arXiv subjects

JunYan Luo

Publications and source records attributed to JunYan Luo.

At least 19 recordsLinked to original sources

arXiv2026

Beyond Photon Shot Noise: Chemical Limits in Spectrophotometric Precision

In this work, we investigate precision limitations in spectrophotometry (i.e., spectroscopic concentration measurements) imposed by chemical processes of molecules. Using the recently developed Photon-resolved Floquet theory, which generalizes Maxwell-Bloch theory for higher-order measurement statistics, we analyze a molecular model system subject to chemical reactions whose electronic and optical properties depend on the chemical state. Analysis of sensitivity bounds reveals: (i) Phase measurements are more sensitive than intensity measurements; (ii) Sensitivity exhibits three regimes: photon-shot-noise limited, chemically limited, and intermediate; (iii) Sensitivity shows a turnover as a function of reaction rate due to the interplay between coherent electronic dynamics and incoherent chemical dynamics. Our findings demonstrate that chemical properties must be considered to estimate ultimate precision limits in optical spectrophotometry.

quant-ph↗

arXiv2026

Heisenberg scaling in optical magnetometry with measurement-induced correlations as a quantum resource

Theoretical proposals to reach the Heisenberg scaling of the measurement precision typically require carefully engineered interactions or initial entanglement. In studying optical magnetometry, we show that the continuous collective measurement process itself can generate the necessary many-body quantum correlations to achieve the elusive Heisenberg scaling of the quantum Fisher information in a dissipative, steady-state system without direct inter-atomic interactions. By contrasting a correlation-neglecting but otherwise consistent semiclassical model, which can violate the quantum Cram\'er-Rao bound (QCRB) by several orders of magnitude, with a collective quantum model, we isolate measurement-induced correlations as the essential mechanism. The violation of the QCRB serves thereby as a fundamental sanity check for semiclassical spectroscopic theories. This work reveals measurement-induced correlations as a widely unexplored quantum resource for quantum-enhanced sensing, establishes a new paradigm for achieving Heisenberg scaling in open quantum systems, and provides a direct path to test the foundations of quantum mechanics using macroscopic atom ensembles.

quant-ph↗

arXiv2025

Full-counting statistics and quantum information of dispersive readout with a squeezed environment

Motivated by the importance of dispersive readout in quantum technology, we study a prototypical dispersive readout setup that is probed by a squeezed vacuum in a time-reversal-symmetric fashion. To this end, we develop a full-counting-statistics framework for dispersive readout and analyze its measurement information, accompanied by a generalized mean-field approach suitable to deal with non-unitary dynamics. Distinct from conventional input-output theory, our full-counting-statistics approach enables the direct calculation of arbitrary-order cumulants for the measured cumulative (i.e., time-integrated) photonic distribution while maintaining applicability to nonlinear systems. The corresponding Fisher information exhibits an exponential dependence on the squeezing parameter and a robustness against residual nonlinearity, which can even approach the quantum Fisher information, setting an upper limit. This work introduces a conceptually streamlined and computationally efficient framework for continuous quantum measurements, making it well suited for widespread adoption in quantum technologies.

quant-ph↗

arXiv2025

Anomalous current-electric field characteristics in transport through a nanoelectromechanical systems

A deep understanding of the correlation between electronic and mechanical degrees of freedom is crucial to the development of quantum devices in a nanoelectromechanical system (NEMS). In this work, we first establish a fully quantum mechanical approach for transport through a NEMS device, which is valid for arbitrary bias voltages, temperatures, and electro-mechanical couplings. We find an anomalous current-electric field characteristics at a low bias, where the current decreases with a rising electric field, associated with the backward tunneling of electrons for a weak mechanical damping. We reveal that this intriguing behavior arises from a combined effect of mechanical motion and Coulomb blockade, where the rapid increase of backward tunneling events at a large oscillation amplitude suppresses the forward current due to prohibition of double occupation. In the opposite limit of strong damping, the oscillator dissipates its energy to the environment and relaxes to the ground state rapidly. Electrons then transport via the lowest vibrational state such that the net current and its corresponding noise have a vanishing dependence on the electric field.

cond-mat.mes-hall↗

arXiv2024

Photon-resolved Floquet theory I: Full-Counting statistics of the driving field in Floquet systems

