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Wenze Lan

Publications and source records attributed to Wenze Lan.

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Excitonic fingerprints of magnetic configurations and switching in multilayer CrSBr

The coupling between electronic states and magnetism provides a route towards optical readout and control of magnetic information. In the magnetic semiconductor CrSBr, excitons are coupled to magnetic order, making their optical response sensitive to the underlying magnetization. Here, we show that the energy and oscillator strength of bulk and surface excitons provide distinct spectroscopic fingerprints of magnetic configurations and switching pathways. We distinguish domain-wall-mediated magnetization reversal, manifested by continuous spectral evolution as a domain wall traverses the optical spot, from abrupt, large-area magnetization reversal. Using the resulting excitonic fingerprints, we reconstruct successive magnetic configurations in 4- and 5-layer CrSBr during the transition from ferromagnetic to antiferromagnetic order. We further find that the sensitivity to magnetic order is strongly exciton-dependent: low-energy excitons resolve intermediate and surface-related configurations, whereas a higher-energy exciton predominantly exhibits a transfer of oscillator strength between ferromagnetic and antiferromagnetic resonances. These results establish excitonic spectroscopy as a sensitive probe of layer-dependent magnetic configurations and their switching pathways in layered magnetic semiconductors.

cond-mat.mtrl-sci

Re-evaluation of bottleneck effect via a coupled monolayer WS_2/photonic crystal heterostructure

Exciton-polariton condensates is an important type of Bose-Einstein condensate whose realization requires efficient relaxation of polaritons to the band-energy minima. However, this process is often obstructed by bottleneck effect near the anticrossing region of polariton dispersion. Although the exciton-polariton bottleneck effect has been extensively observed in various polariton system, but there is no a unified views of physical origin. Here, we construct an exciton-trion-photon coupling system in monolayer WS_2/photonic-crystal slab heterostructures. Momentum-resolved photoluminescence reveals the anticrossing polariton dispersions for the exciton resonance with a ~57 meV Rabi splitting and there is no characteristic anticrossing for trion resonance with a ~5 meV splitting at ~12 K. Enhanced polariton emission is observed around the trion-polariton crossing with elevating temperature. We attributes this exotic phenomenon to bottleneck effect and indicating that small Rabi splitting is the unified origin of bottleneck effect in polariton systems.

physics.optics

Role of a Quarter-Wave Plate in Confocal Microscopy: Signature of Spin-Orbit Interactions

Spin-orbit interactions of light couple polarization and spatial degrees of freedom, underpinning phenomena such as the spin Hall effect of light. Although widely explored at interfaces and in tightly focused beams, their impact in nominally paraxial confocal systems remains largely unexamined. Here we show that a single quarter-wave plate embedded in a simple confocal geometry between polarizers can strongly reshape the transverse structure of a Gaussian beam. We observe an enhancement of the polarization extinction ratio by more than two orders of magnitude, accompanied by a transformation of the Gaussian intensity profile into a first-order Hermite-Gaussian-like two-lobe mode. The orientation of this pattern is continuously tunable via rotation of the wave plate, evidencing polarization-controlled reorientation of the transverse field. To explain these observations, we introduce a minimal extension of Jones matrix formalism incorporating complex parameters that quantitatively reproduces the measurements. Our results uncover a previously overlooked form of spin-orbit-mediated mode control in standard confocal optics and establish a simple route to on-demand spatial mode engineering for applications in resonant spectroscopy, optical imaging and quantum optics.

