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Philip Phillips

Publications and source records attributed to Philip Phillips.

At least 55 records · Page 3Linked to original sources
arXiv2008

Mottness on a triangular lattice

We study the physics on the paramagnetic side of the phase diagram of the cobaltates, $Na_{x}CoO_{2}$, with an implementation of cellular dynamical mean field theory (CDMFT) with the non-crossing approximation (NCA) for the one-band Hubbard model on a triangular lattice. At low doping we find that the low energy physics is dominated by a quasi-dispersionless band. At half-filling, we find a metal-insulator transition at $U_{c}=5.6\pm0.15t$ which depends weakly on the cluster size. The onset of the metallic state occurs through the growth of a coherence peak at the chemical potential. Away from half filling, in the electron-doped regime, the system is metallic with a large, continuous Fermi surface as seen experimentally. Upon hole doping, a quasi non-dispersing band emerges at the top of the lower Hubbard band and controls the low-energy physics. This band is a clear signature of non-Fermi liquid behavior and cannot be captured by any weakly coupled approach. This quasi non-dispersive band, which persists in a certain range of dopings, has been observed experimentally. We also investigate the pseudogap phenomenon in the context of a triangular lattice and we propose a new framework for discussing the pseudogap phenomena in general. This framework involves a momentum-dependent characterization of the low-energy physics and links the appearance of the pseudogap to a reconstruction of the Fermi surface without invoking any long range order or symmetry breaking. Within this framework we predict the existence of a pseudogap for the two dimensional Hubbard model on a triangular lattice in the weakly hole-doped regime.

cond-mat.str-el↗
arXiv2008

Theory of the Magnetic Moment in Iron Pnictides

We show that the combined effects of spin-orbit, monoclinic distortion, and p-d hybridization in tetrahedrally coordinated Fe in LaOFeAs invalidates the naive Hund's rule filling of the Fe d-levels. The two highest occupied levels have one electron each but as a result of the p-d hybridization have very different on-site repulsions. As a result, electrons in the upper level are more itinerant while those in the lower level are more localized. It is the xy-projection of the spin in the lower level that orders antiferromagnetically as the z-components of the spins in the two levels is shown to be vanishingly small in the ground state. The resulting magnetic moment is highly anisotropic with an in-plane value of $0.25-0.35μ_B$ per Fe and a z-projection of $0.06μ_B$, both of which are in agreement with experiment. As a consequence, we arrive the minimal model that describes the electronic properties of LaOFeAs.

cond-mat.str-el↗
arXiv2008

Minimal Model for Disorder-induced Missing Moment of Inertia in Solid $^4$He

The absence of a missing moment inertia in clean solid $^4$He suggests that the minimal experimentally relevant model is one in which disorder induces superfluidity in a bosonic lattice. To this end, we explore the relevance of the disordered Bose-Hubbard model in this context. We posit that a clean array $^4$He atoms is a self-generated Mott insulator, that is, the $^4$He atoms constitute the lattice as well as the `charge carriers'. With this assumption, we are able to interpret the textbook defect-driven supersolids as excitations of either the lower or upper Hubbard bands. In the experiments at hand, disorder induces a closing of the Mott gap through the generation of mid-gap localized states at the chemical potential. Depending on the magnitude of the disorder, we find that the destruction of the Mott state takes place for $d+z>4$ either through a Bose glass phase (strong disorder) or through a direct transition to a superfluid (weak disorder). For $d+z<4$, disorder is always relevant. The critical value of the disorder that separates these two regimes is shown to be a function of the boson filling, interaction and the momentum cut off. We apply our work to the experimentally observed enhancement $^3$He impurities has on the onset temperature for the missing moment of inertia. We find quantitative agreement with experimental trends.

cond-mat.dis-nn↗
arXiv2008

Breakdown of Fermi Liquid Theory in Doped Mott Insulators by Dynamical Spectral Weight Transfer

