantum Monte Carlo simulations of highly frustrated magnets in a cluster basis: The two-dimensional Shastry-Sutherland model

Quantum Monte Carlo (QMC) simulations constitute nowadays one of the most powerful methods to study strongly correlated quantum systems, provided that no "sign problem" arises. However, many systems of interest, including highly frustrated magnets, suffer from an average sign that is close to zero in standard QMC simulations. Nevertheless, a possible sign problem depends on the simulation basis, and here we demonstrate how a suitable choice of cluster basis can be used to eliminate or at least reduce the sign problem in highly frustrated magnets that were so far inaccessible to efficient QMC simulations. We focus in particular on the application of a two-spin (dimer)-based QMC method to the thermodynamics of the spin-1/2 Shastry-Sutherland model for SrCu$_2$(BO$_3$)$_2$.

cond-mat.str-el↗

arXiv2021

Edge states and universality class of the critical two-box symmetric SU(3) chain

We numerically demonstrate that, although it is critical, the two-box symmetric $\mathrm{SU}(3)$ chain possesses edge states in the adjoint representation whose excitation energy scales with the number of sites $N_s$ as $1/(N_s \log N_s)$, in close analogy to those found in half-integer $\mathrm{SU}(2)$ chains with spin $S\ge 3/2$. We further show that these edge states dominate the entanglement entropy of finite chains, explaining why it has been impossible so far to verify with DMRG simulations the field theory prediction that this model is in the $\mathrm{SU}(3)_1$ universality class. Finally, we show that these edge states are very efficiently screened by attaching adjoint representations at the ends of the chain, leading to an estimate of the central charge consistent within 1\% with the prediction $c=2$ for $\mathrm{SU}(3)_1$.

cond-mat.str-el↗

arXiv2021

Artificial out-of-plane Ising antiferromagnet on the kagome lattice with very small further neighbour couplings

Despite their simple formulation, short range classical antiferromagnetic Ising models on frustrated lattices give rise to exotic phases of matter, in particular due to their macroscopic ground state degeneracy. Recent experiments on artificial spin systems comprising arrays of chirally coupled nanomagnets provide a significant strengthening of the nearest neighbour couplings compared to systems with dipolar-coupled nanomagnets. This opens the way to design artificial spin systems emulating Ising models with nearest neighbour couplings. In this paper, we compare the results of an extensive investigation with tensor network and Monte Carlo simulations of the nearest- and further-neighbour ($J_1-J_2-J_{3||}$) kagome Ising antiferromagnet with the experimental spin-spin correlations of a kagome lattice of chirally coupled nanomagnets. Even though the ratios between the further neighbour couplings and the nearest neighbour coupling estimated from micromagnetic simulations are much smaller than for dipolar-coupled nanomagnets, we show that they still play an essential role in the selection of the correlations.

cond-mat.mes-hall↗

arXiv2021

Phase diagram of the Shastry-Sutherland Compound SrCu2(BO3)2 under extreme combined conditions of field and pressure

Motivated by the intriguing properties of the Shastry-Sutherland compound SrCu2(BO3)2 under pressure, with a still debated intermediate plaquette phase appearing at around 20 kbar and a possible deconfined critical point at higher pressure upon entering the antiferromagnetic phase, we have investigated its high-field properties in this pressure range using tunnel diode oscillator (TDO) measurements. The two main new phases revealed by these measurements are fully consistent with those identified by infinite Projected Entangled Pair states (iPEPS) calculations of the Shastry-Sutherland model, a 1/5 plateau and a 10 x 2 supersolid. Remarkably, these phases are descendants of the full-plaquette phase, the prominent candidate for the intermediate phase of SrCu2(BO3)2. The emerging picture for SrCu2(BO3)2 is shown to be that of a system dominated by a tendency to an orthorhombic distortion at intermediate pressure, an important constraint on any realistic description of the transition into the antiferromagnetic phase.

cond-mat.str-el↗

arXiv2021

State selective cooling of $\mathrm{SU}(N)$ Fermi-gases

We investigate a species selective cooling process of a trapped $\mathrm{SU}(N)$ Fermi gas using entropy redistribution during adiabatic loading of an optical lattice. Using high-temperature expansion of the Hubbard model, we show that when a subset $N_A < N$ of the single-atom levels experiences a stronger trapping potential in a certain region of space, the dimple, it leads to improvement in cooling as compared to a $\mathrm{SU}(N_A)$ Fermi gas only. We show that optimal performance is achieved when all atomic levels experience the same potential outside the dimple and we quantify the cooling for various $N_A$ by evaluating the dependence of the final entropy densities and temperatures as functions of the initial entropy. Furthermore, considering ${}^{87}{\rm Sr}$ and ${}^{173}{\rm Yb}$ for specificity, we provide a quantitative discussion of how the state selective trapping can be achieved with readily available experimental techniques.

