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Igor Žutić

Publications and source records attributed to Igor Žutić.

At least 19 recordsLinked to original sources

Magnon Polarization Textures and Transport in Antiferromagnets and Altermagnets

Antiferromagnets (AFMs) host magnons that can exhibit fully circular, elliptic and linear polarizations of sublattice magnetization dynamics. We analyze theoretically different momentum-space magnon polarization textures and magnon transport in collinear AFMs and altermagnets (AMs). The sensitivity of the polarization texture to a magnon momentum direction determines two regimes of magnon polarization kinetics: The Dyakonov-Perel relaxation or its dephasing due to asynchronous Larmor precession. For an easy-axis AFM, magnetic field parallel to the N{é}el vector leads to the suppression of the magnetic dipolar interaction-induced Dyakonov-Perel relaxation, accompanied by the increase in the magnon spin-diffusion length and its counter-intuitive growth with temperature. For a perpendicular orientation, instead, relaxation of circular polarization of magnons is enhanced due to Larmor precession. Finally, extremely anisotropic relaxation of magnon polarization is predicted for AMs or AFMs having Dzyaloshinskii-Morya interaction.

cond-mat.other↗

Ferroelectric switching of odd-parity magnon spin splitting

Magnetic symmetry can lift spin degeneracy in momentum space without producing net magnetization, generating spin textures classified by their parity under momentum reversal. Even-parity textures have well established in altermagnets. Odd-parity spin textures have recently emerged in electronic bands of compensated magnets, but their counterpart in collective bosonic excitations remains experimentally unresolved. Magnons provide a natural setting for this extension because they carry spin angular momentum through insulating magnets without accompanying charge flow. Beyond realizing this missing state, a broader challenge is to program spin splitting with voltage at room temperature. Here we report room-temperature transport evidence for ferroelectric switching odd-parity magnon spin splitting in multiferroic BiFeO3. Symmetry analysis and spin-wave calculations reveal that the cycloidal chirality splits opposite-spin magnon branches with an odd-in-momentum dependence and sets the sign. Experimentally, an injected in-plane-polarized spin current generates an out-of-plane magnon spin component during propagation. This component exhibits the crystalline angular dependence predicted by theory and reverses upon ferroelectric switching, providing a transport fingerprint of the spin-split magnon state. We use the programmed magnon spin to drive deterministic field-free switching of a perpendicular ferromagnet and demonstrate XNOR logic-in-memory. Our results extend odd-parity spin splitting from fermionic electronic states to bosonic collective modes and establish nonvolatile electrical control at room temperature.

cond-mat.mtrl-sci↗

Supercurrent-Driven Néel Torque in Superconductor/Altermagnet Hybrids

We predict a supercurrent-driven Néel spin-orbit torque in a superconductor/$d$-wave altermagnet heterostructure, associated with the emergence of spin-triplet correlations. The effect can be understood as a consequence of the supercurrent-induced spin polarization, owing to the interplay between spin orbit coupling and momentum-dependent spin splitting, as found, for example, in altermagnets. Remarkably, the supercurrent can be tuned by the Néel-vector direction, and the supercurrent-induced torque can both propel magnetic domain walls and reverse the Néel-vector orientation within a domain wall. These findings establish superconductor/altermagnet heterostructures as a versatile platform for the {supercurrent-driven} control of the Néel vector, with potential applications in racetrack memory, dissipationless superconducting electronics, and unconventional computing.

cond-mat.mes-hall↗

Dynamical Josephson Effect Between a Singlet and a Triplet Superconductor

Phase-sensitive Josephson effect has long been central to identifying unconventional pairing symmetries in superconductors. Although the selection rules governing Josephson junctions (JJs) are generally determined by the symmetries of the constituent superconductors, we demonstrate that this paradigm is modified in the dynamic regime. By modeling a JJ where spin-singlet and spin-triplet superconductors are separated by a two-dimensional electron gas, we show that a time-dependent gate voltage qualitatively changes the underlying selection rules. This modification arises as a consequence of the gate-controlled spin-orbit coupling. A harmonic modulation of the gate voltage generates an oscillatory $\cos ϕ$ Josephson component which vanishes in the static limit. The resulting charge current contains both dissipationless and dissipative components, with the latter strongly suppressed at low temperatures. This dynamical Josephson effect could transform the use of JJs in qubits, as sources of spin-triplet currents, and as platforms for proximity effects.

