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Pierre A. Pantaleon

Publications and source records attributed to Pierre A. Pantaleon.

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The First Magic Angle Beyond the Chiral Limit in Twisted Bilayer Graphene

We develop a squared-Hamiltonian description of twisted bilayer graphene beyond the chiral limit to explain why the first magic angle remains robust under lattice relaxation, while higher-order magic angles are strongly destabilized. Starting from the non-chiral Bistritzer--MacDonald model with finite same-sublattice tunneling, we show that lattice relaxation reshapes the effective confinement landscape rather than acting as a simple perturbation of the chiral theory. A central result is that the realistic relaxation-renormalized tunneling ratio lies close to a special confinement point where the oscillatory part of the symmetric confinement potential nearly cancels. This places realistic twisted bilayer graphene near a nearly uniform confinement regime. At the same time, finite same-sublattice tunneling activates an additional inter-sublattice current-like channel that competes with the chiral orbital channel. The first magic angle survives because these confinement and current-like contributions remain balanced, whereas higher-order magic angles lose this balance through stronger remote-band hybridization and enhanced real-space localization around AA regions. Our results provide a single-particle mechanism for the breakdown of the chiral magic-angle hierarchy and clarify why the experimentally relevant first magic angle remains the most stable remnant of the chiral flat-band structure.

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Interaction-driven charge textures and unconventional superconductivity in strained monolayer graphene

Two-dimensional systems with flat bands support correlated phases such as superconductivity. While twisted moiré systems, like twisted bilayer graphene, have revealed such states, they remain complex to control. Here, we study monolayer graphene under uniaxial periodic strain, which forms a quasi-one-dimensional moiré lattice that hosts two flat sublattice-polarized bands. When electron-electron interactions are included at the self-consistent Hartree level, we find features familiar from moiré flat-band systems, such as Fermi-level pinning to the Van Hove singularity and a Kohn-Luttinger-like pairing instability. In addition, we find strong interband enhancement of the pairing scale and higher-energy metastable electrostatic textures in enlarged supercells, with charge localized in selected regions of multiple unit cells.

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Mode-Resolved Multiband Ballistic Transport and Conductance Thresholds in Bilayer Graphene Junctions

We study ballistic transport in bilayer graphene junctions and show how electrostatic gating, interlayer bias, and homogeneous strain provide complementary control over electron transmission. In the absence of strain, transport is governed by symmetry constraints that suppress transmission at specific incidence angles despite the availability of states. An interlayer bias lifts this suppression through mode mixing and opens a tunable transport gap. Within a full four-band description, we identify a distinct conductance threshold that marks the onset of propagation of the upper band inside the barrier. This produces a clear change in the slope of the conductance and serves as an experimentally accessible transport fingerprint of the multiband structure and interlayer coupling. Homogeneous in-plane strain acts as a geometric control mechanism. By reshaping the band structure in momentum space, it redistributes the angular transmission window and suppresses conductance without introducing disorder. Importantly, strain preserves the underlying symmetry-based decoupling responsible for transmission suppression while shifting its condition away from normal incidence. These results provide a unified framework for interpreting angle-resolved transport in bilayer graphene and establish multiband ballistic transport as a practical probe of band-structure geometry.

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Revealing quantum geometry effects in magic angle twisted bilayer graphene using the circular photogalvanic effect

We report a photocurrent studies of a magic angle twisted bilayer graphene device using near infrared light. Through photocurrent imaging and polarization dependence, we separate the photo-thermoelectric effect from the photogalvanic effect. We observe a circular photogalvanic effect (CPGE) over a wide range of doping and temperature. The CPGE at normal incidence constraints the symmetry of the system to C$_1$, and points to a Berry curvature dipole, in agreement with theoretical predictions for strained graphene. Remarkably, the CPGE vanishes for filling $-2.5 < ν< -1.5$, suggesting an additional symmetry breaking in that regime. Insight into this effect is obtained through Berry curvature dipole calculations, which emphasize a novel symmetry breaking effect near $ν=-2$.

