arXiv subjects

M. M. Sharma

Publications and source records attributed to M. M. Sharma.

At least 19 recordsLinked to original sources

arXiv2026

Engineering magnetic anisotropy and ferromagnetism in topological Kagome metal GdV6Sn6 via Nd substitution

Kagome metals with the formula RM6X6 (R = rare-earth, M = 3d transition metal, and X = Sn/Ge) provide a rich platform for exploring magnetic and electronic phenomena, with tunable properties enabled by the combination of rare-earth elements and transition metals. In this study, we report the structural, electrical and magnetic properties of Kagome metal (NdxGd1-x)V6Sn6. We demonstrate that substituting lighter Nd atoms at the Gd site tunes the complex magnetic ground state of GdV6Sn6 into a ferromagnetic-like one. Moreover, the isotropic magnetization of GdV6Sn6 becomes anisotropic, with the c-axis emerging as the easy axis. Transport measurements reveal a strong coupling between magnetism and electronic properties, with negative magnetoresistance observed at low magnetic fields in all compositions. In addition, a fourfold anisotropy component tends to emerge in end compounds at higher magnetic fields. These findings highlight the role of rare-earth substitution in tuning magnetic anisotropy and magneto-transport behaviour in RM6X6 compounds, featuring a non-magnetic Kagome layer, with potential implications for spintronic and topological applications.

cond-mat.mtrl-sci↗

arXiv2026

Chalcogen Doping Effect on the Insulator-to-Metal Transition in GdPS

Topological semimetals offer a rich platform for exploring massless fermion physics and realizing exotic properties with potential technological applications. GdPS, a magnetic semiconductor derived from the nodal-line semimetal ZrSiS family, exhibits a field-induced insulator-to-metal transition driven by exchange splitting. This transition is accompanied by an unusual, isotropic, and gigantic negative magnetoresistance, attributed to negligible magnetic anisotropy resulting from the weak spin-orbit coupling of half-filled Gd3+ 4f orbitals and light S atoms. In this work, we investigate Se substitution, which is expected to enhance spin-orbit coupling. Indeed, we observe slightly increased magnetic anisotropy in magnetotransport. Moreover, Se substitution suppresses the field-induced insulator-to-metal transition, likely due to an enlarged band gap that demands a higher exchange splitting to close. These findings provide deeper insights into the interplay between spin-orbit coupling, magnetic anisotropy, and transport behavior in GdPS, offering guidance for future materials design for desired functionalities.

cond-mat.mtrl-sci↗

arXiv2026

Ferromagnetic Spin Glass State and Anomalous Hall Effect in Topological Semimetal Candidate Mn2Sb2Te5

Materials that intrinsically possess both magnetism and topological states represent a key frontier of quantum materials research. Recently, Mn2(Bi/Sb)2Te5 has emerged as a promising candidate for hosting topological surface states coupled with intrinsic magnetic order, making it a potential magnetic Weyl semimetal. In this study, we investigate the magnetic and transport properties of Mn2Sb2Te5 single crystals. The magnetization measurements reveal a spin glass state with field-induced ferromagnetism. Although heat capacity measurement indicates the absence of long-range order, the intrinsic magnetization in Mn2Sb2Te5 significantly affects its electrical properties, as demonstrated by the anomalous Hall effect. This work provides valuable insights into the magnetism and the electronic properties of Mn2Sb2Te5, establishing Mn2(Bi/Sb)2Te5 system as a compelling platform for exploring the interplay between magnetism and non-trivial band topology, enabling emergent quantum phases and novel transport responses not accessible in non-magnetic systems.

cond-mat.mtrl-sci↗

arXiv2025

Ground-based Observations of Temporal Variation of Cosmic Ray Spectrum during Forbush Decreases

Observations of temporary Forbush decreases (FDs) in the Galactic cosmic ray (GCR) flux due to passage of solar storms are useful for space weather studies and alerts. Here we introduce techniques that use global networks of ground-based neutron monitors and muon detectors to measure variations of GCR rigidity spectra in space during FDs by: A) fitting count rate decreases for power-law rigidity spectra in space with anisotropy up to second order, and B) using the "leader fraction" derived from a single neutron monitor. We demonstrate that both provide consistent results for hourly spectral index variations for five major FDs and they agree with daily space-based data when available from AMS-02. We have also made the neutron monitor leader fraction publicly available in real time. This work verifies that ground-based observations can be used to precisely monitor GCR spectral variation over a wide range of rigidities during space weather events, with results in real time or from short-term post-analysis.

