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Mingliang Tian

Publications and source records attributed to Mingliang Tian.

At least 19 recordsLinked to original sources

N\'eel-Vector Control of the Josephson Diode Effect in $\mathcal{PT}$-symmetric Antiferromagnets

The interplay of superconductivity and magnetism gives rise to rich phenomena in Josephson junctions. In this Letter, we study Josephson junctions formed by conventional $s$-wave superconductors and a $\PT$-symmetric collinear antiferromagnet modeled on CuMnAs. Using microscopic modeling and symmetry analysis, we show that these junctions exhibit both the Josephson diode effect and $\varphi_{0}$-junction states. Remarkably, both effects are controlled by the N\'eel vector: rotating it by $90^{\circ}$ switches off both, while reversing it switches the diode polarity. To reveal the microscopic mechanism, we develop a channel-resolved scattering theory that accurately captures the anomalous phases and establishes the exact condition for the diode effect. The interplay of the channel current-phase relations yields a sizable diode efficiency, tunable by both the magnitude and direction of the exchange field. Furthermore, a Green-function reduction identifies a single renormalized $\PT$-degenerate band as the transport carrier and precisely reproduces the full current amplitudes. Our work establishes $\PT$-symmetric antiferromagnets as versatile platforms for field-free, highly tunable Josephson diodes and $\varphi_{0}$ junctions.

cond-mat.supr-con

Nearly Isotropic Vortex Solid in $\mathbf{(La,Pr)_{3}Ni_{2}O_{7}}$ Thin Films

The discovery of superconductivity in bulk bilayer nickelates has established a new platform for exploring high-$T_c$ superconductivity beyond the cuprates. The role of the Ni $3d_{z^2}$-derived $\gamma$ band in the superconductivity of bilayer nickelates remains unresolved. By performing simultaneous resistance and diamagnetism measurements on (La,Pr)$_3$Ni$_2$O$_7$ thin films, we map the vortex melting phase diagram for both in-plane and out-of-plane magnetic fields. For $H\parallel c$, the geometric confinement effect gives rise to pancake vortices. Remarkably, the anisotropy parameter of the vortex melting field $\gamma_{H_m} \equiv H_m^{ab}/H_m^c$ decreases monotonically with decreasing temperature and approaches unity at low temperatures. Within the anisotropic Ginzburg--Landau scaling, $H_m^{ab}/H_m^c = \sqrt{\rho_s^{ab}/\rho_s^c}$ tracks the superfluid-density anisotropy. Such a vortex solid implies a nearly isotropic superfluid density, which is irreconcilable with the strictly two-dimensional $3d_{x^2-y^2}$-derived bands, but naturally explained by a substantial interlayer superfluid contribution from the $3d_{z^2}$-derived $\gamma$ band. Our results provide thermodynamic evidence for a substantial contribution of the $\gamma$ band to superconductivity in bilayer nickelate thin films.

cond-mat.supr-con

A Unified Symmetry Framework For In-plane Anomalous Hall effect

The in-plane anomalous Hall effect (IPAHE), driven by an in-plane net magnetization or an applied magnetic field, challenges the conventional anomalous Hall paradigm. Despite growing interest, a unified symmetry principle governing these phenomena has remained elusive. Here, we establish a comprehensive symmetry framework that bridges the spin space group, which dictates the magnetic geometry, with the magnetic space group, which governs the anomalous Hall response. We show that spontaneous IPAHE can emerge in ferromagnets when spin-orbit-coupling-induced spin-group symmetry breaking permits additional net magnetization directions. For field-induced IPAHE, we analyze how an applied magnetic field reduces the symmetries of all 122 magnetic point groups and identify 54 groups that support IPAHE. Our framework naturally predicts IPAHE in a broad class of unconventional magnets, including altermagnets and odd-parity magnets. In particular, symmetry analysis reveals characteristic one-, two-, or three-fold angular harmonics of the Hall conductance under an in-plane rotating field, providing a symmetry-resolved fingerprint for unconventional magnetism. Using this framework, we screen the MAGNDATA database and identify candidate materials supporting spontaneous or field-induced IPAHE, encompassing ferromagnets, antiferromagnets, and unconventional magnets. Finally, we validate the symmetry predictions through first-principles calculations for two representative materials.

cond-mat.mtrl-sci

Ferrimagnetic Skyrmions in a Tetragonal Mn1.9Co0.1Sb Single Crystal at Room Temperature