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Mode-selective cloaking and phase-matching cavity resonances in bilayer graphene transport

We study ballistic electron transport through electrostatic barriers in AB-stacked bilayer graphene within a full four-band framework. A mode-resolved analysis reveals how propagating and evanescent channels couple across electrostatic interfaces and how channel selectivity governs transport at normal incidence. We show that perfect transmission can occur at discrete energies due to phase matching of a single internal mode within an individual barrier, without activating the decoupled channels. This effect is interpreted as a phase-matching cavity, namely, an effective cavity formed by internal phase coherence inside the barrier, which yields perfect transmission at discrete energies without true bound states and without opening additional transport channels. For single- and double-barrier geometries, we derive compact analytical expressions for the transmission and identify the corresponding resonance conditions. Extending the analysis to multibarrier structures using a transfer-matrix approach, we demonstrate how perfect resonances driven by internal phase matching coexist with Fabry-Perot-type resonances arising from interbarrier interference. Our results provide a unified, channel-resolved description of tunneling suppression and resonance-assisted transport in bilayer graphene barrier systems.

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Twistraintronics in Square Moire Superlattices of Stacked Graphene Layers

We report the first observation of controlled, strain-induced square moire patterns in stacked graphene. By selectively displacing native wrinkles, we drive a reversible transition from the usual trigonal to square moire order. Scanning tunneling microscopy reveals elliptically shaped AA domains, while spectroscopy shows strong electronic correlation in the form of narrow bands with split Van Hove singularities near the Fermi level. A continuum model with electrostatic interactions reproduces these features under the specific twist-strain combination that minimizes elastic energy. This work demonstrates that the combination of twist and strain, or twistraintronics, enables the realization of highly correlated electronic states in moire heterostructures with geometries that were previously inaccessible.

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Topological phase diagram of twisted bilayer graphene as a function of the twist angle

Twisted bilayer graphene (TBG) hosts a rich landscape of electronic phases arising from the interplay between strong electron-electron interactions and nontrivial band topology. While the flat bands near zero energy are central to many correlated phenomena, their interaction with higher-energy remote bands remains less understood. Here, we investigate these hybridization processes as a function of the twist angle and analyze their impact on the charge distribution, topological properties such as Chern number, quantum metric, and orbital magnetic energy. We identify multiple topological phase transitions between magic angles, driven by band inversions at high-symmetry points in momentum space. Notably, the central bands can exhibit phases with Chern numbers C = 2, revealing previously unreported topological states in TBG.

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Designing Flat Bands and Pseudo-Landau Levels in GaAs with Patterned Gates

We investigate the electronic properties of two-dimensional electron gases (2DEGs) subjected to a periodic patterned gate. By incorporating the superlattice (SL) potential induced by patterning into the Schrodinger equation, we develop a methodology for obtaining exact analytical solutions. These solutions enable us to construct a comprehensive phase diagram illustrating the emergence of narrow bands and pseudo-Landau levels driven by the SL potential. To complement the analytical approach, we employ a standard plane-wave formalism to track the evolution of the band structure as the SL strength increases. By breaking the inversion symmetry of the SL potential, we found a nontrivial Berry curvature. Furthermore, we introduce a self-consistent Hartree screening to account for the interplay between the SL potential and electronic interactions. Our findings not only reveal the emergence of a non-trivial quantum geometry and a competition between SL strength and electron-electron interactions, but also highlight the value of exact analytical solutions for understanding and engineering electronic phases in patterned 2DEG systems.

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Band Renormalization, Quarter Metals, and Chiral Superconductivity in Rhombohedral Tetralayer Graphene

Recently, exotic superconductivity emerging from a spin-and-valley-polarized metallic phase has been discovered in rhombohedral tetralayer graphene. To explain this observation, we study the role of electron-electron interactions in driving flavor symmetry breaking, using the Hartree-Fock (HF) approximation, and in stabilizing superconductivity mediated by repulsive interactions. Though mean-field HF correctly predicts the isospin flavors and reproduces the experimental phase diagram, it overestimates the band renormalization near the Fermi energy and suppresses superconducting instabilities. To address this, we introduce a physically motivated scheme that includes internal screening in the HF calculation. Using this formalism, we find superconductivity arising from the spin-valley polarized phase for a range of electric fields and electron dopings. Our findings reproduce the experimental observations and reveal a p-wave, finite-momentum, time-reversal-symmetry-broken superconducting state, encouraging further investigation into exotic phases in graphene multilayers.

