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Robert S. Whitney

Publications and source records attributed to Robert S. Whitney.

At least 19 recordsLinked to original sources

Improving photovoltaics by adding extra terminals to extract hot carriers

Photovoltaic cells usually have two terminals, one collecting electrons and the other collecting holes. Can more terminals improve such solar cells? Energy-filtering terminals could collect "hot" carriers (electrons or holes not yet relaxed to the band edge), with other terminals for low-energy carriers. When collection is faster than carrier-phonon relaxation, we predict that four-terminal cells have higher power output than optimal two-terminal cells, often 20-40% higher. Similar effects will occur in multi-terminal thermoelectrics exploiting non-equilibrium distributions.

cond-mat.mes-hall

Magic states are rarely the best resource to optimize: An analytical tool for qubit resource estimation in concatenated codes

Concatenated error-correction schemes are well-understood routes to fault-tolerant quantum computing, and research on such schemes continues, including recent claims that they may be competitive with surface codes, and show potential when combined with high-rate Quantum Low Density Parity Check codes. However, there are few tools to evaluate the qubit resources required by concatenated schemes. We propose such a tool here. Its equations are closed-form and remain simple for an arbitrary number of levels of concatenation, making it ideal for comparing and minimizing the resource costs of such schemes. We use this tool to evaluate the resources for gate operations that require the injection of so-called ``magic states'', needed to complete the set of logical operations. It was expected that the complexity of such ``magic operations" would make them dominate the resource costs of a calculation, with numerous works proposing optimizations of these cost. Our work reveals that this expectation is often inaccurate: Magic operations are rarely the dominant cost of concatenated schemes, mirroring similar conclusions from past work for surface codes. Optimizations affecting all operations naturally have more impact than those on magic operations alone, yet we unexpected find that the former can reduce qubit resources by a few orders of magnitude while the latter give only marginal reductions. We show this in detail for a 7-qubit concatenated scheme with Steane error-correction gadgets or flag-qubits gadgets, and argue that our findings are representative of most concatenated schemes.

quant-ph

Going beyond Landauer scattering theory to describe spatially-resolved non-local heating and cooling in quantum thermoelectrics

Spatially-resolved heating and cooling in nanostructures is nowadays measured with various nanoscale thermometry techniques, including scanning thermometry. Yet the most commonly used theory of nanoscale heating and thermoelectricity -- Landauer scattering theory -- is not appropriate to model such measurements. Hence, we analyze a minimal model of spatially-resolved heat transfer between electrons and phonons in simple thermoelectric nanostructures. This combines Landauer scattering formalism with a Boltzmann equation for transport, revealing the non-locality of Joule heating and Peltier cooling induced by a scatterer in a nanowire. The corresponding heating or cooling of the phonons is caused by the voltage drop at the scatterer, but is often maximal at a certain distance from the scatterer. This distance is of the order of the electron-phonon scattering length. Scanning thermal microscopy, such as SQUID-on-tip thermometers, should detect this non-locality as phonon hot spots and cold spots, spatially separated from the scatterer. We provide physical arguments explaining the thermoelectric response of the combined system of wire and scatterer, and in particular, why the resulting heating and cooling is sometimes the opposite to that predicted by the standard Landauer scattering theory.

cond-mat.mes-hall

Reservoir-Free Decoherence in Flying Qubits

An effective time-dependent Hamiltonian can be implemented by making a quantum system fly through an inhomogeneous potential, realizing, for example, a quantum gate on its internal degrees of freedom. However, flying systems have a spatial spread that will generically entangle the internal and spatial degrees of freedom, leading to decoherence in the internal state dynamics, even in the absence of any external reservoir. We provide formulas valid at all times for the dynamics, fidelity, and change of entropy for ballistic particles with small spatial spreads, quantified by $Δx$. This non-Markovian decoherence can be significant for ballistic flying qubits (scaling as $Δx^2$) but usually not for flying qubits carried by a moving potential well (scaling as $Δx^6$). We also discuss a method to completely counteract this decoherence for a ballistic qubit later measured.

quant-ph

Constraints between entropy production and its fluctuations in nonthermal engines