The development of room temperature small-sized ferrimagnetic skyrmion materials is significant for topological spintronic device applications. As a room temperature ferrimagnetic material, the tetragonal Mn1.9Co0.1Sb crystal exhibits multiple phase transitions, including spin reorientation transitions. However, the magnetic spin textures and their evolution mechanisms during magnetic phase transitions in Mn1.9Co0.1Sb crystals remain unexplored. Using Lorentz transmission electron microscopy, we discovered and verified dipolar skyrmion behavior and its magnetic evolution at room temperature. We established a stable phase diagram of magnetic textures as functions of temperature and magnetic field, while also investigating the evolution mechanisms of spin textures across multiple temperature-induced magnetic phase transitions. Through micromagnetic simulations, a ferrimagnetic configuration with in-plane ferromagnetic coupling and interlayer antiferromagnetic arrangement was established, which stands in contrast to synthetic ferrimagnetic/antiferromagnetic systems that exhibit interlayer antiferromagnetic coupling via the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. We determined that the intrinsic frequency of ferrimagnetic skyrmions can reach the THz regime due to strong interlayer antiparallel exchange interactions. These findings highlight the diversity of room temperature ferrimagnetic skyrmion regulation behaviors in Mn1.9Co0.1Sb and their dynamic evolution characteristics, opening new avenues for developing novel spintronic devices with enhanced functionalities capable of operating under ambient conditions.

cond-mat.mtrl-sci

Enhanced Curie temperature and room-temperature 50-nm skyrmions achieved in hexagonal ferromagnet Mn5Ge3+x synthesized via a high-pressure method

The development of new high-temperature ultrasmall-size skyrmion materials holds immense significance for the promising applications of topological spintronic devices. In this study, we demonstrate that a high-pressure synthesis technique can significantly elevate the Curie temperature of Mn5Ge3+x crystals, from 294 K to 350 K. This enhancement is attributed to the combined effects of lattice contraction and increased Ge content, the conclusion supported by Density Functional Theory calculations. Additionally, our real-space magnetic imaging reveals the stability of dipolar skyrmions with diameters of approximately 50 nm at room temperature. Our micromagnetic simulations closely replicate the diverse experimental topological magnetic textures observed. Furthermore, magnetotransport measurements indicate the potential for the electrical distinction between various topological magnetic textures in skyrmion-based devices. We also report deterministic manipulations on single dipolar skyrmions in confined nanostructures by using in-plane currents. The observation, electrical manipulation, and electrical detection of room-temperature ultrasmall topological magnetic textures underscore the potential of Mn5Ge3+x as a promising platform for spintronic device applications.

cond-mat.mtrl-sci

Current-induced creation and dynamics of embedded magnetic skyrmion bags

Magnetic skyrmion bags-vortex-like structures hosting multiple skyrmions with tunable topological charge (Q)-hold significant promise for next-generation spintronic computing. However, while their creation using magnetic fields has been demonstrated, their direct electrical generation remains an outstanding challenge. Here, we report the direct current-induced formation and manipulation of embedded skyrmion bags in a FeGe nanoplate under zero magnetic field. Using in-situ Lorentz transmission electron microscopy, we capture the transformation of a distorted helical ground state into embedded skyrmion bags with diverse configurations, driven by nanosecond current pulses. Theoretical analysis indicates that this process is driven by the spin-transfer-torque-induced fracture of the helical state. Furthermore, we demonstrate electrically-induced transitions between skyrmion bags of different Q, leading to the stabilization of complex three-dimensional topological structures, including experimental signatures of magnetic monopoles and bobbers. Our work establishes a foundation for all-electrical control of high-Q topological spin textures and topological defects, paving the way for their application in functional spintronic devices.

cond-mat.mes-hall

Majorana vortex phases in time-reversal invariant higher-order topological insulators and topologically trivial insulators

Majorana vortex phases have been extensively studied in topological materials with conventional superconducting pairing. Inspired by recent experimental progress in realizing time-reversal invariant higher-order topological insulators (THOTIs) and inducing superconducting proximity effects, we investigate Majorana vortex phases in these systems. We construct THOTIs as two copies of a topological insulator (TI) with time-reversal symmetry-preserving mass terms that anisotropically gap the surface states. We find that these mass terms have a negligible impact on the vortex phase transitions of double TIs when treated as perturbations, and no additional topological phase transitions are induced. Consequently, $\mathbb{Z}_2$-protected Majorana vortex end modes (MVEMs) emerge when the chemical potential lies between the critical chemical potentials $μ_c^{(1)}$ and $μ_c^{(2)}$ of the two TI vortex phase transitions. We demonstrate this behavior across multiple THOTI models, including rotational symmetry-protected THOTI, inversion symmetry-protected THOTI, rotational and inversion symmetries-protected THOTI bismuth, and extrinsic THOTI. Remarkably, MVEMs persist even when all surfaces are gapped with the same sign, rendering the system topologically trivial in both first- and second-order classifications. Our findings establish that MVEMs can be realized in time-reversal invariant systems with fully gapped surfaces, encompassing both topologically nontrivial and trivial insulators, thus significantly broadening the solid state material platforms for hosting Majorana vortex phases.

