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P. W. H. Pinkse

Publications and source records attributed to P. W. H. Pinkse.

At least 19 recordsLinked to original sources

Dispersive Hong-Ou-Mandel Interference with Finite Coincidence Windows

Hong-Ou-Mandel (HOM) interference is a fundamental tool for assessing photon indistinguishability in quantum information processing. While the effect of chromatic dispersion on HOM interference has been widely studied, the interplay between dispersion and the finite detection window of realistic measurement devices remains under-explored. In this work, we demonstrate that the rectangular coincidence window inherent to modern time-tagging modules, which effectively acts as a temporal filter, breaks the standard dispersion cancellation condition and restores sensitivity to symmetric group velocity dispersion. We derive an analytical model for type-II SPDC processes that predicts a modification of the HOM dip shape, specifically the emergence of characteristic oscillations and dip broadening. We experimentally validate this theoretical framework using a ppKTP source and transmission through optical fibers of lengths up to 29 km. The experimental data show excellent agreement with the model, confirming the presence of window-induced oscillations and allowing for the precise extraction of the fiber dispersion parameter. These findings underscore the importance of accounting for finite timing resolution in the design and characterization of dispersive quantum communication links.

quant-ph↗

Quantum simulation of thermodynamics in an integrated quantum photonic processor

One of the core questions of quantum physics is how to reconcile the unitary evolution of quantum states, which is information-preserving and time-reversible, with evolution following the second law of thermodynamics, which, in general, is neither. The resolution to this paradox is to recognize that global unitary evolution of a multi-partite quantum state causes the state of local subsystems to evolve towards maximum-entropy states. In this work, we experimentally demonstrate this effect in linear quantum optics by simultaneously showing the convergence of local quantum states to a generalized Gibbs ensemble constituting a maximum-entropy state under precisely controlled conditions, while introducing an efficient certification method to demonstrate that the state retains global purity. Our quantum states are manipulated by a programmable integrated quantum photonic processor, which simulates arbitrary non-interacting Hamiltonians, demonstrating the universality of this phenomenon. Our results show the potential of photonic devices for quantum simulations involving non-Gaussian states.

quant-ph↗

Clones of the Unclonable: Nanoduplicating Optical PUFs and Applications

Physical unclonable functions (PUFs), physical objects that are practically unclonable because of their andom and uncontrollable manufacturing variations, are becoming increasingly popular as security primitives and unique identifiers in a fully digitized world. One of the central PUF premises states that both friends and foes, both legitimate manufacturers and external attackers alike, cannot clone a PUF, producing two instances that are the same. Using the latest nanofabrication techniques, we show that this premise is not always met: We demonstrate the possibility of effective PUF duplication through sophisticated manufacturers by producing 63 copies of a non-trivial optical scattering structure which exhibit essentially the same scattering behavior. The remaining minuscule differences are close to or below noise levels, whence the duplicates have to be considered fully equivalent from a PUF perspective. The possibility for manufacturer-based optical PUF duplication has positive and negative consequences at the same time: While fully breaking the security of certain schemes, it enables new applications, too. For example, it facilitates unforgeable labels for valuable items; the first key-free group identification schemes over digital networks; or new types of encryption/decryption devices that do not contain secret keys.

cs.CR↗

Boson Sampling in Low-depth Optical Systems

Optical losses are the main obstacle to demonstrating a quantum advantage via boson sampling without leaving open the possibility of classical spoofing. We propose a method for generating low-depth optical circuits suitable for boson sampling with very high efficiencies. Our circuits require only a constant number of optical components (namely three) to implement an optical transformation suitable for demonstrating a quantum advantage. Consequently, our proposal has a constant optical loss regardless of the number of optical modes. We argue that sampling from our family of circuits is computationally hard by providing numerical evidence that our family of circuits converges to that of the original boson sampling proposal in the limit of large optical systems. Our work opens a new route to demonstrate an optical quantum advantage.

quant-ph↗

Deterministic and controllable photonic scattering media via direct laser writing