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Designing Moire Patterns by Shearing

We analyze the elastic properties, structural effects, and low-energy physics of a sheared nanoribbon placed on top of graphene, which creates a gradually changing moire pattern. By means of a classical elastic model we derive the strains in the ribbon and we obtain its electronic energy spectrum with a scaled tight-binding model. The size of the sheared region is determined by the balance between elastic and van der Waals energy, and different regimes are identified. Near the clamped edge, moderate strains and small twist angles lead to one-dimensional channels. Near the sheared edge, a long region behaves like magic angle twisted bilayer graphene (TBG), showing a sharp peak in the density of states, mostly isolated from the rest of the spectrum. We also calculate the band topology along the ribbon and we find that it is stable for large intervals of strains and twist angles. Together with the experimental observations, these results show that the sheared nanoribbon geometry is ideal for exploring superconductivity and correlated phases in TBG in the very sought-after regime of ultralow twist angle disorder.

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Electronic Structure and Kohn-Luttinger Superconductivity of Heavily-Doped Single-Layer Graphene

The existence of superconductivity (SC) in graphene appears to be established in both twisted and non-twisted multilayers. However, whether their building block, single-layer graphene (SLG), can also host SC remains an open question. Earlier theoretical works predicted that SLG could become a chiral d-wave superconductor driven by electronic interactions when doped to its van Hove singularity, but questions such as whether the d-wave SC survives the strong band renormalizations seen in experiments, its robustness against the source of doping, or if it will occur at any reasonable critical temperature (Tc) have remained difficult to answer, in part due to uncertainties in model parameters. In this study, we adopt a random-phase approximation framework based on a Kohn-Luttinger-like mechanism to investigate SC in heavily-doped SLG. We predict that robust d+id topological SC could arise in SLG doped by Tb, with a Tc up to 600 mK. We also investigate the possibility of realizing d-wave SC by employing other dopants, such as Li or Cs. The structural models have been derived from angle-resolved photoemission spectroscopy measurements on Tb-doped graphene and first-principles calculations for Cs and Li doping. We find that dopants that change the lattice symmetry of SLG are detrimental to the d-wave state. The stability of the d-wave SC predicted here in Tb-doped SLG could provide a valuable insight for guiding future experimental efforts aimed at exploring topological superconductivity in monolayer graphene.

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Double-edged Role of Interactions in Superconducting Twisted Bilayer Graphene

For the unconventional superconducting phases in moire materials, a critical question is the role played by electronic interactions in the formation of Cooper pairs. In twisted bilayer graphene (tBLG), the strength of electronic interactions can be reduced by increasing the twist angle or screening provided by the dielectric medium. In this work, we place tBLG at 3-4 nm above bulk SrTiO3 substrates, which have a large yet tunable dielectric constant. By raising the dielectric constant in situ in a magic angle device, we observe suppression of both the height and the width of the entire superconducting dome, thus demonstrating that, unlike conventional superconductors, the pairing mechanism in tBLG is strongly dependent on electronic interactions. Interestingly, in contrast to the absence of superconductivity in devices on SiO2 with angle>1.3 deg, we observe a superconducting pocket in a large-angle (angle=1.4 deg) tBLG/STO device while the correlated insulating states are absent. These experimental results are in qualitative agreement with a theoretical model in which the pairing mechanism arises from Coulomb interactions that are screened by plasmons, electron-hole pairs, and longitudinal acoustic phonons. Our results highlight the unconventional nature of the superconductivity in tBLG, the double-edged role played by electronic interactions in its formation, as well as their complex interplay with the correlated insulating states.

