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L. Dumoulin

Publications and source records attributed to L. Dumoulin.

At least 19 recordsLinked to original sources

The CROSS experiment: detector construction, background projection, and sensitivity to $^{100}$Mo $0\nu2\beta$ decay

The CROSS experiment to search for neutrinoless double-beta ($0\nu2\beta$) decay in $^{100}$Mo with the help of an array of scintillating cryogenic calorimeters, containing 4.9 kg of $^{100}$Mo, has been ongoing in a low-background setup at the Canfranc underground laboratory (Spain) since mid-November 2025. In this paper, we present the construction of the CROSS detector and the description of Geant4-based Monte Carlo simulations of expected background in the region of interest. The simulations predict the background index in a 100-keV-wide interval centered at the $Q$-value of $^{100}$Mo (3034 keV) on the level of 3.2(5) $\times$ 10$^{-3}$ cnts/keV/kg/yr. Taking into account an 18% deadtime induced by the muon veto cut and a typical 90% duty cycle of the facility, such background level would allow to reach the world-leading sensitivity to $^{100}$Mo $0\nu2\beta$ decay (lim $T_{1/2} \sim 4 \times 10^{24}$ yr) in 1 year of data taking. Considering conservatively a factor 3 (10) worse background index due to unpredictable radioactive contamination of construction materials and/or detector performance, a 2-yr-long operation of the CROSS array would be still compatible with the best (competitive) sensitivity to $0\nu2\beta$ decay in $^{100}$Mo.

physics.ins-det

Muon veto system for the CROSS double-beta decay search experiment

In preparation to the CROSS experiment at the Canfranc underground laboratory (Spain) $-$ aiming to search for neutrinoless double-beta ($0\nu\beta\beta$) decay of $^{100}$Mo using low-temperature detectors with heat-scintillation readout $-$ we report on development of a dedicated muon veto system. The need for the muon veto in CROSS is caused by a comparatively high residual cosmic muon flux at the experimental site ($\sim$20 $\mu$/m$^2$/h), being a dominant background in the region of interest (ROI) at $\sim$3 MeV. Thus, we installed the muon veto system around the CROSS low-background setup, forming four lateral, one top, and four bottom sectors. In this paper we describe the design, construction and operation of the CROSS muon veto system, as well as its optimization and validation by comparing dedicated Monte Carlo (MC) simulations of muons with low-temperature measurements in the setup. We demonstrate a stable operation of the veto system with the average trigger rates compatible with MC simulations. Also, we investigated two muon trigger logics based on coincidences with either 2 sectors or a single sector of the veto. The MC study shows that, in combination with the multiplicity cut of thermal detectors, these trigger logics allow to reject 99.2\% and 99.7\% of muon-induced events in the ROI, respectively. Despite a comparatively high dead time ($\sim$18\%) introduced by coincidences with any of nine sectors of the veto $-$ the adopted strategy $-$ the muon-induced background in the ROI of the CROSS experiment can be reduced down to $\sim$2 $\times 10^{-3}$ cnts/keV/kg/yr, i.e., an acceptable level compatible with a high-sensitivity $0\nu\beta\beta$ decay search foreseen in CROSS.

physics.ins-det

Cryogenic light detectors with thermal signal amplification for $0\nu\beta\beta$ search experiments