Floquet theory and other established semiclassical approaches are widely used methods to predict the state of externally-driven quantum systems, yet, they do not allow to predict the state of the photonic driving field. To overcome this shortcoming, the photon-resolved Floquet theory (PRFT) has been developed recently [Phys. Rev. Research 6, 013116], which deploys concepts from full-counting statistics to predict the statistics of the photon flux between several coherent driving modes. In this paper, we study in detail the scaling properties of the PRFT in the semiclassical regime. We find that there is an ambiguity in the definition of the moment-generating function, such that different versions of the moment-generating function produce the same photonic probability distribution in the semiclassical limit, and generate the same leading-order terms of the moments and cumulants. Using this ambiguity, we establish a simple expression for the Kraus operators, which describe the decoherence dynamics of the driven quantum system appearing as a consequence of the light-matter interaction. The PRFT will pave the way for improved quantum sensing methods, e.g., for spectroscopic quantum sensing protocols, reflectometry in semiconductor nanostructures and other applications, where the detailed knowledge of the photonic probability distribution is necessary.

quant-ph↗

arXiv2024

Variational approach to light-matter interaction: Bridging quantum and semiclassical limits

We present a time-dependent variational approach with the multiple Davydov $D_2$ trial state to simulate the dynamics of light-matter systems when the field is in a coherent state with an arbitrary finite mean photon number. The variational approach captures not only the system dynamics but also the field dynamics and is applicable to a variety of quantum models of light-matter interaction such as the Jaynes-Cummings model, Rabi model, and Dicke model, and is feasible to tackle the multimode quantized fields. By comparison of the variational and semiclassical dynamics of both the system and field, we illustrate that the variational dynamics from the quantum models agrees with those from the corresponding semiclassical models as long as the mean number of photons is sufficiently large. Moreover, we illustrate that in the crossover between the quantum and semiclassical limits, the quantum corrections lead to the collapse of the oscillations in dynamics, which is absent in the semiclassical models. The variational approach provides a unified treatment of light-matter interaction from the quantum to the semiclassical limit.

quant-ph↗

arXiv2024

Spin-resolved counting statistics as a sensitive probe of spin correlation in transport through a quantum dot spin valve

We investigate the noise in spin transport through a single quantum dot (QD) tunnel coupled to ferromagnetic electrodes with noncollinear magnetizations. Based on a spin-resolved quantum master equation, auto- and cross-correlations of spin-resolved currents are analyzed to reveal the underlying spin transport dynamics and characteristics for various polarizations. We find the currents of majority and minority spins could be strongly autocorrelated despite uncorrelated charge transfer. The interplay between tunnel coupling and the Coulomb interaction gives rise to an exchange magnetic field, leading to the precession of the accumulated spin in the QD. It strongly suppresses the bunching of spin tunneling events and results in a unique double-peak structure in the noise of the net spin current. The spin autocorrelation is found to be susceptible to magnetization alignments, which may serve as a sensitive tool to measure the magnetization directions between the ferromagnetic electrodes.

cond-mat.mes-hall↗

arXiv2023

Photon-resolved Floquet theory II: Open quantum systems

Photon-resolved Floquet theory keeps track of the photon exchange of a quantum system with a coherent driving field. It thus complements the standard full-counting statistics that counts the number of photons exchanged with incoherent photon modes giving rise to dissipation. In this paper, we introduce a unifying framework describing both situations. We develop methods suitable for an analytical evaluation of low-order cumulants of photonic probability distributions. Within this framework we analyze the two-mode Jaynes-Cummings model to demonstrate that the Photon-resolved Floquet theory and the standard full-counting statistics make consistent statistical predictions. Interestingly, we find that the photon-flux fluctuations diverge for vanishing dissipation, which can be related to an entanglement effect between the driven matter system and the driving field. To substantiate our results, we use our framework to describe efficient photon up-conversion in an ac-driven lambda system, that is characterized by a high signal-to-noise ratio. As the framework is non-perturbative and predicts fluctuations, it paves the way towards non-perturbative spectroscopy, which will assist to improve metrological methods.

quant-ph↗

arXiv2023

Distance-dependent emission spectrum from two qubits in a strong-coupling regime

We study the emission spectrum of two distant qubits strongly coupled to a waveguide by using the numerical and analytical approaches, which are beyond the Markovian approximation and the rotating-wave approximation (RWA). The numerical approach combines the Dirac-Frenkel time-dependent variational principle with the multiple Davydov $D_{1}$ ansatz. A transformed RWA (TRWA) treatment and a standard perturbation (SP) are used to analytically calculate the emission spectrum. It is found that the variational approach and the TRWA treatment yield accurate emission spectra of the two distant qubits in certain strong coupling regimes while the SP breaks down. The emission spectrum is found to be asymmetric irrespective of the two-qubit distance and exhibits a single peak, doublet, and multipeaks depending on the two-qubit distance as well as the initial states. In sharply contrast with the single-qubit case, the excited-state populations of the two qubits can ultraslowly decay due to the subradiance even in the presence of a strong qubit-waveguide coupling, which in turn yields ultranarrow emission line. Our results provide insights into the emission spectral features of the two distant qubits in the strong light-matter coupling regime.

