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Hai-Zhou Lu

Publications and source records attributed to Hai-Zhou Lu.

At least 19 recordsLinked to original sources

Scaling analysis of quantum geometry in second-order nonlinear transport

Quantum geometry encodes the structure of the Hilbert space of Bloch states and can be accessed through nonlinear transport. Yet, disorder-induced mechanisms generically contribute to nonlinear transport, making it difficult to isolate quantum-geometric contributions in experiments. Here we systematically enumerate geometric and disorder-induced mechanisms of the second-order nonlinear Hall effect and derive a scaling law that expresses the nonlinear Hall conductivity as a polynomial of the linear longitudinal conductivity. Crucially, each mechanism carries a distinct "weight fingerprint" in the polynomial, enabling a quantitative disentanglement of quantum geometry from disorder backgrounds in existing experiments, both with and without time-reversal symmetry. Our results provide an implementable workflow for identifying quantum-geometric contributions in nonlinear-transport measurements.

cond-mat.mes-hall

Identifying geometric third-order nonlinear transport in disordered materials

In nonlinear transport, the quantum-geometric effects can generate higher-harmonic voltages in response to a driving current, which has defined a fast-moving field of intense interest. However, in realistic materials where disorder scattering also contributes to nonlinear transport, identifying the geometric mechanisms remains a challenge. In particular, a theoretical framework for data analysis is still lacking for nonlinear transport at any order. Here, we develop a mechanism-resolved and symmetry-guided framework for identifying mechanisms of third-order nonlinear transport in disordered materials. We find a total of 20 mechanisms of third-order nonlinear transport, by treating quantum-geometric and disorder-mediated mechanisms on an equal footing. More importantly, we propose a protocol of data analysis that combines symmetry diagnosis of magnetic point groups and scaling law of relation between the third-order nonlinear Hall conductivity and linear longitudinal conductivity. We identify characteristic fingerprints in the scaling-law weights, which allow the mechanisms to be quantitatively distinguished in experiments. We have applied the protocol to identify the geometric mechanisms in materials with and without time-reversal symmetry, including 2D materials, topological materials, and altermagnets. The theory can be generalized to arbitrary orders of nonlinear transport, further promoting nonlinear transport as a probe of geometric effects and phase transitions in quantum materials.

cond-mat.mes-hall

Giant and Broadband Circular Dichroism from Particle-Hole Symmetry Breaking in Weyl Semimetals

Circular dichroism originates from symmetry breaking of material structure, leading to differential absorption of left- and right-circularly polarized light. However, circular dichroism in most materials is inherently weak and spectrally narrow, especially in the mid-to-far infrared. Here, we uncover giant infrared circular dichroism in the magnetic-field-forced Weyl semimetal Mn(Bi,Sb)2Te4, driven by extreme particle-hole symmetry breaking. Helicity-resolved magneto-infrared spectroscopy reveals circular dichroism exceeding 3000 mdeg (~130 mdeg/nm) with above-degree response extending over the 6-13 μm spectral range. The optical resonances are enhanced by a strong band nesting effect intrinsic to the Landau levels of type-II Weyl dispersion. A symmetry-based kp model reproduces these magneto-infrared responses and demonstrates that magnetization-induced asymmetric spin-orbit coupling generates particle-hole symmetry breaking, suppressing spin-up, parity-even wavefunction components in the valence Landau band and thereby producing pronounced optical helicity selectivity. Our findings establish particle-hole symmetry breaking as an effective route toward helicity-resolved optical control in quantum materials.

cond-mat.mtrl-sci

Anisotropic Surface Spin Waves as Signature of A-type Altermagnets

Altermagnets have attracted intense interest because they have the advantages of both ferromagnets and antiferromagnets. However, their experimental identification remains challenging, in particular for the A-type altermagnets that account for a large group of material candidates. Here, we discover a kind of anisotropic surface spin waves in A-type altermagnets, which is absent in ferromagnets and conventional antiferromagnets. The anisotropic surface spin waves arise directly from the nature of altermagnets, i.e., the spin-opposite sublattices cannot be related by translation or inversion, which breaks the combined spatial-inversion and time-reversal symmetry, leading to the anisotropic surface spin waves with two properties, the chirality-dependent top-bottom positions and chiral split constant frequency contours. We further show that these two properties can be measured experimentally from the stray field and by resonance absorption spectrum, respectively. Our results provide a signature for detecting altermagnets and will inspire spin-based logic and information-storage devices.

