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arXiv · 2009.00136

A Chirality-Based Quantum Leap

Abstract

Chiral degrees of freedom occur in matter and in electromagnetic fields and constitute an area of research that is experiencing renewed interest driven by recent observations of the chiral-induced spin selectivity (CISS) effect in chiral molecules and engineered nanomaterials. The CISS effect underpins the fact that charge transport through nanoscopic chiral structures favors a particular electronic spin orientation, resulting in large room-temperature spin polarizations. Observations of the CISS effect suggest opportunities for spin control and for the design and fabrication of room-temperature quantum devices from the bottom up, with atomic-scale precision. Any technology that relies on optimal charge transport, including quantum devices for logic, sensing, and storage, may benefit from chiral quantum properties. These properties can be theoretically and experimentally investigated from a quantum information perspective, which is presently lacking. There are uncharted implications for the quantum sciences once chiral couplings can be engineered to control the storage, transduction, and manipulation of quantum information. This forward-looking perspective provides a survey of the experimental and theoretical fundamentals of chiral-influenced quantum effects, and presents a vision for their future roles in enabling room-temperature quantum technologies.

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Clarice D. Aiello, Muneer Abbas, John M. Abendroth, Andrei Afanasev, Shivang Agarwal, Amartya S. Banerjee, David N. Beratan, Jason N. Belling, Bertrand Berche, Antia Botana, Justin R. Caram, Giuseppe Luca Celardo, Gianaurelio Cuniberti, Aitzol Garcia-Etxarri, Arezoo Dianat, Ismael Diez-Perez, Yuqi Guo, Rafael Gutierrez, Carmen Herrmann, Joshua Hihath, Suneet Kale, Philip Kurian, Ying-Cheng Lai, Alexander Lopez, Ernesto Medina, Vladimiro Mujica, Ron Naaman, Mohammadreza Noormandipour, Julio L. Palma, Yossi Paltiel, William T. Petuskey, Joao Carlos Ribeiro-Silva, Juan Jose Saenz, Elton J. G. Santos, Maria Solyanik, Volker J. Sorger, Dominik M. Stemer, Jesus M. Ugalde, Ana Valdes-Curiel, Solmar Varela, David H. Waldeck, Paul S. Weiss, Helmut Zacharias, Qing Hua Wang. 2020-08-31. A Chirality-Based Quantum Leap. https://doi.org/10.1021/acsnano.1c01347

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