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Peter Michler

Publications and source records attributed to Peter Michler.

At least 37 records · Page 2Linked to original sources
arXiv2023

Enhancing quantum cryptography with quantum dot single-photon sources

Quantum cryptography harnesses quantum light, in particular single photons, to provide security guarantees that cannot be reached by classical means. For each cryptographic task, the security feature of interest is directly related to the photons' non-classical properties. Quantum dot-based single-photon sources are remarkable candidates, as they can in principle emit deterministically, with high brightness and low multiphoton contribution. Here, we show that these sources provide additional security benefits, thanks to the tunability of coherence in the emitted photon-number states. We identify the optimal optical pumping scheme for the main quantum-cryptographic primitives, and benchmark their performance with respect to Poisson-distributed sources such as attenuated laser states and down-conversion sources. In particular, we elaborate on the advantage of using phonon-assisted and two-photon excitation rather than resonant excitation for quantum key distribution and other primitives. The presented results will guide future developments in solid-state and quantum information science for photon sources that are tailored to quantum communication tasks.

quant-ph↗
arXiv2022

Wavelength-tunable open double-microcavity to enhance two closely spaced optical transitions

Microcavities have long been recognized as indispensable elements in quantum photonic research due to their usefulness for enhanced light extraction and light-matter interaction. A conventional high-Q cavity structure typically allows only a single optical transition to be tuned into resonance with a specific mode. The transition to a more advanced double-cavity structure, however, introduces new and interesting possibilities such as enhancing two spectrally close optical transitions at the same time with two distinct cavity modes. Here, we investigate a cavity structure composed of a monolithic planar cavity enclosed between two semiconductor distributed Bragg reflectors (DBR) and a top dielectric mirror deposited on a fiber tip. While the bottom cavity is formed by the two DBRs, the mirror on the fiber tip and the top DBR of the semiconductor chip create a second tunable cavity. These coupled cavities exhibit mode hybridization when tuned into resonance and their splitting can be adjusted to match with the spectral separation of closely spaced optical transitions by a suitable sample design. Furthermore, we report on the simultaneous resonance tuning of the exciton and biexciton transition of a semiconductor quantum dot, each to a separate mode of the open fiber-based double cavity. Decay time measurements at simultaneous resonance showed a Purcell-factor of $F_P^X$=1.9$\pm$0.4 for the exciton transition.

physics.optics↗
arXiv2022

High emission rate from a Purcell-enhanced, triggered source of pure single photons in the telecom C-band

Several emission features mark semiconductor quantum dots as promising non-classical light sources for prospective quantum implementations. For long-distance transmission [1] and Si-based on-chip processing[2, 3], the possibility to match the telecom C-band [4] stands out, while source brightness and high single-photon purity are key features in virtually any quantum implementation [5, 6]. Here we present an InAs/InGaAs/GaAs quantum dot emitting in the telecom C-band coupled to a circular Bragg grating. The Purcell enhancement of the emission enables a simultaneously high brightness with a fiber-coupled single-photon count rate of 13.9MHz for an excitation repetition rate of 228MHz (first-lens collection efficiency ca. 17% for NA = 0.6), while maintaining a low multi-photon contribution of g(2)(0) = 0.0052. Moreover, the compatibility with temperatures of up to 40K attainable with compact cryo coolers, further underlines the suitability for out-of-the-lab implementations.

quant-ph↗
arXiv2022

Observation of ultrafast interfacial Meitner-Auger energy transfer in a van der Waals heterostructure