cond-mat.supr-con↗

Many-body description of two-dimensional van der Waals ferroelectric $α-$In$_2$Se$_3$

Two-dimensional (2D) van der Waals ferroelectrics are recognized for enabling many applications, from memory and logic to neuromorphic computing, as well as transforming other materials to control electronic phase transitions and topological states. While these materials are typically weakly correlated and expected to have their ground-state properties well described with the commonly used density functional theory, by focusing on bilayers and trilayers of In$_2$Se$_3$ we show that this approach may not be reliable. The underlying electronic structure strongly depends on the polarization structure of the multilayer system and is surprisingly challenging to accurately calculate, requiring a high-fidelity many-body theory of the quasiparticle self-consistent \textit{GW} approximation. We develop this underlying description by extending the capabilities of Green function implementation within the open-source Questaal package. We show that even a sophisticated hybrid functional approach may fail to predict a nonvanishing gap in a bilayer In$_2$Se$_3$ and yields charge density, polarization, and band offsets that strongly deviate from the many-body picture. We discuss the implications of these computational advances for future opportunities in 2D ferroelectrics.

cond-mat.mtrl-sci↗

Valleytronics in 2D Materials Roadmap

Valleytronics exploits non-equivalent energy extrema in the electronic band structure of crystalline solids -- the valley degree of freedom -- to encode, manipulate, and read out information. The advent of 2D materials, first graphene and then transition-metal dichalcogenides, made valley control practical through optical, electrical, and magnetic routes. This foundation has enabled remarkable progress in recent years spanning established frontiers, such as valley exciton physics and valley Hall effects, as well as emerging directions including lightwave valleytronics, nanophotonic integration, flat-band valleytronics, and spin-valley qubits. In parallel, there are sustained efforts to scale up valleytronic materials and to predict new valleytronic platforms. This Roadmap brings together perspectives from leading experts to chart the key opportunities and challenges at the forefront of 2D material valleytronics. Each section captures a snapshot of progress in a key research area, identifies critical open challenges, and outlines pathways toward future valleytronics breakthroughs.

cond-mat.mes-hall↗

Superconducting spintronics with electron symmetry filtering and interfacial spin-orbit coupling

Over the recent years, crossroads of magnetism and superconductivity led to the emerging field of superconducting spintronics. A cornerstone of this venture is the generation of equal-spin triplet Cooper pairs in superconductor-ferromagnet hybrids, enabling long-range spin-polarized supercurrents and magnetic control over superconducting quantum states for the development of energy-efficient cryogenic devices. Until now, nearly all superconducting spintronic devices have relied on direct interfaces between superconductors and ferromagnets, since it was believed that an insulating barrier would decouple spin and charge transport. This assumption, however, appears to be invalid when a thin spin- and orbit-filtering barrier couples epitaxial ferromagnet and the superconductor. Symmetry filtering plays a crucial role in enhancing giant tunneling magnetoresistance (TMR) by selectively allowing specific electronic states to tunnel through the barrier. Such a mechanism is key for high-performance spintronic devices like magnetic random access memories, magnetic sensors or spin-light emitting diodes. This manuscript provides a comprehensive review of superconducting spintronics driven by electron symmetry filtering and interfacial SOC. It emphasizes the critical role of a crystalline MgO barrier in selectively transmitting specific electronic states between V(100) and Fe(100). The manuscript also highlights how interfacial SOC enables symmetry mixing, allowing for the interaction between ferromagnetic and superconducting orderings though MgO(100). This mutual interaction, mediated by interfacial SOC, facilitates the conversion of spin-singlet to spin-triplet Cooper pairs. The work provides key insights into designing SOC based superconductor-ferromagnet hybrid structures for advanced superconducting spintronic functionalities.

cond-mat.supr-con↗

Giant shot noise in superconductor/ferromagnet junctions with orbital-symmetry-controlled spin-orbit coupling

