arXiv subjects

Alessandro Tredicucci

Publications and source records attributed to Alessandro Tredicucci.

At least 19 recordsLinked to original sources

arXiv2025

Coherent absorption reveals colors hidden in a grey Fabry-P\'erot cavity

Thin dielectric films are known to show distinct colors, responsible for the iridescence of various natural and artificial objects such as insect wings and soap bubbles. In the present article we show that a specialized thin film Fabry-P\'erot resonator, that we name conductor-dielectric-conductor (CDC) matched cavity, appears instead completely grey when observed under ordinary conditions (i.e. by analyzing the transmitted or reflected incoherent white light). Nonetheless, the matched CDC cavity still retains spectral information, that clearly appear when the cavity is analyzed by the coherent absorption technique. The CDC system is simply a dielectric thin film sandwiched by two conducting interfaces, whose conductivity shall be appropriately matched depending upon the dielectric refractive index. In practical applications, the ideal conducting interfaces can be safely replaced by thin metal films, making the system easily applicable in particular for cryptographic purposes. We indeed demonstrated experimentally that a visually recognizable thin-film color pattern can be concealed to an ordinary observer, and finally recovered through a dedicated coherent absorption decoding apparatus.

physics.optics↗

arXiv2025

Bridging mid and near infrared by combining optomechanics and self mixing

This work describes a self-mixing-assisted optomechanical platform for transferring information between near- and mid-infrared radiation. In particular, the self-mixing signal of a mid-infrared quantum cascade laser is used to detect the oscillation of a membrane driven by light-induced forces exerted by a near-infrared excitation beam, which is amplitude-modulated at the membrane resonance frequency. This technique benefits from spectral broadness and, therefore, can link different spectral regions from both the excitation and probe sides. This versatility can pave the way for future applications of this self-mixing-assisted optomechanical platform in communication and advanced sensing systems.

physics.optics↗

arXiv2025

Direct Dark Matter searches with Metal Halide Perovskites

Polar materials with optical phonons in the meV range are excellent candidates for both dark matter direct detection (via dark photon-mediated scattering) and light dark matter absorption. In this study, we propose, for the first time, the metal halide perovskites MAPbI$_3$, MAPbCl$_3$, and CsPbI$_3$ for these purposes. Our findings reveal that CsPbI$_3$ is the best material, significantly improving exclusion limits compared to other polar materials. For scattering, CsPbI$_3$ can probe dark matter masses down to the keV range. For absorption, it enhances sensitivity to detect dark photon masses below $\sim 10~{\rm meV}$. The only material which has so far been investigated and that could provide competitive bounds is CsI, which, however, is challenging to grow in kilogram-scale sizes due to its considerably lower stability compared to CsPbI$_3$. Moreover, CsI is isotropic while the anisotropic structure of CsPbI$_3$ enables daily modulation analysis, showing that a significant percentage of daily modulation exceeding 1% is achievable for dark matter masses below $40~{\rm keV}$.

hep-ph↗

arXiv2024

Tailoring coherent charge transport in graphene by deterministic defect generation

Harnessing the wave-nature of charge carriers in solid state devices, electron optics investigates and exploits coherent phenomena, in analogy with optics and photonics. Typically, this requires complex electronic devices leveraging macroscopically coherent charge transport in two-dimensional electron gases and superconductors. Here, collective coherent effects are induced in a simple counterintuitive architecture by defect engineering. Deterministically introduced lattice defects in graphene enable the phase coherent charge transport by playing the role of potential barriers, instead of scattering centres as conventionally considered. Thus, graphene preserves its quasi-ballistic quantum transport and can support phase-matched charge carrier waves. Based on this approach, multiple electronic Fabry-Pèrot cavities are formed by creating periodically alternating defective and pristine nano-stripes through low energy electron-beam irradiation. Indeed, defective stripes behave as partially reflecting mirrors and resonantly confine the charge carrier waves within the pristine areas, giving rise to Fabry-Pèrot resonant modes. These modes experimentally manifest as sheet resistance oscillations, as also confirmed by Landauer-Büttiker simulations. Moreover, these coherent phenomena survive up to 30 K for both polarities of charge carriers, contrarily to traditional monopolar electrostatically created Fabry-Pèrot interferometers. Our study positions defective graphene as an innovative platform for coherent electronic devices, with potential applications in nano and quantum technologies.

