arXiv subjects

Jian-Hao Chen

Publications and source records attributed to Jian-Hao Chen.

At least 19 recordsLinked to original sources

arXiv2026

Correlated Insulating States in Twisted Double Bilayer Graphene Enhanced by Interfacial Effect on CrOCl

Interaction between different two dimensional materials can give rise to many exotic physical phenomena which are rarely observed in intrinsic materials. Recently, several theoretical and experimental works have revealed that magnetic proximity effect between pristine graphene and magnetic substrates can lead to the emergence of quantum anomalous Hall states and quantum spin Hall states. However, interplay between correlated states in graphene-based systems and magnetic materials has seldom been studied. Here we perform the transport measurement at ultrahigh magnetic field of twisted double bilayer graphene (TDBG) on CrOCl (COC) substrate, which is an antiferromagnetic material. Instead of a magnetic-exchange effect on graphene, we observe an enhanced correlated insulating state at half-filling factor of TDBG as a result of the charge-transfer process between TDBG and COC. The temperature and magnetic field dependence of this enhanced state are further studied. Our results demonstrate the influence of charge-related effect at the interface, and shed a light on a new route for manipulating the correlated states in graphene-based moiré systems using interfacial engineering.

cond-mat.mes-hall↗

arXiv2026

Quantum geometry induced anomalous chiral transport and hidden symmetry breaking in centrosymmetric 2M-WS2

Chirality, a widely existing material property in nature involving the breaking of the left-right symmetry, has profound influences in various fields of natural sciences. Nonlinear response, such as electronic magnetochiral anisotropy (eMChA), has been recognized as a sensitive probe for the effects of symmetry breaking and nontrivial quantum geometries in solids. So far, observations of eMChA have primarily been limited to inversion-symmetry broken materials. Here, we report a remarkable chiral transport in centrosymmetric candidate topological superconductor 2M-WS2 flakes observed via second-harmonic generation under an out-of-plane magnetic field. More importantly, the eMChA becomes significant around the crossover temperature TFL ~ 25 K from the Fermi liquid (FL) to strange metal (SM) in the normal state, which interestingly echoes with the anomalously large Nernst response at the same temperature in bulk 2M-WS2. These observations reveal a direct correspondence between the nonlinear response, Nernst response, and FL-SM transition in 2M-WS2. Theoretical analysis indicates that nontrivial quantum geometry is behind the simultaneous response of eMChA and Nernst effects in 2M-WS2 and the contribution from the orbital magnetic moment at the Fermi surface becomes significant during the FL-SM transition. Based on first-principles calculations, a thick-layer-sliding mechanism with minimal energy gain in 2M-WS2 provides one possibility for the generation of such nontrivial quantum geometry. The intertwined physics of remarkable eMChA, Nernst response, and FL-SM transition make 2M-WS2 a rare quantum platform to study the chiral transport and unexplored phenomena in strange metals, which may shed light on the trans-century, unresolved scientific issue in unconventional high-temperature superconductivity.

cond-mat.str-el↗

arXiv2026

Long-distance spin transport in frustrated hyperkagome magnet Gd3Ga5O12

Transport of spin angular momentum over large distance has been a long sought-after goal in the field of spintronics. While the majority of the research effort has been devoted to the spin transport properties of magnetically ordered materials, spin transport in magnetically frustrated materials has received little attention. Here, we report an anomalous state in frustrated hyperkagome magnetic insulator Gd3Ga5O12, where spin angular momenta can be transported over a long distance of 480 μm, far exceeding the transport distance of any diffusive spin current in magnetically ordered materials, to the best of our knowledge. Monte Carlo simulations reveal significant spin fluctuations, spin-spin correlations and an absence of conventional magnons in such anomalous state; while the response of the anomalous state to perturbation is found to be akin to an overdamped forced oscillator. We find close relation of such state to the correlated ``director'' state in the material. Our result provides an effective electrical technique to characterize spin-spin correlations and frustrations; it also unveils the potential of frustrated magnets as powerful channel materials for spin transport.