As a step towards the realization of cryogenic-detector experiments to search for neutrinoless double-beta decay (such as CROSS, BINGO, and CUPID), we investigated a batch of 10 Ge light detectors (LDs) assisted by Neganov-Trofimov-Luke (NTL) signal amplification. Each LD was assembled with a large cubic light-emitting crystal (45 mm side) using the recently developed CROSS mechanical structure. The detector array was operated at milli-Kelvin temperatures in a pulse-tube cryostat at the Canfranc underground laboratory in Spain. We achieved good performance with scintillating bolometers from CROSS, made of Li$_{2}$$^{100}$MoO$_4$ crystals and used as reference detectors of the setup, and with all LDs tested (except for a single device that encountered an electronics issue). No leakage current was observed for 8 LDs with an electrode bias up to 100 V. Operating the LDs at an 80 V electrode bias applied in parallel, we obtained a gain of around 9 in the signal-to-noise ratio of these devices, allowing us to achieve a baseline noise RMS of $O$(10 eV). Thanks to the strong current polarization of the temperature sensors, the time response of the devices was reduced to around half a millisecond in rise time. The achieved performance of the LDs was extrapolated via simulations of pile-up rejection capability for several configurations of the CUPID detector structure. Despite the sub-optimal noise conditions of the LDs (particularly at high frequencies), we demonstrated that the NTL technology provides a viable solution for background reduction in CUPID.

physics.ins-det

Sensitivity of the CUPID experiment to $0\nu\beta\beta$ decay of $^{100}$Mo

CUPID is a next-generation bolometric experiment to search for neutrinoless double-beta decay ($0\nu\beta\beta$) of $^{100}$Mo using Li$_2$MoO$_4$ scintillating crystals. It will operate 1596 crystals at $\sim$10 mK in the CUORE cryostat at the Laboratori Nazionali del Gran Sasso in Italy. Each crystal will be facing two Ge-based bolometric light detectors for $\alpha$ rejection. We compute the discovery and the exclusion sensitivity of CUPID to $0\nu\beta\beta$ in a Frequentist and a Bayesian framework. This computation is done numerically based on pseudo-experiments. For the CUPID baseline scenario, with a background and an energy resolution of $1.0 \times 10^{-4}$ counts/keV/kg/yr and 5 keV FWHM at the Q-value, respectively, this results in a Bayesian exclusion sensitivity (90% c.i.) of $\hat{T}_{1/2} > 1.6 \times 10^{27} \ \mathrm{yr}$, corresponding to the effective Majorana neutrino mass of $\hat{m}_{\beta\beta} < \ 9.6$ -- $28 \ \mathrm{meV}$. The Frequentist discovery sensitivity (3$\sigma$) is $\hat{T}_{1/2}= 1.0 \times 10^{27} \ \mathrm{yr}$, corresponding to $\hat{m}_{\beta\beta}= \ 12$ -- $36 \ \mathrm{meV}$.

nucl-ex

Innovating Bolometers' Mounting: A Gravity-Based Approach

Cryogenic calorimeters, also known as bolometers, are among the leading technologies for searching for rare events. The CUPID experiment is exploiting this technology to deploy a tonne-scale detector to search for neutrinoless double-beta decay of $^{100}$Mo. The CUPID collaboration proposed an innovative approach to assembling bolometers in a stacked configuration, held in position solely by gravity. This gravity-based assembly method is unprecedented in the field of bolometers and offers several advantages, including relaxed mechanical tolerances and simplified construction. To assess and optimize its performance, we constructed a medium-scale prototype hosting 28 Li$_2$MoO$_4$ crystals and 30 Ge light detectors, both operated as cryogenic calorimeters at the Laboratori Nazionali del Gran Sasso (Italy). Despite an unexpected excess of noise in the light detectors, the results of this test proved (i) a thermal stability better than $\pm$0.5 mK at 10 mK, (ii) a good energy resolution of Li$_2$MoO$_4$ bolometers, (6.6 $\pm$ 2.2) keV FWHM at 2615 keV, and (iii) a Li$_2$MoO$_4$ light yield measured by the closest light detector of 0.36 keV/MeV, sufficient to guarantee the particle identification requested by CUPID.

