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Fu-Chun Zhang

Publications and source records attributed to Fu-Chun Zhang.

At least 19 recordsLinked to original sources

Charge imprinting biases topology of correlated insulator in hBN-aligned rhombohedral multilayer graphene

Rhombohedral multilayer graphene aligned with hexagonal boron nitride (RMG-hBN) hosts correlated Chern phases, but the microscopic role of hBN stacking remains unclear, especially when the active carriers are displaced away from the moir\'e interface. Using Hartree-Fock calculations over layer numbers, twist angles, displacement fields, fillings, and hBN alignments, we show that correlated insulators are most robust at small twist angles and intermediate layer number ($N\simeq 6$), where bandwidth suppression is balanced by layer delocalization of the wavefunctions of the active carriers. Under moir\'e-distant conditions at filling $\nu=1$, the topology of the insulating state is strongly biased by charge imprinting: the hBN alignment shapes the occupied valence-band charge texture near the interface via moir\'e potential, which acts through long-range Coulomb interactions as a remote electrostatic template for doped conduction electrons. Depending on the alignment, this template favors either triangular charge localization associated with trivial insulators or honeycomb-like charge networks compatible with Chern insulators. Our results identify valence-band charge textures as a microscopic route by which a remote moir\'e interface controls correlated topology in multilayer graphene.

cond-mat.mes-hall

Gossamer Superconductivity in Moir\'e WSe$_2$ Bilayer

Moir\'e transition metal dichalcogenides have served as a versatile platform for simulating Hubbard physics. Recent experiments have identified robust superconductivity in moir\'e bilayer WSe$_2$ for certain twist angles. Here, we propose the gossamer nature of the superconductivity recently discovered at half-filling and zero displacement field in twisted WSe$_2$. By mapping the moir\'e continuum system to an effective extended single-orbital Hubbard model on the triangular lattice, we employ renormalized mean-field theory to investigate the strong-coupling phase diagram. We find that a moderate Coulomb repulsion partially suppresses charge fluctuations while preserving a finite density of mobile doublons and holes. In this regime, the interplay between extended kinetic hoppings and antiferromagnetic superexchange stabilizes a chiral $d+id$ superconducting phase. Our results naturally account for the twist-angle-dependent evolution from a Mott insulator to a superconductor and eventually to a correlated metal. Furthermore, the model demonstrates that this half-filled pairing state vanishes rapidly upon density doping, consistent with experimental observations.

cond-mat.str-el

Orbital-Selective $d$-wave Superconductivity in the Two-Band $t$-$J$ Model: Possible Applications to La$_3$Ni$_2$O$_7$

We investigate superconductivity in a two-band $t$-$J$ model consisting of an itinerant orbital (orbital-0) and a quasi-localized orbital (orbital-1) using variational Monte Carlo. A robust orbital-selective $d$-wave superconducting state is found to emerge exclusively from the itinerant orbital. An analysis of the superexchange energy hierarchy shows that the quasi-localized orbital-1 competes with superconductivity by favoring local inter-orbital bound states, which act as energy defects and disrupt phase coherence. Consistently, the superconducting order parameter is monotonically suppressed as the occupancy of orbital-1 increases. Motivated by superconductivity in nickelate La$_3$Ni$_2$O$_7$, these results highlight the essential role of multi-orbital physics beyond the single-band $t$-$J$ framework and point to a concrete route to enhance $T_c$: suppressing the involvement of localized $d_{z^2}$-derived orbitals.

cond-mat.str-el

Jahn-Teller distortion on strained La$_3$Ni$_2$O$_7$ thin films

We present a systematic study of the electronic structure of strained La$_3$Ni$_2$O$_7$ thin films. We show that biaxial compressive strain mainly elongates the outer apical Ni-O bond while leaving the inner apical Ni-O bond nearly unchanged. As a result, the Jahn-Teller splitting $\Delta_{JT}$ is strongly enhanced, whereas the interlayer $d_{z^2}$ hopping $t_\perp^z$ changes only weakly. Since superconductivity is widely believed to emerge only below a critical in-plane lattice constant, our results identify the strain-enhanced $\Delta_{JT}$ as the relevant microscopic tuning parameter. Consistently, the calculated Fermi surfaces and Hall response for LaAlO$_3$ and SrLaAlO$_4$ substrates agree with ARPES and Hall measurements. Our results identify Jahn-Teller distortion as a key tuning parameter in strained La$_3$Ni$_2$O$_7$ and support its central role in optimizing superconductivity in bilayer nickelates.