cond-mat.mtrl-sci↗

arXiv2024

Nematic Ising superconductivity with hidden magnetism in few-layer 6R-TaS2

In van der Waals heterostructures (vdWHs), the manipulation of interlayer stacking/coupling allows for the construction of customizable quantum systems exhibiting exotic physics. An illustrative example is the diverse range of states of matter achieved through varying the proximity coupling between two-dimensional (2D) quantum spin liquid (QSL) and superconductors within the TaS2 family. This study presents a demonstration of the intertwined physics of spontaneous rotational symmetry breaking, hidden magnetism, and Ising superconductivity in the three-fold rotationally symmetric, non-magnetic natural vdWHs 6R-TaS2. A distinctive phase emerges in 6R-TaS2 below a characteristic temperature (T*) of approximately 30 K, which is characterized by a remarkable set of features, including a giant extrinsic anomalous Hall effect (AHE), Kondo screening, magnetic field-tunable thermal hysteresis, and nematic magneto-resistance. At lower temperatures, a coexistence of nematicity and Kondo screening with Ising superconductivity is observed, providing compelling evidence of hidden magnetism within a superconductor. This research not only sheds light on unexpected emergent physics resulting from the coupling of itinerant electrons and localized/correlated electrons in natural vdWHs but also emphasizes the potential for tailoring exotic quantum states through the manipulation of interlayer interactions.

cond-mat.str-el↗

arXiv2024

Three-dimensional quantum Griffiths singularity in bulk iron-pnictide superconductors

The quantum Griffiths singularity (QGS) is a phenomenon driven by quenched disorders that break conventional scaling invariance and result in a divergent dynamical critical exponent during quantum phase transitions (QPT). While this phenomenon has been well-documented in low-dimensional conventional superconductors and in three-dimensional (3D) magnetic metal systems, its presence in 3D superconducting systems and in unconventional high-temperature superconductors (high-Tc SCs) remains unclear. In this study, we report the observation of robust QGS in the superconductor-metal transition (SMT) of both quasi-2D and 3D anisotropic unconventional high-Tc superconductor CaFe1-xNixAsF (x < 5%) bulk single crystals, where the QGS states persist to up to 5.3 K. A comprehensive quantum phase diagram is established that delineates the 3D anisotropic QGS of SMT induced by perpendicular and parallel magnetic field. Our findings reveal the universality of QGS in 3D superconducting systems and unconventional high-Tc SCs, thereby substantially expanding the range of applicability of QGS.

cond-mat.str-el↗

arXiv2024

Three-dimensional hidden phase probed by in-plane magnetotransport in kagome metal CsV$_3$Sb$_5$ thin flakes

Transition metal compounds with kagome structure have been found to exhibit a variety of exotic structural, electronic, and magnetic orders. These orders are competing with energies very close to each other, resulting in complex phase transitions. Some of the phases are easily observable, such as the charge density wave (CDW) and the superconducting phase, while others are more challenging to identify and characterize. Here we present magneto-transport evidence of a new phase below ~35 K in the kagome topological metal CsV$_3$Sb$_5$ (CVS) thin flakes between the CDW and the superconducting transition temperatures. This phase is characterized by six-fold rotational symmetry in the in-plane magnetoresistance (MR) and is connected to the orbital current order in CVS. Furthermore, the phase is characterized by a large in-plane negative magnetoresistance, which suggests the existence of a three-dimensional, magnetic field-tunable orbital current ordered phase. Our results highlight the potential of magneto-transport to reveal the interactions between exotic quantum states of matter and to uncover the symmetry of such hidden phases.

cond-mat.str-el↗

arXiv2023

Perpendicular in-plane negative magnetoresistance in ZrTe5

The unique band structure in topological materials frequently results in unusual magneto-transport phenomena, one of which is in-plane longitudinal negative magnetoresistance (NMR) with the magnetic field aligned parallel to the electrical current direction. This NMR is widely considered as a hallmark of chiral anomaly in topological materials. Here we report the observation of in-plane NMR in the topological material ZrTe5 when the in-plane magnetic field is both parallel and perpendicular to the current direction, revealing an unusual case of quantum transport beyond the chiral anomaly. We find that a general theoretical model, which considers the combined effect of Berry curvature and orbital moment, can quantitatively explain this in-plane NMR. Our results provide new insights into the understanding of in-plane NMR in topological materials.

cond-mat.mes-hall↗

arXiv2022

Transport evidence of superlattice Dirac cones in graphene monolayer on twisted boron nitride substrate

