arXiv subjects

Ryan O. Behunin

Publications and source records attributed to Ryan O. Behunin.

At least 19 recordsLinked to original sources

arXiv2026

Nonequilibrium thermodynamics of the acoustoelectric quantum vacuum

The quantum vacuum can assume thermal properties as a consequence of system kinematics, highlighting the nuance of our definition of particles in quantum field theory. Here, we explore this phenomenon in acoustoelectric systems, involving the interaction of phonons and plasmons, where the charge carriers drift at a constant velocity exceeding the speed of sound. Through an open quantum systems analysis, we show that the acoustoelectric quantum vacuum acquires a thermal character with a temperature defined by the drift velocity and the phonon wavevector. Realistic parameters yield effective temperatures of several Kelvin, establishing acoustoelectric systems as a promising platform for the investigation of quantum vacuum effects.

quant-ph↗

arXiv2026

Noise factor of Brillouin amplifiers

Stimulated Brillouin scattering (SBS), an optical nonlinearity arising from photon-phonon interactions, has formed the basis for a large class of optical signal processing devices, including Brillouin amplifiers. A limiting factor of such amplifiers is the noise due to thermal-mechanical fluctuations that the phonons imprint on the optical signal. Prior work has either inferred or experimentally observed a noise factor ($F$) that depends only on the thermal occupation of the phonons ($F\approx 1+n_{th}$). We show that this noise factor results naturally from a Hamiltonian-based spatio-temporal coupled mode treatment in the limit of large Brillouin amplification and when phonon propagation is neglected. Moreover, this theoretical framework allows us to extend our treatment to a much larger and more representative parameter space for emerging SBS systems; specifically, this analysis accounts for the forward or backward nature of the scattering process and the effects of phonon propagation, optical loss, and small Brillouin gains. Our results demonstrate that the noise factor can deviate radically from $F\approx 1+n_{th}$ for a host of modern SBS devices, especially those in which phonon propagation significantly changes the coupled mode dynamics.

physics.optics↗

arXiv2026

Noise and dynamics in acoustoelectric waveguides

We present a quantum field theoretic formulation of acoustoelectric interactions in waveguide-like systems of arbitrary cross-section. Building on an open quantum systems approach, we derive a unified description of plasmon-phonon coupling that incorporates dissipation, noise, and the influence of drift currents. Our analysis captures both bulk and surface plasmon modes, highlighting how drift currents Doppler-shift plasmonic resonances and reshape the phonon noise spectrum. The resulting Heisenberg-Langevin equations yield closed-form expressions for frequency shifts, gain, and noise power spectra, enabling direct evaluation of performance metrics such as the noise factor in acoustoelectric amplifiers and oscillators. In the appropriate limits, this framework reproduces known results while extending them to complex geometries.

physics.optics↗

arXiv2026

Phonon decoherence produced by two-level tunneling states

Phonon modes within pristine crystalline resonators now routinely reach the quantum ground state. Such systems are attractive for quantum information science applications, as advanced fabrication and processing can enable relatively long quantum coherence times, and precision control can be realized through optical, electrical, or qubit coupling. In many state-of-the-art systems, the phonon lifetime is limited by disorder. In particular, native oxides or damaged `dead layers' at surfaces can host two-level tunneling states that lead to a particularly problematic form of dissipation that increases at lower temperatures. As mechanical losses are driven down in systems such as micro-fabricated bulk acoustic wave resonators, tunneling states are expected to emerge as the dominant mechanism for phonon decoherence. A quantitative description of these mesoscopic systems therefore requires a framework that captures interactions between a selected phonon mode and a large ensemble of TLS. Here, we derive a quantum master equation for this coupled system, permitting the phonon decoherence produced by two-level tunneling states to be calculated. As an example, we estimate the lifetime of a variety of quantum states within quartz micro-resonators hosting a thin surface layer of tunneling states. We find that the phonon coherence time is maximized at low temperatures, in spite of increased mechanical dissipation, and that phonon-TLS coupling can be reduced for modes with strain nodes at the surfaces.

