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Xiu-Ping Xie

Publications and source records attributed to Xiu-Ping Xie.

At least 19 recordsLinked to original sources

High-Performance Quantum Frequency Conversion from Ultraviolet to Telecom Band

Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. In this work, we demonstrate a short-wavelength-pumping QFC with the first-order quasi-phase matching period of 3.07 um on thin-film lithium niobate, converting ultraviolet photons to the telecom C-band. By constructing a theoretical model that correlates the normalized conversion efficiency with domain defects in the short-period phase-matched waveguide, we found the critical tolerance of domain defects along the waveguide should be $\le 2$ (excluding the ends). Based on this, we achieved a theoretical limit normalized conversion efficiency of 839%/(W*cm^2) for the fundamental guided mode through fabrication optimization. Furthermore, we propose a robust noise suppression strategy for short-wavelength pumping by utilizing the counter-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion. By combining these advances with ultra-narrowband filtering, we achieve a record-high external efficiency of 28.8% and an ultra-low noise of 35 counts per second. This high-performance QFC connecting ultraviolet and telecom bands satisfies the stringent requirements for long-lived remote ion-ion entanglement in scalable quantum networks [W.-Z. Liu et al., Nature (2026)].

quant-ph

Device-independent quantum key distribution over 100 km with single atoms

Device-independent quantum key distribution (DI-QKD) is a key application of the quantum internet. We report the realization of DI-QKD between two single-atom nodes linked by 100-km fibers. To improve the entangling rate, single-photon interference is leveraged for entanglement heralding, and quantum frequency conversion is used to reduce fiber loss. A tailored Rydberg-based emission scheme suppresses the photon recoil effect on the atom without introducing noise. We achieved high-fidelity atom-atom entanglement and positive asymptotic key rates for fiber lengths up to 100 km. At 11 km, 1.2 million heralded Bell pairs were prepared over 624 hours, yielding an estimated extractable finite-size secure key rate of 0.112 bits per event against general attacks. Our results close the gap between proof-of-principle quantum network experiments and real-world applications.

quant-ph

Metrology-grade mid-infrared spectroscopy for multi-dimensional perception

The mid-infrared spectral window is essential for molecular fingerprinting and atmospheric sensing, yet unlocking its full potential is currently constrained by a fundamental instrumental trade-off: existing systems cannot simultaneously deliver broad bandwidth, high photon flux, and metrological frequency fidelity. Here, we resolve this bottleneck by demonstrating a metrology-grade spectroscopic system based on difference frequency generation, driven by widely tunable, near-infrared diode lasers traceable to atomic standards. Our system achieves continuous tunability across the 3-3.7 $μ$m atmospheric window and delivers output power exceeding 45 mW with an absolute frequency accuracy of 7.2 MHz. We harness this convergence to overcome a critical barrier in integrated photonics, unambiguously identifying and eliminating hydrogen-induced absorption in silicon nitride microresonators to achieve an 88-fold reduction in optical loss. We further reveal multi-phonon absorption in the silica cladding as the fundamental limit to mid-infrared integrated photonics. Finally, we demonstrate the system's versatility through scattering-resilient LiDAR capable of penetrating optically dense fog, and dual-modality sensing that simultaneously retrieves target distance and chemical composition. By unifying the rigor of frequency metrology with the versatility of broadband sensing, this architecture establishes a new paradigm for multi-dimensional perception in complex environments.

physics.optics

Electrically pumped ultra-efficient quantum frequency conversion on thin film lithium niobate chip

Quantum frequency conversion (QFC) plays a crucial role in constructing seamless interconnection between quantum systems operating at different wavelengths. To advance future quantum technology, chip-scale integrated QFC components, featuring high efficiency, small footprint, low power consumption and high scalability, are indispensable. In this work, we demonstrate the first hybrid integrated QFC chip on thin film lithium niobate platform that connects the telecom and visible bands. Benefiting from the periodically poled microring resonator with ulta-high normalized conversion efficiency of 386,000 %/W, an ultra-low pump power of 360 μW is achieved which is more than two orders of magnitude lower than traditional straight waveguide scheme. By injecting current into the chip, an on-chip quantum efficiency of 57% and a noise count of ~ 7k counts per second are achieved. Such an electrically pumped, integrated and scalable QFC chip would significantly advancing the integration of quantum network and the development of chip-scale quantum optical systems.

quant-ph

Realization of an untrusted intermediate relay architecture using a quantum dot single-photon source

