arXiv subjects

S. D. Baranovskii

Publications and source records attributed to S. D. Baranovskii.

At least 19 recordsLinked to original sources

arXiv2023

How to detect the spacetime curvature without rulers and clocks. II. Three-dimensional spacetime

We have generalized the results of the previous work [arXiv:2302.12209] to the case of three-dimensional (3D) spacetime with two spatial and one temporal coordinates. We have found that the flat Minkowski 3D spacetime is "well-stitched", which means that it possesses a structure described by 24 causal relations between 12 events. We have proved that a 3D spacetime is "well-stitched" if and only if it is conformally flat. The concept of a "well-stitched" spacetime does not rely on metrical information about lengths, times, etc., and does not belong to the metric geometry, but rather to geometry of incidence. We therefore have "translated" an important concept of a conformally-flat spacetime from the "metric" language of Riemannian geometry to the "non-metric" language of the geometry of incidence. The results of this paper provide a tool for detecting the curvature of the 3D spacetime on the basis of causal relations only, without any measurement instruments like rulers and clocks, provided that the spacetime is not conformally flat.

gr-qc↗

arXiv2023

Parametrization of the Charge-Carrier Mobility in Organic Disordered Semiconductors. APAE against EGDM

An appropriately parameterized compact analytical equation (APAE) is suggested to account for charge carrier mobility in organic disordered semiconductors (ODSs). This equation correctly reproduces the effects of temperature $T$, carrier concentration $n$, and electric field $F$ on the carrier mobility $μ(T,F,n)$, as evidenced by comparison with analytical theories and Monte Carlo simulations. The set of material parameters responsible for charge transport is proven to be at varience to those used in the so-called extended Gaussian disorder model (EGDM) approach, which is widely exploited in commercially distributed device--simulation algorithms. While EGDM is only valid for cubic lattices with a specific choice of parameters, APAE describes charge transport in systems with spatial disorder in a wide range of parameters. APAE is user-friendly and, thus, suitable for incorporation into device-simulation algorithms.

cond-mat.soft↗

arXiv2023

A pedestrian approach to Einstein's formula $E=mc^2$ with an application to photon dynamics

There are several ways to derive Einstein's celebrated formula for the energy of a massive particle at rest, $E=mc^2$. Noether's theorem applied to the relativistic Lagrange function provides an unambiguous and straightforward access to energy and momentum conservation laws but those tools were not available at the beginning of the twentieth century and are not at hand for newcomers even nowadays. In a pedestrian approach, we start from relativistic kinematics and analyze elastic and inelastic scattering processes in different reference frames to derive the relativistic energy-mass relation. We extend the analysis to Compton scattering between a massive particle and a photon, and a massive particle emitting two photons. Using the Doppler formula, it follows that $E=\hbar ω$ for photons at angular frequency $ω$ where $\hbar$ is the reduced Planck constant. We relate our work to other derivations of Einstein's formula in the literature.

physics.class-ph↗

arXiv2023

How to detect the spacetime curvature without rulers and clocks

We demonstrate how one can distinguish a curved 4-dimensional spacetime from a flat one, when it is possible, relying only on the causality relations between events. It is known that it is possible only for spacetimes that are not conformally flat. We prove that if a spacetime is not conformally flat, then its non-flatness can be verified by only a few (sixteen) measurements of causal relations. Therefore the results of this paper clarify what can be said about flatness or non-flatness of the spacetime after a finite number of measurements of causal relations.

gr-qc↗

arXiv2023

Quantum states in disordered media. I. Low-pass filter approach

The current burst in research activities on disordered semiconductors calls for the development of appropriate theoretical tools that reveal the features of electron states in random potentials while avoiding the time-consuming numerical solution of the Schrödinger equation. Among various approaches suggested so far, the low-pass filter approach of Halperin and Lax (HL) and the so-called localization landscape technique (LLT) have received most recognition in the community. We prove that the HL approach becomes equivalent to the LLT for the specific case of a Lorentzian filter when applied to the Schrödinger equation with a constant mass. Advantageously, the low-pass filter approach allows further optimization beyond the Lorentzian shape. We propose the global HL filter as optimal filter with only a single length scale, namely, the size of the localized wave packets. As an application, we design an optimized potential landscape for a (semi-)classical calculation of the number of strongly localized states that faithfully reproduce the exact solution for a random white-noise potential in one dimension.

cond-mat.dis-nn↗

arXiv2023

Quantum states in disordered media. II. Spatial charge carrier distribution

The space- and temperature-dependent electron distribution $n(\mathbf r,T)$ is essential for the theoretical description of the opto-electronic properties of disordered semiconductors. We present two powerful techniques to access $n(\mathbf r,T)$ without solving the Schrödinger equation. First, we derive the density for non-degenerate electrons by applying the Hamiltonian recursively to random wave functions (RWF). Second, we obtain a temperature-dependent effective potential from the application of a universal low-pass filter (ULF) to the random potential acting on the charge carriers in disordered media. Thereby, the full quantum-mechanical problem is reduced to the quasi-classical description of $n(\mathbf r,T)$ in an effective potential. We numerically verify both approaches by comparison with the exact quantum-mechanical solution. Both approaches prove superior to the widely used localization landscape theory (LLT) when we compare our approximate results for the charge carrier density and mobility at elevated temperatures obtained by RWF, ULF, and LLT with those from the exact solution of the Schrödinger equation.