We show that doped Mott insulators exhibit a collective degree of freedom, not made out of the elemental excitations, because the number of single-particle addition states at low energy per electron per spin is greater than one. The presence of such a collective degree of freedom which is not a consequence of proximity to a phase transition is a consequence of dynamical spectral weight transfer from high to low energies. This physics is captured by the charge $2e$ boson that emerges by explicitly integrating out the high-energy scale in the Hubbard model. The charge $2e$ boson binds to a hole, thereby mediating new charge $e$ states at low energy. It is the presence of such charge $e$ states which have no counterpart in the non-interacting system that provides the general mechanism for the breakdown of Fermi liquid theory in doped Mott insulators. The relationship between the charge $2e$ boson formulation and the standard perturbative treatment is explained.

cond-mat.str-el↗
arXiv2008

Hidden Charge 2e Boson: Experimental Consequences for Doped Mott Insulators

We show here that many of the normal state properties of the cuprates can result from the new charge 2e bosonic field which we have recently (Phys. Rev. Lett. {\bf 99}, 46404 (2007) and Phys. Rev. B 77, 014512 (2008)) shown to exist in the exact low-energy theory of a doped Mott insulator. In particular, the 1) mid-infrared band including the non-vanishing of the restricted f-sum rule in the Mott insulator, 2) the $T^2$ contribution to the thermal conductivity, 3) the pseudogap, 4) the bifurcation of the electron spectrum below the chemical potential as recently seen in angle-resolved photoemission, 5) insulating behaviour away from half-filling, 6) the high and low-energy kinks in the electron dispersion and 7) T-linear resistivity all derive from the charge 2e bosonic field. We also calculate the inverse dielectric function and show that it possesses a sharp quasiparticle peak and a broad particle-hole continuum. The sharp peak is mediated by a new charge e composite excitation formed from the binding of a charge 2e boson and a hole and represents a distinctly new prediction of this theory. It is this feature that is responsible for dynamical part of the spectral weight transferred across the Mott gap. We propose that electron energy loss spectroscopy at finite momentum and frequency can be used to probe the existence of such a sharp feature.

cond-mat.str-el↗
arXiv2008

Exact Integration of the High Energy Scale in Doped Mott Insulators

We expand on our earlier work (cond-mat/0612130, Phys. Rev. Lett. {\bf 99}, 46404 (2007)) in which we constructed the exact low-energy theory of a doped Mott insulator by explicitly integrating (rather than projecting) out the degrees of freedom far away from the chemical potential. The exact low-energy theory contains degrees of freedom that cannot be obtained from projective schemes. In particular a new charge $\pm 2e$ bosonic field emerges at low energies that is not made out of elemental excitations. Such a field accounts for dynamical spectral weight transfer across the Mott gap. At half-filling, we show that two such excitations emerge which play a crucial role in preserving the Luttinger surface along which the single-particle Green function vanishes. In addition, the interactions with the bosonic fields defeat the artificial local SU(2) symmetry that is present in the Heisenberg model. We also apply this method to the Anderson-U impurity and show that in addition to the Kondo interaction, bosonic degrees of freedom appear as well. Finally, we show that as a result of the bosonic degree of freedom, the electron at low energies is in a linear superposition of two excitations--one arising from the standard projection into the low-energy sector and the other from the binding of a hole and the boson.

cond-mat.str-el↗
arXiv2007

Hidden Charge 2e Boson in Doped Mott Insulators: Field Theory of Mottness

We construct the low energy theory of a doped Mott insulator, such as the high-temperature superconductors, by explicitly integrating over the degrees of freedom far away from the chemical potential. For either hole or electron doping, a charge 2e bosonic field emerges at low energy. The charge 2e boson mediates dynamical spectral weight transfer across the Mott gap and creates a new charge e excitation by binding a hole. The result is a bifurcation of the electron dispersion below the chemical potential as observed recently in angle-resolved photoemission on Pb-doped Bi_2Sr_2CaCu_2O_{8+δ} (Pb2212).

cond-mat.str-el↗
arXiv2007

Cracking the Supersolid

We prepresent an overview of the status of experiment and theory on the supersolid state of matter.

