arXiv subjects

Yang-Yang Lv

Publications and source records attributed to Yang-Yang Lv.

11 recordsLinked to original sources

arXiv2020

Kinetics-Limited Two-Step Growth of van der Waals Puckered Honeycomb Sb Monolayer

Puckered honeycomb Sb monolayer, the structural analog of black phosphorene, has been recently successfully grown by means of molecular beam epitaxy. However, little is known to date about the growth mechanism for such puckered honeycomb monolayer. In this study, by using scanning tunneling microscopy in combination with first-principles density functional theory calculations, we unveil that the puckered honeycomb Sb monolayer takes a kinetics-limited two-step growth mode. As the coverage of Sb increases, the Sb atoms firstly form the distorted hexagonal lattice as the half layer, and then the distorted hexagonal half-layer transforms into the puckered honeycomb lattice as the full layer. These results provide the atomic-scale insight in understanding the growth mechanism of puckered honeycomb monolayer, and can be instructive to the direct growth of other monolayers with the same structure.

cond-mat.mtrl-sci↗

arXiv2020

Tuning the electronic structure of α-antimonene monolayer through interface engineering

The interfacial charge transfer from the substrate may influence the electronic structure of the epitaxial van der Waals (vdW) monolayers and thus their further technological applications. For instance, the freestanding Sb monolayer in puckered honeycomb phase (α-antimonene), the structural analog of black phosphorene, was predicted to be a semiconductor, but the epitaxial one behaves as a gapless semimetal when grown on the Td-WTe2 substrate. Here, we demonstrate that interface engineering can be applied to tune the interfacial charge transfer and thus the electron band of epitaxial monolayer. As a result, the nearly freestanding (semiconducting) α-antimonene monolayer with a band gap of ~170 meV was successfully obtained on the SnSe substrate. Furthermore, a semiconductor-semimetal crossover is observed in the bilayer α-antimonene. This study paves the way towards modifying the electron structure in two-dimensional vdW materials through interface engineering.

cond-mat.mtrl-sci↗

arXiv2019

Van der Waals heteroepitaxial growth of monolayer Sb in puckered honeycomb structure

Atomically thin two-dimensional (2D) crystals have gained tremendous attentions owing to their potential impacts to the future electronics technologies, as well as the exotic phenomena emerging in these materials. Monolayer of α phase Sb (α-antimonene) that shares the same puckered structure as black phosphorous, has been predicted to be stable with precious properties. However, the experimental realization still remains challenging. Here, we successfully grow high-quality monolayer α-antimonene, with the thickness finely controlled. The α-antimonene exhibits great stability upon exposure to air. Combining scanning tunneling microscope, density functional theory calculations and transport measurement, it is found that the electron band crossing the Fermi level exhibits a linear dispersion with a fairly small effective mass, and thus a good electrical conductivity. All of these properties make the α-antimonene promising in the future electronic applications.

cond-mat.mtrl-sci↗

arXiv2019

Turning ZrTe5 into semiconductor through atomic intercalation

In this work, we use the liquid ammonia method to successfully intercalate potassium atoms into ZrTe5 single crystal, and find a transition from semimetal to semiconductor at low temperature in the intercalated ZrTe5. The resistance anomalous peak is gradually suppressed and finally disappears with increasing potassium concentration. Whilst, the according sign reversal is always observed in the Hall resistance measurement. We tentatively attribute the semimetal-semiconductor transition to the lattice expansion induced by atomic intercalation and thereby a larger energy band gap.

cond-mat.mtrl-sci↗

arXiv2019

Superconductivity in Potassium-intercalated Td-WTe2

To realize topological superconductor is one of the most attracting topics because of its great potential in quantum computation. In this study, we successfully intercalate potassium (K) into the van der Waals gap of type II Weyl semimetal WTe2, and discover the superconducting state in KxWTe2 through both electrical transport and scanning tunneling spectroscopy measurements. The superconductivity exhibits an evident anisotropic behavior. Moreover, we also uncover the coexistence of superconductivity and the positive magneto-resistance state. Structural analysis substantiates the negligible lattice expansion induced by the intercalation, therefore suggesting K-intercalated WTe2 still hosts the topological nontrivial state. These results indicate that the K-intercalated WTe2 may be a promising candidate to explore the topological superconductor.

cond-mat.supr-con↗

arXiv2018

Experimental evidence of giant chiral magnetic effect in type-II Weyl semimetal WP$_{2+δ}$ crystals

Chiral magnetic effect is a quantum phenomenon that is breaking of chiral symmetry of relativistic Weyl fermions by quantum fluctuation under paralleled electric field E and magnetic field B. Intuitively, Weyl fermions with different chirality, under stimulus of paralleled E and B, will have different chemical potential that gives rise to an extra current, whose role likes a chiral battery in solids. However, up to now, the experimental evidence for chiral magnetic effect is the negative longitudinal magnetoresistance rather than a chiral electric source. Here, totally different from previous reports, we observed the giant chiral magnetic effect evidenced by: 'negative' resistivity and corresponding voltage-current curves lying the second-fourth quadrant in type-II Weyl semimetal WP$_{2+δ}$ under following conditions: the misaligned angle between E and B is smaller than 20$^\circ$, temperature <30 K and externally applied E<50 mA. Phenomenologically, based on macroscopic Chern-Simon-Maxwell equation, the giant chiral magnetic effect observed in WP$_{2+δ}$ is attributed to two-order higher coherent time of chiral Weyl-fermion quantum state over Drude transport relaxation-time. This work demonstrates the giant chiral-magnetic/chiral-battery effect in Weyl semimetals.

