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Lianhe Li

Publications and source records attributed to Lianhe Li.

At least 19 recordsLinked to original sources

Transport-defined photodetection through electrically selectable nonequilibrium carrier transport

Broadband optical fields can change in both intensity and spectral distribution, but a fixed-response detector maps this evolving information onto a single electrical signal. Here we demonstrate transport-defined photodetection, in which electrical bias selects how photoexcited carriers are redistributed, escape and are collected, creating complementary response functions within one shared active region. In a GaAs/AlGaAs semiconductor ratchet, light-driven ratchet transport defines the response at 0 V, whereas the spectral evolution at -2 V is consistent with field-assisted hot-carrier transport. The overlapping states span a measured spectral range of 0.4-94.5 {\mu}m at 5 K, provide state-dependent calculated detection floors and support joint infrared operation at 30 K. Direct optical beat notes at 7.432 GHz in the mid-infrared and 17.103 GHz in the terahertz demonstrate optical-to-electrical conversion. Their common-path outputs recover an imposed spatial temperature gradient and the transient field-of-view-integrated effective radiation temperature of laser-excited graphite. These results establish post-photoexcitation transport as a function-defining design variable for semiconductor photodetectors, complementing structure-defined, field-tuned and optically encoded approaches to reconfigurable photodetection.

physics.optics

Quantum cascade laser roadmap

Quantum cascade lasers (QCLs) are unipolar semiconductor lasers first demonstrated in 1994. Since then, they have played a central role in advancing mid-infrared and terahertz photonics, becoming among the most reliable light sources in these regions of the electromagnetic spectrum. Their importance is further reinforced by their ability to generate self-starting optical frequency combs, whose investigation is motivated both by fundamental physics and by a wide range of applications, including molecular spectroscopy and free-space optical communications. This Roadmap provides a unified overview of current advances and emerging directions in QCL research. The chapters are organized into three main sections: device design and technology; frequency combs and pulse formation; and applications of QCLs. Each chapter reviews the relevant background, summarizes the current state of the art, and identifies key challenges and future directions within its specific research area.

physics.optics

Improving terahertz-detection sensitivity of 8x8 FET arrays through liquid-nitrogen cooling in a compact low-noise cryostat

We show that the sensitivity of antenna-coupled field-effect transistors (FETs) to terahertz (THz) radiation improves continuously with decreasing temperature. The noise-equivalent power (NEP) of 540 GHz patch-antenna-coupled FETs decreases as temperature reduces to 20 K. We project NEP values approaching 1 to 2 pW/sqrt(Hz) under efficient power coupling conditions (e.g., using a superstrate Si-lens), which is comparable to superconducting niobium transition-edge sensors (TESs) at 4 K. Building on these findings, a compact, low-noise, liquid-nitrogen-cooled (77 K) FET-based direct (incoherent) THz-power sensing system} for spectroscopy applications was realized. Here, an 8x8 pixel-binned detector array fabricated in a commercial 65-nm Si-CMOS process, was optimized for operation in the 2.85 to 3.4 THz band. Characterization was performed in the focal plane of a 2.85-THz quantum-cascade laser delivering approx. 2~mW of THz power. A linear dynamic range exceeding 67 dB was achieved without saturation (for 1~Hz-detection bandwidth). The system provides a -3 dB readout bandwidth of 5 MHz, exceeding that of conventional thermal detectors (typically 1 kHz). Combined with its broad temperature operability 20 K to 300 K and compact design, the system is particularly well suited for space- and payload-constrained platforms such as balloon- and satellite-based missions, where deep cryogenic cooling is impractical.

physics.app-ph

Detectorless 3D terahertz imaging: achieving subwavelength resolution with reflectance confocal interferometric microscopy

Terahertz imaging holds great potential for non-destructive material inspection, but practical implementation has been limited by resolution constraints. In this study, we present a single-pixel THz imaging system based on a confocal microscope architecture, utilising a quantum cascade laser as both transmitter and phase-sensitive receiver. Our approach integrates laser feedback interferometry detection to achieve a two-fold improvement in lateral resolution and a two-order-of-magnitude enhancement in axial resolution over conventional imaging through precise interferometric phase measurements. This translates to a lateral resolution near $λ/2$ and a depth of focus better than $λ/5$, significantly outperforming traditional confocal systems. The system can produce a 0.5 Mpixel image in under two minutes, surpassing both raster-scanning single-pixel and multipixel focal-plane array-based imagers. Coherent operation enables simultaneous amplitude and phase image acquisition, and a custom visualisation method links amplitude to image saturation and phase to hue, enhancing material characterisation. A 3D tomographic analysis of a silicon chip reveals subwavelength features, demonstrating the system's potential for high-resolution THz imaging and material analysis. This work sets a new benchmark for THz imaging, overcoming key challenges and opening up transformative possibilities for non-destructive material inspection and characterisation.