cond-mat.quant-gas↗

arXiv2021

Revealing three-dimensional quantum criticality by Sr-substitution in Han Purple

Classical and quantum phase transitions (QPTs), with their accompanying concepts of criticality and universality, are a cornerstone of statistical thermodynamics. An exemplary controlled QPT is the field-induced magnetic ordering of a gapped quantum magnet. Although numerous "quasi-one-dimensional" coupled spin-chain and -ladder materials are known whose ordering transition is three-dimensional (3D), quasi-2D systems are special for several physical reasons. Motivated by the ancient pigment Han Purple (BaCuSi$_{2}$O$_{6}$), a quasi-2D material displaying anomalous critical properties, we present a complete analysis of Ba$_{0.9}$Sr$_{0.1}$CuSi$_{2}$O$_{6}$. We measure the zero-field magnetic excitations by neutron spectroscopy and deduce the magnetic Hamiltonian. We probe the field-induced transition by combining magnetization, specific-heat, torque and magnetocalorimetric measurements with low-temperature nuclear magnetic resonance studies near the QPT. By a Bayesian statistical analysis and large-scale Quantum Monte Carlo simulations, we demonstrate unambiguously that observable 3D quantum critical scaling is restored by the structural simplification arising from light Sr-substitution in Han Purple.

cond-mat.str-el↗

arXiv2021

Lifshitz point at commensurate melting of 1D Rydberg atoms

The recent investigation of chains of Rydberg atoms has brought back the problem of commensurate-incommensurate transitions into the focus of current research. In 2D classical systems, or in 1D quantum systems, the commensurate melting of a period-p phase with p larger than 4 is known to take place through an intermediate floating phase where correlations between domain walls or particles decay only as a power law, but when p is equal to 3 or 4, it has been argued by Huse and Fisher that the transition could also be direct and continuous in a non-conformal chiral universality class with a dynamical exponent larger than 1. This is only possible however if the floating phase terminates at a Lifshitz point before reaching the conformal point, a possibility debated since then. Here we argue that this is a generic feature of models where the number of particles is not conserved because the exponent of the floating phase changes along the Pokrovsky-Talapov transition and can thus reach the value at which the floating phase becomes unstable. Furthermore, we show numerically that this scenario is realized in an effective model of the period-3 phase of Rydberg chains in which hard-core bosons are created and annihilated three by three: The Luttinger liquid parameter reaches the critical value $p^2/8=9/8$ along the Pokrovsky-Talapov transition, leading to a Lifshitz point that separates the floating phase from a chiral transition. Implications beyond Rydberg atoms are briefly discussed.

cond-mat.str-el↗

arXiv2020

Spin-$\frac{1}{2}$ kagome Heisenberg antiferromagnet with strong breathing anisotropy

We study the zero-temperature phase diagram of the spin-$\frac{1}{2}$ Heisenberg model with breathing anisotropy (i.e., with different coupling strength on the upward and downward triangles) on the kagome lattice. Our study relies on large scale tensor network simulations based on infinite projected entangled-pair state and infinite projected entangled-simplex state methods adapted to the kagome lattice. Our energy analysis suggests that the U(1) algebraic quantum spin-liquid (QSL) ground-state of the isotropic Heisenberg model is stable up to very large breathing anisotropy until it breaks down to a critical lattice-nematic phase that breaks rotational symmetry in real space through a first-order quantum phase transition. Our results also provide further insight into the recent experiment on vanadium oxyfluoride compounds which has been shown to be relevant platforms for realizing QSL in the presence of breathing anisotropy.

cond-mat.str-el↗

arXiv2020

Solving frustrated Ising models using tensor networks

Motivated by the recent success of tensor networks to calculate the residual entropy of spin ice and kagome Ising models, we develop a general framework to study frustrated Ising models in terms of infinite tensor networks %, i.e. tensor networks that can be contracted using standard algorithms for infinite systems. This is achieved by reformulating the problem as local rules for configurations on overlapping clusters chosen in such a way that they relieve the frustration, i.e. that the energy can be minimized independently on each cluster. We show that optimizing the choice of clusters, including the weight on shared bonds, is crucial for the contractibility of the tensor networks, and we derive some basic rules and a linear program to implement them. We illustrate the power of the method by computing the residual entropy of a frustrated Ising spin system on the kagome lattice with next-next-nearest neighbour interactions, vastly outperforming Monte Carlo methods in speed and accuracy. The extension to finite-temperature is briefly discussed.

