arXiv subjects

Paul S. Julienne

Publications and source records attributed to Paul S. Julienne.

At least 73 records · Page 4Linked to original sources

arXiv2009

Controlling nuclear spin exchange via optical Feshbach resonances in ${}^{171}$Yb

Nuclear spin exchange occurs in ultracold collisions of fermionic alkaline-earth-like atoms due to a difference between s- and p-wave phase shifts. We study the use of an optical Feshbach resonance, excited on the ${}^1S_0 \to {}^3P_1$ intercombination line of ${}^{171}$Yb, to affect a large modification of the s-wave scattering phase shift, and thereby optically mediate nuclear exchange forces. We perform a full multichannel calculation of the photoassociation resonances and wave functions and from these calculate the real and imaginary parts of the scattering length. As a figure of merit of this interaction, we estimate the fidelity to implement a $\sqrt{SWAP}$ entangling quantum logic gate for two atoms trapped in the same well of an optical lattice. For moderate parameters one can achieve a gate fidelity of $\sim95% $ in a time of $\sim 50 μ$s.

quant-ph↗

arXiv2009

Prediction of Feshbach resonances from three input parameters

We have developed a model of Feshbach resonances in gases of ultracold alkali metal atoms using the ideas of multichannel quantum defect theory. Our model requires just three parameters describing the interactions - the singlet and triplet scattering lengths, and the long range van der Waals coefficient - in addition to known atomic properties. Without using any further details of the interactions, our approach can accurately predict the locations of resonances. It can also be used to find the singlet and triplet scattering lengths from measured resonance data. We apply our technique to $^{6}$Li--$^{40}$K and $^{40}$K--$^{87}$Rb scattering, obtaining good agreement with experimental results, and with the more computationally intensive coupled channels technique.

cond-mat.other↗

arXiv2009

Collisional cooling of ultra-cold atom ensembles using Feshbach resonances

We propose a new type of cooling mechanism for ultra-cold fermionic atom ensembles, which capitalizes on the energy dependence of inelastic collisions in the presence of a Feshbach resonance. We first discuss the case of a single magnetic resonance, and find that the final temperature and the cooling rate is limited by the width of the resonance. A concrete example, based on a p-wave resonance of $^{40}$K, is given. We then improve upon this setup by using both a very sharp optical or radio-frequency induced resonance and a very broad magnetic resonance and show that one can improve upon temperatures reached with current technologies.

cond-mat.other↗

arXiv2009

Molecular states near a collision threshold

This chapter summarizes the properties of near-threshold molecular states that can be formed from ultracold atoms. The properties of the states for a single potential are characterized for different partial waves using the concepts of quantum defect theory for a van der Waals potential. Examples are given for various isotopes of the Yb_2 molecule. Magnetically tunable Feshbach resonances or photoassociation resonances are characterized by the multichannel version of the theory. Examples of the latter are given for the KRb molecule.

physics.atom-ph↗

arXiv2009

Ultracold molecules from ultracold atoms: a case study with the KRb molecule

Ultracold collisions of cold atoms or molecules make the bound states of the collision complex formed from the two colliding species accessible for control and manipulation of the cold species or the complex. Such resonances are best treated by a resonant scattering theory, which in the ultracold domain can take advantage of the properties of the long-range potential and the methods of multichannel quantum defect theory. Coupled channels calculations on the threshold scattering states and bound states of the 40K87Rb molecule illustrate the ideas and methodology of quantum defect theory using the long-range potential and also demonstrate the spin properties of the bound states throughout the spectrum.

physics.atom-ph↗

arXiv2009

Multi-channel modelling of the formation of vibrationally cold polar KRb molecules

We describe the theoretical advances that influenced the experimental creation of vibrationally and translationally cold polar $^{40}$K$^{87}$Rb molecules \cite{nphys08,science08}. Cold molecules were created from very-weakly bound molecules formed by magnetic field sweeps near a Feshbach resonance in collisions of ultra-cold $^{40}$K and $^{87}$Rb atoms. Our analysis include the multi-channel bound-state calculations of the hyperfine and Zeeman mixed X$^1Σ^+$ and a$^3Σ^+$ vibrational levels. We find excellent agreement with the hyperfine structure observed in experimental data. In addition, we studied the spin-orbit mixing in the intermediate state of the Raman transition. This allowed us to investigate its effect on the vibrationally-averaged transition dipole moment to the lowest ro-vibrational level of the X$^1Σ^+$ state. Finally, we obtained an estimate of the polarizability of the initial and final ro-vibrational states of the Raman transition near frequencies relevant for optical trapping of the molecules.