physics.ins-det

CUPID, the CUORE Upgrade with Particle IDentification

CUPID, the CUORE Upgrade with Particle IDentification, is a next-generation experiment to search for neutrinoless double beta decay ($0\nu\beta\beta$) and other rare events using enriched Li$_2$$^{100}$MoO$_4$ scintillating bolometers. It will be hosted by the CUORE cryostat located at the Laboratori Nazionali del Gran Sasso in Italy. The main physics goal of CUPID is to search for $0\nu\beta\beta$\ of $^{100}$Mo with a discovery sensitivity covering the full neutrino mass regime in the inverted ordering scenario, as well as the portion of the normal ordering regime with lightest neutrino mass larger than 10 meV. With a conservative background index of 10$^{-4}$ cnts/(keV$\cdot$kg$\cdot$yr), 240 kg isotope mass, 5 keV FWHM energy resolution at 3 MeV and 10 live-years of data taking, CUPID will have a 90\% C.L. half-life exclusion sensitivity of 1.8 $\cdot$ 10$^{27}$ yr, corresponding to an effective Majorana neutrino mass ($m_{\beta\beta}$) sensitivity of 9--15 meV, and a $3\sigma$ discovery sensitivity of 1 $\cdot$ 10$^{27}$ yr, corresponding to an $m_{\beta\beta}$ range of 12--21 meV.

physics.ins-det

Precise $^{113}$Cd $\beta$ decay spectral shape measurement and interpretation in terms of possible $g_A$ quenching

Highly forbidden $\beta$ decays provide a sensitive test to nuclear models in a regime in which the decay goes through high spin-multipole states, similar to the neutrinoless double-$\beta$ decay process. There are only 3 nuclei ($^{50}$V, $^{113}$Cd, $^{115}$In) which undergo a $4^{\rm th}$ forbidden non-unique $\beta$ decay. In this work, we compare the experimental $^{113}$Cd spectrum to theoretical spectral shapes in the framework of the spectrum-shape method. We measured with high precision, with the lowest energy threshold and the best energy resolution ever, the $\beta$ spectrum of $^{113}$Cd embedded in a 0.43 kg CdWO$_4$ crystal, operated over 26 days as a bolometer at low temperature in the Canfranc underground laboratory (Spain). We performed a Bayesian fit of the experimental data to three nuclear models (IBFM-2, MQPM and NSM) allowing the reconstruction of the spectral shape as well as the half-life. The fit has two free parameters, one of which is the effective weak axial-vector coupling constant, $g_A^{\text{eff}}$, which resulted in $g_A^{\text{eff}}$ between 1.0 and 1.2, compatible with a possible quenching. Based on the fit, we measured the half-life of the $^{113}$Cd $\beta$ decay including systematic uncertainties as $7.73^{+0.60}_{-0.57} \times 10^{15}$ yr, in agreement with the previous experiments. These results represent a significant step towards a better understanding of low-energy nuclear processes.

nucl-ex

Searching for Beyond the Standard Model physics using the improved description of $^{100}$Mo $2νββ$ decay spectral shape with CUPID-Mo

The current experiments searching for neutrinoless double-$β$ ($0νββ$) decay also collect large statistics of Standard Model allowed two-neutrino double-$β$ ($2νββ$) decay events. These can be used to search for Beyond Standard Model (BSM) physics via $2νββ$ decay spectral distortions. $^{100}$Mo has a natural advantage due to its relatively short half-life, allowing higher $2νββ$ decay statistics at equal exposures compared to the other isotopes. We demonstrate the potential of the dual read-out bolometric technique exploiting a $^{100}$Mo exposure of 1.47 kg $\times$ y, acquired in the CUPID-Mo experiment at the Modane underground laboratory (France). We set limits on $0νββ$ decays with the emission of one or more Majorons, on $2νββ$ decay with Lorentz violation, and $2νββ$ decay with a sterile neutrino emission. In this analysis, we investigate the systematic uncertainty induced by modeling the $2νββ$ decay spectral shape parameterized through an improved model, an effect never considered before. This work motivates searches for BSM processes in the upcoming CUPID experiment, which will collect the largest amount of $2νββ$ decay events among the next-generation experiments.