Atomically thin layered van der Waals heterostructures feature exotic and emergent optoelectronic properties. With growing interest in these novel quantum materials, the microscopic understanding of fundamental interfacial coupling mechanisms is of capital importance. Here, using multidimensional photoemission spectroscopy, we provide a layer- and momentum-resolved view on ultrafast interlayer electron and energy transfer in a monolayer-WSe$_2$/graphene heterostructure. Depending on the nature of the optically prepared state, we find the different dominating transfer mechanisms: while electron injection from graphene to WSe$_2$ is observed after photoexcitation of quasi-free hot carriers in the graphene layer, we establish an interfacial Meitner-Auger energy transfer process following the excitation of excitons in WSe$_2$. By analysing the time-energy-momentum distributions of excited-state carriers with a rate-equation model, we distinguish these two types of interfacial dynamics and identify the ultrafast conversion of excitons in WSe$_2$ to valence band transitions in graphene. Microscopic calculations find interfacial dipole-monopole coupling underlying the Meitner-Auger energy transfer to dominate over conventional Förster- and Dexter-type interactions, in agreement with the experimental observations. The energy transfer mechanism revealed here might enable new hot-carrier-based device concepts with van der Waals heterostructures.

cond-mat.mtrl-sci↗
arXiv2021

Thin-Film InGaAs Metamorphic Buffer for telecom C-band InAs Quantum Dots and Optical Resonators on GaAs Platform

The GaAs-based material system is well-known for the implementation of InAs quantum dots (QDs) with outstanding optical properties. However, these dots typically emit at a wavelength of around 900nm. The insertion of a metamorphic buffer (MMB) can shift the emission to the technologically attractive telecom C-band range centered at 1550nm. However, the thickness of common MMB designs limits their compatibility with most photonic resonator types. Here we report on the MOVPE growth of a novel InGaAs MMB with a non-linear indium content grading profile designed to maximize plastic relaxation within minimal layer thickness. Single-photon emission at 1550nm from InAs QDs deposited on top of this thin-film MMB is demonstrated. The strength of the new design is proven by integrating it into a bullseye cavity via nano-structuring techniques. The presented advances in the epitaxial growth of QD/MMB structures form the basis for the fabrication of high-quality telecom non-classical light sources as a key component of photonic quantum technologies.

physics.optics↗
arXiv2021

Optical Charge Injection and Full Coherent Control of Spin-Qubit in the Telecom C-band Emitting Quantum Dot

Solid-state quantum emitters with manipulable spin-qubits are promising platforms for quantum communication applications. Although such light-matter interfaces could be realized in many systems only a few allow for light emission in the telecom bands necessary for long-distance quantum networks. Here, we propose and implement a new optically active solid-state spin-qubit based on a hole confined in a single InAs/GaAs quantum dot grown on an InGaAs metamorphic buffer layer emitting photons in the C-band. We lift the hole spin-degeneracy using an external magnetic field and demonstrate hole injection, initialization, read-out and complete coherent control using picosecond optical pulses. These results showcase a new solid-state spin-qubit platform compatible with preexisting optical fibre networks.

cond-mat.mes-hall↗
arXiv2021

Bright Purcell enhanced single-photon source in the telecom O-band based on a quantum dot in a circular Bragg grating

The combination of semiconductor quantum dots (QDs) with photonic cavities is a promising way to realize non-classical light sources with state-of-the-art performances in terms of brightness, indistinguishability and repetition rate. In the present work we demonstrate the coupling of an InGaAs/GaAs QDs emitting in the telecom O-band to a circular Bragg grating cavity. We demonstrate a broadband geometric extraction efficiency enhancement by investigating two emission lines under above-band excitation, inside and detuned from the cavity mode, respectively. In the first case, a Purcell enhancement of 4 is attained. For the latter case, an end-to-end brightness of 1.4% with a brightness at the first lens of 23% is achieved. Using p-shell pumping, a combination of high count rate with pure single-photon emission (g(2)(0) = 0.01 in saturation) is achieved. Finally a good single-photon purity (g(2)(0) = 0.13) together with a high detector count rate of 191kcps is demonstrated for a temperature of up to 77K.

physics.optics↗
arXiv2020

Delaying two-photon Fock-states in a hot cesium vapor using on-demand generated single-photons from a semiconductor quantum dot