We analyze a mesoscopic conductor autonomously performing a thermodynamically useful task, such as cooling or producing electrical power, in a part of the system -- the working substance -- by exploiting another terminal or set of terminals -- the resource -- that contains a stationary nonthermal (nonequilibrium) distribution. Thanks to the nonthermal properties of the resource, on average no exchange of particles or energy with the working substance is required to fulfill the task. This resembles the action of a demon, as long as only average quantities are considered. Here, we go beyond a description based on average currents and investigate the role of fluctuations in such a system. We show that a minimum level of entropy fluctuations in the system is necessary, whenever one is exploiting a certain entropy production in the resource terminal to perform a useful task in the working substance. For concrete implementations of the demonic nonthermal engine in three- and four-terminal electronic conductors in the quantum Hall regime, we compare the resource fluctuations to the entropy production in the resource and to the useful engine output (produced power or cooling power).

cond-mat.mes-hall

Optimizing resource efficiencies for scalable full-stack quantum computers

In the race to build scalable quantum computers, minimizing the resource consumption of their full stack to achieve a target performance becomes crucial. It mandates a synergy of fundamental physics and engineering: the former for the microscopic aspects of computing performance, and the latter for the macroscopic resource consumption. For this we propose a holistic methodology dubbed Metric-Noise-Resource (MNR) able to quantify and optimize all aspects of the full-stack quantum computer, bringing together concepts from quantum physics (e.g., noise on the qubits), quantum information (e.g., computing architecture and type of error correction), and enabling technologies (e.g., cryogenics, control electronics, and wiring). This holistic approach allows us to define and study resource efficiencies as ratios between performance and resource cost. As a proof of concept, we use MNR to minimize the power consumption of a full-stack quantum computer, performing noisy or fault-tolerant computing with a target performance for the task of interest. Comparing this with a classical processor performing the same task, we identify a quantum energy advantage in regimes of parameters distinct from the commonly considered quantum computational advantage. This provides a previously overlooked practical argument for building quantum computers. While our illustration uses highly idealized parameters inspired by superconducting qubits with concatenated error correction, the methodology is universal -- it applies to other qubits and error-correcting codes -- and provides experimenters with guidelines to build energy-efficient quantum processors. In some regimes of high energy consumption, it can reduce this consumption by orders of magnitudes. Overall, our methodology lays the theoretical foundation for resource-efficient quantum technologies.

quant-ph

Thermodynamic performance of hot-carrier solar cells: A quantum transport model

In conventional solar cells, photogenerated carriers lose part of their energy before they can be extracted to make electricity. The aim of hot-carrier solar cells is to extract the carriers before this energy loss, thereby turning more energy into electrical power. This requires extracting the carriers in a nonequilibrium (nonthermal) energy distribution. Here, we investigate the performance of hot-carrier solar cells for such nonequilibrium distributions. We propose a quantum transport model in which each energy-loss process (carrier thermalization, relaxation, and recombination) is simulated by a Büttiker probe. We study charge and heat transport to analyze the hot-carrier solar cell's power output and efficiency, introducing partial efficiencies for different loss processes and the carrier extraction. We show that producing electrical power from a nonequilibrium distribution has the potential to improve the output power and efficiency. Furthermore, in the limit where the distribution is thermal, we prove that a boxcar-shaped transmission for the carrier extraction maximizes the efficiency at any given output power.

cond-mat.mes-hall

Illusory cracks in the second law of thermodynamics in quantum nanoelectronics

This is a review of the theory of quantum thermodynamic demons; these are quantum systems that look like they violate the laws of thermodynamics, in analogy with Maxwell's demon. It concentrates on autonomous demons that can be made using nanoelectronics. Here ``autonomous'' means that the demon operates without any external measurement or driving, making it possible to model their entire thermodynamic behaviour using Schrödinger's equation. My main aim is to review why cracks in the laws of thermodynamics, sometimes glimpsed in such systems, have turned out to be illusory. For this, I work by example, introducing the methods of quantum thermodynamics via an old thought experiment that appears to break the second law. This thought experiment is usually known as Smoluchowski's trapdoor, although it was first proposed by Maxwell. Smoluchowski showed that the trapdoor's thermal motion complicates its dynamics, but I argue that he did not show that it must obey the second law. This question is now of practical relevance, because a nanoelectronic version of the trapdoor can be made with quantum dots. The methods presented here show that such a quantum trapdoor obeys the laws of thermodynamics. This reviews then addresses other types of autonomous demon that superficially appear to break the laws of thermodynamics, but which do not. These include an experimental demonstration of a Maxwell demon, and a kind of demon that exploit non-equilibrium resources (the N-demon). It discusses a way of classifying different kinds of autonomous demon. It concludes by briefly reviewing how fluctuations affect nanoelectronics, and how their role in stochastic thermodynamics changes our view of entropy.