cond-mat.dis-nn↗

arXiv2022

Comment on "Interplay of Structural and Optoelectronic Properties in Formamidinium Mixed Tin-Lead Triiodide Perovskites"

Studying optoelectronic properties in FAPb$_{1-x}$Sn$_x$I$_3$ perovskites as a function of the lead:tin content, Parrott et al. observed the broadest luminescence linewidth and the largest luminescence Stokes shift in mixed compositions with Sn $ < 25$% and with $> 0.85$%. Since the largest effects of alloy disorder were expected for the 50:50 composition, it was concluded that the revealed disorder effects might arise from extrinsic factors that can be eliminated upon further crystal growth optimization. This comment shows that the largest effects of alloy disorder for perfectly random fluctuations in FAPb$_{1-x}$Sn$_x$I$_3$ perovskite are, in fact, expected for $x < 0.25$ and for $x > 0.85$. Therefore, further crystal growth optimization is futile.

cond-mat.mtrl-sci↗

arXiv2019

Percolation description of charge transport in the random barrier model applied to amorphous oxide semiconductors

Charge transport in amorphous oxide semiconductors is often described as the band transport affected by disorder in the form of random potential barriers (RB). Theoretical studies in the framework of this approach neglected so far the percolation nature of the phenomenon. In this article, a recipe for theoretical description of charge transport in the RB model is formulated using percolation arguments. Comparison with the results published so far evidences the superiority of the percolation approach.

cond-mat.dis-nn↗

arXiv2019

Percolation description of charge transport in amorphous oxide semiconductors

The charge transport mechanism in amorphous oxide semiconductors (AOS) is a matter of controversial debates. Most theoretical studies so far neglected the percolation nature of the phenomenon. In this article, a recipe for theoretical description of charge transport in AOSs is formulated using the percolation arguments. Comparison with the previous theoretical studies shows a superiority of the percolation approach. The results of the percolation theory are compared to experimental data obtained in various InGaZnO materials revealing parameters of the disorder potential in such AOS.

cond-mat.dis-nn↗

arXiv2017

Fundamental characteristic length scale for the field dependence of hopping charge transport in disordered organic semiconductors

Using analytical arguments and computer simulations we show that the dependence of the hopping carrier mobility on the electric field $μ(F)/μ(0)$ in a system of random sites is determined by the localization length $a$, and not by the concentration of sites $N$. This result is in drastic contrast to what is usually assumed in the literature for a theoretical description of experimental data and for device modeling, where $N^{-1/3}$ is considered as the decisive length scale for $μ(F)$. We show that although the limiting value $μ(F \rightarrow 0)$ is determined by the ratio $N^{-1/3}/a$, the dependence $μ(F)/μ(0)$ is sensitive to the magnitude of $a$, and not to $N^{-1/3}$. Furthermore, our numerical and analytical results prove that the effective temperature responsible for the combined effect of the electric field $F$ and the real temperature $T$ on the hopping transport via spatially random sites can contain the electric field only in the combination $eFa$.

cond-mat.mes-hall↗

arXiv2010

Role of Diffusion in Two-dimensional Bimolecular Recombination

Experiments on carrier recombination in two-dimensional organic structures are often interpreted in the frame of the Langevin model with taking into account only the drift of the charge carriers in their mutual electric field. While this approach is well justified for three-dimensional systems, it is in general not valid for two-dimensional structures, where the contribution of diffusion can play a dominant role. We study the two-dimensional Langevin recombination theoretically and find the critical concentration below which diffusion cannot be neglected. For typical experimental conditions, neglecting the diffusion leads to an underestimation of the recombination rate by several times.

cond-mat.dis-nn↗

arXiv2009

Effect of Electric Field on Diffusion in Disordered Materials I. One-dimensional Hopping Transport

An exact analytical theory is developed for calculating the diffusion coefficient of charge carriers in strongly anisotropic disordered solids with one-dimensional hopping transport mode for any dependence of the hopping rates on space and energy. So far such a theory existed only for calculating the carrier mobility. The dependence of the diffusion coefficient on the electric field evidences a linear, non-analytic behavior at low fields for all considered models of disorder. The mobility, on the contrary, demonstrates a parabolic, analytic field dependence for a random-barrier model, being linear, non-analytic for a random energy model. For both models the Einstein relation between the diffusion coefficient and mobility is proven to be violated at any finite electric field. The question on whether these non-analytic field dependences of the transport coefficients and the concomitant violation of the Einstein's formula are due to the dimensionality of space or due to the considered models of disorder is resolved in the following paper [Nenashev et al., arXiv:0912.3169], where analytical calculations and computer simulations are carried out for two- and three-dimensional systems.

