arXiv subjects

Hiroshi Eisaki

Publications and source records attributed to Hiroshi Eisaki.

At least 91 records · Page 5Linked to original sources

arXiv2015

Inequivalence of Single-Particle and Population Lifetimes in a Cuprate Superconductor

We study optimally doped Bi-2212 ($T_\textrm{c}=96$~K) using femtosecond time- and angle-resolved photoelectron spectroscopy. Energy-resolved population lifetimes are extracted and compared with single-particle lifetimes measured by equilibrium photoemission. The population lifetimes deviate from the single-particle lifetimes in the low excitation limit by one to two orders of magnitude. Fundamental considerations of electron scattering unveil that these two lifetimes are in general distinct, yet for systems with only electron-phonon scattering they should converge in the low-temperature, low-fluence limit. The qualitative disparity in our data, even in this limit, suggests that scattering channels beyond electron-phonon interactions play a significant role in the electron dynamics of cuprate superconductors.

cond-mat.supr-con↗

arXiv2015

Resolving unoccupied electronic states with laser ARPES in bismuth-based cuprate superconductors

Angle-resolved photoemission spectroscopy (ARPES) is typically used to study only the occupied electronic band structure of a material. Here we use laser-based ARPES to observe a feature in bismuth-based superconductors that, in contrast, is related to the unoccupied states. Specifically, we observe a dispersive suppression of intensity cutting across the valence band, which, when compared with relativistic one-step calculations, can be traced to two final-state gaps in the bands 6 eV above the Fermi level. This finding opens up possibilities to bring the ultra-high momentum resolution of existing laser-ARPES instruments to the unoccupied electron states. For cases where the final-state gap is not the object of study, we find that its effects can be made to vanish under certain experimental conditions.

cond-mat.supr-con↗

arXiv2014

Identifying the `Fingerprint' of Antiferromagnetic Spin-Fluctuations on Iron-Pnictide Superconductivity

Cooper pairing in the iron-based high-Tc superconductors is often conjectured to involve bosonic fluctuations. Among the candidates are antiferromagnetic spin-fluctuations and d-orbital fluctuations amplified by phonons. Any such electron-boson interaction should alter the electron's `self-energy', and then become detectable through consequent modifications in the energy dependence of the electron's momentum and lifetime. Here we introduce a theoretical/experimental approach aimed at identifying the relevant fluctuations of iron-based superconductors by measuring effects of their self-energy. We use quasiparticle interference (QPI) imaging techniques in LiFeAs to reveal strongly momentum-space anisotropic self-energy signatures that are focused along the Fe-Fe (interband scattering) direction, where the spin fluctuations of LiFeAs are concentrated. These effects coincide in energy with perturbations to the density-of-states N(ω) usually associated with the Cooper pairing interaction. We show that all the measured phenomena comprise the predicted QPI `fingerprint' of a self-energy due to antiferromagnetic spin-fluctuations, thereby distinguishing them as the predominant electron-boson interaction.

cond-mat.supr-con↗

arXiv2014

Photo-enhanced antinodal conductivity in the pseudogap state of high Tc cuprates

A major challenge in understanding the cuprate superconductors is to clarify the nature of the fundamental electronic correlations that lead to the pseudogap phenomenon. Here we use ultrashort light pulses to prepare a non-thermal distribution of excitations and capture novel properties that are hidden at equilibrium. Using a broadband (0.5-2 eV) probe we are able to track the dynamics of the dielectric function, unveiling an anomalous decrease of the scattering rate of the charge carriers in a pseudogap-like region of the temperature ($T$) and hole-doping ($p$) phase diagram. In this region, delimited by a well-defined $T^*_{neq}(p)$ line, the photo-excitation process triggers the evolution of antinodal excitations from gapped (localized) to delocalized quasi-particles characterized by a longer lifetime. The novel concept of photo-enhanced antinodal conductivity is naturally explained within the single-band Hubbard model, in which the short-range Coulomb repulsion leads to a k-space differentiation between "nodal" quasiparticles and antinodal excitations.

cond-mat.str-el↗

arXiv2014

Direct spectroscopic evidence for phase competition between the pseudogap and superconductivity in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$