physics.optics

Ultra-sensitive heterodyne detection at room temperature in the atmospheric windows

We report room temperature heterodyne detection of a quantum cascade laser beaten with a local oscillator on a unipolar quantum photodetector in two different atmospheric windows, at 4.8 $μ$m and 9 $μ$m. A noise equivalent power of few pW is measured by employing an active stabilization technique in which the local oscillator and the signal are locked in phase. The measured heterodyne noise equivalent power is six orders of magnitude lower than that obtained with direct detection.

physics.optics

8x8 Patch-Antenna-Coupled TeraFET Detector Array for Terahertz Quantum-Cascade-Laser Applications

Monolithically integrated, antenna-coupled field-effect transistors (TeraFETs) are rapid and sensitive detectors for the terahertz range (0.3-10~THz) that can operate at room temperature. We conducted experimental characterizations of a single patch-antenna coupled TeraFET optimized for 3.4~THz operation and its integration into an 8x8 multi-element detector configuration. In this configuration, the entire TeraFET array operates as a unified detector element, combining the output signals of all detector elements. Both detectors were realized using a mature commercial Si-CMOS 65-nm process node. Our experimental characterization employed single-mode Quantum-Cascade Lasers (QCLs) emitting at 2.85~THz and 3.4~THz. The 8x8 multi-element detector yields two major improvements for sensitive power detection experiments. First, the larger detector area simplifies alignment and enhances signal stability. Second, the reduced detector impedance enabled the implementation of a TeraFET+QCL system capable of providing a -3~dB modulation bandwidth up to 21~MHz, which is currently limited primarily by the chosen readout circuitry. Finally, we validate the system's performance by providing high resolution gas spectroscopy data for methanol vapor around 3.4~THz, where a detection limit of 1.6e-5 absorbance, or 2.6e11~molecules/cm^3 was estimated under optimal coupling conditions.

physics.ins-det

Ultrafast (10 GHz) mid-IR modulator based on ultra-fast electrical switching of the light-matter coupling

We demonstrate a free-space amplitude modulator for mid-infrared radiation (lambda=9.6 um) that operates at room temperature up to at least 20 GHz (above the -3dB cutoff frequency measured at 8.2 GHz). The device relies on the ultra-fast transition between weak and strong-coupling regimes induced by the variation of the applied bias voltage. Such transition induces a modulation of the device reflectivity. It is made of a semiconductor heterostructure enclosed in a judiciously designed array of metal-metal optical resonators, that - all-together - behave as an electrically tunable surface. At negative bias, it operates in the weak light-matter coupling regime. Upon application of an appropriate positive bias, the quantum wells populate with electrons and the device transitions to the strong-coupling regime. The modulator transmission keeps linear with input RF power in the 0dBm - 9dBm range. The increase of optical powers up to 25 mW exhibit a weak beginning saturation a little bit below.

physics.app-ph

Sculpting harmonic comb states in terahertz quantum cascade lasers by controlled engineering

Optical frequency combs (FCs), that establish a rigid phase-coherent link between the microwave and optical domains of the electromagnetic spectrum, are emerging as a key high-precision tools for the development of quantum technology platforms. These include potential applications for communication, computation, information, sensing and metrology, and can extend from the near-infrared with micro-resonator combs, up to the technologically attractive terahertz (THz) frequency range, with powerful and miniaturized quantum cascade laser (QCL) FCs. The recently discovered ability of the QCLs to produce a harmonic frequency comb (HFC), a FC with large intermodal spacings, has attracted new interest in these devices for both applications and fundamental physics, particularly for the generation of THz tones of high spectral purity for high data rate wireless communication networks, for radiofrequency arbitrary waveform synthesis, and for the development of quantum key distributions. The controlled generation of harmonic states of a specific order remains, however, elusive in THz QCLs. Here we devise a strategy to obtain broadband HFC emission of a pre-defined order in QCL, by design. By patterning n regularly spaced defects on the top-surface of a double-metal Fabry-Perot QCL, we demonstrate harmonic comb emission with modes spaced by (n+1) free spectral range and with a record optical power/mode of ~270 $μW$.

physics.optics

Liquid-Crystal-Based Controllable Attenuators Operating in the 1-4 Terahertz Band

Liquid-crystal devices (LCDs) offer a potential route toward adaptive optical components for use in the < 2 THz band of the electromagnetic spectrum. We demonstrate LCDs using a commercially available material (E7), with unbiased birefringence values of 0.14-0.18 in the 0.3-4 THz band. We exploit the linear dichroism of the material to modulate the emission from a 3.4-THz quantum cascade laser by up to 40%, dependent upon both the liquid-crystal layer thickness and the bias voltage applied.