To fully exploit the potential of quantum technologies, quantum networks are needed to link different systems, significantly enhancing applications in computing, cryptography, and metrology. Central to these networks are quantum relays that can facilitate long-distance entanglement distribution and quantum communication. In this work, we present a modular and scalable quantum relay architecture using a high-quality single-photon source. The proposed network incorporates three untrusted intermediate nodes and is capable of a repetition rate of 304.52 MHz. We use a measurement-device-independent protocol to demonstrate secure key establishment over fibers covering up to 300 kilometers. This study highlights the potential of single-photon sources in quantum relays to enhance information transmission, expand network coverage, and improve deployment flexibility, with promising applications in future quantum networks.

quant-ph

Electrically pumped ultrabright entangled photons on chip

Entangled photon sources (EPS) are essential for quantum science and technology. Despite advancements in integrated optical platforms like thin-film lithium niobate, a scalable, high-performance, chip-scale EPS has remained elusive. We address this by demonstrating an electrically pumped, post-selection-free polarization-EPS, achieved through hybrid integration of a distributed feedback laser with thin-film lithium niobate chip which integrates periodically poled lithium niobate waveguides, beam splitter, and polarization rotator combiner. By injecting current into the chip, we realize a high-performance EPS with a bandwidth of 73 nm and an entanglement pair generation rate of 4.5*10^10 pairs/s/mW. The polarization entanglement shows Bell-state fidelities above 96% across frequency-correlated modes. This compact, integrated EPS enables key applications, including high-speed quantum key distribution via wavelength division multiplexing, satellite-based quantum communication, and entanglement-based quantum metrology.

quant-ph

Silicon single-photon detector achieving over 84% photon detection efficiency with flexible operation modes

Silicon single-photon detectors (Si SPDs) play a crucial role in detecting single photons in the visible spectrum. For various applications, photon detection efficiency (PDE) is the most critical characteristic for effectively collecting photons. Here, we present a Si SPD with a remarkable PDE of up to 84.4% at 785 nm, supporting multiple operation modes. We design and fabricate a thick-junction Si single-photon avalanche diode (SPAD) that enhances the avalanche probability through a backside-illumination structure, while minimizing noise through the design of a doping-compensated avalanche region. To maximize PDE, we implement a readout circuit with a 50 V quenching voltage, enabling operation in free-running, gating, or hybrid modes. The SPAD, along with its readout circuits and affiliated circuits, is integrated into a compact SPD module. In free-running mode, the module achieves a maximum PDE of 84.4%, with a dark count rate of 260 cps, and an afterpulse probability of 2.9% at 268 K. This work provides a practical solution for applications requiring ultra-high-efficiency Si SPD with multiple operation modes.

quant-ph

Ultrabright Entanglement Based Quantum Key Distribution over a 404 km Optical Fiber

Entangled photons are crucial resources for quantum information processing. Here, we present an ultrabright polarization-entangled photon source based on a periodically poled lithium niobate waveguide designed for practical quantum communication networks. Using a 780 nm pump laser, the source achieves a pair generation rate of 2.4 $\times 10^{10}$ pairs/s/mW. Remarkably, the entangled photons are bright enough to be detected by a power meter, reaching a power of 17.9 nW under a pump power of 3.2 mW. We demonstrate the practicality of the source by conducting quantum key distribution experiments over long-distance fiber links. Wavelength-division multiplexing was employed to enhance the key generation, and nonlocal dispersion compensation was implemented to ensure precise timing coincidence measurements across a broad spectral range. By utilizing nine pairs of wavelength channels, the system achieved the applicable secure key rates of up to 440.80 bits/s over 200 km with a 62 dB loss and extended the maximum secure key generation distance to 404 km. These results demonstrate the potential of wavelength-multiplexed polarization-entangled photon sources for high-speed, long-distance quantum communication, positioning them as key components for future large-scale quantum networks.

quant-ph

Entangling quantum memories over 420 km in fiber

Long-distance entanglement is pivotal for quantum communication, distributed quantum computing and sensing. Significant progresses have been made in extending the distribution distance of entangled photons, either in free space or fiber. For future quantum network applications, matter-based entanglement is more favorable since the capability of storage is essential for advanced applications. Extending entanglement distance for memory qubits was partially hindered by the mismatch of its photonic emission wavelength with the low-loss transmission window of optical fiber. By incorporating quantum frequency conversion, memory-memory entanglement has been successfully extended to several tens of kilometers. Here, we make a significant step further by reporting the entanglement between two atomic ensemble quantum memories over 420 km. We convert photons emitted from the memories to telecom S-band, which enable us to exploit the significantly low transmission loss in fiber (0.17 dB/km). We employ the DLCZ scheme for remote entanglement generation, and delicately stabilize the relative phase between the two memories by using fulltime far-off-resonant locking to reduce high-frequency noise and intermittent dual-band locking to compensate low-frequency drift jointly. We demonstrate that the memory-memory entangling probability beats the repeaterless channel capacity for direct entanglement distribution. Our experiment provides a testbed of studying quantum network applications from metropolitan scale to intercity scale.

