SearcharxivSearch

arXiv subjects

S. Patnaik

Publications and source records attributed to S. Patnaik.

At least 19 recordsLinked to original sources

Identification of thermal expansion coefficient in a thermoelastic plate from final time-measured displacement

We investigate a coupled thermoelastic plate system consisting of a fourth-order displacement equation and a heat evolution equation linked through a spatially varying coupling factor $\alpha(x)$. The model accounts for thermoelastic interactions through the operators $\operatorname{div}(\alpha(x)\nabla \theta)$ and $\operatorname{div}(\alpha(x)\nabla u_t)$. We establish the well-posedness of the direct problem under homogeneous Neumann conditions for $u$ and Dirichlet conditions for $\theta$, deriving optimal energy estimates and demonstrating continuous dependence of solutions on the given data. We further introduce an input-output operator corresponding to the considered inverse problem and show that it is compact and Lipschitz continuous, confirming the ill-posed nature of the associated inverse problem. Using these properties, the inverse problem is formulated as a minimization problem for the Tikhonov functional, and we establish the existence of a minimizer.

math.AP

Evidence for fully-gapped superconductivity in BCS superconductor NiBi3

We investigate the physical characteristics, normal state and superconducting properties of NiBi3 single crystals. Measurements of electrical resistivity, magnetization, and London penetration depth demonstrate a superconducting transition temperature, Tc=4.0 K, with a sharp transition in resistivity (Tc = 0.20 K) and RRR = 18, reflecting the high quality of NiBi3 single crystals. With both orientations H perpendicular b and H parallel b of NiBi3 single crystals, we estimated the upper critical field, Hc2, from the magnetization data. In both orientations, Hc2 is significantly smaller than the Pauli limit, suggesting the orbital pair breaking in superconducting state. The coherence length, xi(0) = 26.78 nm, electron-phonon coupling constant, lambda(e-p) = 0.81, and penetration depth, lambda0 = 181.8 nm, suggest type-II superconductivity in NiBi3. In the superconducting state, lambda(T) is best described by an s-wave BCS model and does not have linear or quadratic dependency with T, which is in line with the expectation for a node-less superconducting order parameter. The temperature evolution of the superfluid density, obtained from lambda(T), reveals a fully gapped superconductivity in NiBi3, with a superconducting gap = 4.07. All the results from the present study indicate that NiBi3 is a typical type-II, BCS-like, moderately strong coupled, and fully gapped superconductor in the dirty limit.

cond-mat.supr-con

Evidence for Multiband Superconductivity in 2H-NbSeS

The nature of superconductivity in 2H-NbSe2 has generated sustained debate in the recent past. While angle resolved photoemission spectroscopy data have been interpreted as evidence for multiband superconductivity, the data from scanning tunneling microscope experiments relate to strongly anisotropic single-band superconductivity. In the later case, the charge density wave (CDW) order mimics the multigap character. Because the CDW reconstructs the Fermi surface and modifies the superconducting gap distribution, disentangling intrinsic multiband pairing from CDW-related effects is challenging. To address this issue, we investigate single-crystalline 2H-NbSeS, a mixed-chalcogen analogue of 2H-NbSe2 in which random Se/S substitution suppresses long-range CDW order while preserving the layered crystal structure P63/mmc. The material becomes superconducting below 6.0 K with moderate magnetic anisotropy. The upper critical field exhibits a pronounced upward curvature that cannot be described within a single-band framework but is well captured by a dirty-limit two-band model with a large diffusivity ratio. This indicates strong band-dependent scattering. The in-plane upper critical field exceeds the weak-coupling Pauli limit. Measurements of the lower critical field, superfluid density, and electronic specific heat are consistent with an interpretation of a fully gapped superconducting state with two nodeless gaps of different magnitudes.