physics.optics

Detection of strong light-matter interaction in a single nano-cavity with a thermal transducer

Recently, the concept of strong light-matter coupling has been demonstrated in semiconductor structures, and it is poised to revolutionize the design and implementation of components, including solid state lasers and detectors. We demonstrate an original nanospectroscopy technique that permits to study the light-matter interaction in single subwavelength-sized nano-cavities where far-field spectroscopy is not possible using conventional techniques. We inserted a thin ($\approx$ 150 nm) polymer layer with negligible absorption in the mid-IR (5 $μ$m < $λ$ < 12 $μ$m) inside a metal-insulator-metal resonant cavity, where a photonic mode and the intersubband transition of a semiconductor quantum well are strongly coupled. The intersubband transition peaks at $λ$ = 8.3 $μ$m, and the nano-cavity is overall 270 nm thick. Acting as a non-perturbative transducer, the polymer layer introduces only a limited alteration of the optical response while allowing to reveal the optical power absorbed inside the concealed cavity. Spectroscopy of the cavity losses is enabled by the polymer thermal expansion due to heat dissipation in the active part of the cavity, and performed using an atomic force microscope (AFM). This innovative approach allows the typical anticrossing characteristic of the polaritonic dispersion to be identified in the cavity loss spectra at the single nano-resonator level. Results also suggest that near-field coupling of the external drive field to the top metal patch mediated by a metal-coated AFM probe tip is possible, and it enables the near-field mapping of the cavity mode symmetry including in the presence of strong light-matter interaction.

physics.optics

Ultrashort pulse generation from a graphene-coupled passively mode-locked terahertz laser

The generation of stable trains of ultra-short (fs-ps), terahertz (THz)-frequency radiation pulses, with large instantaneous intensities, is an underpinning requirement for the investigation of light-matter interactions, for metrology and for ultra-high-speed communications. In solid-state electrically-pumped lasers, the primary route for generating short pulses is through passive mode-locking. However, this has not yet been achieved in the THz range, defining one of the longest standing goals over the last two decades. In fact, the realization of passive mode-locking has long been assumed to be inherently hindered by the fast recovery times associated with the intersubband gain of THz lasers. Here, we demonstrate a self-starting miniaturized ultra-short pulse THz laser, exploiting an original device architecture that includes the surface patterning of multilayer-graphene saturable absorbers distributed along the entire cavity of a double-metal semiconductor 2.30-3.55 THz wire laser. Self-starting pulsed emission with 4.0-ps-long pulses in a compact, all-electronic, all-passive and inexpensive configuration is demonstrated.

physics.optics

Ultrabroadband THz/IR upconversion and photovoltaic response in semi-conductor ratchet based upconverter

An ultrabroadband upconversion device is demonstrated by direct tandem integration of a p-type GaAs/AlxGa1-xAs ratchet photodetector (RP) with a GaAs double heterojunction LED (DH-LED) using the molecular beam epitaxy (MBE). An ultrabroadband photoresponse from terahertz (THz) to near infrared (NIR) region (4-200 THz) was realized that covers a much wider frequency range com-pared with the existing upconversion devices. Broadband IR/THz radiation from 1000 K blackbody is successfully upconverted into NIR photons which can be detected by commercial Si-based device. The normal incidence absorption of the RP simplifies the structure of the RP-LED device and make it more compact compared with the inter-subband transition based upconverters. In addition to the up-conversion function, the proposed upconverter is also tested as photovoltaic detectors in the infrared region (15-200 THz) without an applied bias voltage due to the ratchet effect.

physics.app-ph

Realization of ultrabroadband THz/IR photoresponse in a bias-tunable ratchet photodetector

High performance Terahertz (THz) photodetector has drawn wide attention and got great improvement due to its significant application in biomedical, astrophysics, nondestructive inspection, 6th generation communication system as well as national security application. Here we demonstrate a novel broadband photon-type THz/infrared (IR) photodetector based on the GaAs/AlxGa1-xAs ratchet structure. This kind of photodetector realizes a THz photon-response based on the electrically pumped hot hole injection and overcomes the internal workfunction related spectral response limit. An ultrabroadband photoresponse from 4 THz to 300 THz and a peak responsivity of 50.3 mA/W are realized at negative bias voltage of -1 V. The photodetector also presents a bias-tunable photon-response characteristic due to the asymmetric structure. The ratchet structure also induces an evident photocurrent even at zero bias voltage, which indicates the detector can be regard as a broadband photovoltaic-like detector. The rectification characteristic and high temperature operation possibility of the photodetector are also discussed. This work not only demonstrates a novel ultrabroadband THz/IR photodetector, but also provides a new method to study the light-responsive ratchet.