quant-ph↗

arXiv2023

Lamb Shift and the Vacuum Rabi Splitting in a Strongly Dissipative Environment

We study the vacuum Rabi splitting of a qubit ultrastrongly coupled to a high-$Q$ cavity mode and a radiation reservoir. Three methods are employed: a numerically exact variational approach with a multiple Davydov ansatz, the rotating-wave approximation (RWA), and the transformed RWA. Agreement between the variational results and the transformed RWA results is found in the regime of validity of the latter, where the RWA breaks down completely. We illustrate that the Lamb shift plays an essential role in modifying the vacuum Rabi splitting in the ultrastrong coupling regime, leading to off-resonant qubit-cavity coupling even though the cavity frequency equals to the bare transition frequency of the qubit. Specifically, the emission spectrum exhibits one broad low-frequency peak and one narrow high-frequency peak in the presence of relatively weak cavity-qubit coupling. As the cavity-qubit coupling increases, the low-frequency peak narrows while the high-frequency peak broadens until they have similar widths.

quant-ph↗

arXiv2020

Variational approach to time-dependent fluorescence of a driven qubit

We employ the Dirac-Frenkel variational principle and multiple Davydov ansatz to study time-dependent fluorescence spectra of a driven qubit in the weak- to strong qubit-reservoir coupling regimes, where both the Rabi frequency and spontaneous decay rate are comparable to the transition frequency of the qubit. Our method agrees well with the time-local master-equation approach in the weak-coupling regime, and offers a flexible way to compute the spectra from the bosonic dynamics instead of two-time correlation functions. While the perturbative master equation breaks down in the strong-coupling regime, our method actually becomes more accurate due to the use of bosonic coherent states under certain conditions. We show that the counter-rotating coupling between the qubit and the reservoir has considerable contributions to the photon number dynamics and the spectra under strong driving conditions even though the coupling is moderately weak. The time-dependent spectra are found to be generally asymmetric, a feature that is derived from photon number dynamics. In addition, it is shown that the spectral profiles can be dramatically different from the Mollow triplet due to strong dissipation and/or multiphoton processes associated with the strong driving. Our formalism provides a unique perspective to interpret time-dependent spectra.

quant-ph↗

arXiv2020

Role of generalized parity in the symmetry of fluorescence spectrum from two-level systems under periodic frequency modulation

We study the origin of the symmetry of the fluorescence spectrum from the two-level system subjected to a low-frequency periodic modulation and a near-resonant high-frequency monochromatic excitation by using the analytical and numerical methods based on the Floquet theory. We find that the fundamental origin of symmetry of the spectrum can be attributed to the presence of the generalized parity of the Floquet states, which depends on the driving parameters. The absence of the generalized parity can lead to the asymmetry of the spectrum. Based on the generalized parity, the conditions for the symmetry and asymmetry of the spectrum can be derived, which succeeds in predicting symmetry and asymmetry of the spectrum for the harmonic, biharmonic, and multiharmonic modulations. Moreover, we find that the secular approximation widely used in the analytical calculation may lead to artifact symmetry of the spectrum that vanishes when such approximation is avoided. The present study provides a significant perspective on the origin of the symmetry of the spectrum.

quant-ph↗

arXiv2019

Stochastic thermodynamics of an electron-spin-resonance quantum dot system

We present a stochastic thermodynamics analysis of an electron-spin-resonance pumped quantum dot device in the Coulomb-blocked regime, where a pure spin current is generated without an accompanying net charge current. Based on a generalized quantum master equation beyond secular approximation, quantum coherences are accounted for in terms of an effective average spin in the Floquet basis. Elegantly, this effective spin undergoes a precession about an effective magnetic field, which originates from the non-secular treatment and energy renormalization. It is shown that the interaction between effective spin and effective magnetic field may have the dominant roles to play in both energy transport and irreversible entropy production. In the stationary limit, the energy and entropy balance relations are also established based on the theory of counting statistics.

cond-mat.stat-mech↗

arXiv2015

Unraveling of a generalized quantum Markovian master equation and its application in feedback control of a charge qubit

