arXiv subjects

Hyunsoo Yang

Publications and source records attributed to Hyunsoo Yang.

At least 55 records · Page 3Linked to original sources

arXiv2020

Spin-orbit torque magnetization switching in MoTe2/permalloy heterostructures

The ability to switch magnetic elements by spin-orbit-induced torques has recently attracted much attention for a path towards high-performance, non-volatile memories with low power consumption. Realizing efficient spin-orbit-based switching requires harnessing both new materials and novel physics to obtain high charge-to-spin conversion efficiencies, thus making the choice of spin source crucial. Here we report the observation of spin-orbit torque switching in bilayers consisting of a semimetallic film of 1T'-MoTe2 adjacent to permalloy. Deterministic switching is achieved without external magnetic fields at room temperature, and the switching occurs with currents one order of magnitude smaller than those typical in devices using the best-performing heavy metals. The thickness dependence can be understood if the interfacial spin-orbit contribution is considered in addition to the bulk spin Hall effect. Further threefold reduction in the switching current is demonstrated with resort to dumbbell-shaped magnetic elements. These findings foretell exciting prospects of using MoTe2 for low-power semimetal material based spin devices.

cond-mat.mtrl-sci↗

arXiv2020

Optical visualization of the enhanced spin Hall effect in bismuth doped silicon

Direct visualizations of spin accumulation due to the enhanced spin Hall effect (SHE) in bismuth (Bi) - doped silicon (Si) at room temperature are realized by using helicity-dependent photovoltage (HDP) measurements. Under application of a dc current to the Bi-doped Si, clear helicity-dependent photovoltages are detected at the edges of the Si channel, indicating a perpendicular spin accumulation due to the SHE. In contrast, the HDP signals are negligibly small for phosphorus-doped Si. Compared to a platinum channel, which has a large spin Hall angle, more than two-orders of magnitude larger HDP signals are obtained in the Bi-doped Si.

cond-mat.mtrl-sci↗

arXiv2020

Electrical generation and detection of terahertz signal based on spin-wave emission from ferrimagnets

Terahertz (THz) signals, mainly generated by photonic or electronic approaches, are being sought for various applications, whereas the development of magnetic source might be a necessary step to harness the magnetic nature of electromagnetic radiation. We show that the relativistic effect on the current-driven domain-wall motion induces THz spin-wave emission in ferrimagnets. The required current density increases dramatically in materials with strong exchange interaction and rapidly exceeds 1012 A m-2, leading to the device breakdown and thus the lack of experimental evidence. By translating the collective magnetization oscillations into voltage signals, we propose a three-terminal device for the electrical detection of THz spin wave. Through material engineering, wide frequency range from 264 GHz to 1.1 THz and uniform continuous signals with improved output power can be obtained. As a reverse effect, the spin wave generated in this system is able to move ferrimagnetic domain wall. Our work provides guidelines for the experimental verification of THz spin wave, and could stimulate the design of THz spintronic oscillators for wideband applications as well as the all-magnon spintronic devices.

cond-mat.mes-hall↗

arXiv2020

Microscopic Origin of Spin-Orbit Torque in Ferromagnetic Heterostructures: A First Principles Approach

We present an {\it ab initio}-based theoretical framework which elucidates the origin of the spin-orbit torque (SOT) in Normal-Metal(NM)/Ferromagnet(FM) heterostructures. The SOT is decomposed into two contributions, namely, {\it spin-Hall} and the {\it spin-orbital} components. We find that {\it (i)} the Field-Like (FL) SOT is dominated by the spin-orbital component and {\it (ii)} both components contribute to the damping-like torque with comparable magnitude in the limit of thick Pt film. The contribution of the spin-orbital component to the DL-SOT is present only for NMs with strong SOC coupling strength. We demonstrate that the FL-SOT can be expressed in terms of the non-equilibrium spin-resolved orbital moment accumulation. The calculations reveal that the experimentally reported oxygen-induced sign-reversal of the FL-SOT in Pt/Co bilayers is due to the significant reduction of the majority-spin orbital moment accumulation on the interfacial NM atoms.