cond-mat.mes-hall

Limitations in quantum computing from resource constraints

Fault-tolerant schemes can use error correction to make a quantum computation arbitrarily ac- curate, provided that errors per physical component are smaller than a certain threshold and in- dependent of the computer size. However in current experiments, physical resource limitations like energy, volume or available bandwidth induce error rates that typically grow as the computer grows. Taking into account these constraints, we show that the amount of error correction can be opti- mized, leading to a maximum attainable computational accuracy. We find this maximum for generic situations where noise is scale-dependent. By inverting the logic, we provide experimenters with a tool to finding the minimum resources required to run an algorithm with a given computational accuracy. When combined with a full-stack quantum computing model, this provides the basis for energetic estimates of future large-scale quantum computers.

quant-ph

Non-Markovian quantum thermodynamics: laws and fluctuation theorems

This work brings together Keldysh non-equilibrium quantum theory and thermodynamics, by showing that a real-time diagrammatic technique is an equivalent of stochastic thermodynamics for non-Markovian quantum machines (heat engines, refrigerators, etc). Symmetries are found between quantum trajectories and their time-reverses on the Keldysh contour, for any interacting quantum system coupled to ideal reservoirs of electrons, phonons or photons. These lead to quantum fluctuation theorems the same as the well-known classical ones (Jarzynski and Crooks equalities, integral fluctuation theorem, etc), whether the system's dynamics are Markovian or not. Some of these are also shown to hold for non-factorizable initial states. The sequential tunnelling approximation and the cotunnelling approximation are both shown to respect the symmetries that ensure the fluctuation theorems. For all initial states, energy conservation ensures that the first law of thermodynamics holds on average, while the above symmetries ensures that the second law of thermodynamics holds on average, even if fluctuations violate it. [ERRATUM added: March 2021]

cond-mat.mes-hall

Shot-noise of quantum chaotic systems in the classical limit

Semiclassical methods can now explain many mesoscopic effects (shot-noise, conductance fluctuations, etc) in clean chaotic systems, such as chaotic quantum dots. In the deep classical limit (wavelength much less than system size) the Ehrenfest time (the time for a wavepacket to spread to a classical size) plays a crucial role, and random matrix theory (RMT) ceases to apply to the transport properties of open chaotic systems. Here we summarize some of our recent results for shot-noise (intrinsically quantum noise in the current through the system) in this deep classical limit. For systems with perfect coupling to the leads, we use a phase-space basis on the leads to show that the transmission eigenvalues are all 0 or 1 -- so transmission is noiseless [Whitney-Jacquod, Phys. Rev. Lett. 94, 116801 (2005), Jacquod-Whitney, Phys. Rev. B 73, 195115 (2006)]. For systems with tunnel-barriers on the leads we use trajectory-based semiclassics to extract universal (but non-RMT) shot-noise results for the classical regime [Whitney, Phys. Rev. B 75, 235404 (2007)].

cond-mat.mes-hall

Quantifying nonequlibrium thermodynamic operations in a multiterminal mesoscopic system

We investigate a multiterminal mesoscopic conductor in the quantum Hall regime, subject to temperature and voltage biases. The device can be considered as a nonequilibrium resource acting on a working substance. We previously showed that cooling and power production can occur in the absence of energy and particle currents from a nonequilibrium resource (calling this an N-demon). Here we allow energy or particle currents from the nonequilibrium resource and find that the device seemingly operates at a better efficiency than a Carnot engine. To overcome this problem, we define free-energy efficiencies which incorporate the fact that a nonequilibrium resource is consumed in addition to heat or power. These efficiencies are well behaved for equilibrium and nonequilibrium resources and have an upper bound imposed by the laws of thermodynamics. We optimize power production and cooling in experimentally relevant parameter regimes.

cond-mat.mes-hall

Comment on "Inconsistency of the conventional theory of superconductivity" by J.E. Hirsch

J. E. Hirsch [EPL 130 (2020) 17006] claimed an inconsistency between thermodynamics and the theory of superconductivity. We argue that he overlooked a crucial term which determines the supercurrent dynamics and ensures energy conservation by providing an internal energy source for the Joule heating. Thermodynamic consistency is restored by restoring energy conservation. The correct dynamics is given by Maxwell's equations in the superconductor.