cond-mat.supr-con

Dimensional Crossover of Mass Anisotropy in Ta-doped WTe2

The observation of extremely large magnetoresistance in WTe2 has attracted considerable attention towards understanding its underlying origin. With its layered van der Waals structure, the question that remains largely unexplored is whether the three-dimensional anisotropic transport characteristics of WTe2 persists under chemical substitution. Here, we present a systematic angle-dependent magneto-transport study of single-crystalline TaxW1-xTe2 (x = 0, 0.05, 0.1). The results are analysed within a mass anisotropy scaling framework to extract the mass anisotropy parameter {\gamma} as a function of temperature and doping. It is observed that Ta substitution leads to monotonic increase of {\gamma} across all temperatures, indicating a progressive deepening of quasi-two-dimensional Fermi surface character. Ta doping also leads to a substantial improvement in crystalline quality, reflected in a pronounced increase in the residual resistivity ratio. Despite weakening electron-hole compensation, the magnetoresistance rises sharply to ~58,211% at x = 0.1, which is assigned to a substantial enhancement in carrier mobility. Rietveld refinement confirms a systematic c-axis contraction with Ta content, identifying the structural origin of the enhanced anisotropy. The mass anisotropy scaling that holds for x = 0 and x = 0.05 breaks down for x = 0.1, where the angular magneto-resistance anisotropy substantially exceeds single-ellipsoid predictions, pointing to a multi-pocket Fermi surface with distinct anisotropies. Nonlinear Hall resistivity provides independent evidence for the underlying multiband character of transport in this system. These findings demonstrate that Fermi surface anisotropy, carrier compensation, and mobility are independent parameters that can lead to tuneable control of large magnetoresistance in topological semimetal WTe2.

cond-mat.mtrl-sci

Effects of Spin Fluctuation and Disorder on Topological States of Quasi 2D Ferromagnet Fe1/5CrTe2

We present a thorough magnetization and magneto-transport study of the diluted Fe-intercalated CrTe2 family member, Fe1/5CrTe2, a van der Waals ferromagnet. Fe1/5CrTe2 shows an elevated Curie transition temperature of 182 K in comparison to the Fe1/3CrTe2 composition, indicating the sensitive role of Fe concentration in modulating magnetic exchange interactions within the CrTe2 framework. The saturated magnetization exhibits a quadratic dependence with temperature, indicating the presence of long-wavelength spin fluctuations. Analysis of the temperature dependent resistivity reveals a dominant T3/2 contribution over the typical T2 behavior, signaling substantial coupling between conduction electrons and localized spins. The magnetoresistance shows a linear and non-saturating negative field dependency throughout a wide temperature range below TC, which is compatible with the increasing suppression of spin-disorder dispersion related to ferromagnetic spin fluctuations. A thorough analysis of the anomalous Hall effect (AHE) shows that extrinsic skew-scattering contribution, which is associated to Fe-related disorder, dominates the anomalous Hall response. The systematic separation of intrinsic and extrinsic components reveals that, over a wide temperature range, the intrinsic anomalous Hall conductivity scales linearly with the saturation magnetization, despite the substantial extrinsic dominant background. The linear behavior of intrinsic anomalous Hall conductivity with magnetization is in line with a long wavelength spin-fluctuation framework, where thermal spin disorder lowers net magnetization without significantly altering the underlying electronic structure. These findings reveal Fe1/5CrTe2 as a newly investigated van der Waals ferromagnet where spin fluctuations and disorder coexist with a well-defined intrinsic Berry-curvature contribution to the Hall response.

cond-mat.str-el

Multiferroicity in the Presence of Exchange Bias: The Case of Spinel CoMn2O4

Ferrimagnetic spinel materials of formula AB2X4, where A and B are transition metals and X is oxygen or sulphur, hold promise for the realization of multiferroic characteristics. In this work, we report synthesis of spinel CoMn2O4 and explore its magnetic, dielectric, and ferroelectric aspects and their correlations. Polycrystalline CoMn2O4 was synthesized by using the conventional solid-state method. The X-ray diffraction (XRD) and Raman spectroscopy confirmed the phase purity of the synthesized compound. The crystal structure was identified with tetragonal symmetry (I41/amd space group). DC magnetization measurements indicate two magnetic transitions: one at temperature T1 ~ 186 K, followed by another Yafet-Kittel (YK) ferrimagnetic transition at T2 ~ 86 K. A frequency independent anomaly in the temperature dependent dielectric permittivity is observed near the low magnetic ordering temperature (T2). This reflects the possibility of the correlation between lattice dynamics and spin ordering in spinel CoMn2O4. A substantial exchange bias was also observed below T2 ~ 86 K. The change in dielectric permittivity in the presence of applied magnetic field follows the square of the magnetization dependence, which is consistent with Ginzburg-Landau theory. However, the detailed pyroelectric current measurements reveal the absence of intrinsic ferroelectric order.