Strong band engineering in two-dimensional (2D) materials can be achieved by introducing moiré superlattices, leading to the emergence of various novel quantum phases with promising potential for future applications. Presented works to create moiré patterns have been focused on a twist embedded inside channel materials or between channel and substrate. However, the effects of a twist inside the substrate materials on the unaligned channel materials are much less explored. In this work, we report the realization of superlattice multi-Dirac cones with the coexistence of the main Dirac cone in a monolayer graphene (MLG) on a ~0.14° twisted double-layer boron nitride (tBN) substrate. Transport measurements reveal the emergence of three pairs of superlattice Dirac points around the pristine Dirac cone, featuring multiple metallic or insulating states surrounding the charge neutrality point (CNP). Displacement field tunable and electron-hole asymmetric Fermi velocities are indicated from temperature dependent measurements, along with the gapless dispersion of superlattice Dirac cones. The experimental observation of multiple Dirac cones in MLG/tBN heterostructure is supported by band structure calculations employing periodic moiré potential. Our results unveil the potential of using twisted substrate as a universal band engineering technique for 2D materials regardless of lattice matching and crystal orientations, which might pave the way for a new branch of twistronics.

cond-mat.mes-hall↗

arXiv2022

Linear nonsaturating magnetoresistance in kagome superconductor CsV3Sb5 thin flakes

Linear nonsaturating magnetoresistance (LMR) represents a class of anomalous resistivity response to external magnetic field that has been observed in a variety of materials including but not limited to topological semi-metals, high-Tc superconductors and materials with charge/spin density wave (CDW/SDW) orders. Here we report the observation of LMR in layered kagome superconductor and CDW material CsV3Sb5 thin flakes, as well as the dimensional crossover and temperature (T) crossover of such LMR. Specifically, in ultrathin CsV3Sb5 crystals, the magnetoresistance (MR) exhibits a crossover from LMR at low T to quadratic B dependence above the CDW transition temperature; the MR also exhibits a crossover from LMR to sublinear MR for sample thickness at around ~20 nm at low T. We discuss several possible origins of the LMR and attribute the effect to two-dimensional (2D) CDW fluctuations. Our results may provide a new perspective for understanding the interactions between competing orders in kagome superconductors.

cond-mat.supr-con↗

arXiv2021

DyOCl: a rare-earth based two-dimensional van der Waals material with strong magnetic anisotropy

Comparing with the widely known transitional metal based van der Waals (vdW) materials, rare-earth based ones are rarely explored in the research of intrinsic two-dimensional (2D) magnetism. In this work, we report the physical properties of DyOCl, a rare-earth based vdW magnetic insulator with direct band gap of $\sim 5.72~eV$. The magnetic order of bulk DyOCl is determined by neutron scattering as the $A$-type antiferromagnetic structure below the Néel temperature $T_N=10~$K. The large magnetic moment near 10.1 $ μ_{B} $/Dy lies parallel to the $a$-axis with strong uniaxial magnetic anisotropy. At $2~K$, a moderate magnetic field ($\sim 2~T$) applied along the easy axis generates spin-flip transitions and polarizes DyOCl to a ferromagnetic state. Density functional theory calculations reveal an extremely large magnetic anisotropy energy ($-5850~μeV/Dy$) for DyOCl, indicating the great potentials to realize magnetism in 2D limit. Furthermore, the mechanical exfoliation of bulk DyOCl single crystals down to seven layers is demonstrated. Our findings suggest DyOCl is a promising material playground to investigate 2D $f$-electron magnetism and spintronic applications at the nanoscale.

cond-mat.mtrl-sci↗

arXiv2021

Enhancement of spin-orbit coupling and magnetic scattering in hydrogenated graphene

Spin-orbit coupling (SOC) can provide essential tools to manipulate electron spins in two-dimensional materials like graphene, which is of great interest for both fundamental physics and spintronics application. In this paper, we report the low-field magnetotransport of in situ hydrogenated graphene where hydrogen atoms are attached to the graphene surface in continuous low temperature and vacuum environment. Transition from weak localization to weak antilocalization with increasing hydrogen adatom density is observed, indicating enhancing Bychkov-Rashba-type SOC in a mirror symmetry broken system. From the low-temperature saturation of phase breaking scattering rate, the existence of spin-flip scattering is identified, which corroborates the existence of magnetic moments in hydrogenated graphene.

cond-mat.mes-hall↗

arXiv2021

Radiation-hardened and Repairable MoS$_2$ Field Effect Devices with Polymer Solid Electrolyte Gates