cond-mat.supr-con

Discriminating Gap Symmetries of Superconducting La$_3$Ni$_2$O$_7$

The discovery of high-T$_c$ superconductor in Ruddlesden-Popper nickelate materials represented by La$_3$Ni$_2$O$_7$ has opened new directions in the quest for unconventional superconductivity. A central unresolved issue concerns the pairing symmetry of the superconducting order. In this paper, we model the superconducting order of La$_3$Ni$_2$O$_7$ using the established Fermi surface structure together with phenomenological pairing functions belonging to $s_\pm$ and $d$-wave symmetry classes, which are the leading possibilities in the current debate. We compute several experimentally accessible observables-including tunneling density of states, point contact spectroscopy, superfluid density, and Raman spectroscopy-each of which exhibits distinct characteristics for different gap symmetries. These quantities provide a concrete and experimentally testable route for identifying the pairing symmetry of La$_3$Ni$_2$O$_7$ and for clarifying the microscopic nature of nickelate superconductivity.

cond-mat.supr-con

Yamaji effect and quantum oscillation in Yang-Rice-Zhang model of underdoped cuprates

Recent experiments have revealed signatures of small Fermi pockets in the pseudogap phase of cuprate superconductors, most notably the Yamaji effect observed in $\mathrm{HgBa}_2\mathrm{CuO}_{4+\delta}$. The Yang-Rice-Zhang (YRZ) model provides a successful phenomenological description of the pseudogap state and naturally predicts such small pockets. In this work, we use a microscopic framework to calculate angle-dependent magnetoresistance and quantum oscillation within the YRZ model. Our calculations simultaneously reproduce the experimentally observed Yamaji oscillations and the Shubnikov-de Haas oscillation corresponding to a pocket area of about $p/8$, with $p$ the hole density. By further testing the effect of Green's-function zeros, we confirm that isolated zeros leave the oscillation period unchanged, whereas an extended zero segment suppresses and modifies the oscillation. Our findings demonstrate that the YRZ model captures essential features of the pseudogap regime and provides a general quantum approach that can be applied to more complex electronic structures.

cond-mat.supr-con

Inter-orbital spin-triplet superconductivity from altermagnetic fluctuations

Altermagnetic (AM) fluctuations are a new class of collinear spin fluctuations whose role in mediating superconductivity faces a fundamental tension: their $\Gamma$-point peak favors intra-orbital spin-triplet pairing, while their spin compensation favors inter-orbital singlets. Here, we demonstrate that inversion-symmetry-broken AM fluctuations generically resolve this competition in favor of spin-triplet pairing. As a proof of concept, we study a minimal two-orbital model with two van Hove singularities. The broken inversion symmetry induces momentum-orbital locking: the same orbital dominates at opposite momenta, enhancing the triplet channel. Crucially, a subdominant fluctuation channel arising from inter-van-Hove nesting provides an internal Josephson coupling that locks the phase difference between triplet pairs on different orbitals. We find this coupling changes sign ($+$ to $-$) upon a crossover from AM-dominant to ferromagnetic-dominant fluctuations. The resulting $\pi$-phase difference manifests as a $\tau_z$-type order parameter, $c_{k,1\uparrow}c_{-k,1\uparrow} - c_{k,2\uparrow}c_{-k,2\uparrow}$. Although intra-orbital in the original basis, its orbital-nontrivial character, as manifested by its equivalence to inter-orbital pairing under rotation, defines a general \textit{inter-orbital spin-triplet superconductivity}. This state is distinct from the $\tau_0$-triplet pairing mediated by ferromagnetic fluctuations, as evidenced by the canceled intra-orbital supercurrent in a Josephson junction between them.