nucl-ex

Development of large-volume $^{130}$TeO$_2$ bolometers for the CROSS $2\beta$ decay search experiment

We report on the development of thermal detectors based on large-size tellurium dioxide crystals (45x45x45 mm), containing tellurium enriched in $^{130}$Te to about 91%, for the CROSS double-beta decay experiment. A powder used for the crystals growth was additionally purified by the directional solidification method, resulting in the reduction of the concentration of impurities by a factor 10, to a few ppm of the total concentration of residual elements (the main impurity is Fe). The purest part of the ingot (the first ~200 mm, about 80% of the total length of the cylindrical part of the ingot) was determined by scanning segregation profiles of impurities and used for the $^{130}$TeO$_2$ powder production with no evidence of re-contamination. The crystal growth was verified with precursors produced from powder with natural Te isotopic composition, and two small-size (20x20x10 mm) samples were tested at a sea-level laboratory showing high bolometric and spectrometric performance together with acceptable $^{210}$Po content (below 10 mBq/kg). This growth method was then applied for the production of six large cubic $^{130}$TeO$_2$ crystals and 4 of them were taken randomly to be characterized at the Canfranc underground laboratory, in the CROSS-dedicated low-background cryogenic facility. Two $^{130}$TeO$_2$ samples were coated with a thin, $O$(100 nm), metal film in form of Al layer (on 4 sides) or AlPd grid (on a single side) to investigate the possibility to tag surface events by pulse-shape discrimination. Similarly to the small natural precursors, large-volume $^{130}$TeO$_2$ bolometers show high performance and even better internal purity ($^{210}$Po activity $\sim$ 1 mBq/kg, while activities of $^{228}$Th and $^{226}$Ra are below 0.01 mBq/kg), satisfying requirements for the CROSS and, potentially, next-generation experiments.

physics.ins-det

A novel mechanical design of a bolometric array for the CROSS double-beta decay experiment

The CROSS experiment will search for neutrinoless double-beta decay using a specific mechanical structure to hold thermal detectors. The design of the structure was tuned to minimize the background contribution, keeping an optimal detector performance. A single module of the structure holds two scintillating bolometers (with a crystal size of 45x45x45 mm and a Ge slab facing the crystal's upper side) in the Cu frame, allowing for a modular construction of a large-scale array. Two designs are released: the initial $Thick$ version contains around 15% of Cu over the crystal mass (lithium molybdate, LMO), while this ratio is reduced to ~6% in a finer ($Slim$) design. Both designs were tested extensively at aboveground (IJCLab, France) and underground (LSC, Spain) laboratories. In particular, at LSC we used a pulse-tube-based CROSS facility to operate a 6-crystal array of LMOs enriched/depleted in $^{100}$Mo. The tested LMOs show high spectrometric performance in both designs; notably, the measured energy resolution is 5--7 keV FWHM at 2615 keV $\gamma$s, nearby the Q-value of $^{100}$Mo (3034 keV). Due to the absence of a reflective cavity around LMOs, a low scintillation signal is detected by Ge bolometers: ~0.3 keV (150 photons) for 1-MeV $\gamma$($\beta$) LMO-event. Despite that, an acceptable separation between $\alpha$ and $\gamma$($\beta$) events is achieved with most devices. The highest efficiency is reached with light detectors in the $Thick$ design thanks to a lower baseline noise width (0.05--0.09 keV RMS) when compared to that obtained in the $Slim$ version (0.10--0.35 keV RMS). Given the pivotal role of bolometric photodetectors for particle identification and random coincidences rejection, we will use the structure here described with upgraded light detectors, featuring thermal signal amplification via the Neganov-Trofimov-Luke effect, as also demonstrated in the present work.

physics.ins-det

BINGO innovative assembly for background reduction in bolometric $0\nu\beta\beta$ experiments

