arXiv subjects

S. Ishihara

Publications and source records attributed to S. Ishihara.

At least 37 records · Page 2Linked to original sources

arXiv2013

Collective excitation of electric dipole on molecular dimer in organic dimer-Mott insulator

The terahertz (THz) response in 10-100 cm^-1 was investigated in an organic dimer-Mott (DM) insulator kappa-(ET)_2Cu_2(CN)_3 that exhibits a relaxor-like dielectric anomaly. 30 cm^-1 band in the optical conductivity was attributable to collective excitation of the intra-dimer electric dipoles which are formed by an electron correlation. We succeeded in observing photoinduced enhancement of this 30 cm^-1 band, reflecting the growth of the electric dipole cluster in the DM phase. Such optical responses in kappa-(ET)_2Cu_2(CN)_3 reflect instability near the boundary between the DM-ferroelectric charge ordered phases.

cond-mat.str-el↗

arXiv2013

Comparative study of non-invasive force and stress inference methods in tissue

In the course of animal development, the shape of tissue emerges in part from mechanical and biochemical interactions between cells. Measuring stress in tissue is essential for studying morphogenesis and its physical constraints. Experimental measurements of stress reported thus far have been invasive, indirect, or local. One theoretical approach is force inference from cell shapes and connectivity, which is non-invasive, can provide a space-time map of stress and relies on prefactors. Here, to validate force- inference methods, we performed a comparative study of them. Three force-inference methods, which differ in their approach of treating indefiniteness in an inverse problem between cell shapes and forces, were tested by using two artificial and two experimental data sets. Our results using different datasets consistently indicate that our Bayesian force inference, by which cell-junction tensions and cell pressures are simultaneously estimated, performs best in terms of accuracy and robustness. Moreover, by measuring the stress anisotropy and relaxation, we cross-validated the force inference and the global annular ablation of tissue, each of which relies on different prefactors. A practical choice of force-inference methods in distinct systems of interest is discussed.

q-bio.QM↗

arXiv2011

Orbital Compass Model as an Itinerant Electron System

Two-dimensional orbital compass model is studied as an interacting itinerant electron model. A Hubbard-type tight-binding model, from which the orbital compass model is derived in the strong coupling limit, is identified. This model is analyzed by the random-phase approximation (RPA) and the self-consistent RPA methods from the weak coupling. Anisotropy for the orbital fluctuation in the momentum space is qualitatively changed by the on-site Coulomb interaction. This result is explained by the fact that the dominant fluctuation is changed from the intra-band nesting to the inter-band one by increasing the interaction.

cond-mat.str-el↗

arXiv2011

Photo-induced spin-state change in itinerant correlated-electron system

Photo-induced spin-state change in itinerant correlated-electron system is studied. The model Hamiltonians before and after photon-pumping are derived from the two-orbital Hubbard model with crystalline field splitting. A photon introduced in the low-spin band insulator induces a bound state of the high-spin state and a photoexcited hole. This bound state brings a characteristic peak in the optical absorption spectra in the photo-excited state. The resent results well explain the recent experimental results of the ultrafast optical spectroscopy in perovskite cobaltites.

cond-mat.str-el↗

arXiv2010

Polarization-analyzed resonant inelastic x-ray scattering of the orbital excitations in KCuF3

We report a Cu K-edge resonant inelastic x-ray scattering (RIXS) study of orbital excitations in KCuF3 . By performing the polarization analysis of the scattered photons, we disclose that the excitation between the eg orbitals and the excitations from t2g to eg exhibit distinct polarization dependence. The polarization dependence of the respective excitations is interpreted based on a phenomenological consideration of the symmetry of the RIXS process that yields a necessary condition for observing the excitations. In addition, we show that the orbital excitations are dispersionless within our experimental resolution.

cond-mat.str-el↗

arXiv2010

Meson mass spectrum using the Cayley-Dickson algebra

From an injective map between the mass of the meson 16-plet and the eigenvalue of the right multiplication in the Cayley-Dickson algebra, we obtain the mass formula as 2 m_{D_s} = m_{eta_c} + m_{eta'}, which is in excellent agreement with experiment.

math-ph↗

arXiv2010

Numerical Study of Photo-Induced Dynamics in Double-Exchange Model

Photo-induced spin and charge dynamics in double-exchange model are numerically studied. The Lanczos method and the density-matrix renormalization-group method are applied to one-dimensional finite-size clusters. By photon irradiation in a charge ordered (CO) insulator associated with antiferromagnetic (AFM) correlation, both the CO and AFM correlations collapse rapidly, and appearances of new peaks inside of an insulating gap are observed in the optical spectra and the one-particle excitation spectra. Time evolutions of the spin correlation and the in-gap state are correlated with each other, and are governed by the transfer integral of conduction electrons. Results are interpreted by the charge kink/anti-kink picture and their effective motions which depend on the localized spin correlation. Pump-photon density dependence of spin and charge dynamics are also studied. Roles of spin degree of freedom are remarkable in a case of weak photon density. Implications of the numerical results for the pump-probe experiments in perovskite manganites are discussed.