Photonic scattering materials, such as biological tissue and white paper, are made of randomly positioned nanoscale inhomogeneities in refractive index that lead to multiple scattering of light. Typically these materials, both naturally-occurring or man-made, are formed through self assembly of the scattering inhomogeneities, which imposes challenges in tailoring the disorder and hence the optical properties. Here, We report on the nanofabrication of photonic scattering media using direct laser writing with deterministic design. These deterministic scattering media consist of submicron thick polymer nanorods that are randomly oriented within a cubic volume. We study the total transmission of light as a function of the number density of rods and of the sample thickness to extract the scattering and transport mean free paths using radiative transfer theory. Such photonic scattering media with deterministic and controllable properties are model systems for fundamental light scattering in particular with strong anisotropy and offer new applications in solid-state lighting and photovoltaics.

physics.optics↗

Optimizing spontaneous parametric down-conversion sources for boson sampling

An important step for photonic quantum technologies is the demonstration of a quantum advantage through boson sampling. In order to prevent classical simulability of boson sampling, the photons need to be almost perfectly identical and almost without losses. These two requirements are connected through spectral filtering, improving one leads to a decrease of the other. A proven method of generating single photons is spontaneous parametric downconversion (SPDC). We show that an optimal trade-off between indistinguishability and losses can always be found for SPDC. We conclude that a 50-photon scattershot boson-sampling experiment using SPDC sources is possible from a computational complexity point of view. To this end, we numerically optimize SPDC sources under the regime of weak pumping and with a single spatial mode.

quant-ph↗

Spatially encoded light for Large-alphabet Quantum Key Distribution

Most Quantum Key Distribution protocols use a two-dimensional basis such as HV polarization as first proposed by Bennett and Brassard in 1984. These protocols are consequently limited to a key generation density of 1 bit per photon. We increase this key density by encoding information in the transverse spatial displacement of the used photons. Employing this higher-dimensional Hilbert space together with modern single-photon-detecting cameras, we demonstrate a proof-of-principle large-alphabet Quantum Key Distribution experiment with 1024 symbols and a shared information between sender and receiver of 7 bit per photon.

quant-ph↗

Transmitting more than 10 bit with a single photon

Encoding information in the position of single photons has no known limits, given infinite resources. Using a heralded single-photon source and a Spatial Light Modulator (SLM), we steer single photons to specific positions in a virtual grid on a large-area spatially resolving photon-counting detector (ICCD). We experimentally demonstrate selective addressing any location (symbol) in a 9072 size grid (alphabet) to achieve 10.5 bit of mutual information between the sender and receiver per detected photon. Our results set the stage for very-high-dimensional quantum information processing.

quant-ph↗

Looking inside three-dimensional (3D) silicon photonic band gap crystals

We have performed an x-ray holotomography study of a three-dimensional (3D) photonic band gap crystal. The crystals was made from silicon by CMOS-compatible methods. We manage to obtain the 3D material density throughout the fabricated crystal. We observe that the structural design is for most aspects well-realized by the fabricated nanostructure. One peculiar feature is a slight shear-distortion of the cubic crystal structure. We conclude that 3D X-ray tomography has great potential to solve many future questions on optical metamaterials.

cond-mat.other↗

The rotational memory effect of a multimode fiber

We demonstrate the rotational memory effect in a multimode fiber. Rotating the incident wavefront around the fiber core axis leads to a rotation of the resulting pattern of the fiber output without significant changes in the resulting speckle pattern. The rotational memory effect can be exploited for non-invasive imaging or ultrafast high-resolution scanning through a multimode fiber. Our experiments demonstrate this effect over a full range of angles in two experimental configurations.

physics.optics↗

Programming balanced optical beam splitters in white paint

Wavefront shaping allows for ultimate control of light propagation in multiple-scattering media by adaptive manipulation of incident waves. We shine two separate wavefront-shaped beams on a layer of dry white paint to create two enhanced output speckle spots of equal intensity. We experimentally confirm by interference measurements that the output speckle spots are almost correlated like the two outputs of an ideal balanced beam splitter. The observed deviations from the phase behavior of an ideal beam splitter are analyzed with a transmission matrix model. Our experiments demonstrate that wavefront shaping in multiple-scattering media can be used to approximate the functionality of linear optical devices with multiple inputs and outputs.