As human activities expand into naturally or man-made radiation-prone environment, the need for radiation-hardened (Rad-Hard) electronic hardware surged. The state-of-the-art silicon-based and two-dimensional (2D) materials based Rad-Hard transistors can withstand up to 1 Mrad (Si) of total ionization dose (TID), while higher TID tolerance is being heatedly sought after. Here we present few-layer MoS$_2$ Rad-Hard field-effect transistors (FETs) with polymer solid electrolyte (PSE) gate dielectrics. The MoS$_2$ PSE-FETs exhibit a TID tolerance of up to 3.75 Mrad (Si) at a dose rate of 523 rad (Si) s$^{-1}$ and can be repaired with a moderate thermal annealing at 100 $^{\circ}$C for 5 minutes. Combining the excellent intrinsic radiation tolerance and the reparability, the MoS$_2$ PSE-FETs reach a TID tolerance of up to 10 Mrad (Si). Complementary metal-oxide-semiconductor (CMOS)-like MoS$_2$ PSE-inverters have been built and show similar high radiation tolerance. Furthermore, the feasibility of wafer-scale Rad-Hard PSE-inverter array has been demonstrated using chemical vapor deposition (CVD) grown monolayer MoS$_2$. Our studies uncover the potential of 2D materials based PSE devices in future Rad-Hard integrated circuits (ICs).

cond-mat.mtrl-sci↗

arXiv2021

Crossover behavior in the magnetoresistance of thin flakes of the topological material ZrTe5

ZrTe5 is a layered material that exhibits intricate topological effects. Intensive theoretically and experimental efforts have been devoted to try to understand the physics in this materials. In this paper the temperature dependent magneto-transport properties of ZrTe5 thin flakes are investigated. A characteristic temperature T* is observed in the temperature dependence of three different types of magnetoresistance simultaneously, which are the saturated Hall anomaly, the chiral anomaly and the longitudinal magnetoresistance. Furthermore, the value of T* decreases monotonically from 200K to 160K with increasing thickness of the ZrTe5 thin flakes from 42nm to 89nm. Temperature induced topological phase transitions are attributed to the cause of such anomaly in the three types of magnetoresistance at T*. Our findings provide a multi-parameter indicator for the emergence of topological phase transition in ZrTe5 and could be extended to the study of other topological materials. The temperature dependence of the three types of magnetoresistance also shed light on the role of anomalous Hall Effect in the transport properties of ZrTe5.

cond-mat.mtrl-sci↗

arXiv2021

Electrically Switchable van der Waals Magnon Valves

Van der Waals magnets have emerged as a fertile ground for the exploration of highly tunable spin physics and spin-related technology. Two-dimensional (2D) magnons in van der Waals magnets are collective excitation of spins under strong confinement. Although considerable progress has been made in understanding 2D magnons, a crucial magnon device called the van der Waals magnon valve, in which the magnon signal can be completely and repeatedly turned on and off electrically, has yet to be realized. Here we demonstrate such magnon valves based on van der Waals antiferromagnetic insulator MnPS3. By applying DC electric current through the gate electrode, we show that the second harmonic thermal magnon (SHM) signal can be tuned from positive to negative. The guaranteed zero crossing during this tuning demonstrates a complete blocking of SHM transmission, arising from the nonlinear gate dependence of the non-equilibrium magnon density in the 2D spin channel. Using the switchable magnon valves we demonstrate a magnon-based inverter. These results illustrate the potential of van der Waals anti-ferromagnets for studying highly tunable spin-wave physics and for application in magnon-base circuitry in future information technology.

cond-mat.mtrl-sci↗

arXiv2021

Ionic liquid gating induced two superconductor-insulator phase transitions in spinel oxide Li$_{1 \pm x}$Ti$_2$O$_{4-δ}$