BINGO is a project aiming to set the grounds for large-scale bolometric neutrinoless double-beta-decay experiments capable of investigating the effective Majorana neutrino mass at a few meV level. It focuses on developing innovative technologies (a detector assembly, cryogenic photodetectors and active veto) to achieve a very low background index, of the order of $10^{-5}$ counts/(keV kg yr) in the region of interest. The BINGO demonstrator, called MINI-BINGO, is designed to investigate the promising double-beta-decay isotopes $^{100}$Mo and $^{130}$Te and it will be composed of Li$_2$MoO$_4$ and TeO$_2$ crystals coupled to bolometric light detectors and surrounded by a Bi$_4$Ge$_3$O$_{12}$-based veto. This will allow us to reject a significant background in bolometers caused by surface contamination from $\alpha$-active radionuclides by means of light yield selection and to mitigate other sources of background, such as surface contamination from $\beta$-active radionuclides, external $\gamma$ radioactivity, and pile-up due to random coincidence of background events. This paper describes an R\&D program towards the BINGO goals, particularly focusing on the development of an innovative assembly designed to reduce the passive materials within the line of sight of the detectors, which is expected to be a dominant source of background in next-generation bolometric experiments. We present the performance of two prototype modules -- housing four cubic (4.5-cm side) Li$_2$MoO$_4$ crystals in total -- operated in the Canfranc underground laboratory in Spain within a facility developed for the CROSS double-beta-decay experiment.

physics.ins-det

Results from a Prototype TES Detector for the Ricochet Experiment

Coherent elastic neutrino-nucleus scattering (CE$ν$NS) offers valuable sensitivity to physics beyond the Standard Model. The Ricochet experiment will use cryogenic solid-state detectors to perform a precision measurement of the CE$ν$NS spectrum induced by the high neutrino flux from the Institut Laue-Langevin nuclear reactor. The experiment will employ an array of detectors, each with a mass of $\sim$30 g and a targeted energy threshold of 50 eV. Nine of these detectors (the "Q-Array") will be based on a novel Transition-Edge Sensor (TES) readout style, in which the TES devices are thermally coupled to the absorber using a gold wire bond. We present initial characterization of a Q-Array-style detector using a 1 gram silicon absorber, obtaining a baseline root-mean-square resolution of less than 40 eV.

physics.ins-det

Test of $^{116}$CdWO$_4$ and Li$_2$MoO$_4$ scintillating bolometers in the CROSS underground facility with upgraded detector suspension

In preparation to the CROSS $2\beta$ decay experiment, we installed a new detector suspension with magnetic dumping inside a pulse-tube cryostat of a dedicated low-background facility at the LSC (Spain). The suspension was tested with two scintillating bolometers based on large-volume 116CdWO4 (CWO-enr) and Li2MoO4 (LMO) crystals. The former, a reference device, was used for testing new noise conditions and for comparing bolometric performance of an advanced Li2MoO4 crystal developed in the framework of the CLYMENE project, in view of next-generation double-beta decay experiments like CUPID. We cooled down detectors to 15 mK and achieved high performance for all tested devices. In particular both CWO-enr and LMO bolometers demonstrated the energy resolution of 6 keV FWHM for the 2.6 MeV gamma quanta, among the best for thermal detectors based on such compounds. The baseline noise resolution (FWHM) of the CWO-enr detector was improved by 2 keV, compared to the best previous measurement of this detector in the CROSS facility, while the noise of the Ge-based optical bolometer was improved by a factor 2, to 100 eV FWHM. Despite of the evident progress in the improving of noise conditions of the set-up, we see high-frequency harmonics of a pulse-tube induced noise, suggesting a noise pick-up by cabling. Another Ge light detector was assisted with the signal amplification exploiting the Neganov-Trofimov-Luke effect, which allowed to reach 20 eV FWHM noise resolution by applying 60 V electrode bias. Highly-efficient particle identification was achieved with both detectors, despite a low scintillation efficiency of the LMO material. The radiopurity level of the LMO crystal is rather high; only traces of 210Po and 226Ra were detected (0.1 mBq/kg each), while the 228Th activity is expected to be at least an order of magnitude lower, as well as a 40K activity is found to be < 6 mBq/kg.