physics.optics↗

Storage and Adiabatic Cooling of Polar Molecules in a Microstructured Trap

We present a versatile electric trap for the exploration of a wide range of quantum phenomena in the interaction between polar molecules. The trap combines tunable fields, homogeneous over most of the trap volume, with steep gradient fields at the trap boundary. An initial sample of up to 10^8 CH3F molecules is trapped for as long as 60 seconds, with a 1/e storage time of 12 seconds. Adiabatic cooling down to 120 mK is achieved by slowly expanding the trap volume. The trap combines all ingredients for opto-electrical cooling, which, together with the extraordinarily long storage times, brings field-controlled quantum-mechanical collision and reaction experiments within reach.

quant-ph↗

Extraction of optical Bloch modes in a photonic-crystal waveguide

We perform phase-sensitive near-field scanning optical microscopy on photonic-crystal waveguides. The observed intricate field patterns are analyzed by spatial Fourier transformations, revealing several guided TE- and TM-like modes. Using the reconstruction algorithm proposed by Ha, et al. (Opt. Lett. 34 (2009)), we decompose the measured two-dimensional field pattern in a superposition of propagating Bloch modes. This opens new possibilities to study specific modes in near-field measurements. We apply the method to study the transverse behavior of a guided TE-like mode, where the mode extends deeper in the surrounding photonic crystal when the band edge is approached.

physics.optics↗

Photonic-Crystal Waveguides with Disorder: Measurement of a Band-Edge Tail in the Density of States

We measure localized and extended mode profiles at the band edge of slow-light photonic-crystal waveguides using phase-sensitive near-field microscopy. High-resolution band structures are obtained and interpreted, allowing the retrieval of the optical density of states (DOS). This constitutes a first observation of the DOS of a periodic system with weak disorder. The Van Hove singularity in the DOS expected at the band edge of an ideal 1D periodic structure is removed by the disorder. The Anderson-localized states form a "tail" in the density of states, as predicted by Lifshitz for solid-state systems.

physics.optics↗

Opto-Electrical Cooling of Polar Molecules

We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found in symmetric-top rotors comprising six low-field-seeking rovibrational states. A generic trap design is presented. Suitable molecules are identified with vibrational decay rates on the order of 100Hz. A simulation of the cooling process shows that the molecular temperature can be reduced from 1K to 1mK in approximately 10s. The molecules remain electrically trapped during this time, indicating that the ultracold regime can be reached in an experimentally feasible scheme.

quant-ph↗

Electrostatic extraction of cold molecules from a cryogenic reservoir

We present a method which delivers a continuous, high-density beam of slow and internally cold polar molecules. In our source, warm molecules are first cooled by collisions with a cryogenic helium buffer gas. Cold molecules are then extracted by means of an electrostatic quadrupole guide. For ND$_3$ the source produces fluxes up to $(7 \pm ^{7}_{4}) \times 10^{10}$ molecules/s with peak densities up to $(1.0 \pm ^{1.0}_{0.6}) \times 10^9$ molecules/cm$^3$. For H$_2$CO the population of rovibrational states is monitored by depletion spectroscopy, resulting in single-state populations up to $(82 \pm 10)%$.

physics.chem-ph↗

Cold guided beams of water isotopologs

Electrostatic velocity filtering and guiding is an established technique to produce high fluxes of cold polar molecules. In this paper we clarify different aspects of this technique by comparing experiments to detailed calculations. In the experiment, we produce cold guided beams of the three water isotopologs H2O, D2O and HDO. Their different rotational constants and orientations of electric dipole moments lead to remarkably different Stark shift properties, despite the molecules being very similar in a chemical sense. Therefore, the signals of the guided water isotopologs differ on an absolute scale and also exhibit characteristic electrode voltage dependencies. We find excellent agreement between the relative guided fractions and voltage dependencies of the investigated isotopologs and predictions made by our theoretical model of electrostatic velocity filtering.

physics.chem-ph↗

Two-photon gateway in one-atom cavity quantum electrodynamics

Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the quantum anharmonicity of the energy structure of the atom-cavity system. Future applications could include the controlled interaction of two photons by means of one atom.

quant-ph↗