cond-mat.mes-hall↗

arXiv2019

Magnetotransport of Weyl semimetals with tilted Dirac cones

Weyl semimetals (WSM) exhibit chiral anomaly in their magnetotransport due to broken conservation laws. Here, we analyze the magnetotransport of WSM in the presence of the time-reversal symmetry-breaking tilt parameter. The analytical expression for the magnetoconductivity is derived in the small tilt limit using the semiclassical Boltzmann equation. We predict a planar Hall current which flows transverse to the electric field and in the plane containing magnetic and electric fields and scales linearly with the tilt parameter. A tilt-induced transverse conductivity is also present in the case where the electric and magnetic fields are parallel to each other, a scenario where the conventional Hall current completely vanishes.

cond-mat.mes-hall↗

arXiv2019

Nonlinear planar Hall effect

An intriguing property of three-dimensional (3D) topological insulator (TI) is the existence of surface states with spin-momentum locking, which offers a new frontier of exploration in spintronics. Here, we report the observation of a new type of Hall effect in a 3D TI Bi2Se3 film. The Hall resistance scales linearly with both the applied electric and magnetic fields and exhibits a π/2 angle offset with respect to its longitudinal counterpart, in contrast to the usual angle offset of π/4 between the linear planar Hall effect and the anisotropic magnetoresistance. This novel nonlinear planar Hall effect originates from the conversion of a nonlinear transverse spin current to a charge current due to the concerted actions of spin-momentum locking and time reversal symmetry breaking, which also exists in a wide class of non-centrosymmetric materials with a large span of magnitude. It provides a new way to characterize and utilize the nonlinear spin-to-charge conversion in a variety of topological quantum materials.

cond-mat.mes-hall↗

arXiv2019

Nonlinear magnetotransport shaped by Fermi surface topology and convexity in WTe2

The nature of Fermi surface defines the physical properties of conductors and many physical phenomena can be traced to its shape. Although the recent discovery of a current-dependent nonlinear magnetoresistance in spin-polarized non-magnetic materials has attracted considerable attention in spintronics, correlations between this phenomenon and the underlying fermiology remain unexplored. Here, we report the observation of nonlinear magnetoresistance at room temperature in a semimetal WTe2, with an interesting temperature-driven inversion. Theoretical calculations reproduce the nonlinear transport measurements and allow us to attribute the inversion to temperature-induced changes in Fermi surface convexity. We also report a large anisotropy of nonlinear magnetoresistance in WTe2, due to its low symmetry of Fermi surfaces. The good agreement between experiments and theoretical modeling reveals the critical role of Fermi surface topology and convexity on the nonlinear magneto-response. These results lay a new path to explore ramifications of distinct fermiology for nonlinear transport in condensed-matter.

cond-mat.mtrl-sci↗

arXiv2018

Current-enhanced broadband THz emission from spintronic devices

An ultra-broadband THz emitter covering a wide range of frequencies from 0.1 to 10 THz is highly desired for spectroscopy applications. So far, spintronic THz emitters have been proven as one class of efficient THz sources with a broadband spectrum while the performance in the lower frequency range (0.1 to 0.5 THz) limits its applications. In this work, we demonstrate a novel concept of a current-enhanced broad spectrum from spintronic THz emitters combined with semiconductor materials. We observe a 2-3 order enhancement of the THz signals in a lower THz frequency range (0.1 to 0.5 THz), in addition to a comparable performance at higher frequencies from this hybrid emitter. With a bias current, there is a photoconduction contribution from semiconductor materials, which can be constructively interfered with the THz signals generated from the magnetic heterostructures driven by the inverse spin Hall effect. Our findings push forward the utilization of metallic heterostructures-based THz emitters on the ultra-broadband THz emission spectroscopy.

