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Martino Poggio

Publications and source records attributed to Martino Poggio.

At least 19 recordsLinked to original sources

Spatial resolution and point spread function of high-resolution scanning SQUID microscopy probes

Superconducting quantum interference devices (SQUIDs) show exceptional sensitivity to magnetic flux. In scanning SQUID microscopy (SSM), SQUID size and its distance to the sample are minimized in order to map weak magnetic fields with best possible spatial resolution. SQUID-on-lever (SOL) architectures have proven especially effective as SSM probes due to their small sensor size, robustness, and ease of integration with conventional atomic force microscopy hardware. In order to optimize magnetic microscopy carried out with SOL probes and to accurately reconstruct the magnetic fields that they measure, it is essential to know their point spread function (PSF). The size and shape of this PSF are determined by magnetic flux focusing effects, which depend on the characteristic length-scales of the superconductor and the sensor geometry. By simulating the coupling to sources of magnetic flux, this work provides a mathematical description of the SOL PSF, which contains a full description of the probe's magnetic sensitivity and spatial resolution. We then use measurements of a single magnetic skyrmion to measure the magnetic flux response of a real SOL. We demonstrate excellent agreement with flux responses that are obtained from simulations, thereby confirming the calculated PSF and spatial resolution.

cond-mat.supr-con↗

Unresolved-Sideband Optomechanics with Hexagonal Boron Nitride: Induced Transparency, Gain, and Frequency Combs

Optomechanically induced transparency (OMIT) is usually modeled and studied in the resolved-sideband regime, but many compact microcavity platforms operate in the unresolved-sideband limit $(κ\gg Ω_m)$. Here we investigate OMIT in this regime using a tunable fiber-based Fabry-Perot microcavity coupled to a suspended hexagonal boron nitride (hBN) drum resonator in a membrane-in-the-middle geometry. The system achieves a large single-photon coupling rate of $g_0/2π\sim 180$ kHz and exhibits strong radiation-pressure backaction. By measuring OMIT spectra as a function of pump power and cavity detuning, we observe a crossover from a transparency-like dip to a gain feature in the reflected response. These maps are quantitatively reproduced by the full linearized optomechanical response, demonstrating the breakdown of the standard rotating-wave approximation used in the resolved-sideband limit. Finally, we drive the system into a nonlinear regime to generate optomechanical frequency combs. These results establish hBN fiber-cavities as a versatile architecture for unresolved-sideband optomechanics, nonlinear dynamics, and hybrid device integration.

physics.optics↗

Imaging short- and long-range magnetic order in a quantum anomalous Hall insulator

The quantum anomalous Hall effect has been observed in several magnetically doped topological insulators, where its robustness and macroscopic magnetization properties have been taken to suggest the presence of long-range ferromagnetic order. However, experiments in such systems have found evidence for both long- and short-range order, leaving the precise nature of the magnetism in these systems unclear. Here, we use scanning superconducting quantum interference device microscopy to study magnetic domains in V-doped (Bi,Sb)$_2$Te$_3$ exhibiting a quantum anomalous Hall effect with precise quantization. By imaging stray magnetic fields as a function of applied field, we map the formation and evolution of domains through magnetic reversal. We reconstruct the magnetization configuration underlying the measured stray field and find that magnetic domains and crystallographic grains are of similar size. Moreover, magnetic reversal is found to occur through domain expansion, typical of ferromagnets, rather than through nucleation at random sites. Our measurements thus reveal a coexistence of both local magnetic interactions within crystallographic grains and long-range ferromagnetic coupling between grains. This behavior in V-doped (Bi,Sb)$_2$Te$_3$ is markedly distinct from that previously reported for Cr-doped (Bi,Sb)$_2$Te$_3$.