cond-mat.str-el

Robust Majorana Platform Driven by a Meissner-Induced Anisotropic Doppler Shift

The realization of robust Majorana zero modes (MZMs), a cornerstone for fault-tolerant quantum computing, is hindered by the challenge of creating a platform that simultaneously offers a large topological gap, high tunability, and resilience to disorder. A system unifying these properties has remained elusive. Here, we propose and validate a novel platform that harnesses the Meissner effect in a topological insulator (TI) nanowire partially covered by a superconducting (SC) layer. Under an external magnetic field, Meissner screening currents in the SC induce a spatially varying Doppler shift on the TI surface. This effect generates a highly anisotropic effective g-factor, which selectively drives a topological phase transition localized on the nanowire's bottom surface. This mechanism is crucial as it spatially separates the topological phase from the SC/TI interface, permitting strong proximity-induced superconductivity while preventing detrimental band renormalization at the interface from closing the topological gap. Furthermore, by confining the topological superconducting phase to the gate-tunable bottom surface, our platform fully leverages the intrinsic disorder resilience of the TI's topologically protected surface states. Through a combination of supercurrent simulations, self-consistent Schr\"odinger-Poisson calculations, and large-scale tight-binding computations, we validate the platform's robustness. Our work establishes a practical pathway toward Meissner-mediated topological superconductivity for realizing robust MZMs in SC/TI hybrid systems.

cond-mat.mes-hall

Competing $s$-wave pairing in overdoped $t$-$J$ model

The $d$-wave pairing symmetry has long been considered a defining feature of high-temperature superconductivity in cuprates. In this work, we reveal that $s$-wave pairing states exhibit variational energies comparable to the $d$-wave state in a square $t$-$J$ model, particularly at high doping levels ($\delta\gtrsim 15\%$) by using the state-of-the-art tensor network simulation. This surprising result suggests that $s$-wave pairing may play an important role in the cuprate phase diagram, especially for the overdoped region. Our findings provide a potential resolution to discrepancies in recent Josephson tunneling experiments on twisted bilayer cuprates and offer new insights into the evolution of pairing symmetry with doping.

cond-mat.str-el

Spin-Polarized Josephson Supercurrent in Nodeless Altermagnets

Long-range propagation of equal-spin triplet Cooper pairs typically occurs in ferromagnet/$s$-wave superconductor junctions, where net magnetization plays a crucial role. Here, we propose a fundamentally different scenario in which Josephson supercurrents mediated exclusively by spin-triplet pairings emerge in systems with \textit{zero} net magnetization. We identify collinear altermagnets, particularly a subclass termed nodeless altermagnets, as ideal platforms to realize this phenomenon. These materials host spin-split Fermi surfaces that do not intersect altermagnetic nodal lines and support maximal spin-valley polarization, yielding fully spin-polarized electronic states at each valley. Consequently, Josephson junctions based on nodeless altermagnets sustain supercurrents solely through spin-polarized triplet pairing correlations, simultaneously contributed by spin-up Cooper pairs from one valley and spin-down Cooper pairs from the other. Furthermore, controlling the relative local inversion-symmetry breaking at the two interfaces enables a robust 0--$\pi$ transition without fine tuning, while adjusting the junction orientation allows a crossover between pure triplet and mixed singlet-triplet states. Our work thus establishes nodeless altermagnets as a unique platform for altermagnetic superconductors with magnetization-free spin-polarized supercurrents.

cond-mat.supr-con

High Chern Number Quantum Anomalous Hall States in Haldane-Graphene Multilayers

We consider a rhombohedral-stacked $N$-layer graphene coupled to a monolayer of Haldane model. We show that high order Dirac points in multilayer graphene can be gapped out by topological proximity effect of the Haldane model layer, leading to total Chern number $|C|=N+1$ quantum anomalous Hall states. This provides a new way to construct high Chern number quantum anomalous Hall states in realistic crystalline graphene systems.