By measuring the shot noise, a consequence of charge quantization, in superconductor/insulator/ferromagnet (V/MgO/Fe) junctions, we discover a giant increase, orders of magnitude larger than expected. The origin of this giant noise is a peculiar realization of a superconducting proximity effect, where a simple superconductor influences its neighbors. Our measurements reveal largely unexplored implications of orbital-symmetry-controlled proximity effects. The importance of orbital symmetries and the accompanying spin-orbit coupling is manifested by an unexpected emergence of another superconducting region strikingly different from the parent superconductor. Unlike vanadium's common spin-singlet superconductivity, the broken inversion symmetry in V/MgO/Fe junctions and the resulting interfacial spin-orbit coupling leads to the formation of spin-triplet superconductivity across the ferromagnetic iron. Here we show that the enhanced shot noise, known from Josephson junctions with two superconductors, is measured even in a single superconductor, this discovery motivates revisiting how the spin-orbit coupling and superconducting proximity effects can transform many materials.

cond-mat.supr-con↗

The birefringent spin-laser as a system of coupled harmonic oscillators

Adding spin-polarized carriers to semiconductor lasers strongly changes their properties and, through the transfer of angular momentum, leads to the emission of circularly polarized light. In such spin-lasers, the polarization of the emitted light can be modulated an order of magnitude faster than its intensity in the best conventional lasers. This ultrafast operation in spin-lasers relies on large linear birefringence, usually viewed as detrimental in spin and conventional lasers, which couples the two linearly polarized emission modes. We show that the dynamical properties of birefringent spin-lasers under intensity and polarization modulation are accurately described as coupled harmonic oscillators. Our model agrees with the intensity-equation description which, unlike the common complex field components describing the role of birefringence in laser dynamics, uses simpler real quantities and allows analytical solutions. We further predict unexplored operation regimes and elucidate the difference between the weak and strong coupling in spin-lasers.

cond-mat.mes-hall↗

Unconventional Spintronics from Chiral Perovskites

Spintronic devices typically employ heterostructures with ferromagnets which break time-reversal symmetry and have non-vanishing magnetization. With the growing class of materials that support spin-polarized carriers, current, and excitations,it is possible to envision emerging spintronic applications that are not limited to magnetoresistance. Here we focus on chiral perovskites with no net magnetization where the space-inversion and mirror symmetries are broken to induce chiral structure. The known importance of these perovskites is further expanded by the demonstration of the chiral-induced spin selectivity (CISS). However, the generation of the spin-polarized carriers across the interface with these chiral perovskites remains to be fully understood. Our first-principles studies for two-dimensional PbBr$_4$-based chiral perovskites provide their electronic structure and an orbital-based symmetry analysis, which allows us to establish an effective Hamiltonian to elucidate the underlying origin of their chirality. We also use this analysis for the Edelstein effect, responsible for electrical generation of the nonequilibrium spin polarization in many materials, which in chiral perovskites could be a mechanism contributing to CISS. Furthermore, by examining optical properties of chiral perovskites and the opportunity to use them to realize tunable altermagnets, another class of zero-magnetization spintronic materials, we put forth a versatile materials platform for unconventional spintronics.

cond-mat.mtrl-sci↗

Movable Dirac Points with Ferroelectrics: Kink States and Berry Curvature Dipoles

Two-dimensional (2D) Dirac states and Dirac points with linear dispersion are the hallmark of graphene, topological insulators, semimetals, and superconductors. Lowering a symmetry by the ferroelectric polarization opens the gap in Dirac points and introduces finite Berry curvature. Combining this with Dirac points detached from high symmetry points of the Brillouin zone offers additional ways to tailor topological properties. We explore this concept by studying topological phenomena emerging in 2D materials with movable Dirac points and broken out-of-plane mirror reflection. The resulting topological kink states and Berry curvature dipoles are changed by movable 2D Dirac points with experimental signatures in electrical conductance and second-harmonic nonlinear Hall conductivity. We identify materials platforms where our predictions can be realized and support that with the first-principles results for Cl$_2$Rh$_2$S$_2$-GeS junction.

