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Structural, magnetic and transport properties in the Cu-doped manganites La0.85Te0.15Mn1-xCuxO3 (0 \leq x \leq 0.20)

J. Yang·W. H. Song·Y. Q. Ma·R. L. Zhang·B. C. Zhao·Z. G. Sheng·G. H. Zheng·J. M. Dai·Y. P. Sun
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Abstract

The effect of Cu-doping at Mn-site on structural, magnetic and transport properties in electron-doped manganites La0.85Te0.15Mn1-xCuxO3 has been investigated. Based on the analysis of structural parameter variations, the valence state of the Cu ion in Cu-doped manganites is suggested to be +2. All samples undergo the paramagnetic-ferromagnetic (PM-FM) phase transition. The Curie temperature decreases and the transition becomes broader with increasing Cu-doping level, in contrast, the magnetization magnitude of Cu-doping samples at low temperatures increase as x \leq 0.15. The insulator-metal (I-M) transition moves to lower temperatures with increasing Cu-doping content and disappears as x > 0.1. In addition, the higher temperature resistivity r peak in double-peak-like r(T) curves observed in no Cu-doping sample is completely suppressed as Cu-doping level x = 0.1 and r(T) curve only shows single I-M transition at the low temperature well below . The results are discussed according to the change of magnetic exchange interaction caused by Cu-doping.

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J. Yang, W. H. Song, Y. Q. Ma, R. L. Zhang, B. C. Zhao, Z. G. Sheng, G. H. Zheng, J. M. Dai, Y. P. Sun. 2004-09-20. Structural, magnetic and transport properties in the Cu-doped manganites La0.85Te0.15Mn1-xCuxO3 (0 \leq x \leq 0.20). https://doi.org/10.1103/physrevb.70.092504

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