cond-mat.mtrl-sci↗

Magnetic properties of an individual Magnetospirillum gryphiswaldense cell

Many bacteria share the fascinating ability to sense Earth's magnetic field -- a process known as magnetotaxis. These bacteria synthesize magnetic nanoparticles, called magnetosomes, within their own cell body and arrange them to form a linear magnetic chain. The chain, which behaves like a compass needle, aligns the microorganisms with the geomagnetic field. Here, we measure the magnetic hysteresis of an individual bacterium of the species Magnetospirillum gryphiswaldense via ultrasensitive torque magnetometry. These measurements, in combination with transmission electron microscopy and micromagnetic simulations, reveal the magnetic configurations of the magnetosomes, their progression as a function of applied field, as well as the total remanent magnetic moment and effective magnetic anisotropy of a chain within a single bacterium. Knowledge of magnetic properties is crucial both for understanding the mechanisms behind magnetotaxis and for the design of systems exploiting magnetotactic bacteria in biomedical applications.

physics.bio-ph↗

Measuring high field gradients of cobalt nanomagnets in a spin-mechanical setup

Hybrid systems composed of a single nitrogen-vacancy center spin magnetically coupled to a macroscopic mechanical resonator constitute promising platforms for the realization of quantum information protocols and for quantum sensing applications. The magnetic structure that mediates the interaction must ensure high field gradients while preserving the spin and mechanical properties. We present a spin-mechanical setup built around a cobalt nanomagnet grown with focused electron beam-induced deposition. The magnetic structure is fully characterized, and a maximum gradient of $170\,\mathrm{kT/m}$ is directly measured at a spin-oscillator distance of a few hundred nanometers. Spin coherence was preserved at the value of $20\,\mathrm{ μs}$ up to a gradient of $25\,\mathrm{kT/m}$. The effect of the mechanical motion onto the spin dynamics was observed, thus signifying the presence of spin-mechanics coupling. Given the noninvasive nature of the nanomagnet deposition process, we foresee the adoption of such structures in hybrid platforms with high-quality factor resonators, in the "magnet on oscillator" configuration.

cond-mat.mes-hall↗

Advanced SQUID-on-lever scanning probe for high-sensitivity magnetic microscopy with sub-100-nm spatial resolution

Superconducting quantum interference devices (SQUIDs) are exceptionally sensitive magnetometers capable of detecting weak magnetic fields. Miniaturizing these devices and integrating them onto scanning probes enables high-resolution imaging at low-temperature. Here, we fabricate nanometer-scale niobium SQUIDs with inner-loop sizes down to 10 nm at the apex of individual planar silicon cantilevers via a combination of wafer-scale optical lithography and focused-ion-beam (FIB) milling. These robust SQUID-on-lever probes overcome many of the limitations of existing devices, achieving spatial resolution better than 100 nm, magnetic flux sensitivity of $0.3~μΦ_0/\sqrt{\rm{Hz}}$, and operation in magnetic fields up to about 0.5 T at 4.2 K. Nanopatterning via Ne- or He-FIB allows for the incorporation of a modulation line for coupling magnetic flux into the SQUID or a third Josephson junction for shifting its phase. Such advanced functionality, combined with high spatial resolution, large magnetic field range, and the ease of use of a cantilever-based scanning probe, extends the applicability of scanning SQUID microscopy to a wide range of magnetic, normal conducting, superconducting, and quantum Hall systems. We demonstrate magnetic imaging of skyrmions at the surface of bulk Cu$_2$OSeO$_3$. Analysis of the point spread function determined from imaging a single skyrmion yields a full-width-half-maximum of 87 nm. Moreover, we image modulated magnetization patterns with a period of 65 nm.