cond-mat.mes-hall↗

arXiv2025

Noise dynamics in large mode volume Brillouin lasers

Photonic integrated Brillouin lasers have emerged as an important tool to realize a wide range of precision applications, including atomic time-keeping, low-noise microwave signal generation, fiber and quantum sensing, and ultra-high capacity coherent communications. While Brillouin lasers routinely achieve sub-Hz instantaneous linewidths, many of these applications also require exceptional frequency stability and high-power single-mode emission. A recent demonstration showed that extending the resonator length increases the laser power while also improving the frequency stability through suppression of thermorefractive noise. However, as the resonator scales to larger lengths, multiple optical resonances can be found within the Brillouin gain bandwidth, greatly complicating the laser dynamics compared to existing coupled-mode Brillouin laser models. Given the potential to scale lasers of this type to watt-level output powers at sub-mHz linewidths, a theoretical model describing this physics is needed to provide key insights into their performance. Here, we develop a coupled-mode theory of integrated large mode volume Brillouin lasers, accounting for multiple cavity modes with potential to lase within the gain bandwidth. We obtain expressions for the steady-state dynamics, spontaneous spectrum, relative intensity noise, and frequency noise. Our analysis reveals that the broad gain bandwidth results in atypical Brillouin dynamics, giving rise to distinct features in the noise spectra, and consequently modifications of the standard, single-mode fundamental linewidth of Brillouin lasers. Additionally, these features may be used for a variety of tangential applications, such as phonon spectroscopy or quality factor enhancement. Furthermore, we find that the linewidth can be significantly impacted by transferred RIN from the external pump in Brillouin lasers that lack ideal phase matching.

physics.optics↗

arXiv2025

Lifetime-limited Gigahertz-frequency Mechanical Oscillators with Millisecond Coherence Times

High-frequency mechanical oscillators with long coherence times are essential to realizing a variety of high-fidelity quantum sensors, transducers, and memories. However, the unprecedented coherence times needed for quantum applications require exquisitely sensitive new techniques to probe the material origins of phonon decoherence and new strategies to mitigate decoherence in mechanical oscillators. Here, we combine non-invasive laser spectroscopy techniques with materials analysis to identify key sources of phonon decoherence in crystalline media. Using micro-fabricated high-overtone bulk acoustic-wave resonators ($μ$HBARs) as an experimental testbed, we identify phonon-surface interactions as the dominant source of phonon decoherence in crystalline quartz; lattice distortion, subsurface damage, and high concentration of elemental impurities near the crystal surface are identified as the likely causes. Removal of this compromised surface layer using an optimized polishing process is seen to greatly enhance coherence times, enabling $μ$HBARs with Q-factors of > 240 million at 12 GHz frequencies, corresponding to > 6 ms phonon coherence times and record-level f-Q products. Complementary phonon linewidth and time-domain ringdown measurements, performed using a new Brillouin-based pump-probe spectroscopy technique, reveal negligible dephasing within these oscillators. Building on these results, we identify a path to > 100 ms coherence times as the basis for high-frequency quantum memories. These findings clearly demonstrate that, with enhanced control over surfaces, dissipation and noise can be significantly reduced in a wide range of quantum systems.

quant-ph↗

arXiv2025

Large mode volume integrated Brillouin lasers for scalable ultra-Low linewidth and high power