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Designing Band Structures by Patterned Dielectric Superlattices

We investigate the electronic structure of graphene monolayers subjected to patterned dielectric superlattices. Through a quantum capacitance model approach, we simulate realistic devices capable of imposing periodic potentials on graphene. By means of both tight-binding and continuum models, we analyze the electronic structure across varied patterning geometries, including triangular, kagome, and square configurations. We explicitly explore the influence of device parameters such as the superlattice potential strength, geometry, and periodicity on the electronic properties of graphene. By introducing a long-range Coulomb interaction, we found an emergent periodic potential strong enough to open a mass gap, thereby generating a Chern band. Our study highlights the robustness and versatility of patterned dielectric superlattices for band engineering in graphene systems.

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Evolution of Superconductivity in Twisted Graphene Multilayers

The group of moiré graphene superconductors keeps growing, and by now it contains twisted graphene multilayers and twisted double bilayers. We analyze the contribution of long range charge fluctuations in the superconductivity of twisted double graphene bilayers and helical trilayers, and compare the results to twisted bilayer graphene. We apply a diagrammatic approach which depends on a few, well known parameters. We find that the critical temperature and the order parameter differ significantly between twisted double bilayers and helical trilayers on one hand, and twisted bilayer graphene on the other. We show that this trend, consistent with experiments, can be associated to the role played by moiré Umklapp processes in the different systems.

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Superconductivity and correlated phases in non-twisted bilayer and trilayer graphene

Twisted bilayer graphene has a rich phase diagram, including superconductivity. Recently, an unexpected discovery has been the observation of superconductivity in non-twisted graphene bilayers and trilayers. In this Perspective, we give an overview of the search for uncommon phases in non-twisted graphene systems. We first contextualize these recent results within earlier work in the field, before examining the new experimental findings. Finally, we analyse the numerous theoretical models that study the underlying physical processes in these systems

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Narrow bands, electrostatic interactions and band topology in graphene stacks

The occurrence of superconducting and insulating phases is well-established in twisted graphene bilayers, and they have also been reported in other arrangements of graphene layers. We investigate three such arrangements: untwisted AB bilayer graphene on an hBN substrate, two graphene bilayers twisted with respect to each other, and a single ABC stacked graphene trilayer on an hBN substrate. Narrow bands with different topology occur in all cases, producing a high density of states which enhances the role of interactions. We investigate the effect of the long range Coulomb interaction, treated within the self consistent Hartree-Fock approximation. We find that the on-site part of the Fock potential strongly modifies the band structure at charge neutrality. The Hartree part does not significantly modify the shape and width of the bands in the three cases considered here, in contrast to the effect that such a potential has in twisted bilayer graphene.

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Band structure of twisted bilayer graphene on hexagonal boron nitride

The effect of an hexagonal boron nitride (hBN) layer close aligned with twisted bilayer graphene (TBG) is studied. At sufficiently low angles between twisted bilayer graphene and hBN, $θ_{hBN} \lesssim 2^\circ$, the graphene electronic structure is strongly disturbed. The width of the low energy peak in the density of states changes from $W \sim 5 - 10$ meV for a decoupled system to $\sim 20 - 30$ meV. Spikes in the density of states due to van Hove singularities are smoothed out. We find that for a realistic combination of the twist angle in the TBG and the twist angle between the hBN and the graphene layer the system can be described using a single moiré unit cell.

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Topological Magnon Insulator with a Kekule Bond Modulation

We examine the combined effects of a Kekule coupling texture (KC) and a Dzyaloshinskii-Moriya interaction (DMI) in a two-dimensional ferromagnetic honeycomb lattice. By analyzing the gap closing conditions and the inversions of the bulk bands, we identify the parameter range in which the system behaves as a trivial or a nontrivial topological magnon insulator. We find four topological phases in terms of the KC parameter and the DMI strength. We present the bulk-edge correspondence for the magnons in a honeycomb lattice with an armchair or a zigzag boundary. Furthermore, we find Tamm-like edge states due to the intrinsic on-site interactions along the boundary sites. Our results may have significant implications to magnon transport properties in the 2D magnets at low temperatures.

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