physics.app-ph↗

arXiv2018

Long spin coherence length and bulk-like spin-orbit torque in ferrimagnetic multilayers

Ferromagnetic spintronics has been a main focus as it offers non-volatile memory and logic applications through current-induced spin-transfer torques. Enabling wider applications of such magnetic devices requires a lower switching current for a smaller cell while keeping the thermal stability of magnetic cells for non-volatility. As the cell size reduces, however, it becomes extremely difficult to meet this requirement with ferromagnets because spin-transfer torque for ferromagnets is a surface torque due to rapid spin dephasing, leading to the 1/ferromagnet-thickness dependence of the spin-torque efficiency. Requirement of a larger switching current for a thicker and thus more thermally stable ferromagnetic cell is the fundamental obstacle for high-density non-volatile applications with ferromagnets. Theories predicted that antiferromagnets have a long spin coherence length due to the staggered spin order on an atomic scale, thereby resolving the above fundamental limitation. Despite several spin-torque experiments on antiferromagnets and ferrimagnetic alloys, this prediction has remained unexplored. Here we report a long spin coherence length and associated bulk-like-torque characteristic in an antiferromagnetically coupled ferrimagnetic multilayer. We find that a transverse spin current can pass through > 10 nm-thick ferrimagnetic Co/Tb multilayers whereas it is entirely absorbed by 1 nm-thick ferromagnetic Co/Ni multilayer. We also find that the switching efficiency of Co/Tb multilayers partially reflects a bulk-like-torque characteristic as it increases with the ferrimagnet-thickness up to 8 nm and then decreases, in clear contrast to 1/thickness-dependence of Co/Ni multilayers. Our results on antiferromagnetically coupled systems will invigorate researches towards energy-efficient spintronic technologies.

cond-mat.mtrl-sci↗

arXiv2018

Ultrafast Spin-To-Charge Conversion at the Surface of Topological Insulator Thin Films

Strong spin-orbit coupling, resulting in the formation of spin-momentum-locked surface states, endows topological insulators with superior spin-to-charge conversion characteristics, though the dynamics that govern it have remained elusive. Here, we present an all-optical method that enables unprecedented tracking of the ultrafast dynamics of spin-to-charge conversion in a prototypical topological insulator Bi$_2$Se$_3$/ferromagnetic Co heterostructure, down to the sub-picosecond timescale. Compared to pure Bi$_2$Se$_3$ or Co, we observe a giant terahertz emission in the heterostructure than originates from spin-to-charge conversion, in which the topological surface states play a crucial role. We identify a 0.12-picosecond timescale that sets a technological speed limit of spin-to-charge conversion processes in topological insulators. In addition, we show that the spin-to-charge conversion efficiency is temperature independent in Bi$_2$Se$_3$ as expected from the nature of the surface states, paving the way for designing next-generation high-speed opto-spintronic devices based on topological insulators at room temperature.

cond-mat.mtrl-sci↗

arXiv2018

Recent advances in spin-orbit torques: Moving towards device applications

The ability of spintronic devices to utilize an electric current for manipulating the magnetization has resulted in large-scale developments, such as, magnetic random access memories and boosted the spintronic research area. In this regard, over the last decade, magnetization manipulation using spin-orbit torque has been devoted a lot of research attention as it shows a great promise for future ultrafast and power efficient magnetic memories. In this review, we summarize the latest advancements in spin-orbit torque research and highlight some of the technical challenges for practical spin-orbit torque devices. We will first introduce the basic concepts and highlight the latest material choices for spin-orbit torque devices. Then, we will summarize the important advancements in the study of magnetization switching dynamics using spin-orbit torque, which are important from scientific as well as technological aspect. The final major section focuses on the concept of external assist field free spin-orbit torque switching which is a requirement for practical spin-orbit torque devices.