cond-mat.supr-con↗

Magnetically-controlled Vortex Dynamics in a Ferromagnetic Superconductor

Ferromagnetic superconductors are exceptionally rare because the strong ferromagnetic exchange field usually destroys singlet superconductivity. EuFe$_2$(As$_{1-x}$P$_x$)$_2$, an iron-based superconductor with a maximum critical temperature of 25 K, uniquely exhibits full coexistence with ferromagnetic order below $T_\mathrm{FM}$ $\simeq$ $19$ K. The interplay leads to narrowing of ferromagnetic domains at higher temperatures and spontaneous nucleation of vortices/antivortices at lower temperatures. Here we demonstrate how the underlying magnetic structure controls the superconducting vortex dynamics in applied magnetic fields. Just below $T_\mathrm{FM}$ we observe a pronounced peak in the creep activation energy, and magnetic force microscopy measurements reveal the presence of very closely-spaced ($w\ll λ$) vortex clusters. We attribute these observations to the formation of vortex polarons for which we present a theoretical description. In contrast, we link strong magnetic irreversibility at low temperatures to a critical current governed by giant flux creep over an activation barrier for vortex-antivortex annihilation near domain walls. Our work suggests new routes for the magnetic enhancement of vortex pinning with important applications in high-current conductors.

cond-mat.supr-con↗

Imaging magnetic switching in orthogonally twisted stacks of a van der Waals antiferromagnet

Stacking van der Waals magnets holds promise for creating new hybrid materials with properties that do not exist in bulk materials. Here we investigate orthogonally twisted stacks of the van der Waals antiferromagnet CrSBr, aiming to exploit an extreme misalignment of magnetic anisotropy across the twisted interface.Using nitrogen-vacancy centre microscopy, we construct vector maps of the magnetisation, and track their evolution under an external field, in a range of twisted compensated and uncompensated configurations differing by the number of layers. We show that twisted stacking consistently modifies the local magnetic switching behaviour of constituent flakes, and that these modifications are spatially non-uniform. In the case of compensated component flakes (even number of layers), we demonstrate that the combination of dipolar coupling and stacking-induced strain can reduce the switching field by over an order of magnitude. Conversely, in uncompensated component flakes (odd number of layers), we observe indications of a non-zero interlayer exchange interaction between twisted flakes during magnetization reversal, which can persistently modify magnetic order. This work highlights the importance of spatial imaging in investigating stacking-induced magnetic effects, particularly in the case of twistronics where spatial variation is expected and can be conflated with structural imperfections.

cond-mat.mes-hall↗

Simulation and measurement of stray fields for the manipulation of spin-qubits in one- and two-dimensional arrays

The inhomogeneous magnetic stray field of micromagnets has been extensively used to manipulate electron spin qubits. By means of micromagnetic simulations and scanning superconducting quantum interference device microscopy, we show that the polycrystallinity of the magnet and non-uniform magnetization significantly impact the stray field and corresponding qubit properties. We find that the random orientation of the crystal axis in polycrystalline Co magnets alters the qubit frequencies by up to 0.5 GHz, compromising single qubit addressability and single gate fidelities. We map the stray field of Fe micromagnets with an applied magnetic field of up to 500 mT (mimicking conditions when operating qubits), finding field gradients above 1 mT/nm. The measured gradients and the lower magnetocrystalline anisotropy of Fe demonstrate the advantage of using Fe instead of Co for magnets in spin qubit devices. These properties of Fe also enabled us to design a 2D arrangement of nanomagnets for driving spin qubits distributed on a 2D lattice.

cond-mat.mes-hall↗

Imaging strain-controlled magnetic reversal in thin CrSBr

Two-dimensional materials are extraordinarily sensitive to external stimuli, making them ideal for studying fundamental properties and for engineering devices with new functionalities. One such stimulus, strain, affects the magnetic properties of the layered magnetic semiconductor CrSBr to such a degree that it can induce a reversible antiferromagnetic-to-ferromagnetic phase transition. Given the pervasiveness of non-uniform strain in exfoliated two-dimensional magnets, it is crucial to understand its impact on their magnetic behavior. Using scanning SQUID-on-lever microscopy, we directly image the effects of spatially inhomogeneous strain on the magnetization of layered CrSBr as it is polarized by a field applied along its easy axis. The evolution of this magnetization and the formation of domains is reproduced by a micromagnetic model, which incorporates the spatially varying strain and the corresponding changes in the local interlayer exchange stiffness. The observed sensitivity to small strain gradients along with similar images of a nominally unstrained CrSBr sample suggest that unintentional strain inhomogeneity influences the magnetic behavior of exfoliated samples and must be considered in the design of future devices.