cond-mat.supr-con↗
arXiv2007

Mottness

We review several of the normal state properties of the cuprates in an attempt to establish an organizing principle from which pseudogap phenomena, broad spectral features, $T-$linear resistivity, and spectral weight transfer emerge. We first show that standard field theories with a single critical length scale cannot capture the $T-$linear resistivity as long as the charge carriers are critical. What seems to be missing is an additional length scale, which may or may not be critical. Second, we prove a generalised version of Luttinger's theorem for a Mott insulator. Namely, regardless of the spatial dimension, the Fermi surface of the non-interacting system is converted into a surface of zeros of the single-particle Green function when the Mott insulator posesses particle-hole symmetry. Only in the presence of particle-hole symmetry does the volume of the surface of zeros equal the particle density. The surface of zeros persists at finite doping and is shown to provide a framework from which pseudogaps, broad spectral features, spectral weight transfer on the Mott gap scale can be understood.

cond-mat.str-el↗
arXiv2007

Squaring the Triangle: Insulating Ground State of $Na_{0.5}CoO_{2}$

We demonstrate that at a filling of $n=1.5$, an hexatic insulating state obtains in the extended Hubbard model on a triangular lattice. Composed of two tetragonal sublattices with fillings of $n=1$ and $n=2$, the insulating state is charge ordered and possesses an antiferromagnetic superlattice with dimension $a\times\sqrt{3}$. Two distinct energy scales arise in our model, a charge gap for the insulator and the effective exchange interaction in the antiferromagnet. Our model is capable of explaining both qualitatively and quantitatively the Hall coefficient including the sign change, the temperature dependence of the resistivity and the persistence of antiferromagnetism above the insulating state.

cond-mat.str-el↗
arXiv2006

Vortex Glass is a Metal: Unified Theory of the Magnetic Field and Disorder-Tuned Bose Metals

We consider the disordered quantum rotor model in the presence of a magnetic field. We analyze the transport properties in the vicinity of the multicritical point between the superconductor, phase glass and paramagnetic phases. We find that the magnetic field leaves metallic transport of bosons in the glassy phase in tact. In the vicinity of the vicinity of the superconductivity-to-Bose metal transition, the resistitivy turns on as $(H-H_c)^{2}$ with $H_c$. This functional form is in excellent agreement with the experimentally observed turn-on of the resistivity in the metallic state in MoGe, namely $R\approx R_c(H-H_c)^μ$, $1<μ<3$. The metallic state is also shown to presist in three spatial dimensions. In addition, we also show that the metallic state remains intact in the presence of Ohmic dissipation in spite of recent claims to the contrary. As the phase glass in $d=3$ is identical to the vortex glass, we conclude that the vortex glass is, in actuality, a metal rather than a superconductor at T=0. Our analysis unifies the recent experiments on vortex glass systems in which the linear resistivity remained non-zero below the putative vortex glass transition and the experiments on thin films in which a metallic phase has been observed to disrupt the direct transition from a superconductor to an insulator.

cond-mat.supr-con↗
arXiv2005

Breakdown of One-Paramater Scaling in Quantum Critical Scenarios for the High-Temperature Copper-oxide Superconductors

We show that if the excitations which become gapless at a quantum critical point also carry the electrical current, then a resistivity linear in temperature, as is observed in the copper-oxide high-temperature superconductors, obtains only if the dynamical exponent, $z$, satisfies the unphysical constraint, $z<0$. At fault here is the universal scaling hypothesis that, at a continuous phase transition, the only relevant length scale is the correlation length. Consequently, either the electrical current in the normal state of the cuprates is carried by degrees of freedom which do not undergo a quantum phase transition, or quantum critical scenarios must forgo this basic scaling hypothesis and demand that more than a single correlation length scale is necessary to model transport in the cuprates.