cond-mat.mes-hall↗

arXiv2018

Field-free spin-orbit torque switching from geometrical domain wall pinning

Spin-orbit torques, which utilize spin currents arising from the spin-orbit coupling, offer a novel method to electrically switch the magnetization with perpendicular anisotropy. However, the necessity of an external magnetic field to achieve a deterministic switching is an obstacle for realizing practical spin-orbit torque devices with all-electric operation. Here, we report a field-free spin-orbit torque switching by exploiting the domain wall motion in an anti-notched microwire with perpendicular anisotropy, which exhibits multi-domain states stabilized by the domain wall surface tension. The combination of spin-orbit torque, Dzyaloshinskii-Moriya interaction, and domain wall surface tension induced geometrical pinning allows a deterministic control of the domain wall and offers a novel method to achieve a field-free spin-orbit torque switching. Our work demonstrates the proof of concept of a perpendicular memory cell which can be readily adopted in a three-terminal magnetic memory.

cond-mat.mtrl-sci↗

arXiv2018

Terahertz Emission from Compensated Magnetic Heterostructures

Terahertz emission spectroscopy (TES) has recently played an important role in unveiling the spin dynamics at a terahertz (THz) frequency range. So far, ferromagnetic (FM)/nonmagnetic (NM) heterostructures have been intensively studied as THz sources. Compensated magnets such as a ferrimagnet (FIM) and antiferromagnet (AFM) are other types of magnetic materials with interesting spin dynamics. In this work, we study TES from compensated magnetic heterostructures including CoGd FIM alloy or IrMn AFM layers. Systematic measurements on composition and temperature dependences of THz emission from CoGd/Pt bilayer structures are conducted. It is found that the emitted THz field is determined by the net spin polarization of the laser induced spin current rather than the net magnetization. The temperature robustness of the FIM based THz emitter is also demonstrated. On the other hand, an AFM plays a different role in THz emission. The IrMn/Pt bilayer shows negligible THz signals, whereas Co/IrMn induces sizable THz outputs, indicating that IrMn is not a good spin current generator, but a good detector. Our results not only suggest that a compensated magnet can be utilized for robust THz emission, but also provide a new approach to study the magnetization dynamics especially near the magnetization compensation point.

cond-mat.mes-hall↗

arXiv2018

Observation of out-of-plane spin texture in a SrTiO3 (111) two-dimensional electron gas

We explore the second order bilinear magnetoelectric resistance (BMER) effect in the d-electron-based two-dimensional electron gas (2DEG) at the SrTiO3 (111) surface. We find an evidence of a spin-split band structure with the archetypal spin-momentum locking of the Rashba effect for the in-plane component. Under an out-of-plane magnetic field, we find a BMER signal that breaks the six-fold symmetry of the electronic dispersion, which is a fingerprint for the presence of a momentum dependent out-of-plane spin component. Relativistic electronic structure calculations reproduce this spin-texture and indicate that the out-of-plane component is a ubiquitous property of oxide 2DEGs arising from strong crystal field effects. We further show that the BMER response of the SrTiO3 (111) 2DEG is tunable and unexpectedly large.

cond-mat.mes-hall↗

arXiv2018

Direct visualization of current induced spin accumulation in topological insulators

Charge-to-spin conversion in various material systems is the key for the fundamental understanding of spin-orbitronis as well as the development of efficient means to manipulate the magnetization. We report the direct spatial imaging of current induced spin accumulation at the channel edges of Bi2Se3 and BiSbTeSe2 topological insulators by a scanning photovoltage microscope at room temperature. The spin polarization is along the out-of-plane direction with opposite signs for the two channel edges. The accumulated spin direction reverses sign upon changing the current direction and the detected spin signal shows a linear dependence on the magnitude of currents, which indicates that our observed phenomena are the current induced effects. The spin Hall angle of Bi2Se3 and BiSbTeSe2 is determined to be 0.0085 and 0.0616, respectively. We further image the current induced spin accumulation in a Pt heavy metal. Our results open up the possibility of optically detecting the current induced spin accumulations, and thus point towards a better understanding of the interaction between spins and circularly polarized light.