In the high-temperature ($T_{c}$) cuprate superconductors, increasing evidence suggests that the pseudogap, existing below the pseudogap temperature $T$*, has a distinct broken electronic symmetry from that of superconductivity. Particularly, recent scattering experiments on the underdoped cuprates have suggested that a charge ordering competes with superconductivity. However, no direct link of this physics and the important low-energy excitations has been identified. Here we report an antagonistic singularity at $T_{c}$ in the spectral weight of Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ as a compelling evidence for phase competition, which persists up to a high hole concentration $p$ ~ 0.22. Comparison with a theoretical calculation confirms that the singularity is a signature of competition between the order parameters for the pseudogap and superconductivity. The observation of the spectroscopic singularity at finite temperatures over a wide doping range provides new insights into the nature of the competitive interplay between the two intertwined phases and the complex phase diagram near the pseudogap critical point.

cond-mat.supr-con↗

arXiv2014

Two distinct superconducting states in KFe$_2$As$_2$ under high pressure

We report measurements of ac magnetic susceptibility $χ_{ac}$ and de Haas-van Alphen (dHvA) oscillations in KFe$_2$As$_2$ under high pressure up to 24.7 kbar. The pressure dependence of the superconducting transition temperature $T_c$ changes from negative to positive across $P_c \sim 18$ kbar as previously reported. The ratio of the upper critical field to $T_c$, i.e, $B_{c2} / T_c$, is enhanced above $P_c$, and the shape of $χ_{ac}$ vs field curves qualitatively changes across $P_c$. DHvA oscillations smoothly evolve across $P_c$ and indicate no drastic change in the Fermi surface up to 24.7 kbar. Three dimensionality increases with pressure, while effective masses show decreasing trends. We suggest a crossover from a nodal to a full-gap $s$ wave as a possible explanation.

cond-mat.supr-con↗

arXiv2014

Synthesis and physical properties of Ca1-xRExFeAs2 with RE = La ~ Gd

Synthesis of a series of layered iron arsenides Ca1-xRExFeAs2 (112) was attempted by heating at 1000 C under a high-pressure of 2 GPa. The 112 phase successfully forms with RE = La, Ce, Nd, Sm, Eu and Gd, while Tb, Dy and Ho substituted and RE free samples does not contain the 112 phase. The Ce, Nd, Sm, Eu and Gd doped Ca1-xRExFeAs2 are new compounds. All of them exhibit superconducting transition except for the Ce doped sample. The behaviour of the critical temperature, with the RE ionic radii have been investigated.

cond-mat.supr-con↗

arXiv2014

Time- and Momentum-resolved Gap Dynamics in Bi2Sr2CaCu2O8+delta

We use time- and angle-resolved photoemission spectroscopy to characterize the dynamics of the energy gap in superconducting Bi2Sr2CaCu2O8+delta (Bi2212). Photoexcitation drives the system into a nonequilibrium pseudogap state: Near the Brillouin zone diagonal (inside the normal-state Fermi arc), the gap completely closes for a pump fluence beyond F = 15 μJ/cm^2; toward the Brillouin zone face (outside the Fermi arc), it remains open to at least 24 μJ/cm^2. This strongly anisotropic gap response may indicate multiple competing ordering tendencies in Bi2212. Despite these contrasts, the gap recovers with relatively momentum-independent dynamics at all probed momenta, which shows the persistent influence of superconductivity both inside and outside the Fermi arc.

cond-mat.str-el↗

arXiv2013

Thermodynamic Study of Nodal Structure and Multiband Superconductivity of KFe2As2

The temperature, field, and field-orientation dependences of the electronic specific heat Ce of the ironpnictide superconductor KFe2As2 have been investigated. Thermodynamic evidence of the presence of line nodes is obtained from the T and $\sqrt{H}$ linear dependences of Ce/T in the low-T and low-H region. Under a magnetic field rotated within the tetragonal ab plane, a fourfold oscillation is observed in Ce with a sign change at 0.08Tc. On the basis of the Doppler-shift analysis, the observed Ce minima in H // [100] at low T indicate the presence of line nodes somewhere on the Fermi surface where the Fermi velocity is parallel to the [100] direction; this is consistent with the octet-line-node scenario proposed recently by a photoemission experiment. In addition, the low-T Ce/T exhibits an unusual upturn on cooling at moderate fields only for H // ab, which is understood in terms of the strong Pauli paramagnetic effect on multiband superconductivity.

cond-mat.supr-con↗

arXiv2013

Signatures of superconductivity and pseudogap formation in non-equilibrium nodal quasiparticles revealed by ultrafast angle-resolved photoemission