astro-ph.HE↗

arXiv2025

Quantum oscillation studies of the nodal line semimetal Ni3In2S2-xSex

Ternary shandite compounds with the general formula T3M2X2 (T = Ni, Co, Rh or Pd; M = Sn, In or Pb and X = S or Se) have emerged as a large pool of topological semimetals. This family of compounds hosts different topological phases for various combinations of T, M and X. This paper reports the observation of quantum oscillations under the high magnetic fields in Ni3In2S2-xSex single crystals. Angular dependence of oscillation frequency suggests an evolution of the Fermi surface from three-dimensional to two-dimensional on Se substitution for S in Ni3In2S2. The effective mass obtained for each composition by fitting the oscillation amplitude with the Lifshitz-Kosevich formula, shows no significant change, suggesting that the topological phase might be relatively robust against enhanced SOC upon Se doping in Ni3In2S2.

cond-mat.mtrl-sci↗

arXiv2025

Large Negative Magnetoresistance in off-Stochiometric Topological Material PrSbTe

Magnetic topological materials LnSbTe (Ln = lanthanide) have attracted intensive attention because of the presence of interplay between magnetism, topological, and electron correlations depending on the choices of magnetic Ln elements. Varying Sb and Te composition is an efficient approach to control structural, magnetic, and electronic properties. Here we report the composition-dependent properties in PrSbxTe2-x. We identified the tetragonal-to-orthorhombic structure transitions in this material system, and very large negative magnetoresistance in the x = 0.3 composition, which might be ascribed to the coupling between magnetism and transport. Such unusual magnetotransport enables PrSbxTe2-x topological materials as a promising platform for device applications.

cond-mat.mtrl-sci↗

arXiv2025

Large Negative Magnetoresistance in Antiferromagnetic Gd2Se3

Rare earth chalcogenides provide a great platform to study exotic quantum phenomena such as superconductivity and charge density waves. Among various interesting properties, the coupling between magnetism and electronic transport has attracted significant attention. Here, we report the investigation of such coupling in {alpha}-Gd2Se3 single crystals through magnetic, calorimetric, and transport property measurements. {alpha}-Gd2Se3 is found to display an antiferromagnetic ground state below 11 K with metamagnetic spin-flop transitions. The magnetic fluctuations remain strong above the transition temperature. Transport measurements reveal an overall metallic transport behavior with a large negative magnetoresistance of ~ 65% near the magnetic transition temperature, together with positive MR near the field-induced spin-flop transitions, which can be understood in terms of the suppression of spin scattering by the magnetic field.

cond-mat.mtrl-sci↗

arXiv2024

Global analysis of the extended cosmic-ray decreases observed with world-wide networks of neutron monitors and muon detectors; temporal variation of the rigidity spectrum and its implication

This paper presents the global analysis of two extended decreases of the galactic cosmic ray intensity observed by world-wide networks of ground-based detectors in 2012. This analysis is capable of separately deriving the cosmic ray density (or omnidirectional intensity) and anisotropy each as a function of time and rigidity. A simple diffusion model along the spiral field line between Earth and a cosmic-ray barrier indicates the long duration of these events resulting from about 190$^\circ$ eastern extension of a barrier such as an IP-shock followed by the sheath region and/or the corotating interaction region (CIR). It is suggested that the coronal mass ejection merging and compressing the preexisting CIR at its flank can produce such the extended barrier. The derived rigidity spectra of the density and anisotropy both vary in time during each event period. In particular we find that the temporal feature of the ``phantom Forbush decrease'' reported in an analyzed period is dependent on rigidity, looking quite different at different rigidities. From these rigidity spectra of the density and anisotropy, we derive the rigidity spectrum of the average parallel mean-free-path of pitch angle scattering along the spiral field line and infer the power spectrum of the magnetic fluctuation and its temporal variation. Possible physical cause of the strong rigidity dependence of the ``phantom Forbush decrease'' is also discussed. These results demonstrate the high-energy cosmic rays observed at Earth responding to remote space weather.

astro-ph.HE↗

arXiv2024

Medium-entropy Engineering of magnetism in layered antiferromagnet CuxNi2(1-x)CrxP2S6