cond-mat.mes-hall↗

arXiv2018

FMR-related phenomena in spintronic devices

Spintronic devices, such as non-volatile magnetic random access memories and logic devices, have attracted considerable attention as potential candidates for future high efficient data storage and computing technology. In a heavy metal or other emerging material with strong spin-orbit coupling (SOC), the charge currents induce spin currents or spin accumulations via SOC. The generated spin currents can exert spin-orbit torques (SOTs) on an adjacent ferromagnet, which opens up a new way to realize magnetization dynamics and switching of the ferromagnetic layer for spintronic devices. In the SOT scheme, the charge-to-spin interconversion efficiency (SOT efficiency) is an important figure of merit for applications. For the effective characterization of this efficiency, the ferromagnetic resonance (FMR) based methods, such as the spin transfer torque ferromagnetic resonance (ST-FMR) and the spin pumping, are common utilized in addition to low frequency harmonic or dc measurements. In this review, we focus on the ST-FMR measurements for the evaluation of the SOT efficiency. We provide a brief summary of the different ST-FMR setups and data analysis methods. We then discuss ST-FMR and SOT studies in various materials, including heavy metals and alloys, topological insulators, two dimensional (2D) materials, interfaces with strong Rashba effect, antiferromagnetic materials, two dimensional electron gas (2DEG) in oxide materials and oxidized nonmagnetic materials.

cond-mat.mtrl-sci↗

arXiv2018

Effect of capping layer on spin-orbit torques

In order to enhance the magnitude of spin-orbit torque (SOT), considerable experimental works have been devoted to studying the thickness dependence of the different layers in multilayers consisting of heavy metal (HM), ferromagnet (FM) and capping layers. Here we present a theoretical model based on the spin-drift-diffusion (SDD) formalism to investigate the effect of the capping layer properties such as its thickness on the SOT observed in experiments. It is found that the spin Hall-induced SOT can be significantly enhanced by incorporating a capping layer with opposite spin Hall angle to that of the HM layer. The spin Hall torque can be maximized by tuning the capping layer thickness. However, in the absence of the spin Hall effect (SHE) in the capping layer, the torque decreases monotonically with capping layer thickness. Conversely, the spin Hall torque is found to decrease monotonically with the FM layer thickness, irrespective of the presence or absence of SHE in the capping layer. All these trends are in correspondence with experimental observations. Finally, our model suggests that capping layers with long spin diffusion length and high resistivity would also enhance the spin Hall torque.

physics.app-ph↗

arXiv2018

Room-temperature nanoseconds spin relaxation in WTe2 and MoTe2 thin films

The Weyl semimetal WTe2 and MoTe2 show great potential in generating large spin currents since they possess topologically-protected spin-polarized states and can carry a very large current density. In addition, the intrinsic noncentrosymmetry of WTe2 and MoTe2 endows with a unique property of crystal symmetry-controlled spin-orbit torques. An important question to be answered for developing spintronic devices is how spins relax in WTe2 and MoTe2. Here, we report a room-temperature spin relaxation time of 1.2 ns (0.4 ns) in WTe2 (MoTe2) thin film using the time-resolved Kerr rotation (TRKR). Based on ab initio calculation, we identify a mechanism of long-lived spin polarization resulting from a large spin splitting around the bottom of the conduction band, low electron-hole recombination rate and suppression of backscattering required by time-reversal and lattice symmetry operation. In addition, we find the spin polarization is firmly pinned along the strong internal out-of-plane magnetic field induced by large spin splitting. Our work provides an insight into the physical origin of long-lived spin polarization in Weyl semimetals which could be useful to manipulate spins for a long time at room temperature.

cond-mat.mtrl-sci↗