cond-mat.mes-hall

3D Quantum Hall Effect with Two Distinct Plateaus

The recent discovery of the 3D quantum Hall effect in $\mathrm{HfTe_5}$ has also revealed puzzling signatures of possible 3D fractionalization. Beyond the first plateau associated with the lowest Landau band, Hall conductivity exhibits a second plateau with a value of about $3/5$ of the first, accompanied by a suppressed longitudinal resistivity. Here, we attribute this second plateau to an insulating ground state arising from spin-density-wave order. We show that a magnetic-field-driven Lifshitz transition causes the spin-down holelike zeroth Landau band to cross the Fermi energy and that the resulting nesting between the lowest spin-up and spin-down Landau bands induces a spin-density wave. We calculate the Hall and longitudinal resistivity and reproduce the experimental behaviors. Our renormalization-group analysis further supports this insulating ground state. Our work reveals that the tunability of Landau bands along the magnetic-field direction endows the 3D quantum Hall effect with a broader phenomenology than its 2D counterpart and merits further exploration.

cond-mat.mes-hall

Nernst Plateau in the Quantum Limit of Low-Carrier-Density Topological Insulators

Nernst effect, a transverse electric current induced by a temperature gradient, is a promising tool for revealing emergent phases of condensed matter. We find a Nernst coefficient plateau in low carrier density topological insulators, as a signature of 1D Weyl points in the quantum limit of the weak topological insulator. The plateau height is inversely proportional to the impurity density, suggesting a way to engineer infinitely large Nernst effects. The Nernst plateau also exists in strong topological insulators, at the bottom of the lowest Landau band. We show that these plateaus have been overlooked in the previous experiments and we highlight the experimental conditions to observe them. Our results may inspire more investigations of employing anomalous Nernst effect to identify emergent phases of condensed matter.

cond-mat.mes-hall

Enhanced Anomalous Nernst Effect in the Ferromagnetic Kondo Lattice CeCo2As2

The anomalous Nernst effect (ANE), generating a voltage perpendicular to a temperature gradient due to magnetization, is closely linked to the Berry curvature (BC) near the Fermi energy in topological magnets. We report an enhanced spontaneous ANE in the ferromagnetic Kondo lattice CeCo2As2, which features Kondo-screened cerium-based 4f moments embedded in a ferromagnetic d-electron framework. The observed large anomalous Nernst coefficient, greater than the Seebeck coefficient, is attributed to the strong BC present in the f-orbital-dominated flat bands. The enhanced ANE in CeCo2As2 serves as a signature of the Fermi energy pinning within the topological flat band, highlighting the correlation-driven topology in the Kondo lattice.

cond-mat.str-el

Quantum Christoffel Nonlinear Magnetization

The Christoffel symbol is an essential quantity in Einstein's general theory of relativity. We discover that an electric field can induce a nonlinear magnetization in quantum materials, described by a Christoffel symbol defined in the Hilbert space of quantum states (quantum Christoffel symbol). Quite different from the previous scenarios, this orbital magnetization does not need spin-orbit coupling and inversion symmetry breaking. Through symmetry analysis and first-principles calculations, we identify a number of point groups and 2D material candidates (e.g., BiF$_3$, ZnI$_2$, and Ru$_4$Se$_5$) that host this quantum Christoffel nonlinear magnetization. More importantly, this nonlinear magnetization allows the quantum Christoffel symbol to be probed by optical techniques such as magneto-optical Kerr spectroscopy or transport measurements such as tunneling magneto-resistance. This quantum Christoffel nonlinear magnetization gives a paradigm of how geometry dictates physics.

cond-mat.mes-hall

Probing quantum geometric nonlinear magnetization via second-harmonic magneto-optical Kerr effect

Quantum geometry provides an intrinsic framework for characterizing the geometric structure of quantum states. It highlights its relevance to various aspects of fundamental physics. However, its direct implications for magnetic phenomena remain largely unexplored. Here, we report the observation of electric-field-induced nonlinear magnetization in the nonmagnetic semimetal WTe$_2$ by using a second-harmonic magneto-optical Kerr effect (SMOKE) spectroscopy. We observe a robust nonlinear SMOKE signal that scales quadratically with current and persists up to 200 K. Theoretical modeling and scaling analysis indicate that this nonlinear magnetization is dominated by the orbital contribution and is intrinsically linked to the quantum Christoffel symbol. Just as the Christoffel symbol is a fundamental quantity encoding spacetime geometry in Einstein's general relativity, our work establishes a direct link between quantum geometry and nonlinear magnetization, and provides a geometric perspective for designing future orbitronic devices.