Engineering magnetism in layered magnets could result in novel phenomena related to two-dimensional (2D) magnetism, which can be useful for fundamental research and practical applications. Extensive doping efforts such as substitution and intercalation have been adopted to tune antiferromagnetic (AFM) properties in M2P2X6 compounds. The substitutional doping in this material family has mainly focused on bimetallic substitution. Recently, the metal substitution can also be extended to more than two metal elements, leading to medium and high-entropy alloys (MEAs and HEAs), which are fairly underexplored in layered magnetic systems including M2P2X6. In this work, we explored the magnetic properties of the previously unreported Cu- and Cr-substituted Ni2P2S6 i.e., CuxNi2(1-x)CrxP2S6. Our study reveals a relatively systematic evolution of AFM phases with substitution than that observed in traditional bimetallic substitution in M2P2X6. Furthermore, the Cu and Cr substitutions in Ni2P2S6 are found to enhance the ferromagnetic (FM) correlation, which is also accompanied by a possible weak FM phase at low temperatures for the intermediate compositions from 0.32 to 0.80. Our work provides a strategy to establish ferromagnetism in AFM M2P2X6 that can also be used for property tuning in other layered magnets.

cond-mat.mtrl-sci↗

arXiv2024

Tuning Magnetism in Ising-type van der Waals Magnet FePS3 by Lithium Intercalation

Recently, layered materials transition metal thiophosphate MPX3 (M = transition metals, X = S or Se) have gained significant attention because of their rich magnetic, optical, and electronic properties. Specifically, the diverse magnetic structures and the robustness of magnetism in the two-dimensional limit have made them prominent candidates to study two-dimensional magnetism. Numerous efforts such as substitutions and interlayer intercalations have been made to tune the properties of these materials, which has greatly deepened the understanding of the underlying mechanisms that govern the properties. In this work, we focus on modifying the magnetism of Ising-type antiferromagnet FePS3 using electrochemical lithium intercalation. Our work unveils the effectiveness of electrochemical intercalation as a controllable tool to modulating magnetism, including tuning magnetic ordering temperature and inducing low temperature spin-glass state, offering an approach for implementing this material into applications.

cond-mat.mtrl-sci↗

arXiv2024

Normal state magneto transport properties of FeSe$_{0.5}$Te$_{0.5}$ superconductor: The role of topological surface states

Doped Iron Chalcogenide (FeCh) superconductors are extensively studied in the context of topological superconductivity. However, the evidence of topological surface states in electrical transport measurements of the doped FeCh system is yet warranted. In the present letter, we performed angle-dependent magneto transport measurements on a single crystal of a doped FeCh system, i.e., FeSe$_{0.5}$Te$_{0.5}$. A non-saturating linear magnetoresistance (MR) has been observed under the magnetic field up to 14 T in the normal state of FeSe$_{0.5}$Te$_{0.5}$. The MR is shown to possess anisotropy, which indicates the presence of topological surface states in FeSe$_{0.5}$Te$_{0.5}$. Angle-dependent Magneto-conductivity (MC) at low magnetic fields has been modelled by Hikami Larkin Nagaoka (HLN) formalism, which shows the presence of weak antilocalization (WAL) effect in FeSe$_{0.5}$Te$_{0.5}$. The observed WAL effect is found to be 2D in nature through angle-dependent magneto transport measurements. Theoretical calculations based on Density Functional Theory (DFT) are also performed to get more confidence on the presence of topological surface states in FeSe$_{0.5}$Te$_{0.5}$.