Generating ultra-low linewidths and high output power in an integrated single mode laser remains a critical challenge for future compact, portable, precision applications. Moreso, achieving these characteristics in a laser design that enables scaling to lower linewidths and higher power, and implementation in a wafer-scale integration platform that can operate from visible to near-IR and be integrated with other components. Such an advance could impact a wide array of applications including atomic and quantum sensing and computing, metrology, coherent fiber communications and sensing, and ultra-low-noise mmWave and RF generation. Yet, achieving these goals in an integrated laser has remained elusive. Here, we report a class of integrated laser that overcomes these limitations, with demonstration of a 31 mHz instantaneous linewidth, the lowest linewidth to date to the best of our knowledge, with 41 mW output power and 73 dB sidemode suppression ratio and can be tuned across a 22.5 nm range. This performance is possible due to Brillouin nonlinear dynamics that occurs within a large mode volume, nonlinear photon-phonon, MHz-scale-FSR, ultra-low loss silicon nitride resonator cavity. This laser design can scale to a new operating regime of mHz fundamental linewidth and Watt class lasers. Such lasers hold promise to unlock new sensitivity and fidelity for precision quantum experiments, portable precision applications, and atomic, molecular, and optical physics.

physics.optics↗

arXiv2024

Frequency entangled W states and quantum frequency translation protocols via forward Brillouin interactions

Complex quantum states of light are not only central to advancing our understanding of quantum mechanics, but are also necessary for a variety of quantum protocols. High-dimensional, or multipartite, quantum states are of specific interest, as they can exhibit unique properties both fundamentally and in application. The synthesis of high-dimensional, entangled photonic states can take the form of various schemes, which result in varying forms of entanglement. Frequency-entanglement is specifically attractive due to compatibility with integrated systems and resistance to decoherence in fiber transportation; however, increasing the dimension of frequency-entangled states requires a system that offers quantum interactions between a large set of distinct frequencies. Here, we show how the phonon-photon interactions of forward Brillouin scattering, which offer access to a ladder of optical resonances permitted by a single mechanical mode, can be used for fast-synthesis of frequency-entangled, single-photon W states. In our proposed system, simultaneous laser pulses of different frequencies dynamically evolve either an injected single photon or a heralded single phonon, generating W states of selected dimension and output frequency. This method enables the synthesis of `perfect' W states by adjusting the pulse amplitudes. In addition, we show how this system can be used for quantum frequency translation.

quant-ph↗

arXiv2024

Multi-phonon Fock state heralding with single-photon detection

Recognized as a potential resource for quantum technologies and a possible testbed for fundamental physics, the control and preparation of nonclassical states of mechanical oscillators has been explored extensively. Within optomechanics, quantum state synthesis can be realized by entangling photonic and phononic degrees of freedom followed by optical detection. Single-photon detection enables one of the most powerful forms of such heralded quantum state preparation, permitting the creation of single phonon states when applied to conventional cavity optomechanical systems. As the complexity of optomechanical systems increases, single-photon detection may provide heralded access to a larger class of exotic quantum states. Here, we examine the quantum dynamics of optomechanical systems that permit forward Brillouin scattering, where a single phonon mode mediates transitions between a collection of equally spaced optical resonances. Solving both the Schrodinger equation and the Lindblad master equation for this system, we find that initial states comprised of single photons or weak laser pulses evolve into complex quantum states where the frequency of single photon states and the phonon occupation number are entangled. Physically, these interactions permit a single photon to scatter to lower frequencies, where phonon excitation occurs for each scattering event. Combining this result with frequency filtering, we show how single-photon detection can herald selected multi-phonon Fock states, even in the presence of optical losses. We also present an approach for quantum tomography of the heralded phonon states.

quant-ph↗

arXiv2023

Laser cooling of traveling wave phonons in an optical fiber

In recent years, optical control of mechanical oscillators has emerged as a critical tool for everything from information processing to laser cooling. While traditional forms of optomechanical cooling utilize systems comprised of discrete optical and mechanical modes, it has recently been shown that cooling can be achieved in a chip-based system that possesses a continuum of modes. Through Brillouin-mediated phonon-photon interactions, cooling of a band of traveling acoustic waves can occur when anti-Stokes scattered photons exit the system more rapidly than the relaxation rate of the mechanical waves -- to a degree determined by the acousto-optic coupling. Here, we demonstrate that a continuum of traveling wave phonons can be cooled within an optical fiber, extending this physics to macroscopic length scales. Leveraging the large acousto-optic coupling permitted within a liquid-core optical fiber, heterodyne spectroscopy reveals power-dependent changes in spontaneous Brillouin scattering spectra that indicate a reduction of the thermal phonon population by 21K using 120 mW of injected laser power.