cond-mat.mtrl-sci

Coexistence of Nodal and Nodeless Pairing Symmetry in Superconducting 6R-SnNbSe2

Majorana fermions, a fundamental idea to fault-tolerant quantum computing, can emerge in systems where superconductivity coexists with nontrivial band topology. One promising route to realizing such topological superconductors (TSCs) involves inducing superconductivity in topological materials, particularly in systems lacking inversion symmetry. In this study, we report the synthesis and detailed characterization of Sn-intercalated NbSe2, forming a new polytype, 6R-SnNbSe2. This compound crystallizes in the non-centrosymmetric space group R3m and exhibits bulk superconductivity below Tc around 4 K. Structural, electronic, and magnetic measurements confirm the emergence of a superconducting phase derived from Sn intercalation into the non-superconducting 3R-NbSe2. Temperature-dependent magnetic penetration depth and superfluid density measurements down to 1.5 K are performed using the tunnel diode oscillator technique. The findings suggest the mixing of nodal and nodeless superconductivity in 6R-SnNbSe2. Given the non-centrosymmetric nature of the crystal structure and the theoretical prediction of topological nodal-line features in SnNbSe2, it is an interesting candidate to investigate unconventional pairing mechanisms. Our findings highlight the potential of this material to host nontrivial superconducting states among the transition-metal dichalcogenides.

cond-mat.supr-con

Unconventional Relaxation Dynamics in Co_8Zn_7Mn_5 and Co_8Zn_8Mn_4: Evidence of Inertial Effects

Magnetization relaxation dynamics serve as an essential tool for uncovering the intrinsic mechanisms governing the magnetic response and energy dissipation in magnetic systems. In this work, we examine the relaxation dynamics for Beta Mn type Co_8Zn_7Mn_5 and Co_8Zn_8Mn_4 across a frequency range of 1 kHz to 10 kHz, spanning different magnetic phases. While most magnetic systems tend to follow the Debye-like relaxation with non-zero distribution or the Cole-Cole formalism, our analysis reveal that these conventional models fail to capture frequency dependence of ac susceptibility across different magnetic phases in Co_8Zn_7Mn_5 and Co_8Zn_8Mn_4. Instead, an inertial component is needed to successfully describe the dynamics, suggesting the presence of unconventional relaxation behavior. The characteristic relaxation time is found to be of the order of 10^-5 s for both the compositions. The field dependent variation of relaxation time exhibits a non-monotonic nature, with the double peak like structure at the skyrmion phase transitions, implying slower relaxation dynamics at the phase boundaries. Furthermore, the presence of non-zero difference between isothermal and adiabatic susceptibility in the pure phases implies slower relaxation dynamics, which is consistent with the presence of finite dissipation in pure phases. The inertial term has been previously invoked to describe the dynamics in spin ice systems due to the propagation of magnetic monopoles. However, its necessity in this system, points to a wider significance in magnetization dynamics that goes beyond the conventional spin ices and skyrmions.

cond-mat.mtrl-sci

Magneto transport and first principle study of strong topological insulator gray Arsenic

This article reports the synthesis of a single crystalline gray Arsenic (As) via the Bismuth flux method. The X-ray Diffraction (XRD) pattern revealed the single phase of the grown crystal, which crystallized in the rhombohedral structure with the space group R3m. The sharp XRD peaks observed on mechanically exfoliated thin flakes of the same ensured high crystallinity of the same with growth direction along the c-axis. The resistivity measurements illustrated its metallic nature throughout, right from 300K down to 2K. The measured residual resistivity ratio of the sample is 180, which endorses the high metallic nature of the as-synthesized As single crystal. The transverse magnetic field-dependent resistivity (RH) measurements elucidated huge magneto-resistance (MR) at 2K and 14Tesla transverse magnetic fields. Also seen are the SDH oscillations, indicating the presence of topological surface states. The non-trivial band topology and edge states in As are confirmed by first principle calculations.

cond-mat.mtrl-sci

Disorder Induced Superconductivity in TiSe_1.2S_0.8

Disorder can be utilized as an effective parameter to probe the interplay between two long range orders such as superconductivity and charge density wave. In the present work, we report on the experimental evidence for filamentary superconductivity in polycrystalline TiSe1.2S0.8 with superconducting transition Tc ~ 7K. This is validated from magnetization and magneto-transport measurements. Strain induced dislocations, substitutional defects, and randomly distributed Ti ions (with local moments) are considered as possible sources of disorder. A detailed analysis of the temperature dependent resistivity evaluates the degree of disorder and the consequent localization effects. The findings are in striking contrast to the fact that superconductivity has not been reported in single crystals of TiSe2-xSx system. It is established that disorder serves as a stabilizing factor for the superconducting phase due to in-commensuration of the charge density wave.