cond-mat.supr-con↗

arXiv2024

Superconductivity at 9 K in Pb-Bi Alloy

In the present work, we report the synthesis of Pb-Bi alloy with enhanced Tc of up to 9K, which is higher than that of Pb. The alloy is synthesized via a solid-state reaction route in the vacuum-encapsulated quartz tube at 7000C in an automated furnace. The synthesized sample is characterized by X-ray Diffraction(XRD) and Energy dispersive X-ray analysis(EDAX) for its phase purity and elemental composition. Rietveld refinement of XRD reveals that the end product is a majority hexagonal Pb7Bi3, with minor rhombohedral Bi. The electronic transport measurement shows metallic behavior with the Debye temperature of 108K and a superconductivity transition temperature (Tc) below 9K, which is the maximum to date for any reported Pb-Bi alloy, Pb or Bi at ambient pressure. Partial substitution of Bi at the Pb site may modify the free density of electronic states within the BCS model to attain the optimum Tc, which is higher by around 2K from the reported Tc of Pb. The superconductor phase diagram derived from magneto-transport measurements reveals that the synthesized alloy is a conventional superconductor with an upper critical field (Hc2) of 3.9 Tesla, which lies well within the Pauli paramagnetic limit. The magnetization measurements carried out following ZFC(Zero Field Cool) protocols infer that the synthesized alloy is a bulk superconductor below 9K. The isothermal M-H(Magnetization vs. Field) measurements performed below Tc establish it as a type-II superconductor. The specific heat capacity measurements show that the Pb-Bi alloy is a strongly coupled bulk superconductor below around 9K with possibly two superconducting gaps.

cond-mat.supr-con↗

arXiv2024

Anisotropy in Electronic and Magneto-transport of 2D superconductor NbSe$_2$

This article reports the successful synthesis of single crystalline two-dimensional thin flakes of NbSe$_2$. The XRD pattern of the grown crystal ensured its crystallization in a single phase with a hexagonal structure. The EDAX endorsed the stoichiometry of the as grown sample. To study the vibrational modes, the Raman spectra were recorded, which exhibited the expected four Raman active modes. The resistance vs temperature measurement showed a well-established superconducting transition (Tc) at 7.3 K. The ZFC (Zero-Field Cooled) & FC (Field Cooled) magnetization curves, as well as the isothermal MH (Magnetization vs. field) measurements, have been performed for both in plane and out-of-plane H directions. Distinct anisotropy is observed in both magnetization and magneto-transport measurements with field direction, leading to different critical fields (Hc). Out-of-plane magneto-transport data hints towards the existence of a filamentary state. The density functional theory (DFT) has been used to study the band structure of NbSe$_2$. Although the bulk band structure confirmed metallic behavior, the same for mono-layers of NbSe$_2$ within the GGA+U framework showed a band gap of 1.17eV. The article addresses the anisotropy in the electronic and magneto-transport of 2D superconductor NbSe$_2$.

cond-mat.supr-con↗

arXiv2023

Weak Antilocalization and topological edge states in PdSn$_4$

Here we report, the successful synthesis of single crystals of topological semimetal (TSM) candidate, PdSn$_4$ using the self-grown route. The synthesized crystal is well characterized through X-ray diffraction (XRD), field emission scanning electron microscopy (FESEM), and X-ray photoelectron spectroscopy (XPS). Detailed Rietveld analysis of the powder XRD pattern of PdSn$_4$ confirmed the same to crystallize in the Aea2 space group instead of reported Ccce. A large magnetoresistance (MR) along with Subnikov-de Haas oscillations have been observed in magnetotransport measurements at 2K. The presence of a weak antilocalization (WAL) effect in synthesized PdSn$_4$ crystal is confirmed and analyzed using Hikami Larkin Nagaoka (HLN) formalism, being applied on magnetoconductivity of the same at the low magnetic field. An extended Kohler rule is implemented on MR data, to determine the role of the scattering process and temperature-dependent carrier density on transport phenomenon in PdSn$_4$. Further, the non-trivial band topology and presence of edge states are shown through density functional theory (DFT) based theoretical calculations. All calculations are performed considering the Aea2 space group symmetry. The calculated Z2 invariants suggest the presence of weak topological insulating properties in PdSn$_4$. Clear evidence of topological edge states at the $Γ$ point is visible in calculated edge state spectra. This is the first report on PdSn$_4$, showing the presence of SdH oscillation in magneto transport measurement.

cond-mat.mtrl-sci↗

arXiv2023

Two-fold anisotropic superconducting state in topological superconductor Sn$_4$Au

Here we report the anisotropic magnetotransport properties in the superconducting state of Sn$_4$Au single crystal. Sn$_4$Au single crystal is synthesized through an easy melt growth method. Superconducting properties are evidenced by resistivity vs. temperature and DC magnetization measurements. Isothermal magnetization measurements hint toward type-II superconductivity in Sn$_4$Au. In-plane and out-of-plane resistivity measurements show anisotropic behavior of the upper critical field at temperatures below superconducting transition (T$_c$ = 2.3 K). The observed anisotropy is more elucidated in resistivity measurements performed below Tc at different tilt angles. The anisotropy parameter is found to be 1.26. The observed results show the presence two-fold anisotropic superconducting state in Sn$_4$Au single crystal, which may be induced due to the layered structure of synthesized Sn$_4$Au single crystal.

