arXiv subjects

Sukhdeep Dhillon

Publications and source records attributed to Sukhdeep Dhillon.

12 recordsLinked to original sources

arXiv2026

Optimizing spin-based terahertz emission from magnetic heterostructures

Terahertz radiation pulses can be generated efficiently through femtosecond laser excitation of a ferromagnetic/nonmagnetic heterostructure, wherein an ultrafast laser-induced spin current results in an electromagnetic THz pulse due to spin-charge conversion. It is, however, still poorly understood how the THz emission amplitude and its bandwidth can be optimized. Here, we perform a systematic analysis of the THz emission from various magnetic heterostructures. The dynamics of the spin current is described by the semiclassical, superdiffusive spin-transport model and the energy dependence of the spin Hall effect of hot electrons is taken into account, leading to emission profiles for Co(2 nm)/Pt(4 nm) bilayer in good agreement with experiment. To identify the optimal {conditions} for THz emission, {we study} the properties of the emitted THz wave profile by systematically varying the layer thicknesses of metallic bilayers, their interfacial spin-current transmission properties, their materials' dependence, and influence of the pump laser-pulse width, allowing us to give optimization guidelines. We find that thin nonmagnetic layer thicknesses of 5-6 nm provide the largest bandwidth in the case of Co/Pt and that the peak frequency of the THz emission depends only on the geometry of the emitter and not on the laser pulse width. The THz bandwidth {is conversely found to} depend on several factors such as exciting laser pulse width, layers' thicknesses, and interface transmission-reflection properties, with the limitation that an increase in the bandwidth by tuning the interface properties comes with a trade-off in the energy efficiency of the emitter. Lastly, we propose a double pulse excitation protocol of a trilayer system that could provide broadband THz emission with a large bandwidth. {Our results contribute to establishing guidelines for optimizing spintronic THz generation.

cond-mat.mtrl-sci↗

arXiv2026

Thickness-Dependent Spintronic Terahertz Emission in MBE-Grown PtTe$_2$: From Semiconductor to Type-II Dirac Semimetal

Spintronic terahertz (THz) emitters have established themselves as among the most practical broadband THz sources available, yet their performance remains fundamentally limited by the spin Hall conductivity of the nonmagnetic conversion layer - a quantity that is fixed once the material is chosen. Here, we demonstrate that in PtTe$_2$, a type-II Dirac semimetal within the transition metal dichalcogenide family, this limitation can be circumvented by exploiting the dramatic thickness-driven electronic phase evolution of the material itself. Using molecular beam epitaxy to grow PtTe$_2$ films with single-monolayer precision from 1 to 20 ML, we show that the spintronic THz emission tracks the underlying electronic phase diagram directly: it is absent in the single-layer semiconducting phase, turns on sharply at the semimetal transition near 2 ML, and reaches a peak amplitude six times that of an equivalent Pt reference at 10 ML, before declining at larger thicknesses due to THz reabsorption in the increasingly metallic film. This non-monotonic behavior is inconsistent with a bulk inverse spin Hall mechanism and instead reflects a multi-channel spin-to-charge conversion process in which spin-momentum-locked topological surface states and a thickness-dependent interfacial Rashba splitting both contribute and strengthen as the type-II Dirac band structure develops. First-principles calculations of the interfacial spin accumulation reproduce the experimental trend quantitatively, confirming this physical picture. These findings introduce thickness engineering of van der Waals semimetals as a new and accessible route to optimizing spintronic THz emitters and spin-orbit torques in magnetic memories (SOT-MRAMs), with direct implications for the broader class of dimensionally tunable topological materials.