In the context of a charge qubit under continuous monitoring by a single electron transistor, we propose an unraveling of the generalized quantum Markovian master equation into an ensemble of individual quantum trajectories for stochastic point process. A suboptimal feedback algorism is implemented into individual quantum trajectories to protect a desired pure state. Coherent oscillations of the charge qubit could be maintained in principle for an arbitrarily long time in case of sufficient feedback strength. The effectiveness of the feedback control is also reflected in the detector's noise spectrum. The signal-to-noise ratio rises significantly with increasing feedback strength such that it could even exceed the Korotkov-Averin bound in quantum measurement, manifesting almost ideal quantum coherent oscillations of the qubit. The proposed unraveling and feedback protocol may open up the prospect to sustain ideal coherent oscillations of a charge qubit in quantum computation algorithms.

cond-mat.mes-hall↗

arXiv2015

Qubit detection with a T-shaped double quantum dot detector

We propose to continuously monitor a charge qubit by utilizing a T-shaped double quantum dot detector, in which the qubit and double dot are arranged in such a unique way that the detector turns out to be particularly susceptible to the charge states of the qubit. Special attention is paid to the regime where acquisition of qubit information and backaction upon the measured system exhibit nontrivial correlation. The intrinsic dynamics of the qubit gives rise to dynamical blockade of tunneling events through the detector, resulting in a super-Poissonian noise. However, such a pronounced enhancement of detector's shot noise does not necessarily produce a rising dephasing rate. In contrast, an inhibition of dephasing is entailed by the reduction of information acquisition in the dynamically blockaded regimes. We further reveal the important impact of the charge fluctuations on the measurement characteristics. Noticeably, under the condition of symmetric junction capacitances the noise pedestal of circuit current is completely suppressed, leading to a divergent signal-to-noise ratio, and eventually to a violation of the Korotkov-Averin bound in quantum measurement. Our study offers the possibility for a double dot detector to reach the quantum limited effectiveness in a transparent manner.

cond-mat.mes-hall↗

arXiv2014

Conditional spin counting statistics as a probe of Coulomb interaction and spin-resolved bunching

Full counting statistics is a powerful tool to characterize the noise and correlations in transport through mesoscopic systems. In this work, we propose the theory of conditional spin counting statistics, i.e., the statistical fluctuations of spin-up (down) current given the observation of the spin-down (up) current. In the context of transport through a single quantum dot, it is demonstrated that a strong Coulomb interaction leads to a conditional spin counting statistics that exhibits a substantial change in comparison to that without Coulomb repulsion. It thus can be served as an effective way to probe the Coulomb interactions in mesoscopic transport systems. In case of spin polarized transport, it is further shown that the conditional spin counting statistics offers a transparent tool to reveal the spin-resolved bunching behavior.

cond-mat.mes-hall↗

arXiv2013

Non-Markovian dynamics and noise characteristics in continuous measurement of a solid-state charge qubit

We investigate the non-Markovian characteristics in continuous measurement of a charge qubit by a quantum point contact. The backflow of information from the reservoir to the system in the non-Markovian domain gives rise to strikingly different qubit relaxation and dephasing in comparison with the Markovian case. The intriguing non-Markovian dynamics is found to have a direct impact on the output noise feature of the detector. Unambiguously, we observe that the non-Markovian memory effect results in an enhancement of the signal-to-noise ratio, which can even exceed the upper limit of ``4'', leading thus to the violation of the Korotkov-Averin bound in quantum measurement. Our study thus may open new possibilities to improve detector's measurement efficiency in a direct and transparent way.

cond-mat.mes-hall↗

arXiv2013

Spin-resolved bunching and noise characteristics in double quantum dots coupled to ferromagnetic electrodes

We study spin-resolved noise in Coulomb blockaded double quantum dots coupled to ferromagnetic electrodes. The modulation of the interdot coupling and spin polarization in the electrodes gives rise to an intriguing dynamical spin $\uparrow$-$\uparrow$ ($\downarrow$-$\downarrow$) blockade mechanism: Bunching of up (down) spins due to dynamical blockade of an up (down) spin. In contrast to the conventional dynamical spin $\uparrow$-$\downarrow$ bunching (bunching of up spins entailed by dynamical blockade of a down spin), this new bunching behavior is found to be intimately associated with the spin mutual-correlation, i.e., the noise fluctuation between opposite spin currents. We further demonstrate that the dynamical spin $\uparrow$-$\uparrow$ and $\uparrow$-$\downarrow$ bunching of tunneling events may be coexistent in the regime of weak interdot coupling and low spin polarization.

cond-mat.mes-hall↗