The associations between emergent physical phenomena (e.g., superconductivity) and orbital, charge, and spin degrees of freedom of $3d$ electrons are intriguing in transition metal compounds. Here, we successfully manipulate the superconductivity of spinel oxide Li$_{1\pm x}$Ti$_2$O$_{4-δ}$ (LTO) by ionic liquid gating. A dome-shaped superconducting phase diagram is established, where two insulating phases are disclosed both in heavily electron-doping and hole-doping regions. The superconductor-insulator transition (SIT) in the hole-doping region can be attributed to the loss of Ti valence electrons. In the electron-doping region, LTO exhibits an unexpected SIT instead of a metallic behavior despite an increase in carrier density. Furthermore, a thermal hysteresis is observed in the normal state resistance curve, suggesting a first-order phase transition. We speculate that the SIT and the thermal hysteresis stem from the enhanced $3d$ electron correlations and the formation of orbital ordering by comparing the transport and structural results of LTO with the other spinel oxide superconductor MgTi$_2$O$_4$, as well as analysing the electronic structure by first-principles calculations. Further comprehension of the detailed interplay between superconductivity and orbital ordering would contribute to the revealing of unconventional superconducting pairing mechanism.

cond-mat.supr-con↗

arXiv2021

Electron-electron interactions and weak anti-localization in few-layer ZrTe5 devices

Much effort has been devoted to the electronic properties of relatively thick ZrTe5 crystals, focusing on their three-dimensional topological effects. Thin ZrTe5 crystals, on the other hand, were much less explored experimentally. Here we present detailed magnetotransport studies of few-layer ZrTe5 devices, in which electron-electron interactions and weak anti-localization are observed. The coexistence of the two effects manifests themselves in corroborating evidence presented in the temperature and magnetic field dependence of the resistance. Notably, the temperature-dependent phase coherence length extracted from weak anti-localization agrees with strong electron-electron scattering in the sample. Meanwhile, universal conductance fluctuations have temperature and gate voltage dependence that is similar to that of the phase coherence length. Lastly, all the transport properties in thin ZrTe5 crystals show strong two-dimensional characteristics. Our results provide new insight into the highly intricate properties of topological material ZrTe5.

cond-mat.mtrl-sci↗

arXiv2020

Evidence of tunable magnetic coupling in hydrogenated graphene

A lot of efforts have been devoted to understanding the origin and effects of magnetic moments induced in graphene with carbon atom vacancy, or light adatoms like hydrogen or fluorine. At the meantime, the large negative magnetoresistance (MR) widely observed in these systems is not well understood, nor had it been associated with the presence of magnetic moments. In this paper, we study the systematic evolution of the large negative MR of in-situ hydrogenated graphene in ultra-high vacuum (UHV) environment. We find for most combination of electron density ($n_e$) and hydrogen density ($n_H$), MR at different temperature can be scaled to $α=(μ_BB)/[k_B(T-T^*)]$, where $T^*$ is the Curie-Weiss temperature. The sign of $T^*$ indicates the existence of tunable ferromagnetic-like ($T^* >0$) and anti-ferromagnetic-like ($T^* <0$) coupling in hydrogenated graphene. However, the lack of hysteresis of MR or anomalous Hall effect below $|T^*|$ points to the fact that long-range magnetic order did not emerge, which we attribute to the competition of different magnetic orders and disordered arrangement of magnetic moments on graphene. We also find that localized impurity states introduced by H adatoms could modify the capacitance of hydrogenated graphene. This work provides a new way to extract information from large negative MR behavior and can be a key to help understanding interactions of magnetic moments in graphene.

cond-mat.mes-hall↗

arXiv2019

Robust edge photocurrent response on layered Type II Weyl semimetal WTe2

Photo sensing and energy harvesting based on exotic properties of quantum materials and new operation principles have great potentials to break the fundamental performance limit of conventional photodetectors and solar cells. As topological nontrivial materials, Weyl semimetals have demonstrated novel optoelectronic properties that promise potential applications in photo detection and energy harvesting arising from their gapless linear dispersion near Weyl nodes and Berry field enhanced nonlinear optical effect at the vicinity of Weyl nodes. In this work, we demonstrate robust photocurrent generation from charge separation of photoexctied electron-hole pairs at the edge of Td-WTe2, a type-II Weyl semimetal, due to crystalline-symmetry breaking along certain crystal fracture directions and possibly enhanced by robust fermi-arc type surface states. Using scanning photocurrent microscopy (SPCM) measurements, we further demonstrate that the edge current response is robust over a wide excitation photon energy. We find that this robust feature is highly generic, and shall arise universally in a wide class of quantum materials with similar crystal symmetries. In addition, possible connections between these edge photocurrents and topological properties of Weyl semimetals are explored. The robust and generic edge current response demonstrated in this work provides a new type of charge separation mechanism for photosensing and energy harvesting over broad wavelength range.

cond-mat.mes-hall↗