cond-mat.mtrl-sci↗

arXiv2026

Rashba engineering at van der Waals interfaces

Two-dimensional transition metal dichalcogenide (TMD) interfaces offer a versatile platform for studying emergent quantum phenomena and enabling novel device functionalities. When distinct TMD monolayers are stacked vertically or laterally stitched, their interfaces can exhibit unique electronic band alignments, giving rise to long-lived interlayer excitons, charge transfer effects, and moiré superlattices with correlated states. Here, we demonstrate that the interface between a large variety of two different epitaxially grown TMD monolayers controls the intensity and sign of the Rashba spin splitting, which is probed using THz spintronic emission. Optimized TMD heterobilayers, such as HfSe$_2$/PtSe$_2$, show enhanced THz emission that surpass the spin-to-charge conversion efficiency of bulk TMDs, confirming the presence of Rashba states with large spin splitting at the interface. By combining spin- and angle-resolved photoemission spectroscopy with density functional theory, we reveal that the electronic hybridization between the two different TMD monolayers gives rise to extended in-gap states with strong Rashba spin-orbit coupling. The choice of TMD layers enables to engineer the sign and strength of spin-to-charge conversion in van der Waals heterobilayers opening up perspectives to build efficient and tunable THz spintronic emitters.

cond-mat.mes-hall↗

arXiv2026

Quantum cascade laser roadmap

Quantum cascade lasers (QCLs) are unipolar semiconductor lasers first demonstrated in 1994. Since then, they have played a central role in advancing mid-infrared and terahertz photonics, becoming among the most reliable light sources in these regions of the electromagnetic spectrum. Their importance is further reinforced by their ability to generate self-starting optical frequency combs, whose investigation is motivated both by fundamental physics and by a wide range of applications, including molecular spectroscopy and free-space optical communications. This Roadmap provides a unified overview of current advances and emerging directions in QCL research. The chapters are organized into three main sections: device design and technology; frequency combs and pulse formation; and applications of QCLs. Each chapter reviews the relevant background, summarizes the current state of the art, and identifies key challenges and future directions within its specific research area.

physics.optics↗

arXiv2025

Phonon-tunable THz magnonic emission in multiferroic heterostructures

Collective excitations such as magnons and polar phonons provide natural access to the terahertz (THz) regime, but efficient generation and tunability remain elusive. Multiferroic BiFeO3 combines both orders at room temperature, offering a unique platform for narrowband THz emission. Here, we achieve efficient sub-bandgap optical rectification of coupled phonon-polaritons near 2 THz in bare epitaxial thin films. In Pt/BiFeO3 bilayers, we demonstrate that coupling the electromagnon branch with ultrafast strain waves, optically generated in Pt layers with various thicknesses, can produce tunable and narrowband emission between 0.4-0.8 THz. These results uncover the intertwined role of phonons, magnons, and magneto-acoustic dynamics in antiferromagnetic multiferroics, and establish these hybrid platforms as versatile engineered narrowband THz sources.

cond-mat.mes-hall↗

arXiv2025

Mid-Infrared Frequency Combs and Pulse Generation based on Single Section Interband Cascade Lasers

Interband Cascade Lasers (ICLs) are semiconductor lasers emitting in the mid-wave infrared (MWIR 3-6 μm) and can operate as frequency combs (FCs). These demonstrations are based on double section cavities that can reduce dispersion and/or are adapted for radio-frequency operation. Here we show that ICLs FCs at long wavelengths, where the refractive index dispersion reduces, can be realized in a single long section cavity. We show FC generation for ICLs operating at λ ~ 4.2 μm, demonstrating narrow electrical beatnotes over a large current range. We also reconstruct the ultrafast temporal response through a modified SWIFT spectroscopy setup with two fast MWIR detectors, which shows a frequency modulated response in free-running operation. Further, we show that, through active modelocking, the ICL can be forced to generate short pulses on the order of 3 ps. This temporal response is in agreement with Maxwell Bloch simulations, highlighting that these devices possess long dynamics (~100ps) and potentially makes them appropriate for the generation of large peak powers in the MWIR.

physics.optics↗

arXiv2024

Quantum transport signature of strain-induced scalar and pseudo-vector potentials in a crenellated hBN-graphene heterostructure