cond-mat.supr-con↗

arXiv2022

Detailed structural and topological analysis of SnBi2Te4 single crystal

We report herein the successful synthesis of the topological material SnBi2Te4 in single-crystal form. Phase purity and unidirectional growth are evident from X-ray diffraction (XRD) patterns acquired from a powdered sample and a crystal flake. The crystalline morphology has also been visualized by acquiring a field-emission scanning electron microscope (FESEM) image. The crystal has been thoroughly characterized by means of Raman spectroscopy and X ray photoelectron spectroscopy (XPS) measurements. The topological properties of SnBi2Te4 have been probed through magneto-transport measurements. SnBi2Te4 has been found to exhibit a small but non-saturating magneto-resistance (MR) up to 12 T. The low-field magnetoconductivity (MC) of SnBi2Te4 at 2 K can be well explained through the Hikami Larkin Nagaoka (HLN) formalism, which confirms the presence of a weak anti-localization (WAL) effect in its crystal. Moreover, the non-trivial topological character has been evidenced through first-principles calculations using density functional theory (DFT), with and without spin-orbit coupling (SOC) protocols. A significant change in the bulk electronic band structure is observed upon the inclusion of SOC parameters, signifying the topological properties of SnBi2Te4. Its topological non-trivial character has also been verified through the calculation of Z2 invariants and the surface states spectrum in the (111) plane.

cond-mat.mtrl-sci↗

arXiv2022

Weak antilocalization and ferromagnetism in magnetic Weyl semimetal Co3Sn2S2

Here we report successful synthesis of single crystalline magnetic Weyl semimetal Co3Sn2S2. The synthesized crystal is characterized through various tools viz. X-ray diffraction, field emission electron microscopy and X-ray photoelectron spectroscopy. A clear ferromagnetic transition is observed in magnetization and heat capacity at around 175K, which is further verified through electrical transport measurements. Hysteresis is observed in R-T measurements in cooling and warming cycle, showing the presence of first order phase transition and charge ordering in the synthesized sample. The synthesized Co3Sn2S2 exhibits high magnetoresistance of around 230% at 2K. The transport phenomenon in synthesized Co3Sn2S2 appears to have contributions from topological surface states at low temperature below say 70 K, and above that the same is found to be strongly dependent on its bulk magnetic state. Magnetoconductivity data at low fields of up to plus minus 1T (Tesla) is fitted with Hikami Larkin Nagaoka model, which shows the presence of weak antilocalization effect in synthesized Co3Sn2S2 crystal at low temperatures below 30K.

cond-mat.mtrl-sci↗

arXiv2022

Large amplitude bidirectional anisotropy of cosmic-ray intensity observed with world-wide networks of ground-based neutron monitors and muon detectors in November, 2021

We analyze the cosmic-ray variations during a significant Forbush decrease observed with world-wide networks of ground-based neutron monitors and muon detectors during November 3-5, 2021. Utilizing the difference between primary cosmic-ray rigidities monitored by neutron monitors and muon detectors, we deduce the rigidity spectra of the cosmic-ray density (or omnidirectional intensity) and the first- and second-order anisotropies separately, for each hour of data. A clear two-step decrease is seen in the cosmic-ray density with the first $\sim2\%$ decrease after the interplanetary shock arrival followed by the second $\sim5\%$ decrease inside the magnetic flux rope (MFR) at 15 GV. Most strikingly, a large bidirectional streaming along the magnetic field is observed in the MFR with a peak amplitude of $\sim5\%$ at 15 GV which is comparable to the total density decrease inside the MFR. The bidirectional streaming could be explained by adiabatic deceleration and/or focusing in the expanding MFR, which have stronger effects for pitch angles near 90$^\circ$, or by selective entry of GCRs along a leg of the MFR. The peak anisotropy and density depression in the flux rope both decrease with increasing rigidity. The spectra vary dynamically indicating that the temporal variations of density and anisotropy appear different in neutron monitor and muon detector data.

astro-ph.HE↗