cond-mat.mes-hall↗

arXiv2024

Yellow diode-pumped lasing of femtosecond-laser-written Dy,Tb:LiLuF4 waveguide

In this article we report the fabrication of a diode-pumped Dy,Tb:LiLuF4 waveguide laser operating in the yellow region of the visible spectrum. The circular depressed-cladding waveguides have been fabricated by direct femtosecond laser writing, and showed propagation losses as low as 0.07 dB/cm. By employing these structures, we obtain a maximum output power of 86 mW at 574 nm from a 60 {\mu}m diameter waveguide, and a highest slope efficiency of 19% from a 80 {\mu}m diameter depressed cladding waveguide. In addition, we demonstrate lasing at 574 nm from a half-ring surface waveguide, with a maximum output power of 12 mW. Moreover, we also obtained dual wavelength operation at 568-574 nm, with a maximum output power of 15 mW, and stable lasing at 578 nm, with an output power of 100 mW. The latter wavelength corresponds to the main transition of the atomic clock based on the neutral ytterbium atom. To the best of the authors' knowledge, this is the first demonstration of a yellow waveguide laser based on Dy-doped materials.

physics.optics↗

arXiv2023

Gigahertz modulation of a fully dielectric nonlocal metasurface

Nonlocal metasurfaces are currently emerging as advanced tools for the manipulation of electromagnetic radiation, going beyond the widely explored Huygens metasurface concept. Nonetheless, the lack of an unified approach for their fast and efficient tunability still represents a serious challenge to overcome. In this article we report on gigahertz modulation of a dielectric slab-based, nonlocal (i.e. angle-dispersive) metasurface, whose operation relies on the optomechanical coupling with a mechanical wave excited piezoelectrically by a transducer integrated on the same chip. Importantly, the metasurface region is free from any conductive material, thus eliminating optical losses, and making our device of potential interest for delicate environments such as high-power apparatuses or quantum optical systems.

physics.optics↗

arXiv2023

Operability timescale of defect-engineered graphene

Defects in the lattice are of primal importance to tune graphene chemical, thermal and electronic properties. Electron-beam irradiation is an easy method to induce defects in graphene following pre-designed patterns, but no systematic study of the time evolution of the resulting defects is available. In this paper, the change over time of defected sites created in graphene with low-energy ($\leq 20$ keV) electron irradiation is studied both experimentally via micro-Raman spectroscopy for a period of $6\times 10^3$ hours and through molecular dynamics simulations. During the first 10 h, the structural defects are stable at the highest density value. Subsequently, the crystal partially reconstructs, eventually reaching a stable, less defected condition after more than one month. The simulations allow the rationalization of the processes at the atomic level and confirm that the irradiation induces composite clusters of defects of different nature rather than well-defined nanoholes as in the case of high-energy electrons. The presented results identify the timescale of the defects stability, thus establishing the operability timespan of engineerable defect-rich graphene devices with applications in nanoelectronics. Moreover, long-lasting chemical reactivity of the defective graphene is pointed out. This property can be exploited to functionalize graphene for sensing and energy storage applications.

cond-mat.mtrl-sci↗

arXiv2023

Optical grade bromide-based thin film electrolytes

Controlling the charge density in low-dimensional materials with an electrostatic potential is a powerful tool to explore and influence their electronic and optical properties. Conventional solid gates impose strict geometrical constraints to the devices and often absorb electromagnetic radiation in the infrared (IR) region. A powerful alternative is ionic liquid (IL) gating. This technique only needs a metallic electrode in contact with the IL and the highest achievable electric field is limited by the electrochemical interactions of the IL with the environment. Despite the excellent gating properties, a large number of ILs is hardly exploitable for optical experiments in the mid-IR region, because they typically suffer from low optical transparency and degradation in ambient conditions. Here, we report the realization of two electrolytes based on bromide ILs dissolved in polymethyl methacrylate (PMMA). We demonstrate that such electrolytes can induce state-of-the-art charge densities as high as $20\times10^{15}\ \mathrm{cm^{-2}}$. Thanks to the low water absorption of PMMA, they work both in vacuum and in ambient atmosphere after a simple vacuum curing. Furthermore, our electrolytes can be spin coated into flat thin films with optical transparency in the range from 600 cm$^{-1}$ to 4000 cm$^{-1}$. Thanks to these properties, the electrolytes are excellent candidates to fill the gap as versatile gating layers for electronic and mid-IR optoelectronic devices.