Single photons from solid-state quantum emitters are playing a crucial role in the development of photonic quantum technologies. Higher order states, such as N-photon Fock-states allow for applications e.g. in quantum-enhanced sensing. In this study, we utilize the dispersion of a hot cesium vapor at the D1 lines to realize a temporal delay for one and two-photon Fock-states as a result of the slow-light effect. Single photons are generated on-demand from an InGaAs quantum dot, while their quantum interference at a beam splitter is used to generate a two-photon Fockstate. We verify the successful propagation and temporal delay of both the one and two-photon Fock-states, while a significant delay (5x initial photon length) with simultaneous high transmission (~90 %) is achieved.

quant-ph↗
arXiv2020

3D printed micro-optics for quantum technology: Optimized coupling of single quantum dot emission into a single mode fiber

Future quantum technology relies crucially on building quantum networks with high fidelity. To achieve this challenging goal, it is of utmost importance to connect single quantum systems in a way such that their emitted single-photons overlap with the highest possible degree of coherence. This requires perfect mode overlap of the emitted light of different emitters, which necessitates the use of single mode fibers. Here we present an advanced manufacturing approach to accomplish this task: we combine 3D printed complex micro-optics such as hemispherical and Weierstrass solid immersion lenses as well as total internal reflection solid immersion lenses on top of single InAs quantum dots with 3D printed optics on single mode fibers and compare their key features. Interestingly, the use of hemispherical solid immersion lenses further increases the localization accuracy of the emitters to below 1 nm when acquiring micro-photoluminescence maps. The system can be joined together and permanently fixed. This integrated system can be cooled by dipping into liquid helium, by a Stirling cryocooler or by a closed-cycle helium cryostat without the necessity for optical windows, as all access is through the integrated single mode fiber. We identify the ideal optical designs and present experiments that prove excellent high-rate single-photon emission by high-contrast Hanbury Brown and Twiss experiments.

physics.app-ph↗
arXiv2020

Quantum dot single-photon emission coupled into single-mode fibers with 3D printed micro-objectives

User-friendly single-photon sources with high photon-extraction efficiency are crucial building blocks for photonic quantum applications. For many of these applications, such as long-distance quantum key distribution, the use of single-mode optical fibers is mandatory, which leads to stringent requirements regarding the device design and fabrication. We report on the on-chip integration of a quantum dot microlens with a 3D-printed micro-objective in combination with a single-mode on-chip fiber coupler. The practical quantum device is realized by deterministic fabrication of the QD-microlens via in-situ electron-beam lithography and 3D two-photon laser writing of the on-chip micro-objective and fiber-holder. The QD with microlens is an efficient single-photon source, whose emission is collimated by the on-chip micro-objective. A second polymer microlens is located at the end facet of the single-mode fiber and ensures that the collimated light is efficiently coupled into the fiber core. For this purpose, the fiber is placed in the on-chip fiber chuck, which is precisely aligned to the QD-microlens thanks to the sub-$μ$m processing accuracy of high-resolution two-photon direct laser writing. This way, we obtain a fully integrated high-quality quantum device with broadband photon extraction efficiency, a single-mode fiber-coupling efficiency of 26%, a single-photon flux of 1.5 MHz at single-mode fibre output and a multi-photon probability of 13 % under pulsed optical excitation. In addition, the stable design of the developed fiber-coupled quantum device makes it highly attractive for integration into user-friendly plug-and-play quantum applications.

physics.app-ph↗
arXiv2019

Extending Quantum Links: Modules for Fiber- and Memory-Based Quantum Repeaters

We analyze elementary building blocks for quantum repeaters based on fiber channels and memory stations. Implementations are considered for three different physical platforms, for which suitable components are available: quantum dots, trapped atoms and ions, and color centers in diamond. We evaluate and compare the performances of basic quantum repeater links for these platforms both for present-day, state-of-the-art experimental parameters as well as for parameters that could in principle be reached in the future. The ultimate goal is to experimentally explore regimes at intermediate distances, up to a few 100 km, in which the repeater-assisted secret key transmission rates exceed the maximal rate achievable via direct transmission. We consider two different protocols, one of which is better adapted to the higher source clock rate and lower memory coherence time of the quantum dot platform, while the other circumvents the need of writing photonic quantum states into the memories in a heralded, non-destructive fashion. The elementary building blocks and protocols can be connected in a modular form to construct a quantum repeater system that is potentially scalable to large distances.

