Van der Waals Engineering of Ferromagnetic Semiconductor Heterostructures for Spin and Valleytronics

Ding Zhong; Kyle L. Seyler; Xiayu Linpeng; Ran Cheng; Nikhil Sivadas; Bevin Huang; Emma Schmidgall; Takashi Taniguchi; Kenji Watanabe; Michael A. McGuire; Wang Yao; Di Xiao; Kai-Mei C. Fu; Xiaodong Xu

doi:10.1126/sciadv.1603113

arXiv · 1704.00841

Van der Waals Engineering of Ferromagnetic Semiconductor Heterostructures for Spin and Valleytronics

Ding Zhong·Kyle L. Seyler·Xiayu Linpeng·Ran Cheng·Nikhil Sivadas·Bevin Huang·Emma Schmidgall·Takashi Taniguchi·Kenji Watanabe·Michael A. McGuire·Wang Yao·Di Xiao·Kai-Mei C. Fu·Xiaodong Xu

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Abstract

The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. Here we create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI3 and a monolayer of WSe2. We observe unprecedented control of the spin and valley pseudospin in WSe2, where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe2 valley splitting and polarization via flipping of the CrI3 magnetization. The WSe2 photoluminescence intensity strongly depends on the relative alignment between photo-excited spins in WSe2 and the CrI3 magnetization, due to ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure.

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Ding Zhong, Kyle L. Seyler, Xiayu Linpeng, Ran Cheng, Nikhil Sivadas, Bevin Huang, Emma Schmidgall, Takashi Taniguchi, Kenji Watanabe, Michael A. McGuire, Wang Yao, Di Xiao, Kai-Mei C. Fu, Xiaodong Xu. 2017-04-04. Van der Waals Engineering of Ferromagnetic Semiconductor Heterostructures for Spin and Valleytronics. https://doi.org/10.1126/sciadv.1603113

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