cond-mat.stat-mech↗

arXiv2020

Haldane Gap of the Three-Box Symmetric $\mathrm{SU}(3)$ Chain

Motivated by the recent generalization of the Haldane conjecture to $\mathrm{SU}(3)$ chains [M. Lajkó et al., Nucl. Phys. B924, 508 (2017)] according to which a Haldane gap should be present for symmetric representations if the number of boxes in the Young diagram is a multiple of three, we develop a density matrix renormalization group algorithm based on standard Young tableaus to study the model with three boxes directly in the representations of the global $\mathrm{SU}(3)$ symmetry. We show that there is a finite gap between the singlet and the symmetric $[3\,0\,0]$ sector $Δ_{[3\,0\,0]}/J = 0.040\pm0.006$ where $J$ is the antiferromagnetic Heisenberg coupling, and we argue on the basis of the structure of the low energy states that this is sufficient to conclude that the spectrum is gapped.

cond-mat.str-el↗

arXiv2020

Kibble-Zurek exponent and chiral transition of the period-4 phase of Rydberg chains

Chains of Rydberg atoms have emerged as an amazing playground to study quantum physics in 1D. Playing with inter-atomic distances and laser detuning, one can in particular explore the commensurate-incommensurate transition out of charge-density waves through the Kibble-Zurek mechanism, and the possible presence of a chiral transition with dynamical exponent $z>1$. Here we address this problem theoretically with effective blockade models where the short-distance repulsions are replaced by a constraint of no double occupancy. For the period-4 phase, we show there is an Ashkin-Teller transition point with exponent $ν=0.78$ surrounded by a direct chiral transition with a dynamical exponent $z=1.14$ and a Kibble-Zurek exponent $μ=0.4$. For Rydberg atoms with a van der Waals potential, we suggest that the experimental value $μ=0.25$ is due to a chiral transition with $z\simeq 1.9$ and $ν\simeq 0.47$ surrounding an Ashkin-Teller transition close to the 4-state Potts universality.

cond-mat.str-el↗

arXiv2020

Identifying the Huse-Fisher universality class of the three-state chiral Potts model

Using the corner-transfer matrix renormalization group approach, we revisit the three-state chiral Potts model on the square lattice, a model proposed in the eighties to describe commensurate-incommensurate transitions at surfaces, and with direct relevance to recent experiments on chains of Rydberg atoms. This model was suggested by Huse and Fisher to have a chiral transition in the vicinity of the Potts point, a possibility that turned out to be very difficult to definitely establish or refute numerically. Our results confirm that the transition changes character at a Lifshitz point that separates a line of Pokrosky-Talapov transition far enough from the Potts point from a line of direct continuous order-disorder transition close to it. Thanks to the accuracy of the numerical results, we have been able to base the analysis entirely on effective exponents to deal with the crossovers that have hampered previous numerical investigations. The emerging picture is that of a new universality class with exponents that do not change between the Potts point and the Lifshitz point, and that are consistent with those of a self-dual version of the model, namely correlation lengths exponents $ν_x=2/3$ in the direction of the asymmetry and $ν_y=1$ perpendicular to it, an incommensurability exponent $\bar β=2/3$, a specific heat exponent that keeps the value $α=1/3$ of the three-state Potts model, and a dynamical exponent $z=3/2$. These results are in excellent agreement with experimental results obtained on reconstructed surfaces in the nineties, and shed light on recent Kibble-Zurek experiments on the period-3 phase of chains of Rydberg atoms.

cond-mat.stat-mech↗

arXiv2020

SrCu$_2$(BO$_3$)$_2$ under pressure: a first-principle study

Using density-functional theory (DFT) band-structure calculations, we study the crystal structure, the lattice dynamics, and the magnetic interactions in the Shastry-Sutherland magnet SrCu$_2$(BO$_3$)$_2$ under pressure, concentrating on experimentally relevant pressures up to 4 GPa. All tendencies inside the candidate intermediate phases are thoroughly worked out, including specific predictions for some Raman active phonon modes that could be used to pin down the nature of the intermediate phase.