physics.optics↗

arXiv2022

Quantum optomechanics in tripartite systems

Owing to their long-lifetimes at cryogenic temperatures, mechanical oscillators are recognized as an attractive resource for quantum information science and as a testbed for fundamental physics. Key to these applications is the ability to prepare, manipulate and measure quantum states of mechanical motion. Through an exact formal solution to the Schrodinger equation, we show how tripartite optomechanical interactions, involving the mutual coupling between two distinct optical modes and an acoustic resonance enables quantum states of mechanical oscillators to be synthesized and interrogated.

quant-ph↗

arXiv2021

Thermal and driven noise in Brillouin Lasers

Owing to their highly coherent emission and compact form factor, Brillouin lasers have been identified as a valuable asset for applications including portable atomic clocks, precision sensors, coherent microwave synthesis and energy-efficient approaches to coherent communications. While the fundamental emission linewidth of these lasers can be very narrow, noise within dielectric materials leads to drift in the carrier frequency, posing vexing challenges for applications requiring ultra-stable emission. A unified understanding of Brillouin laser performance may provide critical insights to reach new levels of frequency stability, however existing noise models focus on only one or a few key noise sources, and do not capture the thermo-optic drift in the laser frequency produced by thermal fluctuations or absorbed power. Here, we develop a coupled mode theory of Brillouin laser dynamics that accounts for dominant forms of noise in non-crystalline systems, capturing the salient features of the frequency and intensity noise for a variety of systems. As a result, theory and experiment can be directly compared to identify key sources of noise and the frequency bands they impact, revealing strategies to improve the performance of Brillouin lasers and pave the way for highly-coherent sources of light on a chip.

physics.optics↗

arXiv2021

Modulation of Brillouin optomechanical interactions via acoustoelectric phonon-electron coupling

Optomechanical Brillouin nonlinearities -- arising from the coupling between traveling photons and phonons -- have become the basis for a range of powerful optical signal processing and sensing technologies. The dynamics of such interactions are largely set and limited by the host material's elastic, optical, and photo-elastic properties, which are generally considered intrinsic and static. Here we show for the first time that it is feasible to dynamically reconfigure the Brillouin nonlinear susceptibility in transparent semiconductors through acoustoelectric phonon-electron coupling. Acoustoelectric interactions permit a wide range of tunability of the phonon dissipation rate and velocity, perhaps the most influential parameters in the Brillouin nonlinear susceptibility. We develop a Hamiltonian-based analysis that yields self-consistent dynamical equations and noise coupling, allowing us to explore the physics of such acoustoelectrically enhanced Brillouin (AEB) interactions and show that they give rise to a dramatic enhancement of the performance of Brillouin-based photonic technologies. Moreover, we show that these AEB effects can drive systems into new regimes of fully-coherent scattering that resemble the dynamics of optical parametric processes, dramatically different than the incoherent traditional Brillouin limit. We propose and computationally explore a particular semiconductor heterostructure in which the acoustoelectric interaction arises from a piezoelectric phonon-electron coupling. We find that this system provides the necessary piezoelectric and carrier response ($k^2\approx 6 \%$), favorable semiconductor materials properties, and large optomechanical confinement and coupling ($|g_0|\approx8000$ (rad/s)$\sqrt{\text{m}}$) sufficient to demonstrate these new AEB enhanced optomechanical interactions.

physics.optics↗

arXiv2021

Photonic circuits for laser stabilization with ultra-low-loss and nonlinear resonators