cond-mat.mes-hall

Vortex States and Coherence Lengths in Flat-Band Superconductors

Superconductivity in flat-band systems, governed by quantum metric of Bloch states rather than the BCS framework, exhibits unique phenomena due to the vanishing electron group velocity. Here, we propose the vortex states and vortex size as direct probes to explore the quantum geometry effects in flat-band superconductors. We show that flat-band vortex bound states are sharply localized near the vortex core, and the energy gap between the lowest two bound states is on the order of the bulk superconducting gap. Both the spatial spread and energy scales of bound states are controlled by the flat-band's quantum metric length. Moreover, the vortex size at zero temperature, set by the quantum metric length, is atomic in scale and independent of interaction strength. Near $T_c$, the vortex size corresponds to the Ginzburg-Landau coherence length, diverges as $\xi\sim \sqrt{T_c/(T_c-T)}\xi_0$, where $\xi_0$ depends linearly on the quantum metric length. Thus, the quantum metric serves as the lower bound for vortex state spread and vortex size. We also introduce perturbations to make the flat band dispersive, and distinguish flat-band vortices from BCS-like vortices. Our results establish vortices as universal probes of quantum geometry in flat-band superconductors.

cond-mat.supr-con

Anisotropic and tunable vortex topology in multiband iron-based superconductors

Building on the multiband nature of iron-based superconductors (FeSCs), we have uncovered pronounced anisotropy in Majorana vortex topology arising from the interaction between vortex orientation and multiple electronic topologies. This anisotropy manifests in two distinct vortex configurations: the z-vortex and x-vortex, oriented perpendicular and parallel to the Dirac axis (z-axis for FeSCs), respectively. The x-vortex exhibits a unique duality, displaying two distinct topological phase diagrams. One is strikingly simple, comprising only trivial and topological superconducting phases, and remains resilient to multiband entanglement. The other mirrors the z-vortex's complex diagram, featuring alternating trivial, topological crystalline and topological superconducting phases. Crucially, the former is exclusive to the x-vortex and supports unpaired Majorana vortices across a wide parameter range, even with Dirac nodes in electronic bands. Notably, uniaxial strain can modulate these x-vortex phases, enabling the x-vortex to support both stable Majorana vortices and rich exotic physics in a controllable manner. Moreover, we propose that the x-vortex offers promising advantages for developing iron-based superconducting quantum devices. Our findings introduce a novel paradigm in vortex topology within multiband superconducting systems, highlighting the x-vortex as a promising platform for exploring Majorana physics and advancing iron-based superconducting quantum technology.

cond-mat.supr-con

Self-doped Molecular Mott Insulator for Bilayer High-Temperature Superconducting La3Ni2O7

The bilayer structure of recently discovered high-temperature superconducting nickelates La$_3$Ni$_2$O$_7$ provides a new platform for investigating correlation and superconductivity. Starting from a bilayer Hubbard model, we show that there is a molecular Mott insulator limit formed by the bonding band owing to Hubbard interaction $U$ and large interlayer coupling. This molecular Mott insulator becomes self-doped due to electrons transferred to the antibonding bands at a weaker interlayer coupling strength. The self-doped molecular Mott insulator is similar to the doped Mott insulator studied in cuprates. We propose La$_3$Ni$_2$O$_7$ to be a self-doped molecular Mott insulator, whose molecular Mott limit is formed by two nearly degenerate antisymmetric $d_{x^2-y^2}$ and $d_{z^2}$ orbitals. Partial occupation of higher energy symmetric $d_{x^2-y^2}$ orbital leads to self-doping, which may be responsible for high-temperature superconductivity in La$_3$Ni$_2$O$_7$. The effects of Hund's coupling $J_H$ on the low-energy spectra are also studied via exact diagonalization. The proposed low-energy theory for La$_3$Ni$_2$O$_7$ is found to be valid in a wide range of $U$ and $J_H$.

cond-mat.str-el

Directly visualizing nematic superconductivity driven by the pair density wave in NbSe$_2$