We use time- and angle-resolved photoemission to measure the nodal non-equilibrium electronic states in various dopings of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. We find that the initial pump-induced transient signal of these ungapped states is strongly affected by the onset of the superconducting gap at $T_c$, superconducting pairing fluctuations at $T_p$, and the pseudogap at $T^*$. Moreover, $T_p$ marks a suggestive threshold in the fluence-dependent transient signal, with the appearance of a critical fluence below $T_p$ that corresponds to the energy required to break apart all Cooper pairs. These results challenge the notion of a nodal-antinodal dichotomy in cuprate superconductors by establishing a new link between nodal quasiparticles and the cuprate phase diagram.

cond-mat.supr-con↗

arXiv2013

Discovery of New Layered Iron Arsenide Superconductor (Ca,Pr)FeAs2

A new iron-based superconductor (Ca,Pr)FeAs2 was discovered. Plate-like crystals of the new phase were obtained and crystal structure was investigated by single-crystal X-ray diffraction analysis. The structure was identified as the monoclinic system with space group P21/m, and is composed of two Ca(Pr) planes, anti-fluorite Fe2As2 layers, and As2 zigzag chain layers. Plate-like crystals composed of the new phase showed superconductivity with Tc ~20 K in both magnetization and resistivity measurements.

cond-mat.supr-con↗

arXiv2013

Fermi surface in KFe2As2 determined via de Haas-van Alphen oscillation measurements

We have completely determined the Fermi surface in KFe$_2$As$_2$ via de Haas-van Alphen (dHvA) measurements. Fundamental frequencies $ε$, $α$, $ζ$, and $β$ are observed in KFe$_2$As$_2$. The first one is attributed to a hole cylinder near the X point of the Brillouin zone, while the others to hole cylinders at the $Γ$ point. We also observe magnetic breakdown frequencies between $α$ and $ζ$ and suggest a plausible explanation for them. The experimental frequencies show deviations from frequencies predicted by band structure calculations. Large effective masses up to 19 $m_e$ for $B \parallel c$ have been found, $m_e$ being the free electron mass. The carrier number and Sommerfeld coefficient of the specific heat are estimated to be 1.01 -- 1.03 holes per formula unit and 82 -- 94 mJmol$^{-1}$K$^{-2}$, respectively, which are consistent with the chemical stoichiometry and a direct measure of 93 mJmol$^{-1}$K$^{-2}$ [H. Fukazawa \textit{et al}., J. Phys. Soc. Jpn. \textbf{80SA}, SA118 (2011)]. The Sommerfeld coefficient is about 9 times enhanced over a band value, suggesting the importance of low-energy spin and/or orbital fluctuations, and places KFe$_2$As$_2$ among strongly correlated metals. We have also performed dHvA measurements on Ba$_{0.07}$K$_{0.93}$Fe$_2$As$_2$ and have observed the $α$ and $β$ frequencies.

cond-mat.supr-con↗

arXiv2013

Hysteretic superconducting resistive transition in Ba0.07K0.93Fe2As2

We have observed hysteresis in superconducting resistive transition curves of Ba$_{0.07}$K$_{0.93}$Fe$_2$As$_2$ ($T_c\sim$8 K) below about 1 K for in-plane fields. The hysteresis is not observed as the field is tilted away from the $ab$ plane by 20$^{\circ}$ or more. The temperature and angle dependences of the upper critical field indicate a strong paramagnetic effect for in-plane fields. We suggest that the hysteresis can be attributed to a first-order superconducting transition due to the paramagnetic effect. Magnetic torque data are also shown.

cond-mat.supr-con↗

arXiv2013

Effect of doping on the magnetostructural ordered phase of iron arsenides: A comparative study of the resistivity anisotropy in the doped BaFe$_2$As$_2$ with doping into three different sites

In order to unravel a role of doping in the iron-based superconductors, we investigated the in-plane resistivity for BaFe$_2$As$_2$ doped at either of the three different lattice sites, Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, BaFe$_2$(As$_{1-x}$P$_x$)$_2$, and Ba$_{1-x}$K$_x$Fe$_2$As$_2$, focusing on the doping effect in the low-temperature antiferromagnetic/orthorhombic (AFO) phase. A major role of doping in the high-temperature paramagnetic/tetragonal (PT) phase is known to change the Fermi surface by supplying charge carriers or by exerting chemical pressure. In the AFO phase, we found a clear correlation between the magnitude of residual resistivity and resistivity anisotropy. This indicates that the resistivity anisotropy originates from the anisotropic impurity scattering from dopant atoms. The magnitude of residual resistivity is also found to be a parameter controlling the suppression rate of AFO ordering temperature $T_s$. Therefore, the dominant role of doping in the AFO phase is to introduce disorder to the system, distinct from that in the PT phase.