Laser-frequency stabilization with on-chip photonic integrated circuits will provide compact, low cost solutions to realize spectrally pure laser sources. Developing high-performance and scalable lasers is critical for applications including quantum photonics, precision navigation and timing, spectroscopy, and high-capacity fiber communications. We demonstrate a significant advance in compact, stabilized lasers to achieve a record low integral emission linewidth and precision carrier stabilization by combining integrated waveguide nonlinear Brillouin and ultra-low loss waveguide reference resonators. Using a pair of 56.4 Million quality factor (Q) Si$_3$N$_4$ waveguide ring-resonators, we reduce the free running Brillouin laser linewidth by over an order of magnitude to 330 Hz integral linewidth and stabilize the carrier to 6.5$\times$10$^{-13}$ fractional frequency at 8 ms, reaching the cavity-intrinsic thermorefractive noise limit for frequencies down to 80 Hz. This work demonstrates the lowest linewidth and highest carrier stability achieved to date using planar, CMOS compatible photonic integrated resonators, to the best of our knowledge. These results pave the way to transfer stabilized laser technology from the tabletop to the chip-scale. This advance makes possible scaling the number of stabilized lasers and complexity of atomic and molecular experiments as well as reduced sensitivity to environmental disturbances and portable precision atomic, molecular and optical (AMO) solutions.

physics.optics↗

arXiv2021

Integrated Reference Cavity for Dual-mode Optical Thermometry and Frequency Stabilization

Optical frequency stabilization is a critical component for precision scientific systems including quantum sensing, precision metrology, and atomic timekeeping. Ultra-high quality factor photonic integrated optical resonators are a prime candidate for reducing their size, weight and cost as well as moving these systems on chip. However, integrated resonators suffer from temperature-dependent resonance drift due to the large thermal response as well as sensitivity to external environmental perturbations. Suppression of the cavity resonance drift can be achieved using precision interrogation of the cavity temperature through the dual-mode optical thermometry. This approach enables measurement of the cavity temperature change by detecting the resonance difference shift between two polarization or optical frequency modes. Yet this approach has to date only been demonstrated in bulk-optic whispering gallery mode and fiber resonators. In this paper, we implement dual-mode optical thermometry using dual polarization modes in a silicon nitride waveguide resonator for the first time, to the best of our knowledge. The temperature responsivity and sensitivity of the dual-mode TE/TM resonance difference is 180.7$\pm$2.5 MHz/K and 82.56 $μ$K, respectively, in a silicon nitride resonator with a 179.9E6 intrinsic TM mode Q factor and a 26.6E6 intrinsic TE mode Q factor. Frequency stabilization is demonstrated by locking a laser to the TM mode cavity resonance and applying the dual-mode resonance difference to a feedforward laser frequency drift correction circuit with a drift rate improvement to 0.31 kHz/s over the uncompensated 10.03 kHz/s drift rate. Allan deviation measurements with dual-mode feedforward-correction engaged shows that a fractional frequency instability of 9.6E-11 over 77 s can be achieved.

physics.ins-det↗

arXiv2021

Visible light photonic integrated Brillouin laser

Narrow linewidth visible light lasers are critical for atomic, molecular and optical (AMO) applications including atomic clocks, quantum computing, atomic and molecular spectroscopy, and sensing. Historically, such lasers are implemented at the tabletop scale, using semiconductor lasers stabilized to large optical reference cavities. Photonic integration of high spectral-purity visible light sources will enable experiments to increase in complexity and scale. Stimulated Brillouin scattering (SBS) is a promising approach to realize highly coherent on-chip visible light laser emission. While progress has been made on integrated SBS lasers at telecommunications wavelengths, barriers have existed to translate this performance to the visible, namely the realization of Brillouin-active waveguides in ultra-low optical loss photonics. We have overcome this barrier, demonstrating the first visible light photonic integrated SBS laser, which operates at 674 nm to address the 88Sr+ optical clock transition. To guide the laser design, we use a combination of multi-physics simulation and Brillouin spectroscopy in a 2 meter spiral waveguide to identify the 25.110 GHz first order Stokes frequency shift and 290 MHz gain bandwidth. The laser is implemented in an 8.9 mm radius silicon nitride all-waveguide resonator with 1.09 dB per meter loss and Q of 55.4 Million. Lasing is demonstrated, with an on-chip 14.7 mW threshold, a 45% slope efficiency, and linewidth narrowing as the pump is increased from below threshold to 269 Hz. To illustrate the wavelength flexibility of this design, we also demonstrate lasing at 698 nm, the wavelength for the optical clock transition in neutral strontium. This demonstration of a waveguide-based, photonic integrated SBS laser that operates in the visible, and the reduced size and sensitivity to environmental disturbances, shows promise for diverse AMO applications.