cond-mat.supr-con

Kondo Effect in Micron Size Device Fabricated From Flakes of Mn Doped Bi2Se3 Topological Insulator

Single crystals of Mn0.03Bi1.97Se3 were synthesized by modified Bridgman technique and phase purity was confirmed via XRD analysis. EDAX analysis has verified the stoichiometric ratio of elements in the sample. Sample flakes were transferred to the SiO2/Si n-type substrate by mechanical exfoliation technique. Four probe gold contacts were etched with the help of e-beam lithography by masking and lift off process. Resistivity measurement was performed in four probe configurations in 2-300 K temperature range. We report evidence for Kon-do effect in Mn0.03Bi1.97Se3 micro-flakes with Tmin of 14.4 K.

cond-mat.mes-hall

Quantum Linear Magnetoresistance and Fermi Liquid Behavior in Kagome Metal Ni3In2S2

Kagome metals gain attention as they manifest a spectrum of quantum phenomena, including superconductivity, charge order, frustrated magnetism, and intertwined correlated states of condensed matter. With regard to electronic band structure, several of the them exhibit non-trivial topological characteristics. Here, we present a thorough investigation on the growth and the physical properties of single crystals of Ni3In2S2 which is established to be a Dirac nodal line Kagome metal. Extensive characterization is attained through temperature and field-dependent resistivity, angle-dependent magnetoresistance and specific heat measurements. In most metals, the Fermi liquid behaviour is mostly restricted to a narrow range of temperature. In Ni3In2S2, this characteristic feature has been observed for an extensive temperature range of 82 K. This is attributed to the strong electron-electron correlation in the material. Specific heat measurements reveal a high Kadowaki-Woods ratio which is in good agreement with strongly correlated systems. Almost linear positive magnetoresistance follows the conventional Kohler scaling which depicts the applicability of semi-classical theories. The angle-dependent magneto-resistance been explained using the Voigt-Thomson formula. Furthermore, de-Haas van Alphen oscillations are observed in magnetization vs. magnetic field measurement which shed light on the topological features in the Shandite Ni3In2S2.

cond-mat.str-el

Electromagnetic properties of copper doped lead apatite Pb9Cu(PO4)6O

We report on the structural, electrical and magnetic measurements in as-grown polycrystalline samples of Pb10-xCux(PO4)6O. This compound has been recently reported to be a room temperature superconductor. Our as-grown specimen has excellent XRD matching with the original submission of Lee et al. This sample has 1.5% of Cu2S as an impurity phase. A resistive transition around 380 K, possibly corresponding to structural transitions of Cu2S, is observed. No evidence of superconducting to normal state transitions in I-V characteristics at room temperature is obtained. Magnetization measurements show linear diamagnetic behavior that cannot be associated to the superconducting state. Hall measurements provide evidence of hole doping through Cu substitution. In summary, we find no evidence for room temperature ambient pressure superconductivity in Cu doped lead apatite Pb9Cu(PO4)6O.

cond-mat.mtrl-sci

Effect of Spin Fluctuations on Magnetoresistance and Anomalous Hall Effect in the Chiral Magnet Co8Zn8Mn4

The beta Mn type Co-Zn-Mn alloys have seized significant attention due to their ability to host skyrmions at room temperature. Here we analyse the unconventional magneto-transport properties of Co8Zn8Mn4 single crystals with a Curie temperature of 275 K. A negative magnetoresistance is obtained over a wide temperature range of 50K to 300K. The deviation of the isothermal magnetoresistance (MR) curves from linearity to non-linearity as one approaches higher temperatures points towards the transition from the dominance of magnons to spin fluctuations. In the paramagnetic phase, the change in the shape of the MR curve has been explained using the Khosla and Fischer model. The relationship between the anomalous Hall effect (AHE) and longitudinal resistivity reveals the dominance of the skew-scattering mechanism, which is inexplicable based on the theories of semi-classical magneto-transport. We experimentally determine that the spin fluctuation is the source of the skew-scattering mechanism in Co8Zn8Mn4. In general skew-scattering mechanisms predominate in compounds with high conductivity, but our findings demonstrate that this is not always the case and that other aspects also require equal consideration. Our work throws new light on the predominant scattering mechanism in chiral magnets with skyrmionics phase at low conductivity.