physics.app-ph

A "Janus" double sided mid-IR photodetector based on a MIM architecture

We present a mid-IR ($λ\approx$ 8.3 $μ$m) quantum well infrared photodetector (QWIP) fabricated on a mid-IR transparent substrate, allowing photodetection with illumination from either the front surface or through the substrate. The device is based on a 400 nm-thick GaAs/AlGaAs semiconductor QWIP heterostructure enclosed in a metal-insulator-metal (MIM) cavity and hosted on a mid-IR transparent ZnSe substrate. Metallic stripes are symmetrically patterned by e-beam lithography on both sides of the active region. The detector spectral coverage spans from $λ\approx 7.15$ $μ$m to $λ\approx 8.7$ $μ$m by changing the stripe width L - from L = 1.0 $μ$m to L = 1.3 $μ$m - thus frequency-tuning the optical cavity mode. Both micro-FTIR passive optical characterizations and photocurrent measurements of the two-port system are carried out. They reveal a similar spectral response for the two detector ports, with an experimentally measured T$_{BLIP}$ of $\approx$ 200K.

physics.app-ph

Chip-scale terahertz frequency combs through integrated intersubband polariton bleaching

Quantum cascade lasers (QCLs) represent a fascinating accomplishment of quantum engineering and enable the direct generation of terahertz (THz) frequency radiation from an electrically-biased semiconductor heterostructure. Their large spectral bandwidth, high output powers and quantum-limited linewidths have facilitated the realization of THz pulses by active mode-locking and passive generation of optical frequency combs (FCs) through intracavity four-wave-mixing, albeit over a restricted operational regime. Here, we conceive an integrated architecture for the generation of high power (10 mW) THz FCs comprising an ultrafast THz polaritonic reflector, exploiting intersubband cavity polaritons, and a broad bandwidth (2.3-3.8 THz) heterogeneous THz QCL. Quantum cascade lasers (QCLs) represent a fascinating accomplishment of quantum engineering and enable the direct generation of terahertz (THz) frequency radiation from an electrically-biased semiconductor heterostructure. By tuning the group delay dispersion in an integrated geometry, through the exploitation of light induced bleaching of the intersubband-based THz polaritons, we demonstrate spectral reshaping of the QCL emission and stable FC operation over an operational dynamic range of up to 38%, characterized by a single and narrow (down to 700 Hz) intermode beatnote. Our concept provides design guidelines for a new generation of compact, cost-effective, electrically driven chip-scale FC sources based on ultrafast polariton dynamics, paving the way towards the generation of mode locked THz micro-lasers that will strongly impact a broad range of applications in ultrafast sciences, data storage, high-speed communication and spectroscopy.

physics.optics

High temperature metamaterial terahertz quantum detector

We demonstrate a high temperature performance quantum detector of Terahertz (THz) radiation based on three-dimensional metamaterial. The metamaterial unit cell consists of an inductor-capacitor (LC) resonator laterally coupled with antenna elements. The absorbing region, consisting of semiconductor quantum wells is contained in the strongly ultra-subwavelength capacitors of the LC structure. The high radiation loss of the antenna allows strongly increased collection efficiency for the incident THz radiation, while the small effective volume of the LC resonator allows intense light-matter coupling with reduced electrical area. As a result, our detectors operates at much higher temperatures than conventional quantum well detectors demonstrated so far.

physics.optics

Tunable, grating-gated, graphene-on-polyimide terahertz modulators

We present an electrically switchable graphene terahertz (THz) modulator with a tunable-by-design optical bandwidth and we exploit it to compensate the cavity dispersion of a quantum cascade laser (QCL). Electrostatic gating is achieved by a metal-grating used as a gate electrode, with an HfO2/AlOx gate dielectric on top. This is patterned on a polyimide layer, which acts as a quarter wave resonance cavity, coupled with an Au reflector underneath. We get 90% modulation depth of the intensity, combined with a 20 kHz electrical bandwidth in the 1.9 _ 2.7 THz range. We then integrate our modulator with a multimode THz QCL. By adjusting the modulator operational bandwidth, we demonstrate that the graphene modulator can partially compensates the QCL cavity dispersion, resulting in an integrated laser behaving as a stable frequency comb over 35% of the laser operational range, with 98 equidistant optical modes and with a spectral coverage of ~ 1.2 THz. This has significant potential for frontier applications in the terahertz, as tunable transformation-optics devices, active photonic components, adaptive and quantum optics, and as a metrological tool for spectroscopy at THz frequencies.

physics.app-ph