cond-mat.mes-hall↗

arXiv2023

Magnetic-field-induced cavity protection for intersubband polaritons

We analyse the effect of a strong perpendicular magnetic field on an intersubband transition in a disordered doped quantum well strongly coupled to an optical cavity. The magnetic field changes the lineshape of the intersubband optical transition due to the interface roughness of the quantum well from a Lorentzian to a Gaussian one. In this regime, a novel form of magnetic-field-induced cavity protection sets in, which strongly reduces the polariton linewidth to the cavity contribution only. Implications of our results for fundamental studies of nonlinear polariton dynamics and for technological applications to polariton lasers are finally highlighted.

cond-mat.mes-hall↗

arXiv2022

Strain-engineered wrinkles on graphene using polymeric actuators

The electronic and optical properties of graphene can be precisely tuned by generating deterministic arrangements of strain features. In this paper, we report the formation of widespread and controlled buckling delamination of monolayer graphene deposited on hexagonal boron-nitride promoted by a significant squeezing of the graphene flake and induced by polymeric micro-actuators. The flexibility of this method offers a promising technique to create arbitrary buckling geometries and arrays of wrinkles which could also be subjected to iterative folding-unfolding cycles. Further development of this method could pave the way to tune the properties of several kinds of other two-dimensional materials, such as transition metal dichalcogenides, by tailoring their surface topography.

cond-mat.mtrl-sci↗

arXiv2022

Cryptographic Strain-Dependent Light Pattern Generators

Refractive freeform components are becoming increasingly relevant for generating controlled patterns of light, because of their capability to spatially-modulate optical signals with high efficiency and low background. However, the use of these devices is still limited by difficulties in manufacturing macroscopic elements with complex, 3-dimensional (3D) surface reliefs. Here, 3D-printed and stretchable magic windows generating light patterns by refraction are introduced. The shape and, consequently, the light texture achieved can be changed through controlled device strain. Cryptographic magic windows are demonstrated through exemplary light patterns, including micro-QR-codes, that are correctly projected and recognized upon strain gating while remaining cryptic for as-produced devices. The light pattern of micro-QR-codes can also be projected by two coupled magic windows, with one of them acting as the decryption key. Such novel, freeform elements with 3D shape and tailored functionalities is relevant for applications in illumination design, smart labels, anti-counterfeiting systems, and cryptographic communication.

physics.optics↗

arXiv2022

Materials and devices for fundamental quantum science and quantum technologies

Technologies operating on the basis of quantum mechanical laws and resources such as phase coherence and entanglement are expected to revolutionize our future. Quantum technologies are often divided into four main pillars: computing, simulation, communication, and sensing & metrology. Moreover, a great deal of interest is currently also nucleating around energy-related quantum technologies. In this Perspective, we focus on advanced superconducting materials, van der Waals materials, and moiré quantum matter, summarizing recent exciting developments and highlighting a wealth of potential applications, ranging from high-energy experimental and theoretical physics to quantum materials science and energy storage.

quant-ph↗

arXiv2022

Unexpected Electron Transport Suppression in a Heterostructures Graphene MoS2 Multiple Field-Effect Transistor Architecture

We demonstrate a graphene-MoS2 architecture integrating multiple field-effect transistors and we independently probe and correlate the conducting properties of van der Waals coupled graphene-MoS2 contacts with the ones of the MoS2 channels. Devices are fabricated starting from high-quality single-crystal monolayers grown by chemical vapor deposition and characterized by scanning Raman and photoluminescence spectroscopies. Transconductance curves of MoS2 are compared with the current-voltage characteristics of graphene contact stripes, revealing a significant suppression of transport on the n-side of the transconductance curve. Based on ab-initio modeling, the effect is understood in terms of trapping by sulfur vacancies, which counter-intuitively depends on the field-effect, even though the graphene contact layer is positioned between the backgate and the MoS2 channel.

cond-mat.mes-hall↗

arXiv2021

Micromechanical bolometers for sub-Terahertz detection at room temperature

Fast, room temperature imaging at THz and sub-THz frequencies is an interesting feature which could unleash the full potential of plenty applications in security, healthcare and industrial production. In this Letter we introduce micromechanical bolometers based on silicon nitride trampoline membranes as broad-range detectors, down to the sub-THz frequencies. They show, at the largest wavelengths, room-temperature noise-equivalent-powers comparable to state-of-the-art commercial devices (~100 pW Hz-1/2); adding the good operation speed and the easy, large-scale fabrication process, the trampoline membrane could be the next candidate for cheap, room temperature THz imaging and related applications.