quant-ph↗

arXiv2008

Quantum theory of ultracold atom-ion collisions

We study atom-ion scattering in the ultracold regime. To this aim, an analytical model based on the multichannel quantum defect formalism is developed and compared to close-coupled numerical calculations. We investigate the occurrence of magnetic Feshbach resonances focusing on the specific 40Ca+ - Na system. The presence of several resonances at experimentally accessible magnetic fields should allow the atom-ion interaction to be precisely tuned. A fully quantum-mechanical study of charge exchange processes shows that charge-exchange rates should remain small even in the presence of resonance effects. Most of our results can be cast in a system-independent form and are important for the realization of the charge-neutral ultracold systems.

physics.atom-ph↗

arXiv2008

Avoided crossings between bound states of ultracold Cesium dimers

We present an efficient new computational method for calculating the binding energies of the bound states of ultracold alkali-metal dimers in the presence of magnetic fields. The method is based on propagation of coupled differential equations and does not use a basis set for the interatomic distance coordinate. It is much more efficient than the previous method based on a radial basis set and allows many more spin channels to be included. This is particularly important in the vicinity of avoided crossings between bound states. We characterize a number of different avoided crossings in Cs_2 and compare our converged calculations with experimental results. Small but significant discrepancies are observed in both crossing strengths and level positions, especially for levels with l symmetry (rotational angular momentum L=8). The discrepancies should allow the development of improved potential models in the future.

physics.chem-ph↗

arXiv2008

Coherent, adiabatic and dissociation regimes in coupled atomic-molecular Bose-Einstein condensates

We discuss the dynamics of a Bose-Einstein condensate of atoms which is suddenly coupled to a condensate of molecules by an optical or magnetic Feshbach resonance. Three limiting regimes are found and can be understood from the transient dynamics occuring for each pair of atoms. This transient dynamics can be summarised into a time-dependent shift and broadening of the molecular state. A simple Gross-Pitaevskii picture including this shift and broadening is proposed to describe the system in the three regimes. Finally, we suggest how to explore these regimes experimentally.

cond-mat.other↗

arXiv2008

Two-body transients in coupled atomic-molecular BECs

We discuss the dynamics of an atomic Bose-Einstein condensate when pairs of atoms are converted into molecules by single-color photoassociation. Three main regimes are found and it is shown that they can be understood on the basis of time-dependent two-body theory. In particular, the so-called rogue dissociation regime [Phys. Rev. Lett., 88, 090403 (2002)], which has a density-dependent limit on the photoassociation rate, is identified with a transient regime of the two-atom dynamics exhibiting universal properties. Finally, we illustrate how these regimes could be explored by photoassociating condensates of alkaline-earth atoms.

physics.atom-ph↗

arXiv2007

Effective-range description of a Bose gas under strong one- or two-dimensional confinement

We point out that theories describing s-wave collisions of bosonic atoms confined in one- or two-dimensional geometries can be extended to much tighter confinements than previously thought. This is achieved by replacing the scattering length by an energy-dependent scattering length which was already introduced for the calculation of energy levels under 3D confinement. This replacement accurately predicts the position of confinement-induced resonances in strongly confined geometries.

physics.atom-ph↗

arXiv2007

Two-color photoassociation spectroscopy of ytterbium atoms and the precise determinations of s-wave scattering lengths

By performing high-resolution two-color photoassociation spectroscopy, we have successfully determined the binding energies of several of the last bound states of the homonuclear dimers of six different isotopes of ytterbium. These spectroscopic data are in excellent agreement with theoretical calculations based on a simple model potential, which very precisely predicts the s-wave scattering lengths of all 28 pairs of the seven stable isotopes. The s-wave scattering lengths for collision of two atoms of the same isotopic species are 13.33(18) nm for ^{168}Yb, 3.38(11) nm for ^{170}Yb, -0.15(19) nm for ^{171}Yb, -31.7(3.4) nm for ^{172}Yb, 10.55(11) nm for ^{173}Yb, 5.55(8) nm for ^{174}Yb, and -1.28(23) nm for ^{176}Yb. The coefficient of the lead term of the long-range van der Waals potential of the Yb_2 molecule is C_6=1932(30) atomic units $(E_h a_0^6 \approx 9.573\times 10^{-26}$ J nm^6).