physics.optics

Twist-tuned exchange and hysteresis in a bilayer van der Waals magnet

Moiré superlattices in twisted bilayers enable profound reconstructions of the electronic bandstructure, giving rise to correlated states with remarkable tunability. Extending this paradigm to van der Waals magnets, twisting creates spatially varying interlayer exchange interactions that stabilize emergent spin textures and the coexistence of ferromagnetic and antiferromagnetic domains. Here, we demonstrate the emergence of robust magnetic hysteresis in bilayer CrSBr upon twisting by an angle of ~ 3°. This is observed as the corresponding hysteretic evolution of the exciton energy, that directly correlates with the bilayer magnetic state, in magnetic field dependent photoluminescence measurements. A two-sublattice model captures this behavior, attributing it to the twist-induced reduction of interlayer exchange that stabilizes both parallel and antiparallel spin configurations across a broad field range. Comparison with experiment enables quantitative extraction of the effective exchange strength. Remarkably, the system exhibits coherent averaging across the moiré supercell, yielding an effective monodomain response characterized by switching into the antiferromagnetic state, rather than forming spin textures or fragmented domains. Spatially resolved measurements further uncover local variations in hysteresis loops, consistent with position-dependent modulation of the average exchange interaction. Our results establish twist engineering as a powerful route to programmable magnetic memories in two-dimensional magnets, harnessing the robustness of antiferromagnetic order.

cond-mat.mtrl-sci

Visualization of Photonic Band Structures via Far-field Measurements in SiNx Photonic Crystal Slabs

The band structures of the photonic crystal slabs play a significant role in manipulating the flow of light and pre-dicting exotic physics in photonics. In this letter, we show that the key features of photonic band structures can be achieved experimentally by the polarization- and momentum-resolved photoluminescence spectroscopy utilizing the light emission properties of SiNx. The two-dimensional spectra clearly reveal the energy-momentum dispersion of band structures which is in perfect agreement with the simulation results. The isofrequency contours can be measured easily by adding a bandpass filter with a desired photon energy. Furthermore, it is convenient to observe clearly and directly the optical singularity -- the optical bound states in the continuum featured by dark point in three-dimensional photoluminescence spectra. The polarization-resolved isofrequency contours clearly show that this dark point is the center of an azimuthally polarized vortex. Finally, the helical topological edge states can be easily observed in photonic topological insulators with deformed hexagonal lattices. Our work provides a simple and effective approach for exploring topological photonics and other intriguing phenomena hidden in the photonic crystal slabs.

physics.optics

Probing Phase Transition of Band Topology via Radiation Topology

Topological photonics has received extensive attention from researchers because it provides brand new physical principles to manipulate light. Band topology of optical materials is characterized using the Berry phase defined by Bloch states. Until now, the criteria for experimentally probing the topological phase transition of band topology has always been relatively lacking in topological physics. Moreover, radiation topology can be aroused by the far-field polarizations of the radiating Bloch states, which is described by the Stokes phase. Although such two types of topologies are both related to Bloch states on the band structure, it is rather surprising that their development is almost independent. Here, we reveal that the phase transition of band topology can be probed by the radiation topology. We theoretically design and experimentally demonstrate such an intriguing phenomenon by constructing photonic crystals that support optical analogs of quantum spin Hall effects. The results show that the topological charge of the far-field polarization vortex changes from +1 to -2 or from -2 to +1 when the band topology changes from trivial to non-trivial, which provides a new criterion to probe the phase transition of band topology using radiation topology. Our findings not only provide an insightful understanding of band topology and radiation topology, but also can serve as a novel route to manipulate the near and far fields of light.

physics.optics

Polarized exciton emission enhancement of monolayer MoS2 coupled with plasmonic Salisbury-type absorber

The plasmon-mediated manipulation of light-matter interaction in two-dimensional atomically transition-metal dichalcogenides (TMDs) critically depends on the design of plasmonic nanostructures to achieve the maximum optical field in TMDs. Here, a metal-isolator-metal Salisbury-type perfect absorber was fabricated to serve as a generator of the localized surface plasmons. The significant photoluminescence (PL) enhancement up to 60-fold was observed experimentally in the monolayer (ML) MoS2 on the top of this gold plasmonic hybrid nanostructures. Furthermore, the PL linear polarization can approach ~60 % around the peak of exciton emission and is independent on the polarization of the excitation laser. This Salisbury-type plasmon-exciton hybrid system paves a new way to develop optoelectronic devices based on TMDs.

physics.optics