cond-mat.mtrl-sci↗

arXiv2018

Elliptical vortex and oblique vortex lattice in the FeSe superconductor based on the nematicity and mixed superconducting orders

The electronic nematic phase is characterized as an ordered state of matter with rotational symmetry breaking, and has been well studied in the quantum Hall system and the high-$T_c$ superconductors, regardless of cuprate or pnictide family. The nematic state in high-$T_c$ systems often relates to the structural transition or electronic instability in the normal phase. Nevertheless, the electronic states below the superconducting transition temperature is still an open question. With high-resolution scanning tunneling microscope measurements, direct observation of vortex core in FeSe thin films revealed the nematic superconducting state by Song \emph{et al}. Here, motivated by the experiment, we construct the extended Ginzburg-Landau free energy to describe the elliptical vortex, where a mixed \emph{s}-wave and \emph{d}-wave superconducting order is coupled to the nematic order. The nematic order induces the mixture of two superconducting orders and enhances the anisotropic interaction between the two superconducting orders, resulting in a symmetry breaking from $C_4$ to $C_2$. Consequently, the vortex cores are stretched into an elliptical shape. In the equilibrium state, the elliptical vortices assemble a lozenge-like vortex lattice, being well consistent with experimental results.

cond-mat.supr-con↗

arXiv2017

Nematic superconducting state in iron pnictide superconductors

Nematic order often breaks the tetragonal symmetry of iron-based superconductors. It arises from regular structural transition or electronic instability in the normal phase. Here, we report the observation of a nematic superconducting state, by measuring the angular dependence of the in-plane and out-of-plane magnetoresistivity of Ba0.5K0.5Fe2As2 single crystals. We find large twofold oscillations in the vicinity of the superconducting transition, when the direction of applied magnetic field is rotated within the basal plane. To avoid the influences from sample geometry or current flow direction, the sample was designed as Corbino-shape for in-plane and mesa-shape for out-of-plane measurements. Theoretical analysis shows that the nematic superconductivity arises from the weak mixture of the quasi-degenerate s-wave and d-wave components of the superconducting condensate, most probably induced by a weak anisotropy of stresses inherent to single crystals.

cond-mat.supr-con↗

arXiv2016

Experimental observation of anisotropic Adler-Bell-Jackiw anomaly in type-II Weyl semimetal WTe$_{1.98}$ crystals at the quasi-classical regime

The asymmetric electron dispersion in type-II Weyl semimetal theoretically hosts anisotropic transport properties. Here we observe the significant anisotropic Adler-Bell-Jackiw (ABJ) anomaly in the Fermi-level delicately adjusted WTe$_{1.98}$ crystals. Quantitatively, $C_w$ , a coefficient representing intensity of ABJ anomaly, along a- and b-axis of WTe$_{1.98}$ are 0.030 and 0.051 T$^{-2}$ at 2 K, respectively. We found that temperature-sensitive ABJ anomaly is attributed to topological phase transition from type-II Weyl semimetal to trivial semimetal, which is verified by first-principles calculation using experimentally determined lattice parameters at different temperatures. Theoretical electrical transport study reveals that observation of ansotropic ABJ both along a- and b-axis in WTe$_{1.98}$ is attributed to electrical transport in the quasi-classical regime. Our work may suggest that electron-doped WTe$_2$ is an ideal playground to explore the novel properties in type-II Weyl semimetals.

cond-mat.mtrl-sci↗

arXiv2016

Extremely large and significantly anisotropic magnetoresistance in ZrSiS single crystals

Recently, the extremely large magnetoresistance observed in transition metal telluride, like WTe$_2$, attracted much attention because of the potential applications in magnetic sensor. Here we report the observation of extremely large magnetoresistance as 3.0$\times$10$^4$ % measured at 2 K and 9 T magnetic field aligned along [001]-ZrSiS. The significant magnetoresistance change (~1.4$\times$10$^4$ %) can be obtained when the magnetic field is titled from [001] to [011]-ZrSiS. These abnormal magnetoresistance behaviors in ZrSiS can be understood by electron-hole compensation and the open orbital of Fermi surface. Because of these superior MR properties, ZrSiS may be used in the novel magnetic sensors.

cond-mat.mtrl-sci↗

arXiv2016

Robust topological edge states at the perfect surface step edge of topological insulator ZrTe$_5$

We report an atomic-scale characterization of ZrTe$_5$ by using scanning tunneling microscopy. We observe a bulk bandgap of ~80 meV with topological edge states at the step edge, and thus demonstrate ZrTe$_5$ is a two dimensional topological insulator. It is also found that an applied magnetic field induces energetic splitting and spatial separation of the topological edge states, which can be attributed to a strong link between the topological edge states and bulk topology. The perfect surface steps and relatively large bandgap make ZrTe$_5$ be a potential candidate for future fundamental studies and device applications.

cond-mat.mtrl-sci↗