physics.ins-det↗

arXiv2021

Electron localization in periodically strained graphene

Pseudo-magnetic field (PMF) in deformed graphene has been proposed as a promising and flexible method to quantum-confine electronic states and create gaps in the local density of states. Motivated by this perspective, we numerically analyze various different configurations leading to electronic localization and band flattening in periodically strained graphene. In particular, we highlight the existence of a fine structure in the pseudo-Landau levels confined in large-PMF regions, the emergence of states confined to PMF nodes as well as of snake-like orbits. In our paper, we further analyze the importance of the relative rotation and asymmetry of the strain lattice with respect to the atomic lattice and show how it can be used to modulate the PMF periodicity and to create localized orbits far from the strain points. Possible implementations and applications of the simulated structures are discussed.

cond-mat.mes-hall↗

arXiv2020

Stress-strain in electron-beam activated polymeric micro-actuators

Actuation of thin polymeric films via electron irradiation is a promising avenue to realize devices based on strain engineered two dimensional (2D) materials. Complex strain profiles demand a deep understanding of the mechanics of the polymeric layer under electron irradiation; in this article we report a detailed investigation on electron-induced stress on poly-methyl-methacrylate (PMMA) thin film material. After an assessment of stress values using a method based on dielectric cantilevers, we directly investigate the lateral shrinkage of PMMA patterns on epitaxial graphene, which reveals a universal behavior, independent of the electron acceleration energy. By knowing the stress-strain curve, we finally estimate an effective Young's modulus of PMMA on top of graphene which is a relevant parameter for PMMA based electron-beam lithography and strain engineering applications.

cond-mat.mes-hall↗

arXiv2019

Local tuning of WS2 photoluminescence using polymeric micro-actuators in a monolithic van der Waals heterostructure

The control of the local strain profile in 2D materials offers an invaluable tool for tailoring the electronic and photonic properties of solid-state devices. In this paper, we demonstrate a local engineering of the exciton photoluminescence (PL) energy of monolayer tungsten disulfide (WS2) by means of strain. We apply a local uniaxial stress to WS2 by exploiting electron-beam patterned and actuated polymeric micrometric artificial muscles (MAMs), which we implement onto monolithic synthetic WS2/graphene heterostructures. We show that MAMs are able to induce an in-plane stress to the top WS2 layer of the van der Waals heterostructure and that the latter can slide on the graphene underneath with negligible friction. As a proof of concept for the local strain-induced PL shift experiments, we exploit a two-MAM configuration in order to apply uniaxial tensile stress on well-defined micrometric regions of WS2. Remarkably, our architecture does not require the adoption of fragile suspended microstructures. We observe a spatial modulation of the excitonic PL energy of the WS2 monolayers under stress, which agrees with the expected strain profile and attains a maximum redshift of about 40 meV at the maximum strain intensity point. After the actuation, a time-dependent PL blueshift is observed in agreement with the viscoelastic properties of the polymeric MAMs. Our approach enables inducing local and arbitrary deformation profiles and circumvents some key limitations and technical challenges of alternative strain engineering methods requiring the 2D material transfer and production of suspended membranes.

cond-mat.mes-hall↗

arXiv2019

Photonic bands, superchirality, and inverse design of a chiral minimal metasurface

Photonic band structures are a typical fingerprint of periodic optical structures, and are usually observed in spectroscopic quantities such as transmission, reflection and absorption. Here we show that also the chiro-optical response of a metasurface constituted by a lattice of non-centrosymmetric, L-shaped holes in a dielectric slab shows a band structure, where intrinsic and extrinsic chirality effects are clearly recognized and connected to localized and delocalized resonances. Superchiral near-fields can be excited in correspondence to these resonances, and anomalous behaviors as a function of the incidence polarization occur. Moreover, we introduce a singular value decomposition (SVD) approach to show that the above mentioned effects are connected to specific fingerprints of the SVD spectra. Finally, we demonstrate by means of an inverse design technique that the metasurface based on an L-shaped hole array is a minimal one. Indeed, its unit cell geometry depends on the smallest number of parameters needed to implement arbitrary transmission matrices compliant with the general symmetries for 2d-chiral structures. These observations enable more powerful wave operations in a lossless photonic environment.

physics.optics↗