cond-mat.mes-hall

Quantum Geometric Origin of Orbital Magnetization

The exploration of the Riemannian structure of the Hilbert space has led to the concept of quantum geometry, comprising geometric quantities exemplified by Berry curvature and quantum metric. While this framework has profoundly advanced the understanding of various electronic phenomena, its potential for illuminating magnetic phenomena has remained less explored. In this Perspective, we highlight how quantum geometry paves a new way for understanding magnetization within a single-particle framework. We first elucidate the geometric origin of equilibrium magnetization in the modern theory of magnetization, then discuss the role of quantum geometry in kinetic magnetization, and finally outline promising future directions at the frontier of quantum geometric magnetization.

cond-mat.mes-hall

Exploration of Altermagnetism in $\mathrm{RuO_{2}}$

The fundamental role of magnetic materials in modern science and technology has driven a rapid surge in research on unconventional magnetism in recent years. In particular, altermagnets, which simultaneously exhibit zero net magnetization in real space and anisotropic spin splitting in momentum space, have garnered significant interest for both fundamental physics and technological applications. Among these, $\mathrm{RuO_{2}}$ stands as the pioneering and most extensively studied altermagnet. While the intrinsic magnetic order of $\mathrm{RuO_{2}}$ is still a subject of active debate, numerous exotic phenomena characteristic of altermagnetism have been observed in $\mathrm{RuO_{2}}$ samples. In this review, we explore each facet of the altermagnetism through specific case studies in $\mathrm{RuO_{2}}$, systematically surveying its crystal and magnetic structures, electronic band properties, and transport phenomena. We critically assess the debate surrounding the intrinsic magnetism in $\mathrm{RuO_{2}}$, incorporating evidence from altermagnetic signatures in transport, as well as contrasting results from magnetic and spectroscopic measurements. Finally, possible future research directions in this field are discussed.

cond-mat.mes-hall

Linear magnetoresistance of two-dimensional massless Dirac fermions in the quantum limit

Linear magnetoresistance is a hallmark of 3D Weyl metals in the quantum limit. Recently, a pronounced linear magnetoresistance has also been observed in 2D graphene [Xin et al., Nature 616, 270 (2023)]. However, a comprehensive theoretical understanding remains elusive. By employing the self-consistent Born approximation, we derive the analytical expressions for the magnetoresistivity of 2D massless Dirac fermions in the quantum limit. Notably, our result recovers the minimum conductivity in the clean limit and reveals a linear dependence of resistivity on the magnetic field for Gaussian impurity potentials, in quantitative agreement with experiments. These findings shed light on the magnetoresistance behavior of 2D Dirac fermions under ultra-high magnetic fields.

cond-mat.mes-hall

A Clarification on Quantum-Metric-Induced Nonlinear Transport

Over the years, Berry curvature, which is associated with the imaginary part of the quantum geometric tensor, has profoundly impacted many branches of physics. Recently, quantum metric, the real part of the quantum geometric tensor, has been recognized as indispensable in comprehensively characterizing the intrinsic properties of condensed matter systems. The intrinsic second-order nonlinear conductivity induced by the quantum metric has attracted significant recent interest. However, its expression varies across the literature. Here, we reconcile this discrepancy by systematically examining the nonlinear conductivity using the standard perturbation theory, the wave packet dynamics, and the Luttinger-Kohn approach. Moreover, inspired by the Dirac model, we propose a toy model that suppresses the Berry-curvature-induced nonlinear transport, making it suitable for studying the quantum-metric-induced nonlinear conductivity. This work provides a clearer and more unified understanding of the quantum-metric contributions to nonlinear transport. It also establishes a solid foundation for future theoretical developments and experimental explorations in this highly active and rapidly evolving field.