physics.ins-det

Measurement of the $2νββ$ decay rate and spectral shape of $^{100}$Mo from the CUPID-Mo experiment

Neutrinoless double beta decay ($0νββ$) is a yet unobserved nuclear process which would demonstrate Lepton Number violation, a clear evidence of beyond Standard Model physics. The process two neutrino double beta decay ($2νββ)$ is allowed by the Standard Model and has been measured in numerous experiments. In this letter, we report a measurement of $2νββ$ decay half-life of $^{100}$Mo to the ground state of $^{100}$Ru of $(7.07~\pm~0.02~\text{(stat.)}~\pm~0.11~\text{(syst.)})~\times~10^{18}$~yr by the CUPID-Mo experiment. With a relative precision of $\pm~1.6$ \% this is the most precise measurement to date of a $2νββ$ decay rate in $^{100}$Mo. In addition, we constrain higher-order corrections to the spectral shape which provides complementary nuclear structure information. We report a novel measurement of the shape factor $ξ_{3,1}=0.45~\pm 0.03~\text{(stat.)} \ \pm 0.05 \ \text{(syst.)}$, which is compared to theoretical predictions for different nuclear models. We also extract the first value for the effective axial vector coupling constant obtained from a spectral shape study of $2νββ$ decay.

nucl-ex

First demonstration of 30 eVee ionization energy resolution with Ricochet germanium cryogenic bolometers

The future Ricochet experiment aims to search for new physics in the electroweak sector by measuring the Coherent Elastic Neutrino-Nucleus Scattering process from reactor antineutrinos with high precision down to the sub-100 eV nuclear recoil energy range. While the Ricochet collaboration is currently building the experimental setup at the reactor site, it is also finalizing the cryogenic detector arrays that will be integrated into the cryostat at the Institut Laue Langevin in early 2024. In this paper, we report on recent progress from the Ge cryogenic detector technology, called the CryoCube. More specifically, we present the first demonstration of a 30~eVee (electron equivalent) baseline ionization resolution (RMS) achieved with an early design of the detector assembly and its dedicated High Electron Mobility Transistor (HEMT) based front-end electronics. This represents an order of magnitude improvement over the best ionization resolutions obtained on similar heat-and-ionization germanium cryogenic detectors from the EDELWEISS and SuperCDMS dark matter experiments, and a factor of three improvement compared to the first fully-cryogenic HEMT-based preamplifier coupled to a CDMS-II germanium detector. Additionally, we discuss the implications of these results in the context of the future Ricochet experiment and its expected background mitigation performance.

astro-ph.IM

The background model of the CUPID-Mo $0νββ$ experiment

CUPID-Mo, located in the Laboratoire Souterrain de Modane (France), was a demonstrator for the next generation $0νββ$ decay experiment, CUPID. It consisted of an array of 20 enriched Li$_{2}$$ ^{100}$MoO$_4$ bolometers and 20 Ge light detectors and has demonstrated that the technology of scintillating bolometers with particle identification capabilities is mature. Furthermore, CUPID-Mo can inform and validate the background prediction for CUPID. In this paper, we present a detailed model of the CUPID-Mo backgrounds. This model is able to describe well the features of the experimental data and enables studies of the $2νββ$ decay and other processes with high precision. We also measure the radio-purity of the Li$_{2}$$^{100}$MoO$_4$ crystals which are found to be sufficient for the CUPID goals. Finally, we also obtain a background index in the region of interest of 3.7$^{+0.9}_{-0.8}$(stat)$^{+1.5}_{-0.7}$(syst)$\times10^{-3}$counts/$Δ$E$_{FWHM}$/mol$_{iso}$/yr, the lowest in a bolometric $0νββ$ decay experiment.