cond-mat.str-el↗

arXiv2020

Reduction of the sign problem near $T=0$ in quantum Monte Carlo simulations

Building on a recent investigation of the Shastry-Sutherland model [S. Wessel et al., Phys. Rev. B 98, 174432 (2018)], we develop a general strategy to eliminate the Monte Carlo sign problem near the zero temperature limit in frustrated quantum spin models. If the Hamiltonian of interest and the sign-problem-free Hamiltonian---obtained by making all off-diagonal elements negative in a given basis---have the same ground state and this state is a member of the computational basis, then the average sign returns to one as the temperature goes to zero. We illustrate this technique by studying the triangular and kagome lattice Heisenberg antiferrromagnet in a magnetic field above saturation, as well as the Heisenberg antiferromagnet on a modified Husimi cactus in the dimer basis. We also provide detailed appendices on using linear programming techniques to automatically generate efficient directed loop updates in quantum Monte Carlo simulations.

cond-mat.str-el↗

arXiv2020

Magnetic field induced bound states in spin-$\frac{1}{2}$ ladders

Motivated by the intriguing mode splittings in a magnetic field recently observed with inelastic neutron scattering in the spin ladder compound (C$_5$H$_{12}$N)$_2$CuBr$_4$ (BPCB), we investigate the nature of the spin ladder excitations using DMRG and analytical arguments. Starting from the fully frustrated ladder, for which we derive the low-energy spectrum, we show that bound states are generically present close to $k=0$ in the dynamical structure factor of spin ladders above $H_{c 1}$, and that they are characterized by a field-independent binding energy and an intensity that grows with $H-H_{c 1}$. These predictions are shown to explain quantitatively the split modes observed in BPCB.

cond-mat.str-el↗

arXiv2020

Floating, critical and dimerized phases in a frustrated spin-3/2 chain

We study spontaneous dimerization and emergent criticality in a spin-3/2 chain with antiferromagnetic nearest-neighbor $J_1$, next-nearest-neighbor $J_2$ and three-site $J_3$ interactions. In the absence of three-site interaction $J_3$, we provide evidence that the model undergoes a remarkable sequence of three phase transitions as a function of $J_2/J_1$, going successively through a critical commesurate phase, a partially dimerized gapped phase, a critical floating phase with quasi-long-range incommensurate order, to end up in a fully dimerized phase at very large $J_2/J_1$. In the field theory language, this implies that the coupling constant of the marginal operator responsible for dimerization changes sign three times. For large enough $J_3$, the fully dimerized phase is stabilized for all $J_2$, and the phase transitions between the critical phases and this phase are both Wess-Zumino-Witten (WZW) SU(2)$_3$ along part of the boundary and turn first order at some point due to the presence of a marginal operator in the WZW SU(2)$_3$ model. By contrast, the transition between the two dimerized phase is always first order, and the phase transitions between the partially dimerized phase and the critical phases are Kosterlitz-Thouless. Finally, we discuss the intriguing spin-1/2 edge states that emerge in the partially dimerized phase for even chains. Unlike their counterparts in the spin-1 chain, they are not confined and disappear upon increasing $J_2$ in favour of a reorganization of the dimerization pattern.

cond-mat.str-el↗

arXiv2019

Perturbative approach to quantum tunneling and quantum interferences in spin clusters

Collective tunneling is a ubiquitous phenomenon in finite-size spin clusters that shows up in systems as diverse as molecular magnets or spin clusters adsorbed at surfaces. The problem we explore is to understand how small flipping terms can cooperate to flip a large spin to the opposite direction or a cluster of interacting elementary Ising spins into the time-reversed state. These high order processes will involve at least two channels, a single spin-flip channel due to a transverse field and a two-spin flip channel due to exchange or due to single-ion anisotropies. In the present paper, we show that high-order perturbation theory can be formulated and evaluated with the help of simple recurrence relations, leading to a compact theory of tunnelling in macroscopic spins, in one-dimensional clusters, as well as in small higher-dimensional clusters. This is demonstrated explicitly in the case of the Ising model with a transverse field and transverse exchange, and in the case of macroscopic spins with uniaxial anisotropy. Our approach provides a transparent theory of level crossings, where the tunneling between time reversed configurations vanishes as a function of the external field. The crossings result from destructive quantum interferences between competing flipping channels. Our theory consistently predicts N crossings in chains of N Ising spins, 2S crossings in single spins of magnitude S, and yields explicit analytical formulae for the level crossings of open chains and macroscopic spins. Disorder can be easily implemented in this perturbative formalism. Leading disorder effects can be treated analytically for spin rings. At the smallest transverse field crossing, the suppression of tunneling is most robust with respect to disorder. We briefly discuss the implications of our findings for the use of realistic spin clusters on surfaces to store information.

cond-mat.str-el↗