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arXiv · 2405.12811

Engineering band structures of two-dimensional materials with remote moire ferroelectricity

Jing Ding·Hanxiao Xiang·Wenqiang Zhou·Naitian Liu·Xinjie Fang·Kangyu Wang·Linfeng Wu·Kenji Watanabe·Takashi Taniguchi·Shuigang Xu
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Abstract

The stacking order and twist angle provide abundant opportunities for engineering band structures of two-dimensional materials, including the formation of moire bands, flat bands, and topologically nontrivial bands. The inversion symmetry breaking in rhombohedral-stacked transitional metal dichalcogenides (TMDCs) endows them with an interfacial ferroelectricity associated with an out-of-plane electric polarization. By utilizing twist angle as a knob to construct rhombohedral-stacked TMDCs, antiferroelectric domain networks with alternating out-of-plane polarization can be generated. Here, we demonstrate that such spatially periodic ferroelectric polarizations in parallel-stacked twisted WSe2 can imprint their moire potential onto a remote bilayer graphene. This remote moire potential gives rise to pronounced satellite resistance peaks besides the charge-neutrality point in graphene, which are tunable by the twist angle of WSe2. Our observations of ferroelectric hysteresis at finite displacement fields suggest the moire is delivered by a long-range electrostatic potential. The constructed superlattices by moire ferroelectricity represent a highly flexible approach, as they involve the separation of the moire construction layer from the electronic transport layer. This remote moire is identified as a weak potential and can coexist with conventional moire. Our results offer a comprehensive strategy for engineering band structures and properties of two-dimensional materials by utilizing moire ferroelectricity.

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Jing Ding, Hanxiao Xiang, Wenqiang Zhou, Naitian Liu, Xinjie Fang, Kangyu Wang, Linfeng Wu, Kenji Watanabe, Takashi Taniguchi, Shuigang Xu. 2024-05-21. Engineering band structures of two-dimensional materials with remote moire ferroelectricity. https://doi.org/10.1038/s41467-024-53440-w

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