physics.optics↗

arXiv2021

Optically synchronized fiber links with spectrally pure integrated lasers

Precision frequency and phase synchronization between distinct fiber interconnected nodes is critical for a wide range of applications, including atomic timekeeping, quantum networking, database synchronization, ultra-high-capacity coherent optical communications and hyper-scale data centers. Today, many of these applications utilize precision, tabletop laser systems, and would benefit from integration in terms of reduced size, power, cost, and reliability. In this paper we report a record low 3x10^-4 rad^2 residual phase error variance for synchronization based on independent, spectrally pure, ultra-high mutual coherence, photonic integrated lasers. This performance is achieved with stimulated Brillouin scattering lasers that are stabilized to independent microcavity references, realizing sources with 30 Hz integral linewidth and a fractional frequency instability less than or equal to 2x10^-13 at 50 ms. This level of low phase noise and carrier stability enables a new type of optical-frequency-stabilized phase-locked loop (OFS-PLL) that operates with a less than 800 kHz loop bandwidth, eliminating traditional power consuming high bandwidth electronics and digital signal processors used to phase lock optical carriers. Additionally, we measure the residual phase error down to a received carrier power of -34 dBm, removing the need to transmit in-band or out-of-band synchronized carriers. These results highlight the promise for a path to spectrally pure, ultra-stable, integrated lasers for network synchronization, precision time distribution protocols, quantum-clock networks, and multiple-Terabit per second coherent DSP-free fiber-optic interconnects.

physics.optics↗

arXiv2020

422 Million Q Planar Integrated All-Waveguide Resonator with a 3.4 Billion Absorption Limited Q and Sub-MHz Linewidth

High Q optical resonators are a key component for ultra-narrow linewidth lasers, frequency stabilization, precision spectroscopy and quantum applications. Integration of these resonators in a photonic waveguide wafer-scale platform is key to reducing their cost, size and power as well as sensitivity to environmental disturbances. However, to date, the intrinsic Q of integrated all-waveguide resonators has been relegated to below 150 Million. Here, we report an all-waveguide Si3N4 resonator with an intrinsic Q of 422 Million and a 3.4 Billion absorption loss limited Q. The resonator has a 453 kHz intrinsic linewidth and 906 kHz loaded linewidth, with a finesse of 3005. The corresponding linear loss of 0.060 dB/m is the lowest reported to date for an all-waveguide design with deposited upper cladding oxide. These are the highest intrinsic and absorption loss limited Q factors and lowest linewidth reported to date for a photonic integrated all-waveguide resonator. This level of performance is achieved through a careful reduction of scattering and absorption loss components. We quantify, simulate and measure the various loss contributions including scattering and absorption including surface-state dangling bonds that we believe are responsible in part for absorption. In addition to the ultra-high Q and narrow linewidth, the resonator has a large optical mode area and volume, both critical for ultra-low laser linewidths and ultra-stable, ultra-low frequency noise reference cavities. These results demonstrate the performance of bulk optic and etched resonators can be realized in a photonic integrated solution, paving the way towards photonic integration compatible Billion Q cavities for precision scientific systems and applications such as nonlinear optics, atomic clocks, quantum photonics and high-capacity fiber communications systems on-chip.

physics.optics↗