cond-mat.supr-con

Multiple perfectly-transmitting states of a single-level at strong coupling

We study transport through a single-level system placed between two reservoirs with band-structure, taking strong level-reservoir coupling of the order of the energy-scales of these band-structures. An exact solution in the absence of interactions gives the nonlinear Lamb shift. As expected, this moves the perfectly-transmitting state (the reservoir state that flows through the single-level without reflection), and can even turn it into a bound-state. However, here we show that it can also create additional pairs of perfectly-transmitting states at other energies, when the coupling exceeds critical values. Then the single-level's transmission function resembles that of a multi-level system. Even when the discrete level is outside the reservoirs' bands, additional perfectly-transmitting states can appear inside the band when the coupling exceeds a critical value. We propose observing the bosonic version of this in microwave cavities, and the fermionic version in the conductance of a quantum dot coupled to 1D or 2D reservoirs.

cond-mat.mes-hall

Non-equilibrium System as a Demon

Maxwell demons are creatures that are imagined to be able to reduce the entropy of a system without performing any work on it. Conventionally, such a Maxwell demon's intricate action consists of measuring individual particles and subsequently performing feedback. Here we show that much simpler setups can still act as demons: we demonstrate that it is sufficient to exploit a non-equilibrium distribution to seemingly break the second law of thermodynamics. We propose both an electronic and an optical implementation of this phenomenon, realizable with current technology.

cond-mat.mes-hall

Signature of the transition to a bound state in thermoelectric quantum transport

We study a quantum dot coupled to two semiconducting reservoirs, when the dot level and the electrochemical potential are both close to a band edge in the reservoirs. This is modelled with an exactly solvable Hamiltonian without interactions (the Fano-Anderson model). The model is known to show an abrupt transition as the dot-reservoir coupling is increased into the strong-coupling regime for a broad class of band structures. This transition involves an infinite-lifetime bound state appearing in the band gap. We find a signature of this transition in the continuum states of the model, visible as a discontinuous behaviour of the dot's transmission function. This can result in the steady-state DC electric and thermoelectric responses having a very strong dependence on coupling close to critical coupling. We give examples where the conductances and the thermoelectric power factor exhibit huge peaks at critical coupling, while the thermoelectric figure of merit ZT grows as the coupling approaches critical coupling, with a small dip at critical coupling. The critical coupling is thus a sweet spot for such thermoelectric devices, as the power output is maximal at this point without a significant change of efficiency.

cond-mat.mes-hall

Adiabatic almost-topological pumping of fractional charges in non-interacting quantum dots

We use exact techniques to demonstrate theoretically the pumping of fractional charges in a single-level non-interacting quantum dot, when the dot-reservoir coupling is adiabatically driven from weak to strong coupling. The pumped charge averaged over many cycles is quantized at a fraction of an electron per cycle, determined by the ratio of Lamb shift to level-broadening; this ratio is imposed by the reservoir band-structure. For uniform density of states, half an electron is pumped per cycle. We call this "adiabatic almost-topological pumping", because the pumping's Berry curvature is sharply peaked in the parameter space. Hence, so long as the pumping contour does not touch the peak, the pumped charge depends only on how many times the contour winds around the peak (up to exponentially small corrections). However, the topology does not protect against non-adiabatic corrections, which grow linearly with pump speed. In one limit the peak becomes a delta-function, so the adiabatic pumping of fractional charges becomes entirely topological. Our results show that quantization of the adiabatic pumped charge at a fraction of an electron does not require fractional particles or other exotic physics.

cond-mat.mes-hall

Thermoelectric coefficients and the figure of merit for large open quantum dots

We consider the thermoelectric response of chaotic or disordered quantum dots in the limit of phase-coherent transport, statistically described by random matrix theory. We calculate the full distribution of the thermoelectric coefficients (Seebeck $S$ and Peltier $Π$), and the thermoelectric figure of merit $ZT$, for large open dots at arbitrary temperature and external magnetic field, when the number of modes in the left and right leads ($N_{\rm L}$ and $N_{\rm R}$) are large. Our results show that the thermoelectric coefficients and $ZT$ are maximal when the temperature is half the Thouless energy, and the magnetic field is negligible. They remain small, even at their maximum, but they exhibit a type of universality at all temperatures, in which they do not depend on the asymmetry between the left and right leads $(N_{\rm L}-N_{\rm R})$, even though they depend on $(N_{\rm L}+N_{\rm R})$.

cond-mat.mes-hall