cond-mat.supr-con

Unconventional Magnetism: Symmetry Classification, Hybrid-parity and Unconstrained-parity Classes

Unconventional magnetism has emerged as a transformative frontier in condensed matter physics. Such phases are characterized by substantial non-relativistic spin splitting (NSS) in symmetry-compensated magnets. They have been classified by the parity of their spin textures under momentum inversion, leading to the paradigms of altermagnets (even-parity) and odd-parity magnets. However, the full symmetry landscape remains largely unexplored. In this Letter, we present a systematic classification framework for unconventional magnetism based on the representation theory of the spin textures and the associated parity properties. Within this framework, we predict two previously unidentified classes beyond the established pure-parity categories: hybrid-parity magnets (HPMs) and unconstrained-parity magnets (UPMs), where the spin textures exhibit contrasting parities among their Cartesian components and the parity of the spin textures is ill-defined, respectively. We derive universal symmetry criteria that categorize HPMs into three distinct types. Importantly, by combining the spin splitting characteristics of altermagnets and odd-parity magnets, HPMs can enable the coexistence of the spin current and Edelstein effects. Taking FePO4 as an example, we perform first-principles calculations to demonstrate this coexistence. Finally, we discuss the potential applications of HPMs in spintronic devices. Our work provides a comprehensive symmetry classification of unconventional magnetism and establishes HPMs as a promising platform for multi-functional spintronics.

cond-mat.mtrl-sci

High-Pressure Tuning of Electrical Transport in Freestanding Oxide Films

Electrical transport in oxide thin films under high pressure remains largely unexplored due to the lack of a universal experimental strategy. Here we develop an approach that enables high-pressure transport measurements in freestanding oxide films by enhancing their mechanical robustness and integrating them with nanoscale high-pressure devices. As a demonstration, we investigate the resistivity of perovskite SrIrO3 films under hydrostatic pressure and uncover a pressure-driven semimetal-insulator transition near 2.5 GPa, followed by an insulator-metal transition around 9 GPa. In the monolayer limit, SrIrO3 remains insulating and robust against pressure up to 5.5 GPa. The contrasting pressure-dependent phase diagrams of three- and two-dimensional iridates reveal a strong interplay between dimensionality and hydrostatic pressure in correlated oxides. Our work establishes a general platform for exploring pressure-driven phenomena in low-dimensional quantum materials.

cond-mat.mtrl-sci

Electrical Transport and Quantum Oscillations in the Metallic Spin Supersolid EuCo2Al9

The discovery of spin supersolid and its giant magnetocaloric effect has opened a new arena in frustrated quantum magnets and cutting-edge cryogenics. The intermetallic EuCo2Al9 (ECA), for the first time, extends this intriguing phase from Mott insulators to a highly conductive metal [1]. In this work, we systematically study the electrical transport properties of ECA, where itinerant electrons serve as a sensitive probe for the spin supersolid states. We observe anomalies both in the temperature-dependent resistivity and field-dependent magnetoresistance and Hall signals, which are attributed to response of electrons to the Eu2+ spins and their fluctuations. Moreover, Shubnikov-de Haas quantum oscillations at high magnetic field reveal pronounced band splitting in the spin polarized state. Our results reveal an intimate correspondence between electrical transport and magnetic transitions in ECA, deepening the understanding of this metallic spin supersolid.

cond-mat.str-el

Hidden Zeeman Field in Odd-Parity Magnets: An Ideal Platform for Topological Superconductivity