cond-mat.mes-hall↗

Terahertz Spin-Light Coupling in Proximitized Dirac Materials

The two-dimensional (2D) materials are highly susceptible to the influence of their neighbors, thereby enabling the design by proximity phenomena. We reveal a remarkable terahertz (THz) spin-light interaction in 2D Dirac materials that arises from magnetic and spin-orbital proximity effects. The dynamical realization of the spin-charge conversion, the electric dipole spin resonance (EDSR), of Dirac electrons displays distinctive THz features, upon emerging spin-pseudospin proximity terms in the Hamiltonian. To capture the effect of fast pseudospin dynamics on the electron spin, we develop a mean-field theory and complement it with a quantum-mechanical treatment. As a specific example, we investigate the THz response of a single graphene layer proximitized by a magnetic substrate. Our analysis demonstrates a strong enhancement and anomalous polarization structure of the THz-light absorption which can enable THz detection and efficient generation and control of spins in spin-based quantum devices. The identified coupled spin-pseudospin dynamics is not limited to EDSR and may influence a broad range of optical, transport, and ultrafast phenomena.

cond-mat.mes-hall↗

Anisotropic spin dynamics in antiferromagnets with a nonrelativistic spin splitting

Antiferromagnets (AFM) with a nonrelativistic spin splitting (NSS) of electronic bands expand the range of spin-dependent phenomena and their applications. A crucial understanding for both of them pertains to the inherent spin dynamics. We demonstrate that the $d$-wave NSS gives rise to extremely anisotropic spin dynamics of carriers driven by the relaxation induced by motional narrowing. In contrast to the no relaxation of the spin polarization along the Neel vector, the dynamics of perpendicular spin components greatly varies from a long relaxation for a weak NSS to the fast-decaying oscillations for a strong NSS, a regime relevant to AFM with the $d$-wave NSS. The extreme anisotropy of the spin relaxation is transformed by the external magnetic field, which triggers the relaxation of the parallel spin component and also suppresses all the relaxation rates at larger magnitudes. The predicted spin dynamics of the $d$-wave NSS, known also from altermagnets, can be used as their experimental fingerprints and guide future applications.

cond-mat.mes-hall↗

Signatures of enhanced spin-triplet superconductivity induced by interfacial properties

While spin-triplet pairing remains elusive in nature, there is a growing effort to realize proximity-induced equal-spin triplet superconductivity in junctions with magnetic regions or an applied magnetic field and common $s$-wave superconductors. To enhance such spin-triplet contribution, it is expected that junctions with a weak interfacial barrier and strong spin-orbit coupling are desirable. Intuitively, a weak interfacial barrier enables a robust proximity-induced superconductivity and strong spin-orbit coupling promotes spin mixing, converting spin-singlet into spin-triplet superconductivity. In contrast, we reveal a nonmonotonic spin-triplet contribution with the strength of the interfacial barrier and spin-orbit coupling. This picture is established by considering different signatures in conductance and superconducting correlations, as well as by performing self-consistent calculations. As a result, we identify a strongly enhanced spin-triplet superconductivity, realized for an intermediate strength of interfacial barrier and spin-orbit coupling. In junctions with magnetic regions, an enhanced spin-triplet superconductivity leads to a large magnetoanisotropy of conductance and superconducting correlations. This picture of an enhanced spin-triplet superconductivity is consistent with experiments demonstrating a huge increase in the conductance magnetoanisotropy, which we predict can be further enhanced at a finite bias.

cond-mat.supr-con↗

Microwave Signatures of Topological Superconductivity in Planar Josephson Junctions