cond-mat.mtrl-sci

On the Experimental Evidence for Possible Superconductivity in LK99

The desire to create an energy efficient world is bound to be incomplete without the discovery of a room temperature superconductor at ambient pressure. A recent report on the room-temperature ambient-pressure superconductor has inspired scientists to study the Cu doped Lead apatite named as LK-99. Here, we have synthesized Cu doped LK-99 and Ni-doped LK-99 compounds and studied their temperature dependent transport and magnetization behavior. In spite of the presence of impurity phase Cu$_2$S, the temperature dependent resistance shows an insulating nature of the sample. The radio frequency penetration depth measurement unveils the absence of diamagnetic flux expulsion in this sample. The temperature dependent ac susceptibility measurements reveal the paramagnetic nature of the Ni doped LK-99.

cond-mat.supr-con

Conventional Type-II Superconductivity in 2H-TaSeS

Superconductors based on transition metal dichalcogenides are of substantial current relevance, towards attaining topological superconductivity. Here we report a detailed study on the synthesis and electromagnetic characterization of high-quality single crystals of TaSeS. A superconducting transition is confirmed at 4.15K with coexisting charge density wave onset at 66K. The temperature dependence of RF penetration depth indicates s-wave characteristics in the weak coupling limit. A moderate electronic anisotropy is observed in upper critical fields with a value of 1.52. DFT calculations confirm the possibility of superconducting behavior of TaSeS and also suggest that the most stable structure belongs to P63mc space group. Negative values in phonon dispersion curves verify the possibility of co-existing CDW in 2H-TaSeS. Arrhenius plots show power law dependence of activation energy with respect to magnetic field. Overall all characteristics imply TaSeS to be a classic Type-II superconductor without any evidence for topological superconductivity.

cond-mat.supr-con

Two-fold anisotropic superconducting state in topological superconductor Sn$_4$Au

Here we report the anisotropic magnetotransport properties in the superconducting state of Sn$_4$Au single crystal. Sn$_4$Au single crystal is synthesized through an easy melt growth method. Superconducting properties are evidenced by resistivity vs. temperature and DC magnetization measurements. Isothermal magnetization measurements hint toward type-II superconductivity in Sn$_4$Au. In-plane and out-of-plane resistivity measurements show anisotropic behavior of the upper critical field at temperatures below superconducting transition (T$_c$ = 2.3 K). The observed anisotropy is more elucidated in resistivity measurements performed below Tc at different tilt angles. The anisotropy parameter is found to be 1.26. The observed results show the presence two-fold anisotropic superconducting state in Sn$_4$Au single crystal, which may be induced due to the layered structure of synthesized Sn$_4$Au single crystal.

cond-mat.supr-con

Crystal orientation dependent spin pumping in Bi0.1Y2.9Fe5O12/Pt interface

Ferromagnetic resonance (FMR) based spin pumping is a versatile tool to quantify the spin mixing conductance and spin to charge conversion (S2CC) efficiency of ferromagnet/normal metal (FM/NM) heterostructure. The spin mixing conductance of FM/NM interface can also be tuned by the crystal orientation symmetry of epitaxial FM. In this work, we study the S2CC in epitaxial Bismuth substituted Yttrium Iron Garnet (Bi0.1Y2.9Fe5O12) thin films Bi-YIG (100 nm) interfaced with heavy metal platinum (Pt (8 nm)) deposited by pulsed laser deposition process on different crystal orientation Gd3Ga5O12 (GGG) substrates i.e. [100] and [111]. The crystal structure and surface roughness characterized by X-Ray diffraction and atomic force microscopy measurements establish epitaxial Bi-YIG[100], Bi-YIG[111] orientations and atomically flat surfaces respectively. The S2CC quantification has been realized by two complimentary techniques, (i) FMR-based spin pumping and inverse spin Hall effect (ISHE) at GHz frequency and (ii) temperature dependent spin Seebeck measurements. FMR-ISHE results demonstrate that the [111] oriented Bi-YIG/Pt sample shows significantly higher values of spin mixing conductance ((2.31+-0.23)x10^18 m^-2) and spin Hall angle (0.01+-0.001) as compared to the [100] oriented Bi-YIG/Pt. A longitudinal spin Seebeck measurement reveals that the [111] oriented sample has higher spin Seebeck coefficient (106.40+-10 nV mm-1 K-1). This anisotropic nature of spin mixing conductance and spin Seebeck coefficient in [111] and [100] orientation has been discussed using the magnetic environment elongation along the surface normal or parallel to the growth direction. Our results aid in understanding the role of crystal orientation symmetry in S2CC based spintronics devices.

cond-mat.mtrl-sci