cond-mat.supr-con↗

arXiv2013

Understanding the re-entrant superconducting phase diagram of an iron-pnictide Ca$_4$Al$_2$O$_6$Fe$_2$(As$_{1-x}$P$_x$)$_2$

Recently, a very rich phase diagram has been obtained for an iron-based superconductor Ca4Al2O6Fe2(As1-xPx)2. It has been revealed that nodeless (x=0) and nodal (x = 1) superconductivity are separated by an antiferromagnetic phase. Here we study the origin of this peculiar phase diagram using a five orbital model constructed from first principles band calculation, and applying the fluctuation exchange approximation assuming spin fluctuation mediated pairing. Based on the calculation results, we propose a scenario where the frustration in momentum space degrades superconductivity in the intermediate x regime, while antiferromangetism takes place due to a very good nesting. In order to see whether the present theoretical scenario is consistent with the actual nature of the competition between superconductivity and antiferromagnetism, we also perform hydrostatic pressure experiment for Ca4Al2O6Fe2(As1-xPx)2. In the intermediate x regime where antiferromagnetism occurs at ambient pressure, applying hydrostatic pressure smears out the antiferromagnetic transition, but superconductivity does not take place. This supports our scenario that superconductivity is suppressed by the momentum space frustration in the intermediate x regime, apart from the presence of the antiferromangnetism.

cond-mat.supr-con↗

arXiv2013

In search for the pairing glue in cuprates by non-equilibrium optical spectroscopy

In strongly correlated materials the electronic and optical properties are significantly affected by the coupling of fermionic quasiparticles to different degrees of freedom, such as lattice vibrations and bosonic excitations of electronic origin. Broadband ultrafast spectroscopy is emerging as the premier technique to unravel the subtle interplay between quasiparticles and electronic or phononic collective excitations, by their different characteristic timescales and spectral responses. By investigating the femtosecond dynamics of the optical properties of Y-Bi2212 crystals over the 0.5-2 eV energy range, we disentangle the electronic and phononic contributions to the generalized electron-boson Eliashberg function, showing that the spectral distribution of the electronic excitations, such as spin fluctuations and current loops, and the strength of their interaction with quasiparticles can account for the high critical temperature of the superconducting phase transition. Finally, we discuss how the use of this technique can be extended to the underdoped region of the phase diagram of cuprates, in which a pseudogap in the quasiparticle density of states opens. The microscopic modeling of the interaction of ultrashort light pulses with unconventional superconductors will be one of the key challenges of the next-years materials science, eventually leading to the full understanding of the role of the electronic correlations in controlling the dynamics on the femtosecond timescale.

cond-mat.supr-con↗

arXiv2012

Multiplet resonance lifetimes in resonant inelastic X-ray scattering involving shallow core levels

Resonant inelastic X-ray scattering (RIXS) spectra of model copper- and nickel-based transition metal oxides are measured over a wide range of energies near the M-edge (h$ν$=60-80eV) to better understand the properties of resonant scattering involving shallow core levels. Standard multiplet RIXS calculations are found to deviate significantly from the observed spectra. However, by incorporating the self consistently calculated decay lifetime for each intermediate resonance state within a given resonance edge, we obtain dramatically improved agreement between data and theory. Our results suggest that these textured lifetime corrections can enable a quantitative correspondence between first principles predictions and RIXS data on model multiplet systems. This accurate model is also used to analyze resonant elastic scattering, which displays the elastic Fano effect and provides a rough upper bound for the core hole shake-up response time.

cond-mat.str-el↗

arXiv2012

Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission

In high-temperature superconductivity, the process that leads to the formation of Cooper pairs, the fundamental charge carriers in any superconductor, remains mysterious. We use a femtosecond laser pump pulse to perturb superconducting Bi2Sr2CaCu2O8+δ, and study subsequent dynamics using time- and angle-resolved photoemission and infrared reflectivity probes. Gap and quasiparticle population dynamics reveal marked dependencies on both excitation density and crystal momentum. Close to the d-wave nodes, the superconducting gap is sensitive to the pump intensity and Cooper pairs recombine slowly. Far from the nodes pumping affects the gap only weakly and recombination processes are faster. These results demonstrate a new window into the dynamical processes that govern quasiparticle recombination and gap formation in cuprates.

cond-mat.supr-con↗