The sharp Dirac cone of the electronic dispersion confers to graphene a remarkable sensitivity to strain. It is usually encoded in scalar and pseudo-vector potentials, induced by the modification of hopping parameters, which have given rise to new phenomena at the nanoscale such as giant pseudomagnetic fields and valley polarization. Here, we unveil the effect of these potentials on the quantum transport across a succession of strain-induced barriers. We use high-mobility, hBN-encapsulated graphene, transferred over a large (10x10 $μ$m$^{2}$) crenellated hBN substrate. We show the emergence of a broad resistance ancillary peak at positive energy that arises from Klein tunneling barriers induced by the tensile strain at the trench edges. Our theoretical study, in quantitative agreement with experiment, highlights the balanced contributions of strain-induced scalar and pseudo-vector potentials on ballistic transport. Our results establish crenellated van der Waals heterostructures as a promising platform for strain engineering in view of applications and basic physics.

cond-mat.mes-hall↗

arXiv2023

Atomic Layer-controlled Nonlinear Terahertz Valleytronics in Dirac Semi-metal and Semiconductor PtSe2

Platinum diselenide (PtSe2) is a promising two-dimensional (2D) material for the terahertz (THz) range as, unlike other transition metal dichalcogenides (TMDs), its bandgap can be uniquely tuned from a semiconductor in the near-infrared to a semimetal with the number of atomic layers. This gives the material unique THz photonic properties that can be layer-engineered. Here, we demonstrate that a controlled THz nonlinearity - tuned from monolayer to bulk PtSe2 - can be realised in wafer size polycrystalline PtSe2 through the generation of ultrafast photocurrents and the engineering of the bandstructure valleys. This is combined with the PtSe2 layer interaction with the substrate for a broken material centro-symmetry permitting a second order nonlinearity. Further, we show layer-dependent circular dichroism, where the sign of the ultrafast currents and hence the phase of the emitted THz pulse can be controlled through the excitation of different bandstructure valleys. In particular, we show that a semimetal has a strong dichroism that is absent in the monolayer and few layer semiconducting limit. The microscopic origins of this TMD bandstructure engineering is highlighted through detailed DFT simulations and show that circular dichroism can be controlled when PtSe2 becomes a semimetal and when the K-valleys can be excited. As well as showing that PtSe2 is a promising material for THz generation through layer controlled optical nonlinearities, this work opens up new class of circular dichroism materials beyond the monolayer limit that has been the case of traditional TMDs, and impacting a range of domains from THz valleytronics, THz spintronics to harmonic generation.

cond-mat.mtrl-sci↗

arXiv2022

Self-Kerr effect across the yellow $\mathrm{Cu_2O}$ Rydberg series

We investigate the nonlinear refraction induced by Rydberg excitons in $\mathrm{Cu_2O}$. Using a high-precision interferometry imaging technique that spatially resolves the nonlinear phase shift, we observe significant shifts at extremely low laser intensity near each exciton resonance. From this, we derive the nonlinear index $\mathrm{n_2}$, present the $\mathrm{n_2}$ spectrum for $n\geq 5$ and report large $\mathrm{n_2}$ values of order $10^{-3}$ mm$^2$/mW. Moreover, we observe a rapid saturation of the Kerr nonlinearity and find that the saturation intensity $\mathrm{I_{sat}}$ decreases as $n^{-7}$. We explain this with the Rydberg blockade mechanism, whereby giant Rydberg interactions limit the exciton density, resulting in a maximum phase shift of 0.5 rad in our setup.

quant-ph↗

arXiv2021

Chip-scale terahertz frequency combs through integrated intersubband polariton bleaching