cond-mat.dis-nn↗

arXiv2009

Effect of Electric Field on Diffusion in Disordered Materials II. Two- and Three-dimensional Hopping Transport

In the previous paper [Nenashev et al., arXiv:0912.3161] an analytical theory confirmed by numerical simulations has been developed for the field-dependent hopping diffusion coefficient D(F) in one-dimensional systems with Gaussian disorder. The main result of that paper is the linear, non-analytic field dependence of the diffusion coefficient at low electric fields. In the current paper, an analytical theory is developed for the field-dependent diffusion coefficient in three- and two-dimensional Gaussian disordered systems in the hopping transport regime. The theory predicts a smooth parabolic field dependence for the diffusion coefficient at low fields. The result is supported by Monte Carlo computer simulations. In spite of the smooth field dependences for the mobility and for the longitudinal diffusivity, the traditional Einstein form of the relation between these transport coefficients is shown to be violated even at very low electric fields.

cond-mat.dis-nn↗

arXiv2008

Hopping conduction in strong electric fields: Negative differential conductivity

Effects of strong electric fields on hopping conductivity are studied theoretically. Monte-Carlo computer simulations show that the analytical theory of Nguyen and Shklovskii [Solid State Commun. 38, 99 (1981)] provides an accurate description of hopping transport in the limit of very high electric fields and low concentrations of charge carriers as compared to the concentration of localization sites and also at the relative concentration of carriers equal to 0.5. At intermediate concentrations of carriers between 0.1 and 0.5 computer simulations evidence essential deviations from the results of the existing analytical theories. The theory of Nguyen and Shklovskii also predicts a negative differential hopping conductivity at high electric fields. Our numerical calculations confirm this prediction qualitatively. However the field dependence of the drift velocity of charge carriers obtained numerically differs essentially from the one predicted so far. Analytical theory is further developed so that its agreement with numerical results is essentially improved.

cond-mat.dis-nn↗

arXiv2008

Effective temperature for hopping transport in a Gaussian DOS

For hopping transport in disordered materials, the mobility of charge carriers is strongly dependent on temperature and the electric field. Our numerical study shows that both the energy distribution and the mobility of charge carriers in systems with a Gaussian density of states, such as organic disordered semiconductors, can be described by a single parameter - effective temperature, dependent on the magnitude of the electric field. Furthermore, this effective temperature does not depend on the concentration of charge carriers, while the mobility does depend on the charge carrier concentration. The concept of the effective temperature is shown to be valid for systems with and without space-energy correlations in the distribution of localized states.

cond-mat.dis-nn↗

arXiv2008

Spin-dependent transition rates through exchange coupled localized spin pairs during coherent spin excitation

The effect of exchange interactions within spin pairs on spin-dependent transport and recombination rates through localized states in semiconductors during coherent electron spin resonant excitation is studied theoretically. It is shown that for identical spin systems, significant quantitative differences are to be expected between the results of pEDMR/pODMR experiments were permutation symmetry is the observable as compared to pESR experiments with polarization as the observable. It is predicted that beat oscillations of the spin nutations and not the nutations themselves dominate the transport or recombination rates when the exchange coupling strength or the field strength of the exciting radiation exceed the difference of the Zeeman energies within the spin pair. Furthermore, while the intensities of the rate oscillations decrease with increasing exchange within the spin pairs, the singlet and triplet signals retain their relative strength. This means that pEDMR and pODMR experiments could allow better experimental access to ESR forbidden singlet transitions which are hardly or not at all accessible with conventional pulsed electron spin resonance spectroscopy.

cond-mat.mtrl-sci↗

arXiv2005

Simulation of the phononless hopping in a Coulomb glass

The phononless hopping conductivity of a disordered system with localized states is studied in a broad range of frequencies by straightforward computer simulations taking into account Coulomb interactions. At sufficiently low temperatures, the conductivity is determined by the zero-phonon absorption of the photon by pairs of states. The laser frequency dependence of the conductivity is examined and compared with the analytical model of Efros and Shklovskii and with recent experimental data obtained on Si:P. The range of parameters is determined, for which the conductivity dependence on photon energy best reproduces the experimental results.

cond-mat.dis-nn↗

arXiv1999

Fluctuation-Stimulated Variable-Range Hopping

Qualitatively new transport mechanism is suggested for hopping of carriers according to which the variable-range hopping (VRH) arises from the resonant tunneling between transport states brought into resonance by Coulomb potentials produced by surrounding sites with fluctuating occupations. A semiquantitative description of the hopping transport is given based on the assumption that fluctuations of energies of hopping sites have spectral density 1/f.

cond-mat.dis-nn↗