quant-ph↗
arXiv2019

Delay and polarization routing of single photons

The full control of single photons is important in quantum information and quantum networking. A convenient storage device for photons is the key to memory assisted quantum communication and computing. While even a simple optical fiber can act as a convenient and reliable storage device, its storage time is tightly fixed and cannot be adapted. Therefore, the photon storage should ideally be actively controllable by external means, such as magnetic or electric control fields. In order to multiplex several photons, an active routing would also be desirable. Here we show that single photons of a semiconductor quantum dot can be deliberately delayed by an atomic vapor. Also, the output path can be selected, depending on an external magnetic field. By selecting the input polarization of the photons and by aligning the external magnetic field of the hot atomic vapor, the delay-based storage can be fine tuned to a deliberate value. With an overall delay of 25 ns, we are able to fine tune by more than 600 ps. Depending on the input polarization, the photons are routed into different output ports. The experimental data is fully resembled by a theoretical model, which describes the group velocity delay under consideration of spectral diffusion and considers the complex refractive index of the atomic vapor. The present results enable the use of an atomic vapor as a wavelength selective delay and allows for routing the single photons according to their polarization and an external magnetic field.

quant-ph↗
arXiv2019

Characterization of a photon-number resolving SNSPD using Poissonian and sub-Poissonian light

Photon-number resolving (PNR) single-photon detectors are of interest for a wide range of applications in the emerging field of photon based quantum technologies. Especially photonic integrated circuits will pave the way for a high complexity and ease of use of quantum photonics. Superconducting nanowire single-photon detectors (SNSPDs) are of special interest since they combine a high detection efficiency and a high timing accuracy with a high count rate and they can be configured as PNR-SNSPDs. Here, we present a PNR-SNSPD with a four photon resolution suitable for waveguide integration operating at a temperature of 4 K. A high statistical accuracy for the photon number is achieved for a Poissonian light source at a photon flux below 5 photons/pulse with a detection efficiency of 22.7 +- 3.0% at 900 nm and a pulse rate frequency of 76 MHz. We demonstrate the ability of such a detector to discriminate a sub-Poissonian from a Poissonian light source.

physics.ins-det↗
arXiv2019

Single-photon light emitting diodes based on pre-selected quantum dots using a deterministic lithography technique

In the present study, we developed a fabrication process of an electrically driven single-photon LED based on InP QDs emitting in the red spectral range, the wavelength of interest coinciding with the high efficiency window of Si APDs. A deterministic lithography technique allowed for the pre-selection of a suitable QD, here exclusively operated under electrical carrier injection. The final device was characterized under micro-electroluminescence in direct current, as well as in pulsed excitation mode. In particular, under pulsed excitation of one device, single-photon emission of a spectral line, identified as an exciton, has been observed with $g^{(2)}_\mathrm{raw}(0)=0.42\pm0.02$, where the non-zero $g^{(2)}$-value is mainly caused by background contribution in the spectrum and re-excitation processes due to the electrical pulse length. The obtained results constitute an important step forward in the fabrication of electrically driven single-photon sources, where deterministic lithography techniques can be used to sensibly improve the device performances. In principle, the developed process can be extended to any desired emitter wavelength above $600\,\mathrm{nm}$ up to the telecom bands.

cond-mat.mes-hall↗
arXiv2019

Highly indistinguishable single photons from incoherently and coherently excited GaAs quantum dots