Quantum cascade lasers (QCLs) represent a fascinating accomplishment of quantum engineering and enable the direct generation of terahertz (THz) frequency radiation from an electrically-biased semiconductor heterostructure. Their large spectral bandwidth, high output powers and quantum-limited linewidths have facilitated the realization of THz pulses by active mode-locking and passive generation of optical frequency combs (FCs) through intracavity four-wave-mixing, albeit over a restricted operational regime. Here, we conceive an integrated architecture for the generation of high power (10 mW) THz FCs comprising an ultrafast THz polaritonic reflector, exploiting intersubband cavity polaritons, and a broad bandwidth (2.3-3.8 THz) heterogeneous THz QCL. Quantum cascade lasers (QCLs) represent a fascinating accomplishment of quantum engineering and enable the direct generation of terahertz (THz) frequency radiation from an electrically-biased semiconductor heterostructure. By tuning the group delay dispersion in an integrated geometry, through the exploitation of light induced bleaching of the intersubband-based THz polaritons, we demonstrate spectral reshaping of the QCL emission and stable FC operation over an operational dynamic range of up to 38%, characterized by a single and narrow (down to 700 Hz) intermode beatnote. Our concept provides design guidelines for a new generation of compact, cost-effective, electrically driven chip-scale FC sources based on ultrafast polariton dynamics, paving the way towards the generation of mode locked THz micro-lasers that will strongly impact a broad range of applications in ultrafast sciences, data storage, high-speed communication and spectroscopy.

physics.optics↗

arXiv2021

Spin injection efficiency at metallic interfaces probed by THz emission spectroscopy

Terahertz (THz) spin-to-charge conversion has become an increasingly important process for THz pulse generation and as a tool to probe ultrafast spin interactions at magnetic interfaces. However, its relation to traditional, steady state, ferromagnetic resonance techniques is poorly understood. Here we investigate nanometric trilayers of Co/X/Pt (X=Ti, Au or Au0:85W0:15) as a function of the 'X' layer thickness, where THz emission generated by the inverse spin Hall effect is compared to the Gilbert damping of the ferromagnetic resonance. Through the insertion of the 'X' layer we show that the ultrafast spin current injected in the non-magnetic layer defines a direct spin conductance, whereas the Gilbert damping leads to an effective spin mixing-conductance of the trilayer. Importantly, we show that these two parameters are connected to each other and that spin-memory losses can be modeled via an effective Hamiltonian with Rashba fields. This work highlights that magneto-circuits concepts can be successfully extended to ultrafast spintronic devices, as well as enhancing the understanding of spin-to-charge conversion processes through the complementarity between ultrafast THz spectroscopy and steady state techniques.

cond-mat.mes-hall↗

arXiv2021

Tamm Cavity in the Terahertz Spectral Range

Electromagnetic resonators, which are based on optical cavities or electronic circuits, are key elements to enhance and control light-matter interaction. In the THz range, current optical cavities exhibit very high-quality factors with $(λ/2)^3$ mode volumes limited by diffraction, whereas resonant electronic circuits show low quality factor but provide strong subwavelength effective volume ($10^{-6} λ^3$). To overcome the limitations of each type of resonator, great efforts are being devoted to improving the performances of current methods or to the emergence of original approaches. Here, we report on an optical resonator based on Tamm modes newly applied to the THz range, comprising a metallic layer on a distributed Bragg reflector and demonstrating a high-quality factor of 230 at $\sim$1 THz. We further experimentally and theoretically show a fine-tuning of the Tamm mode frequency (over a 250 GHz range) and polarization sensitivity by subwavelength structuration of the metallic layer. Electromagnetic simulations also reveal that THz Tamm modes are confined over a $λ$/2 length within the distributed Bragg reflector and can be ideally coupled to both bulk materials and 2D materials. These THz Tamm cavities are therefore attractive as basic building blocks of lasers, for the development of advanced THz optoelectronic devices such as sensitive detectors, high-contrast modulators, narrow filters, and polarizers, as well as for THz cavity quantum electrodynamics in nanostructures.

physics.optics↗