cond-mat.mes-hall↗

Nanoscale magnetism and magnetic phase transitions in atomically thin CrSBr

Since their first observation in 2017, atomically thin van der Waals (vdW) magnets have attracted significant fundamental, and application-driven attention. However, their low ordering temperatures, $T_c$, sensitivity to atmospheric conditions and difficulties in preparing clean large-area samples still present major limitations to further progress. The remarkably stable high-$T_c$ vdW magnet CrSBr has the potential to overcome these key shortcomings, but its nanoscale properties and rich magnetic phase diagram remain poorly understood. Here we use single spin magnetometry to quantitatively characterise saturation magnetization, magnetic anisotropy constants, and magnetic phase transitions in few-layer CrSBr by direct magnetic imaging. We show pristine magnetic phases, devoid of defects on micron length-scales, and demonstrate remarkable air-stability down the monolayer limit. We address the spin-flip transition in bilayer CrSBr by direct imaging of the emerging antiferromagnetic (AFM) to ferromagnetic (FM) phase wall and elucidate the magnetic properties of CrSBr around its ordering temperature. Our work will enable the engineering of exotic electronic and magnetic phases in CrSBr and the realisation of novel nanomagnetic devices based on this highly promising vdW magnet.

cond-mat.mes-hall↗

Roadmap on Nanoscale Magnetic Resonance Imaging

The field of nanoscale magnetic resonance imaging (NanoMRI) was started 30 years ago. It was motivated by the desire to image single molecules and molecular assemblies, such as proteins and virus particles, with near-atomic spatial resolution and on a length scale of 100 nm. Over the years, the NanoMRI field has also expanded to include the goal of useful high-resolution nuclear magnetic resonance (NMR) spectroscopy of molecules under ambient conditions, including samples up to the micron-scale. The realization of these goals requires the development of spin detection techniques that are many orders of magnitude more sensitive than conventional NMR and MRI, capable of detecting and controlling nanoscale ensembles of spins. Over the years, a number of different technical approaches to NanoMRI have emerged, each possessing a distinct set of capabilities for basic and applied areas of science. The goal of this roadmap article is to report the current state of the art in NanoMRI technologies, outline the areas where they are poised to have impact, identify the challenges that lie ahead, and propose methods to meet these challenges. This roadmap also shows how developments in NanoMRI techniques can lead to breakthroughs in emerging quantum science and technology applications.

cond-mat.mes-hall↗

Coupling trapped ions to a nanomechanical oscillator

Cold ions in traps are well-established, highly controllable quantum systems with a wide variety of applications in quantum information, precision spectroscopy, clocks and chemistry. Nanomechanical oscillators are used in advanced sensing applications and for exploring the border between classical and quantum physics. Here, we report on the implementation of a hybrid system combining a metallic nanowire with laser-cooled ions in a miniaturised ion trap. We demonstrate resonant and off-resonant coupling of the two systems and the coherent motional excitation of the ion by the mechanical drive of the nanowire. The present results open up avenues for mechanically manipulating the quantum motion of trapped ions, for the development of ion-mechanical hybrid quantum systems and for the sympathetic cooling of mechanical systems by trapped ions and vice versa.

physics.atom-ph↗

Visualizing thickness-dependent magnetic textures in few-layer $\text{Cr}_2\text{Ge}_2\text{Te}_6$