cond-mat.str-el↗
arXiv2005

Doped Mott insulators are insulators: hole localization in the cuprates

We demonstrate that a Mott insulator lightly doped with holes is still an insulator at low temperature even without disorder. Hole localization obtains because the chemical potential lies in a pseudogap which has a vanishing density of states at zero temperature. The energy scale for the pseudogap is set by the nearest-neighbour singlet-triplet splitting. As this energy scale vanishes if transitions, virtual or otherwise, to the upper Hubbard band are not permitted, the fundamental length scale in the pseudogap regime is the average distance between doubly occupied sites. Consequently, the pseudogap is tied to the non-commutativity of the two limits $U\to\infty$ ($U$ the on-site Coulomb repulsion) and $L\to\infty$ (the system size).

cond-mat.str-el↗
arXiv2004

Breakdown of Strong-Coupling Perturbation Theory in Doped Mott Insulators

We show that doped Mott insulators, such as the copper-oxide superconductors, are asymptotically slaved in that the quasiparticle weight, $Z$, near half-filling depends critically on the existence of the high energy scale set by the upper Hubbard band. In particular, near half filling, the following dichotomy arises: $Z\ne 0$ when the high energy scale is integrated out but Z=0 in the thermodynamic limit when it is retained. Slavery to the high energy scale arises from quantum interference between electronic excitations across the Mott gap. Broad spectral features seen in photoemission in the normal state of the cuprates are argued to arise from high energy slavery.

cond-mat.str-el↗
arXiv2004

Higher order effective low-energy theories

Three well-known perturbative approaches to deriving low-energy effective theories, the degenerate Brillouin-Wigner perturbation theory (projection method), the canonical transformation, and the resolvent methods are compared. We use the Hubbard model as an example to show how, to fourth order in hopping t, all methods lead to the same effective theory, namely the t-J model with ring exchange and various correlated hoppings. We emphasize subtle technical difficulties that make such a derivation less trivial to carry out for orders higher than second. We also show that in higher orders, different approaches can lead to seemingly different forms for the low-energy Hamiltonian. All of these forms are equivalent since they are connected by an additional unitary transformation whose generator is given explicitly. The importance of transforming the operators is emphasized and the equivalence of their transformed structure within the different approaches is also demonstrated.

cond-mat.str-el↗
arXiv2004

The Full Mottness

Though most fermionic Mott insulators order at low temperatures, ordering is ancillary to their insulating behaviour. Our emphasis here is on disentangling ordering from the intrinsic strongly correlated physics of a doped half-filled band. To this end, we focus on the 2D Hubbard model. Because the charge gap arises from on-site correlations, we implement a non-perturbative approach which incorporates local physics. Crucial to this method is a self-consistent two-site dynamical cluster expansion which builds in the nearest-neighbour energy scale, $J$. At half-filling, we find that the spectral function possesses a gap of order $U$ and is devoid of any coherent quasi-particle peaks. In the doped case, we find that the Fermi surface exceeds the Luttinger volume. Additionally in the underdoped regime, we find that a pseudogap opens in the single particle density of states.The pseudogap closes above optimal doping and hence our proposal is not inconsistent with that of Loram. In analogy with the Mott gap and antiferromagnetism, we propose that ordering may also accompany the formation of a pseudogap. We suggest a current pattern within a 1-band model that preserves translational but breaks time-reversal symmetry along the canonical x and y axes but not along $x=\pm y$ that is consistent with the experimental observations. Finally, we show that the Hall coefficient in a doped Mott insulator must change sign at a doping level $x<1/3$. The sign change is tied to a termination of strong correlation physics in the doped Mott state.

cond-mat.str-el↗
arXiv2003

The Elusive Bose Metal

The conventional theory of metals is in crisis. In the last 15 years, there has been an unexpected sprouting of metallic states in low dimensional systems directly contradicting conventional wisdom. For example, bosons are thought to exist in one of two ground states: condensed in a superconductor or localized in an insulator. However, several experiments on thin metal alloy films have observed that a metallic phase disrupts the direct transition between the superconductor and the insulator. We analyze the experiments on the insulator-superconductor transition and argue that the intervening metallic phase is bosonic. All relevant theoretical proposals for the Bose metal are discussed, particularly the recent idea that the metallic phase is glassy. The implications for the putative vortex glass state in the copper-oxide superconductors are examined.

cond-mat.supr-con↗