cond-mat.str-el↗

arXiv2009

Dynamical coupling and separation of multiple degrees of freedom in a photoexcited double-exchange system

We present a theory of ultrafast photo-induced dynamics in a spin-charge coupled system, motivated by pump-probe experiments in perovskite manganites. A microscopic picture for multiple dynamics in spin and charge degrees is focused on. Real-time simulations are carried out by two complimentary methods. Our calculation demonstrates that electron motion governs a short-time scale where charge and spin dynamics are combined strongly, while, in a long-time scale controlled by spin relaxation, charge sector does not follow remarkable change in spin sector. Present results are in contrast to a conventional double-exchange picture in equilibrium states.

cond-mat.str-el↗

arXiv2008

Doubly degenerate orbital system in honeycomb lattice: implication of orbital state in layered iron oxide

We study a doubly-degenerate orbital model on a honeycomb attice. This is a model for orbital states in multiferroic layered iron oxides. The classical and quantum models are analyzed by spin-wave approximation, Monte-Carlo simulation and Lanczos method. A macroscopic number of degeneracy exists in the classical ground state. In the classical model, a peak in the specific heat appears at a temperature which is much lower than the mean-field ordering one. Below this temperature, angle of orbital pseudo-spin is fixed, but conventional orbital orders are not suggested. The degeneracy in the ground state is partially lifted by thermal fluctuation. We suggest a role of zero-dimensional fluctuation in hexagons on a low-temperature orbital structure. Lifting of the degeneracy also occurs at zero temperature due to the quantum zero-point fluctuation. We show that the ground-state wave function is well represented by a linear combination of the states where a honeycomb lattice is covered by nearest-neighboring pairs of orbitals with the minimum bond energy.

cond-mat.str-el↗

arXiv2007

Theory of Layered Iron Oxide on Frustrated Geometry: Electric Polarization, Magnetoelectric Effect and Orbital State

A layered iron oxide \rfeo ($R$: rare-earth elements) is an exotic dielectric material with charge-order (CO) driven electric polarization and magnetoelectric effect caused by spin-charge coupling. In this paper, a theory of electronic structure and dielectric property in \rfeo is presented. Charge frustration in paired-triangular lattices allows a charge imbalance without inversion symmetry. Spin frustration induces reinforcement of this polar CO by a magnetic ordering. We also analyze an orbital model for the Fe ion which does not show a conventional long-range order.

cond-mat.str-el↗

arXiv2005

Randomly Diluted e_g Orbital-Ordered Systems

Dilution effects on the long-range ordered state of the doubly degenerate $e_g$ orbital are investigated. Quenched impurities without the orbital degree of freedom are introduced in the orbital model where the long-range order is realized by the order-from-disorder mechanism. It is shown by the Monte-Carlo simulation and the cluster-expansion method that a decrease in the orbital ordering temperature by dilution is remarkable in comparison with that in the randomly diluted spin models. Tiltings of orbitals around impurity cause this unique dilution effects on the orbital systems. The present theory provides a new view point for the recent experiments in KCu$_{1-x}$Zn$_x$F$_3$.

cond-mat.str-el↗

arXiv2004

Resonant inelastic x-ray scattering study of hole-doped manganites La1-xSrxMnO3 (x=0.2 and 0.4)

Electronic excitations near the Fermi energy in the hole doped manganese oxides (La1-xSrxMnO3, x=0.2 and 0.4) have been elucidated by using the resonant inelastic x-ray scattering (RIXS) method. A doping effect in the strongly correlated electron systems has been observed for the first time. The scattering spectra show that a salient peak appears in low energies indicating the persistence of the Mott gap. At the same time, the energy gap is partly filled by doping holes and the energy of the spectral weight shifts toward lower energies. The excitation spectra show little change in the momentum space as is in undoped LaMnO3, but the scattering intensities in the low energy excitations of x=0.2 are anisotropic as well as temperature dependent, which indicates a reminiscence of the orbital nature.