physics.atom-ph↗

arXiv2007

Excited Thomas-Efimov levels in ultracold gases

Since the early days of quantum physics, the complex behavior of three interacting particles has been the subject of numerous experimental and theoretical studies. In a recent Letter to Nature, Kraemer et al. [Nature (London) 440, 315 (2006)] report on experimental ``evidence for Efimov quantum states'' in an ultracold gas of cesium atoms. Such quantum states refer to an infinite series of energy levels of three identical Bose particles, accumulating at the threshold for dissociation as the scattering length of each pair is tuned to infinity. Whereas the existence of a single Efimov state has been predicted for three helium atoms, earlier experimental studies concluded that this elusive state had not been found. In this paper we show by an intuitive argument and full numerical calculations that the helium and cesium experiments actually provide evidence of the same, ground state of this trimer spectrum, which the helium experimentalists and pioneering theoretical studies had not associated with Efimov's effect. Unlike the helium trimer, the observed 133Cs_3 resonance refers to a Borromean molecular state. We discuss how as yet unobserved, excited Efimov quantum states might be detected in ultracold gases of 85Rb and of 133Cs at magnetic field strengths in the vicinity of 0.08 T (800 G).

cond-mat.other↗

arXiv2006

Production of cold molecules via magnetically tunable Feshbach resonances

Magnetically tunable Feshbach resonances were employed to associate cold diatomic molecules in a series of experiments involving both atomic Bose as well as two spin component Fermi gases. This review illustrates theoretical concepts of both the particular nature of the highly excited Feshbach molecules produced and the techniques for their association from unbound atom pairs. Coupled channels theory provides the rigorous formulation of the microscopic physics of Feshbach resonances in cold gases. Concepts of dressed versus bare energy states, universal properties of Feshbach molecules, as well as the classification in terms of entrance- and closed-channel dominated resonances are introduced on the basis of practical two-channel approaches. Their significance is illustrated for several experimental observations, such as binding energies and lifetimes with respect to collisional relaxation. Molecular association and dissociation are discussed in the context of techniques involving linear magnetic field sweeps in cold Bose and Fermi gases as well as pulse sequences leading to Ramsey-type interference fringes. Their descriptions in terms of Landau-Zener, two-level mean field as well as beyond mean field approaches are reviewed in detail, including the associated ranges of validity.

cond-mat.other↗

arXiv2006

Quantum Scattering of Distinguishable Bosons using an Ultracold Atom Collider

We describe a new implementation of magnetic collider for investigating cold collisions between ultracold atomic clouds in different spin states, and we use this to investigate scattering involving both even and odd order partial waves. Our method relies on the axial assymetry of a double-well magnetic trap to selectively prepare the spin state in each cloud. We measure the energy dependence of s, p and d partial wave phase shifts in collisions up to 300 microKelvin between ^{87}Rb atoms in the 5S_{1/2}, F=1, m_F=-1 and 5S_{1/2}, F=2, m_F=1 states.

cond-mat.other↗

arXiv2006

Optical Feshbach resonances of Alkaline-Earth atoms in a 1D or 2D optical lattice

Motivated by a recent experiment by Zelevinsky et al. [Phys. Rev. Lett. 96, 203201], we present the theory for photoassociation and optical Feshbach resonances of atoms confined in a tight one-dimensional (1D) or two-dimensional (2D) optical lattice. In the case of an alkaline-earth intercombination resonance, the narrow natural width of the line makes it possible to observe clear manifestations of the dimensionality, as well as some sensitivity to the scattering length of the atoms. Among possible applications, a 2D lattice may be used to increase the spectroscopic resolution by about one order of magnitude. Furthermore, a 1D lattice induces a shift which provides a new way of determining the strength of a resonance by spectroscopic measurements.

physics.atom-ph↗

arXiv2006

Simple Theoretical Models for Resonant Cold Atom Interactions

Magnetically tunable scattering resonances have been used with great success for precise control of s-wave scattering lengths in ultracold atomic collisions. We describe relatively simple yet quite powerful analytic treatments of such resonances based on the analytic properties of the van der Waals long range potential. This theory can be used to characterize a number of properties of specific resonances that have been used successfully in various experiments with $^{87}$Rb, $^{85}$Rb, $^{40}$K, and $^{6}$Li. Optical Feshbach resonances are also possible and may be practical with narrow intercombination line photoassociative transitions in species like Sr and Yb.

physics.atom-ph↗

arXiv2006

A two-channel R-matrix analysis of magnetic field induced Feshbach resonances

A Feshbach resonance arises in cold atom scattering due to the complex interplay between several coupled channels. However, the essential physics of the resonance may be encapsulated in a simplified model consisting of just two coupled channels. In this paper we describe in detail how such an effective Feshbach model can be constructed from knowledge of a few key parameters, characterizing the atomic Born-Oppenheimer potentials and the low energy scattering near the resonance. These parameters may be obtained either from experiment or full coupled channels calculations. Using R-matrix theory we analyze the bound state spectrum and the scattering properties of the two-channel model, and find it to be in good agreement with exact calculations.

cond-mat.other↗