hep-ex

Li$_2$$^{100\textrm{depl}}$MoO$_4$ Scintillating Bolometers for Rare-Event Search Experiments

We report on the development of scintillating bolometers based on lithium molybdate crystals containing molybdenum depleted in the double-$\beta$ active isotope $^{100}$Mo (Li$_2$$^{100\textrm{depl}}$MoO$_4$). We used two Li$_2$$^{100\textrm{depl}}$MoO$_4$ cubic samples, 45 mm side and 0.28 kg each, produced following purification and crystallization protocols developed for double-$\beta$ search experiments with $^{100}$Mo-enriched Li$_2$MoO$_4$ crystals. Bolometric Ge detectors were utilized to register scintillation photons emitted by the Li$_2$$^{100\textrm{depl}}$MoO$_4$ crystal scintillators. The measurements were performed in the CROSS cryogenic set-up at the Canfranc underground laboratory (Spain). We observed that the Li$_2$$^{100\textrm{depl}}$MoO$_4$ scintillating bolometers are characterized by excellent spectrometric performance ($\sim$3--6 keV FWHM at 0.24--2.6 MeV $\gamma$'s), moderate scintillation signal ($\sim$0.3--0.6 keV/MeV depending on light collection conditions) and high radiopurity ($^{228}$Th and $^{226}$Ra activities are below a few $\mu$Bq/kg), comparable to the best reported results of low-temperature detectors based on Li$_2$MoO$_4$ with natural or $^{100}$Mo-enriched molybdenum content. Prospects of Li$_2$$^{100\textrm{depl}}$MoO$_4$ bolometers for use in rare-event search experiments are briefly discussed.

physics.ins-det

ZnO-based scintillating bolometers: New prospects to study double beta decay of $^{64}$Zn

The first detailed study on the performance of a ZnO-based cryogenic scintillating bolometer as a detector to search for rare processes in zinc isotopes was performed. A 7.2 g ZnO low-temperature detector, containing more than 80\% of zinc in its mass, exhibits good energy resolution of baseline noise 1.0--2.7 keV FWHM at various working temperatures resulting in a low-energy threshold for the experiment, 2.0--6.0 keV. The light yield for $β$/$γ$ events was measured as 1.5(3) keV/MeV, while it varies for $α$ particles in the range of 0.2--3.0 keV/MeV. The detector demonstrate an effective identification of the $β$/$γ$ events from $α$ events using time-properties of only heat signals. %(namely, Rise time parameter). The radiopurity of the ZnO crystal was evaluated using the Inductively Coupled Plasma Mass Spectrometry, an ultra-low-background High Purity Ge $γ$-spectrometer, and bolometric measurements. Only limits were set at the level of $\mathcal{O}$(1--100) mBq/kg on activities of \Nuc{K}{40}, \Nuc{Cs}{137} and daughter nuclides from the U/Th natural decay chains. The total internal $α$-activity was calculated to be 22(2) mBq/kg, with a major contribution caused by 6(1) mBq/kg of \Nuc{Th}{232} and 12(2) mBq/kg of \Nuc{U}{234}. Limits on double beta decay (DBD) processes in \Nuc{Zn}{64} and \Nuc{Zn}{70} isotopes were set on the level of $\mathcal{O}(10^{17}$--$10^{18})$ yr for various decay modes profiting from 271 h of acquired background data in the above-ground lab. This study shows a good potential for ZnO-based scintillating bolometers to search for DBD processes of Zn isotopes, especially in \Nuc{Zn}{64}, with the most prominent spectral features at $\sim$10--20 keV, like the two neutrino double electron capture. A 10 kg-scale experiment can reach the experimental sensitivity at the level of $\mathcal{O}(10^{24})$ yr.

physics.ins-det