quant-ph

An alkali-referenced vector spectrum analyzer for visible-light integrated photonics

Integrated photonics has reformed our information society by offering on-chip optical signal synthesis, processing and detection with reduced size, weight and power consumption. As such, it has been successfully established in the near-infrared (NIR) telecommunication bands. With the soaring demand in miniaturized systems for biosensing, quantum information and transportable atomic clocks, extensive endeavors have been stacked on translating integrated photonics into the visible spectrum, i.e. visible-light integrated photonics. Various innovative visible-light integrated devices have been demonstrated, such as lasers, frequency combs, and atom traps, highlighting the capacity and prospect to create chip-based optical atomic clocks that can make timing and frequency metrology ubiquitous. A pillar to the development of visible-light integrated photonics is characterization techniques featuring high frequency resolution and wide spectral coverage, which however remain elusive. Here, we demonstrate a vector spectrum analyzer (VSA) for visible-light integrated photonics, offering spectral bandwidth from 766 to 795 nm and frequency resolution of 415 kHz. The VSA is rooted on a widely chirping, high-power, narrow-linewidth, mode-hop-free laser around 780 nm, which is frequency-doubled from the near-infrared via an efficient, broadband CPLN waveguide. The VSA is further referenced to hyperfine structures of rubidium and potassium atoms, enabling 8.1 MHz frequency accuracy. We apply our VSA to showcase the characterization of loss, dispersion and phase response of passive integrated devices, as well as densely spaced spectra of mode-locked lasers. Combining operation in the NIR and visible spectra, our VSA allows characterization bandwidth exceeding an octave and can be an invaluable diagnostic tool for spectroscopy, nonlinear optical processing, imaging and quantum interfaces to atomic devices.

physics.optics

A multinode quantum network over a metropolitan area

Towards realizing the future quantum internet, a pivotal milestone entails the transition from two-node proof-of-principle experiments conducted in laboratories to comprehensive, multi-node setups on large scales. Here, we report on the debut implementation of a multi-node entanglement-based quantum network over a metropolitan area. We equipped three quantum nodes with atomic quantum memories and their telecom interfaces, and combined them into a scalable phase-stabilized architecture through a server node. We demonstrated heralded entanglement generation between two quantum nodes situated 12.5 km apart, and the storage of entanglement exceeding the round-trip communication time. We also showed the concurrent entanglement generation on three links. Our work provides a metropolitan-scale testbed for the evaluation and exploration of multi-node quantum network protocols and starts a new stage of quantum internet research.

quant-ph

Quantum frequency conversion and single-photon detection with lithium niobate nanophotonic chips

In the past few years, the lithium niobate on insulator (LNOI) platform has revolutionized lithium niobate materials, and a series of quantum photonic chips based on LNOI have shown unprecedented performances. Quantum frequency conversion (QFC) photonic chips, which enable quantum state preservation during frequency tuning, are crucial in quantum technology. In this work, we demonstrate a low-noise QFC process on an LNOI nanophotonic platform designed to connect telecom and near-visible bands with sum-frequency generation by long-wavelength pumping. An internal conversion efficiency of 73% and an on-chip noise count rate of 900 counts per second (cps) are achieved. Moreover, the on-chip preservation of quantum statistical properties is verified, showing that the QFC chip is promising for extensive applications of LNOI integrated circuits in quantum information. Based on the QFC chip, we construct an upconversion single-photon detector with the sum-frequency output spectrally filtered and detected by a silicon single-photon avalanche photodiode, demonstrating the feasibility of an upconversion single-photon detector on-chip with a detection efficiency of 8.7% and a noise count rate of 300 cps. The realization of a low-noise QFC device paves the way for practical chip-scale QFC-based quantum systems in heterogeneous configurations.