cond-mat.mes-hall

Emergence of Nodal-Knot Transitions by Disorder

Under certain symmetries, degenerate points in three-dimensional metals form one-dimensional nodal lines. These nodal lines sometimes exhibit intricate knotted structures and have been studied in various contexts. As one of the most common physical perturbations, disorder effects often trigger novel quantum phase transitions. For nodal-knot phases, whether disorder can drive knot transitions remains an open and intriguing question. Employing renormalization-group calculations, we demonstrate that nodal-knot transitions emerge in the presence of weak disorder. Specifically, both chemical-potential-type and magnetic-type disorders can induce knot transitions, resulting in the emergence of distinct knot topologies. The transition can be quantitatively characterized by changes in topological invariants such as the knot Wilson loop integrals. Our findings open up a new avenue for manipulating the topology of nodal-knot phases through disorder effects.

cond-mat.mes-hall

Quantum oscillation in Hopf-link semimetals

Since the discovery of the relation between the Chern number and quantum Hall effect, searching for observables of topological invariants has been an intriguing topic. Topological Hopf-link semimetals have attracted tremendous interest, in which the conduction and valence energy bands touch at linked nodal lines. However, it is challenging to identify this sophisticated topology. We propose to use the quantum oscillation in strong magnetic fields to probe the Hopf links. For a generic model of Hopf-link semimetal that captures the linked-trivial phase transition, we figure out the phase shifts of oscillation for all Fermi pockets in all magnetic-field directions, by presenting self-consistent results from the Fermi surface tomography, Landau fan diagram, and electrical resistivity. As the magnetic field is rotated, the phase shifts exhibit a unique pattern, which could help to identify Hopf links in real materials, such as those in Li$_2$NaN.

cond-mat.mes-hall

Electrical switching of altermagnetism

Switching magnetism using only electricity is of great significance for industrial applications but remains challenging. We find that, altermagnetism, as a newly discovered unconventional magnetism, may open an avenue along this effort. Specifically, to have deterministic switching, i.e., reversing current direction must reverse magnetic structure, parity symmetry has to be broken. We discover that, due to their symmetry which depends on chemical environments, altermagnet devices may naturally carry the parity symmetry breaking required for deterministic electrical switching of magnetism. More importantly, we identify MnTe bilayers (Te-Mn-Te-Mn-Te) as candidate devices, with the help of symmetry analysis, first-principles calculations, and magnetic dynamics simulations. This scheme will inspire further explorations on unconventional magnetism.

cond-mat.mes-hall

Coulomb Drag in Altermagnets

An altermagnet is a newly discovered antiferromagnet, characterized by unique anisotropic spin-split energy bands. It has attracted tremendous interest, because of its promising potential in information storage and processing. However, measuring the distinctive spin-split energy bands arising from altermagnetism remains a challenge. Here, we propose to employ the Coulomb drag to probe altermagnetism. In the Coulomb drag, an electric current in an active layer of electron gases can induce currents in a close but well-isolated passive layer, due to interlayer Coulomb interactions. We find that the Coulomb drag effects in altermagnets are highly sensitive to the orientation of the spin-split Fermi surfaces. As a result, transverse currents can be dragged in the passive layer, leading to Hall drag effects even in absence of spin-orbit coupling, a feature quite different from all previous systems. More importantly, all the drag effects of altermagnets have unique angle dependence, which can be measured in a multi-terminal setup to serve as signatures for altermagnetism. This proposal will inspire increasing explorations on emergent magnetism.

cond-mat.mes-hall

Dispersions and magnetism of strain-induced pseudo Landau levels in Bernal-stacked bilayer graphene

Elastic strain can displace the massless Dirac fermions in monolayer graphene in a space-dependent fashion, similar to the effect of an external magnetic field, thus giving rise to Landau quantization. We here show that the strain-induced Landau quantization can also take place in Bernal-stacked bilayer graphene, where the low-energy excitations are massive rather than Dirac-like. The zigzag ribbon of Bernal-stacked bilayer graphene realizes a two-legged Su-Schrieffer-Heeger model with a domain wall, which coincides with the guiding center of the strain-induced pseudo Landau levels. We reduce the lattice model of the ribbon in the vicinity of the guiding center into an exactly solvable coupled Dirac model and analytically derive the dispersions of the strain-induced pseudo Landau levels. Remarkably, the zeroth and first pseudo Landau levels are dispersionless and sublattice-polarized. We elucidate that the interaction on these two pseudo Landau levels results in a global antiferromagnetic order. Our study extends the strain-induced Landau quantization to the massive excitations and indicates strain as a tuning knob of magnetism.

cond-mat.mes-hall