Semiconductor quantum dots are converging towards the demanding requirements of photonic quantum technologies. Among different systems, quantum dots with dimensions exceeding the free-exciton Bohr radius are appealing because of their high oscillator strengths. While this property has received much attention in the context of cavity quantum electrodynamics, little is known about the degree of indistinguishability of single photons consecutively emitted by such dots and on the proper excitation schemes to achieve high indistinguishability. A prominent example is represented by GaAs quantum dots obtained by local droplet etching, which recently outperformed other systems as triggered sources of entangled photon pairs. On these dots, we compare different single-photon excitation mechanisms, and we find (i) a "phonon bottleneck" and poor indistinguishability for conventional excitation via excited states and (ii) photon indistinguishablilities above 90% for both strictly resonant and for incoherent acoustic- and optical-phonon-assisted excitation. Among the excitation schemes, optical phonon-assisted excitation enables straightforward laser rejection without a compromise on the source brightness together with a high photon indistinguishability.

cond-mat.mes-hall↗
arXiv2018

Fully on-chip single-photon Hanbury-Brown and Twiss experiment on a monolithic semiconductor-superconductor platform

Photonic quantum technologies such as quantum cryptography, photonic quantum metrology, photonic quantum simulators and computers will largely benefit from highly scalable and small footprint quantum photonic circuits. To perform fully on-chip quantum photonic operations, three basic building blocks are required: single-photon sources, photonic circuits and single-photon detectors. Highly integrated quantum photonic chips on silicon and related platforms have been demonstrated incorporating only one or two of these basic building blocks. Previous implementations of all three components were mainly limited by laser stray light, making temporal filtering necessary or required complex manipulation to transfer all components onto one chip. So far, a monolithic, simultaneous implementation of all elements demonstrating single-photon operation remains elusive. Here, we present a fully-integrated Hanbury-Brown and Twiss setup on a micron-sized footprint, consisting of a GaAs waveguide embedding quantum dots as single-photon sources, a waveguide beamsplitter and two superconducting nanowire single-photon detectors. This enables a second-order correlation measurement at the single-photon level under both continuous-wave and pulsed resonant excitation.

physics.app-ph↗
arXiv2018

Two-photon interference in the telecom C-band after frequency conversion of photons from remote quantum emitters

Efficient fiber-based long-distance quantum communication via quantum repeaters relies on deterministic single-photon sources at telecom wavelengths, with the potential to exploit the existing world-wide infrastructures. For upscaling the experimental complexity in quantum networking, two-photon interference (TPI) of remote non-classical emitters in the low-loss telecom bands is of utmost importance. With respect to TPI of distinct emitters, several experiments have been conducted, e.g., using trapped atoms [Beugnon2006], ions [Maunz2007], NV-centers [Bernien2012, Sipahigil2012], SiV-centers [Sipahigil2014], organic molecules [Lettow2010] and semiconductor quantum dots (QDs) [Patel2010, Flagg2010, He2013b, Gold2014, Giesz2015, Thoma2017, Reindl2017, Zopf2017]; however, the spectral range was far from the highly desirable telecom C-band. Here, we report on TPI at 1550 nm between down-converted single photons from remote QDs [Michler2017Book], demonstrating quantum frequency conversion [Zaske2012, Ates2012, Kambs2016] as precise and stable mechanism to erase the frequency difference between independent emitters. On resonance, a TPI-visibility of (29+-3)% has been observed, being only limited by spectral diffusion processes of the individual QDs [Robinson2000, Kuhlmann2015]. Up to 2-km of additional fiber channel has been introduced in both or individual signal paths with no influence on TPI-visibility, proving negligible photon wave-packet distortion. The present experiment is conducted within a local fiber network covering several rooms between two floors of the building. Our studies pave the way to establish long-distance entanglement distribution between remote solid-state emitters including interfaces with various quantum hybrid systems [DeGreve2012,Maring2017,Bock2017,Maring2018].

quant-ph↗