Planar Josephson junctions provide a platform to host topological superconductivity which, through manipulating Majorana bound states (MBS), could enable fault-tolerant quantum computing. However, what constitutes experimental signatures of topological superconductivity and how MBS can be detected remains strongly debated. In addition to spurious effects that mimic MBS, there is a challenge to discern the inherent topological signals in realistic systems with many topologically-trivial Andreev bound states, determining the transport properties of Josephson junctions. Guided by the advances in microwave spectroscopy, we theoretically study Al/InAs-based planar Josephson junction embedded into a radio-frequency superconducting quantum interference device to identify microwave signatures of topological superconductivity. Remarkably, by exploring the closing and reopening of a topological gap, we show that even in a wide planar Josephson junction with many Andreev bound states, such a topological signature is distinguishable in the resonance frequency shift of a microwave drive and the ``half-slope'' feature of the microwave absorption spectrum. Our findings provide an important step towards experimental detection of non-Abelian statistics and implementing scalable topological quantum computing.

cond-mat.mes-hall↗

Colloquium: Spin-orbit effects in superconducting hybrid structures

Spin-orbit coupling (SOC) relates to the interaction between an electron's motion and its spin, and is ubiquitous in solid-state systems. Although the effect of SOC in normal-state phenomena has been extensively studied, its role in superconducting hybrid structures and devices opens many unexplored questions. In conjunction with broken symmetries and material inhomogeneities within superconducting hybrid structures, SOC may have additional contributions, beyond its effects in homogenous materials. Remarkably, even with well-established magnetic or nonmagnetic materials and conventional s-wave spin-singlet superconductors, SOC leads to emergent phenomena including equal-spin triplet pairing and topological superconductivity (hosting Majorana states), a modified current-phase relationship in Josephson junctions, and nonreciprocal transport. SOC is also responsible for transforming quasiparticles in superconducting structures which enhances the spin Hall effect and changes spin dynamics. Taken together, SOC in superconducting hybrid structures and the potential for electric tuning of the SOC strength, creates fascinating possibilities to advance superconducting spintronic devices for energy-efficient computing, and enable topological fault-tolerant quantum computing. By providing a description of experimental techniques and theoretical methods to study SOC, this Colloquium describes the current understanding of resulting phenomena in superconducting structures and offers a framework to select and design a growing class of materials systems where SOC plays an important role.

cond-mat.supr-con↗

Phase jumps in Josephson junctions with time-dependent spin-orbit coupling

Planar Josephson junctions (JJs), based on common superconductors and III-V semiconductors, are sought for Majorana states and fault-tolerant quantum computing. However, with gate-tunable spin-orbit coupling (SOC), we show that the range of potential applications of such JJs becomes much broader. The time-dependent SOC offers unexplored mechanisms for switching JJs, accompanied by the $2π$-phase jumps and the voltage pulses corresponding to the single-flux-quantum transitions, key to high-speed and low-power superconducting electronics. In a constant applied magnetic field, with Rashba and Dresselhaus SOC, anharmonic current-phase relations, calculated microscopically in these JJs, yield a nonreciprocal transport and superconducting diode effect. Together with the time-dependent SOC, this allows us to identify a switching mechanism at no applied current bias which supports fractional-flux-quantum superconducting circuits and neuromorphic computing.

cond-mat.supr-con↗

Beyond the standard model of topological Josephson junctions: From crystalline anisotropy to finite-size and diode effects

A planar Josephson junction is a versatile platform to realize topological superconductivity over a large parameter space and host Majorana bound states. With a change in Zeeman field, this system undergoes a transition from trivial to topological superconductivity accompanied by a jump in the superconducting phase difference between the two superconductors. A standard model of these Josephson junctions, which can be fabricated to have a nearly perfect interfacial transparency, predicts a simple universal behavior. In that model, at the same value of Zeeman field for the topological transition, there is a $π$ phase jump and a minimum in the critical superconducting current, while applying a controllable phase difference yields a diamond-shaped topological region as a function of that phase difference and a Zeeman field. In contrast, even for a perfect interfacial transparency, we find a much richer and nonuniversal behavior as the width of the superconductor is varied or the Dresselhaus spin-orbit coupling is considered. The Zeeman field for the phase jump, not necessarily $π$, is different from the value for the minimum critical current, while there is a strong deviation from the diamond-like topological region. These Josephson junctions show a striking example of a nonreciprocal transport and superconducting diode effect, revealing the importance of our findings not only for topological superconductivity and fault-tolerant quantum computing, but also for superconducting spintronics.

cond-mat.mes-hall↗