Pair density wave (PDW) is a distinct superconducting state characterized by a periodic modulation of its order parameter in real space. Its intricate interplay with the charge density wave (CDW) state is a continuing topic of interest in condensed matter physics. While PDW states have been discovered in cuprates and other unconventional superconductors, the understanding of diverse PDWs and their interactions with different types of CDWs remains limited. Here, utilizing scanning tunneling microscopy, we unveil the subtle correlations between PDW ground states and two distinct CDW phases -- namely, anion-centered-CDW (AC-CDW) and hollow-centered-CDW (HC-CDW) -- in 2H-NbSe$_2$. In both CDW regions, we observe coexisting PDWs with a commensurate structure that aligns with the underlying CDW phase. The superconducting gap size, $\Delta(r)$, related to the pairing order parameter is in phase with the charge density in both CDW regions. Meanwhile, the coherence peak height, $H(r)$, qualitatively reflecting the electron-pair density, exhibits a phase difference of approximately $2\pi/3$ relative to the CDW. The three-fold rotational symmetry is preserved in the HC-CDW region but is spontaneously broken in the AC-CDW region due to the PDW state, leading to the emergence of nematic superconductivity.

cond-mat.supr-con

The electronic and magnetic structures of bilayer La$_3$Ni$_2$O$_7$ at ambient pressure

We carry out a systematic study of the electronic and magnetic structure of the ambient-pressure bilayer La$_3$Ni$_2$O$_7$. Employing the hybrid exchange-correlation functional, we show that the exchange-correlation pushes the bonding $d_{z^2}$ bands below the Fermi level to be fully occupied. The calculated Fermi surfaces and the correlation normalized band structure match well with the experimental findings at ambient pressure. Moreover, the electronic susceptibility calculated for this new band structure features nesting-induced peaks near the wave vector $Q=(\pi/2, \pi/2)$, suggesting a possible density wave instability in agreement with recent experiments. Through a mean field study and DFT+U calculation introducing a Hubbard U interaction within conventional density functional theory, we confirm the spin-charge intertwined double stripe order is the magnetic ground state. Our results provide a faithful description for the low-pressure La$_3$Ni$_2$O$_7$ electronic structure.

cond-mat.supr-con

Tunable even- and odd-denominator fractional quantum Hall states in trilayer graphene

The fractional quantum Hall (FQH) states are exotic quantum many-body phases whose elementary charged excitations are neither bosons nor fermions but anyons, obeying fractional braiding statistics. While most FQH states are believed to have Abelian anyons, the Moore-Read type states with even denominators, appearing at half filling of a Landau level (LL), are predicted to possess non-Abelian excitations with appealing potentials in topological quantum computation. These states, however, depend sensitively on the orbital contents of the single-particle LL wavefunction and the mixing between different LLs. Although they have been observed in a few materials, their non-Abelian statistics still awaits experimental confirmation. Here we show magnetotransport measurements on Bernal-stacked trilayer graphene (TLG), whose unique multiband structure facilitates the interlaced LL mixing, which can be controlled by external magnetic and displacement fields. We observe a series of robust FQH states including even-denominator ones at filling factors $\nu=-9/2$, $-3/2$, $3/2$ and $9/2$. In addition, we are able to finetune the LL mixing and crossings to drive quantum phase transitions of these half-filling states and their neighboring odd-denominator ones, exhibiting a related emerging and waning behavior. Our results establish TLG as a controllable system for tuning the weights of LL orbitals and mixing strength, and a fresh platform to seek for non-Abelian quasi-particles.

cond-mat.mes-hall

Inter-layer valence bonds and two-component theory for high-$T_c$ superconductivity of La$_{3}$Ni$_{2}$O$_{7}$ under pressure

The recent discovery of high-$T_{c}$ superconductivity in bilayer nickelate La$_{3}$Ni$_{2}$O$_{7}$ under high pressure has stimulated great interest concerning its pairing mechanism. We argue that the weak coupling model from the almost fully-filled $d_{z^{2}}$ bonding band cannot give rise to its high $T_{c}$, and thus propose a strong coupling model based on local inter-layer spin singlets of Ni-$d_{z^{2}}$ electrons due to their strong on-site Coulomb repulsion. This leads to a minimal effective model that contains local pairing of $d_{z^{2}}$ electrons and a considerable hybridization with near quarter-filled itinerant $d_{x^{2}-y^{2}}$ electrons on nearest-neighbor sites. Their strong coupling provides a unique two-component scenario to achieve high-$T_{c}$ superconductivity. Our theory highlights the importance of the bilayer structure of superconducting La$_{3}$Ni$_{2}$O$_{7}$ and points out a potential route for the exploration of more high-$T_{c}$ superconductors.

cond-mat.supr-con