cond-mat.str-el↗

arXiv2003

Ferromagnetic insulating phase in Pr{1-x}Ca{x}MnO3

A ferromagnetic insulating (FM-I) state in Pr0.75Ca0.25MnO3 has been studied by neutron scattering experiment and theoretical calculation. The insulating behavior is robust against an external magnetic field, and is ascribed to neither the phase separation between a ferromagnetic metallic (FM-M) phase and a non-ferromagnetic insulating one, nor the charge ordering. We found that the Jahn-Teller type lattice distortion is much weaker than PrMnO3 and the magnetic interaction is almost isotropic. These features resembles the ferromagnetic metallic state of manganites, but the spin exchange interaction J is much reduced compared to the FM-M state. The theoretical calculation based on the staggered type orbital order well reproduces several features of the spin and orbital state in the FM-I phase.

cond-mat.str-el↗

arXiv2003

Distorted Perovskite with e_g^1 Configuration as a Frustrated Spin System

The evolution of spin- and orbital-ordered states has been systematically investigated for a series of insulating perovskites $R$MnO$_3$ ($R$=La,Pr,Nd,...). $R$MnO$_3$ with a large GdFeO$_3$-type distortion is regarded as a frustrated spin system having ferromagnetic nearest-neighbor and antiferromagnetic (AF) next-nearest-neighbor (NNN) interactions within a MnO$_2$ plane. The staggered orbital order associated with the GdFeO$_3$-type distortion induces the anisotropic NNN interaction, and yields the unique sinusoidal and $E$-type ("up-up-down-down") AF ordered states in the distorted perovskites with $e_g^1$ configuration.

cond-mat.str-el↗

arXiv2001

Magnetic Ordering, Orbital Ordering and Resonant X-ray Scattering in Perovskite Titanates

The effective Hamiltonian for perovskite titanates is derived by taking into account the three-fold degeneracy of $t_{2g}$ orbitals and the strong electron-electron interactions. The magnetic and orbital ordered phases are studied in the mean-field approximation applied to the effective Hamiltonian. A large degeneracy of the orbital states in the ferromagnetic phase is found in contrast to the case of the doubly degenerate $e_g$ orbitals. Lifting of this orbital degeneracy due to lattice distortions and spin-orbit coupling is examined. A general form for the scattering cross section of the resonant x-ray scattering is derived and is applied to the recent experimental results in YTiO$_3$. The spin wave dispersion relation in the orbital ordered YTiO$_3$ is also studied.

cond-mat.str-el↗

arXiv2001

Observation of the antiferroquadrupolar order in DyB2C2 by resonant x-ray scattering

We have investigated the antiferroquadrupolar(AFQ) order in DyB$_2$C$_2$ by resonant x-ray scattering. X-rays with energies near the $L_3$ absorption edge of Dy were employed. Superlattice peaks that correspond to three kinds of propagation vectors of (1 0 0), (1 0 1/2) and (0 0 1/2) were investigated in detail with polarization analyses. The experimental results are analyzed using a formalism on resonant x-ray scattering and a model of the AFQ order. The magnetic and quadrupolar scatterings are explained by the model satisfactorily. A detailed investigation on the critical behavior of the AFQ ordering is also reported. The critical exponent $β$ is deduced to be 0.35, not far from the three-dimensional Heisenberg system. We have also succeeded in detecting the diffuse scattering above $T_{Q}$.

cond-mat.str-el↗

arXiv2001

Orbital excitations in CMR progenitor of LaMnO3 studied by resonant inelastic x-ray scattering

We report resonant inelastic x-ray scattering experiments of the orbital ordered manganite LaMnO3. When the incident photon energy is tuned near the Mn K absorption edge, the spectra reveal three features at 2.5 eV, 8 eV and 11 eV. The 8 eV and 11 eV peaks are considered charge-transfer type excitations. On the other hand, theoretical calculations identify the 2.5 eV peak as an orbital excitation across the Mott gap, i.e. an electron excitation from the lower Hubbard band with the d3x2-r2 and d3y2-r2 orbital characters to the upper Hubbard band with the dy2-z2 and dz2-x2 ones. The observed weak dispersion and characteristic azimuthal angle dependence of this new type of excitations are well reproduced by the theory which includes orbital degeneracy and strong electron correlation.

cond-mat.str-el↗

arXiv2001

Role of electron-phonon interaction in the strongly correlated cuprates superconductors

Using high resolution angle-resolved photoemission data in conjunction with that from neutron and other probes, we show that electron-phonon (el-ph) coupling is strong in cuprates superconductors and it plays an important role in pairing. In addition to the strong electron correlation, the inclusion of phonons provides a theoretical framework explaining many important phenomena that cannot be understood by a strongly correlated electronic model alone. Especially it is indispensable to explain the difference among materials. The phonons with the wave number around the (0,qx) and (qx,0) axes create the d-wave pairing while that near (pi,pi) are pair breaking. Therefore the half-breathing mode of the oxygen motions helps d-wave superconductivity.

cond-mat.supr-con↗