Magnetic ordering in two-dimensional (2D) materials has recently emerged as a promising platform for data storage, computing, and sensing. To advance these developments, it is vital to gain a detailed understanding of how the magnetic order evolves on the nanometer-scale as a function of the number of atomic layers and applied magnetic field. Here, we image few-layer $\text{Cr}_2\text{Ge}_2\text{Te}_6$ using a combined scanning superconducting quantum interference device and atomic force microscopy probe. Maps of the material's stray magnetic field as a function of applied magnetic field reveal its magnetization per layer as well as the thickness-dependent magnetic texture. Using a micromagnetic model, we correlate measured stray-field patterns with the underlying magnetization configurations, including labyrinth domains and skyrmionic bubbles. Comparison between real-space images and simulations demonstrates that the layer dependence of the material's magnetic texture is a result of the thickness-dependent balance between crystalline and shape anisotropy. These findings represent an important step towards 2D spintronic devices with engineered spin configurations and controlled dependence on external magnetic fields.

cond-mat.mes-hall↗

Exchange energy of the ferromagnetic electronic ground-state in a monolayer semiconductor

Mobile electrons in the semiconductor monolayer-MoS$_2$ form a ferromagnetic state at low temperature. The Fermi sea consists of two circles, one at the $K$-point, the other at the $\tilde{K}$-point, both with the same spin. Here, we present an optical experiment on gated MoS$_2$ at low electron-density in which excitons are injected with known spin and valley quantum numbers. The resulting trions are identified using a model which accounts for the injection process, the formation of antisymmetrized trion states, electron-hole scattering from one valley to the other, and recombination. The results are consistent with a complete spin polarization. From the splittings between different trion states, we measure the exchange energy, $Σ$, the energy required to flip a single spin within the ferromagnetic state, as well as the intervalley Coulomb exchange energy, $J$. We determine $Σ=11.2\,$meV and $J=5\,$meV at $n=1.5 \times 10^{12}\,$cm$^{-2}$, and find that $J$ depends strongly on the electron density, $n$.

cond-mat.str-el↗

Scanning NV magnetometry of focused-electron-beam-deposited cobalt nanomagnets

Focused-electron-beam-induced deposition is a promising technique for patterning nanomagnets for spin qubit control in a single step. We fabricate cobalt nanomagnets in such a process, obtaining cobalt contents and saturation magnetizations comparable to or higher than those typically obtained using electron-beam lithography. We characterize the nanomagnets using transmission electron microscopy and image their stray magnetic field using scanning NV magnetometry, finding good agreement with micromagnetic simulations. The magnetometry reveals the presence of magnetic domains and halo side-deposits, which are common for this fabrication technique. Finally, we estimate dephasing times for electron spin qubits in the presence of disordered stray fields due to these side-deposits.

cond-mat.mtrl-sci↗

Mechanical mode imaging of a high-Q hybrid hBN/Si$_3$N$_4$ resonator

We image and characterize the mechanical modes of a 2D drum resonator made of hBN suspended over a high-stress Si$_3$N$_4$ membrane. Our measurements demonstrate hybridization between various modes of the hBN resonator and those of the Si$_3$N$_4$ membrane. The measured resonance frequencies and spatial profiles of the modes are consistent with finite-element simulations based on an idealized geometry. Spectra of the thermal motion reveal that, depending on the degree of hybridization with modes of the heavier and higher-quality-factor Si$_3$N$_4$ membrane, the quality factors and the motional mass of the hBN drum modes can be shifted by orders of magnitude. This effect could be exploited to engineer hybrid drum/membrane modes that combine the low motional mass of 2D materials with the high quality factor of Si$_3$N$_4$ membranes for optomechanical or sensing applications.

cond-mat.mes-hall↗

Electron-beam lithography of nanostructures at the tips of scanning probe cantilevers

We developed a process to fabricate nanoscale metallic gate electrodes on scanning probe cantilevers, including on the irregular surface of protruding cantilever tips. The process includes a floating-layer technique to coat the cantilevers in electron-beam resist. We demonstrate gate definition through a lift-off process, as well as through an etching process. The cantilevers maintain a high force sensitivity after undergoing the patterning process. Our method allows the patterning of nanoscale devices on fragile scanning probes, extending their functionality as sensors.

physics.ins-det↗