Odd-parity magnets (OPMs) have emerged as a fundamental class of unconventional magnetisms, characterized by time-reversal-preserving non-relativistic spin splitting (NSS). Despite growing interest, the fundamental understanding of OPMs remains critically incomplete, as previous studies have focused exclusively on NSS while overlooking the intrinsically broken time-reversal symmetry ($\mathcal{T}$) inherent to magnetic order. In this work, we reveal that OPMs universally host a hidden Zeeman field rooted in this $\mathcal{T}$-breaking, which fundamentally reshapes their band structure. Through an analytical $f$-wave magnet model, we show that NSS microscopically originates from an emergent gauge field, manifesting as a real-space spin loop current order. Crucially, the large NSS (eV scale) enables conventional superconductivity to coexist robustly with the hidden Zeeman field, with Zeeman splitting reaches hundreds of meV. This unique band structure establishes OPMs as an ideal platform for topological superconductors (TSCs), supporting large topological regions. Based on OPMs, we engineer a series of TSCs hosting distinct Majorana boundary modes, including unidirectional Majorana edge states. Our work corrects a fundamental misconception about OPMs and establishes them as a versatile platform for field-free and robust TSCs.

cond-mat.supr-con

Deterministic Switching of the Néel Vector by Asymmetric Spin Torque

Néel vector, the order parameter of collinear antiferromagnets, serves as a state variable in associated antiferromagnetic (AFM) spintronic devices to encode information. A deterministic switching of Néel vector is crucial for the write-in operation, which, however, remains a challenging problem in AFM spintronics. Here we demonstrate, based on analytical derivation and macro-spin simulations, that Néel vector switching can be generally achieved via a current-induced spin torque, provided the spin accumulations responsible for this torque are non-identical between opposite sublattices. This condition occurs widely in AFM films, as symmetry equivalence between sublattice-dependent spin accumulations is usually absent, allowing unequal spin accumulations induced by Edelstein effect or a spin current. Unlike previously studied spin torques induced by uniform or staggered spin accumulations -- where either the field-like or damping-like component dominates exclusively -- the asymmetric spin torque features cooperative contributions from both components, leading to Néel vector dynamics that are fundamentally distinct from previous expectations. Crucially, the static states stabilized by the asymmetric spin torque enable versatile Néel vector switching strategies -- field-free spin-transfer torque switching during current application, as well as field-free or field-assisted spin-orbit torque switching after the current pulse -- demonstrating that established spin torque techniques from ferromagnetic spintronics can be directly adapted to AFM systems, a capability absent in previous theoretical frameworks. Our work establishes a general mechanism for current-induced Néel vector switching, which is in principle feasible for all collinear antiferromagnets, and thus paves the route to realize efficient writing in AFM spintronics.

cond-mat.mtrl-sci

Interface-Controlled Antiferromagnetic Tunnel Junctions based on a metallic van der Waals A-type Antiferromagnet

Magnetic tunnel junctions (MTJs) are crucial components in high-performance spintronic devices. Traditional MTJs rely on ferromagnetic (FM) materials but significant improvements in speed and packing density could be enabled by exploiting antiferromagnetic (AFM) compounds instead. Here, we report all-collinear AFM tunnel junctions (AFMTJs) fabricated with van der Waals A-type AFM metal (Fe0.6Co0.4)5GeTe2 (FCGT) electrodes and nonmagnetic semiconducting WSe2 tunnel barriers. The AFMTJ heterostructure device achieves a tunneling magnetoresistance (TMR) ratio of up to 75% in response to magnetic field switching. Our results demonstrate that the TMR exclusively emerges in the AFM state of FCGT, rather than during the AFM-to-FM transition. By engineering FCGT electrodes with either even- or odd-layer configurations, volatile or non-volatile TMR could be selected, consistent with an entirely interfacial effect. TMR in the even-layer devices arose by Néel vector switching. In the odd-layer devices, TMR stemmed from interfacial spin-flipping. Experimental and theoretical analyses reveal a new TMR mechanism associated with interface-driven spin-polarized transport, despite the spin-independent nature of bulk FCGT. Our work demonstrates that collinear AFMTJs can provide comparable performance to conventional MTJs and introduces a new paradigm for AFM spintronics, in which the spin-dependent properties of AFM interfaces are harnessed.

cond-mat.mes-hall

Deterministic Electrical Control of Single Magnetic Bubbles in Nanostructured Cells

Localized particle-like spin textures have been found to exhibit emergent electromagnetic properties, which hold promise for the development of intriguing spintronic devices. Among these textures, magnetic bubbles represent localized spin configurations that could serve as data bits. However, the precise methods for their electrical manipulation remain uncertain. Here, we demonstrate the deterministic electrical manipulations and detections of single magnetic bubbles in kagome-latticed Fe3Sn2 magnetic nanostructured cells. The current-induced dynamics of magnetic bubbles were explored using nanosecond pulsed currents. We show single pulsed currents with low and high densities can be applied for the creation and deletion of a single bubble, respectively. The mutual writing-deleting operations on single bubbles are attributed to the thermal heating and non-thermal spin-transfer torque effects in combination with micromagnetic simulations. We also realized the in-situ detection of a single bubble using the anisotropic magnetoresistance effect through a standard four-probe method. Our results could propel the development of bubble-based spintronic devices.