quant-ph

Entangling metropolitan-distance separated quantum memories

Quantum internet gives the promise of getting all quantum resources connected, and it will enable applications far beyond a localized scenario. A prototype is a network of quantum memories that are entangled and well separated. Previous realizations are limited in the distance. In this paper, we report the establishment of remote entanglement between two atomic quantum memories physically separated by 12.5 km directly in a metropolitan area. We create atom-photon entanglement in one node and send the photon to a second node for storage. We harness low-loss transmission through a field-deployed fiber of 20.5 km by making use of frequency down-conversion and up-conversion. The final memory-memory entanglement is verified to have a fidelity of 90% via retrieving to photons. Our experiment paves the way to study quantum network applications in a practical scenario.

quant-ph

Non-line-of-sight imaging with picosecond temporal resolution

Non-line-of-sight (NLOS) imaging enables monitoring around corners and is promising for diverse applications. The resolution of transient NLOS imaging is limited to a centimeter scale, mainly by the temporal resolution of the detectors. Here, we construct an up-conversion single-photon detector with a high temporal resolution of ~1.4 ps and a low noise count rate of 5 counts per second (cps). Notably, the detector operates at room temperature, near-infrared wavelength. Using this detector, we demonstrate high-resolution and low-noise NLOS imaging. Our system can provide a 180 μm axial resolution and a 2 mm lateral resolution, which is more than one order of magnitude better than that in previous experiments. These results open avenues for high-resolution NLOS imaging techniques in relevant applications.

physics.optics

Improved Spatial Resolution Achieved by Chromatic Intensity Interferometry

Interferometers are widely used in imaging technologies to achieve enhanced spatial resolution, but require that the incoming photons be indistinguishable. In previous work, we built and analyzed color erasure detectors which expand the scope of intensity interferometry to accommodate sources of different colors. Here we experimentally demonstrate how color erasure detectors can achieve improved spatial resolution in an imaging task, well beyond the diffraction limit. Utilizing two 10.9 mm-aperture telescopes and a 0.8 m baseline, we measure the distance between a 1063.6 nm source and a 1064.4 nm source separated by 4.2 mm at a distance of 1.43 km, which surpasses the diffraction limit of a single telescope by about 40 times. Moreover, chromatic intensity interferometry allows us to recover the phase of the Fourier transform of the imaged objects - a quantity that is, in the presence of modest noise, inaccessible to conventional intensity interferometry.

quant-ph

Entanglement of two quantum memories via fibers over dozens of kilometres

Quantum internet will enable a number of revolutionary applications. It relies on entanglement of remote quantum memories over long distances. Despite enormous progresses so far, the maximal physical separation achieved between two nodes is 1.3 km, and challenges for long distance remain. Here we make a significant step forward by entangling two atomic ensembles in one lab via photon transmission through metropolitan-scale fibers. We use cavity enhancement to create bright atom-photon entanglement, and harness quantum frequency conversion to shift the atomic wavelength to telecom. We realize entanglement over 22 km field-deployed fibers via two-photon interference, and entanglement over 50 km coiled fibers via single-photon interference. Our experiment can be extended to physically separated nodes with similar distance as a functional segment for atomic quantum networks, thus paving the way towards establishing atomic entanglement over many nodes and over much longer distance.

quant-ph

Two-photon comb with wavelength conversion and 20-km distribution for quantum communication

Quantum computing and quantum communication, have been greatly developed in recent years and expected to contribute to quantum internet technologies, including cloud quantum computing and unconditionally secure communication. However, long-distance quantum communication is challenging mainly because of optical fiber losses; quantum repeaters are indispensable for fiber-based transmission because unknown quantum states cannot be amplified with certainty. In this study, we demonstrate a versatile entanglement source in the telecom band for fiber-based quantum internet, which has a narrow linewidth of sub-MHz range, entanglement fidelity of more than 95%, and Bell-state generation even with frequency multimode. Furthermore, after a total distribution length of 20-km in fiber, two-photon correlation is observed with an easily identifiable normalized correlation coefficient, despite the limited bandwidth of the wavelength converter. The presented implementation promises an efficient method for entanglement distribution that is compatible with quantum memory and frequency-multiplexed long-distance quantum communication applications.

quant-ph

Chromatic interferometry with small frequency differences

By developing a `two-crystal' method for color erasure, we can broaden the scope of chromatic interferometry to include optical photons whose frequency difference falls outside of the 400 nm to 4500 nm wavelength range, which is the passband of a PPLN crystal. We demonstrate this possibility experimentally, by observing interference patterns between sources at 1064.4 nm and 1063.6 nm, corresponding to a frequency difference of about 200 GHz.

quant-ph