cond-mat.mes-hall

Fresnel Magnetic Imaging of Ultrasmall Skyrmion Lattices

Magnetic skyrmions with ultrasmall nanometric dimensions hold significant promise for next-generation high-density spintronic devices. Direct real-space imaging of these topological spin textures is critical for elucidating their emergent properties at the nanoscale. Here, we present Lorentz transmission electron microscopy studies of nanometric skyrmion lattices in B20-structured Mn0.5Fe0.5Ge crystals using Fresnel mode. According to conventional chiral discrimination methods relying on static bright-dark contrast, we demonstrate an abnormal periodic chiral-reversal phenomenon retrieved through the transport of intensity equation analysis of defocus-dependent Fresnel images. Through systematic off-axis electron holography experiments and numerical simulations, we attribute these chiral misinterpretations to the sinusoidal modulation mechanism of the contrast transfer functionthat correlates with both defocus values and skyrmion dimensions. Our findings establish quantitative limitations of conventional Fresnel contrast analysis for ultrasmall skyrmions while revealing fundamental insights into defocus-mediated phase-to-intensity conversion processes in nanoscale magnetic imaging.

cond-mat.mtrl-sci

Stable skyrmion bundles at room temperature and zero magnetic field in a chiral magnet

Topological spin textures are characterized by topological magnetic charges, Q, which govern their electromagnetic properties. Recent studies have achieved skyrmion bundles with arbitrary integer values of Q, opening possibilities for exploring topological spintronics based on Q. However, the realization of stable skyrmion bundles in chiral magnets at room temperature and zero magnetic field - the prerequisite for realistic device applications - has remained elusive. Here, through the combination of pulsed currents and reversed magnetic fields, we experimentally achieve skyrmion bundles with different integer Q values - reaching a maximum of 24 at above room temperature and zero magnetic field - in the chiral magnet Co8Zn10Mn2. We demonstrate the field-driven annihilation of high-Q bundles and present a phase diagram as a function of temperature and field. Our experimental findings are consistently corroborated by micromagnetic simulations, which reveal the nature of the skyrmion bundle as that of skyrmion tubes encircled by a fractional Hopfion.

cond-mat.mes-hall

Creating and Deleting a Single Dipolar Skyrmion by Surface Spin Twists

We report deterministic operations on single dipolar skyrmions confined in nanostructured cuboids using in-plane currents. We achieve highly reversible writing and deleting of skyrmions in the simple cuboid without any artificial defects or pinning sites. The current-induced creation of skyrmions is well-understood through the spin-transfer torque acting on surface spin twists of the spontaneous 3D ferromagnetic state, caused by the magnetic dipole-dipole interaction of the uniaxial Fe3Sn2 magnet with a low-quality factor. Current-induced deletions of skyrmions result from the combined effects of magnetic hysteresis and Joule thermal heating. Our results are replicated consistently through 3D micromagnetic simulations. Our approach offers a viable method for achieving reliable single-bit operations in skyrmionic devices for applications such as random-access memories.

cond-mat.mes-hall

Skyrmion Sliding Switch in a 90-nm-Wide Nanostructured Chiral Magnet

Magnetic skyrmions, renowned for their fascinating electromagnetic properties, hold potential for next-generation topological spintronic devices. Recent advancements have unveiled a rich tapestry of 3D topological magnetism. Nevertheless, the practical application of 3D topological magnetism in the development of topological spintronic devices remains a challenge. Here, we showcase the experimental utilization of 3D topological magnetism through the exploitation of skyrmion-edge attractive interactions in 90-nm-wide confined chiral FeGe and CoZnMn magnetic nanostructures. These attractive interactions result in two degenerate equilibrium positions, which can be naturally interpreted as binary bits for a skyrmion sliding switch. Our theory and simulation reveal current-driven spiral motions of skyrmions, governed by the anisotropic gradient of the potential landscape. Our experiments validate the theory that predicts a tunable threshold current density via magnetic field and temperature modulation of the energy barrier. Our results offer an approach for implementing universal on-off switch functions in 3D topological spintronic devices.

cond-mat.mes-hall