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Alessandro Tredicucci

Publications and source records attributed to Alessandro Tredicucci.

At least 37 records · Page 2Linked to original sources

Optomechanical response with nanometer resolution in the self-mixing signal of a terahertz quantum cascade laser

The effectiveness of self-mixing interferometry has been demonstrated across the electromagnetic spectrum, from visible to microwave frequencies, in a plethora of sensing applications, ranging from distance measurement to material analysis, microscopy and coherent imaging. Owing to their intrinsic stability to optical feedback, quantum cascade lasers (QCLs) represent a source that offers unique and versatile characteristics to further improve the self-mixing functionality at mid infrared and terahertz (THz) frequencies. Here, we show the feasibility of detecting with nanometer precision deeply subwalength (< λ/6000) mechanical vibrations of a suspended Si3N4-membrane used as the external element of a THz QCL feedback interferometric apparatus. Besides representing a platform for the characterization of small displacements, our self-mixing configuration can be exploited for the realization of optomechanical systems, where several laser sources can be linked together through a common mechanical microresonator actuated by radiation pressure.

physics.optics↗

Optomechanics of chiral dielectric metasurfaces

Electromagnetic fields coupled with mechanical degrees of freedom have recently shown exceptional and innovative applications, ultimately leading to mesoscopic optomechanical devices operating in the quantum regime of motion. Simultaneously, micromechanical elements have provided new ways to enhance and manipulate the optical properties of passive photonic elements. Following this concept, in this article we show how combining a chiral metasurface with a GaAs suspended micromembrane can offer new scenarios for controlling the polarization state of near-infrared light beams. Starting from the uncommon properties of chiral metasurface to statically realize target polarization states and circular and linear dichroism, we report mechanically induced, ~300 kHz polarization modulation, which favorably compares, in terms of speed, with liquid-crystals commercial devices. Moreover, we demonstrate how the mechanical resonance can be non-trivially affected by the input light polarization (and chiral state) via a thermoelastic effect triggered by intracavity photons. This work inaugurates the field of Polarization Optomechanics, which could pave the way to fast polarimetric devices, polarization modulators and dynamically tunable chiral state generators and detectors, as well as giving access to new form of polarization nonlinearities and control.

physics.optics↗

Gate-tunable spatial modulation of localized plasmon resonances

Nanoplasmonics exploits the coupling between light and collective electron density oscillations (plasmons) to bypass the stringent limits imposed by diffraction. This coupling enables confinement of light to sub-wavelength volumes and is usually exploited in nanostructured metals. Substantial efforts are being made at the current frontier of the field to employ electron systems in semiconducting and semimetallic materials since these add the exciting possibility of realizing electrically tunable and/or active nanoplasmonic devices. Here we demonstrate that a suitable design of the doping profile in a semiconductor nanowire (NW) can be used to tailor the plasmonic response and induce localization effects akin to those observed in metal nanoparticles. Moreover, by field-effect carrier modulation, we demonstrate that these localized plasmon resonances can be spatially displaced along the nanostructure body, thereby paving the way for the implementation of spatially tunable plasmonic circuits.

cond-mat.mes-hall↗

Black-Phosphorus Terahertz Photodetectors

The discovery of graphene and the related fascinating capabilities have triggered an unprecedented interest in inorganic two-dimensional (2D) materials. Despite the impressive impact in a variety of photonic applications, the absence of energy gap has hampered its broader applicability in many optoelectronic devices. The recent advance of novel 2D materials, such as transition-metal dichalcogenides or atomically thin elemental materials, (e.g. silicene, germanene and phosphorene) promises a revolutionary step-change. Here we devise the first room-temperature Terahertz (THz) frequency detector exploiting few-layer phosphorene, e.g., a 10 nm thick flake of exfoliated crystalline black phosphorus (BP), as active channel of a field-effect transistor (FET). By exploiting the direct band gap of BP to fully switch between insulating and conducting states and by engineering proper antennas for efficient light harvesting, we reach detection performance comparable with commercial detection technologies, providing the first technological demonstration of a phosphorus-based active THz device.

cond-mat.other↗

Stretching graphene using polymeric micro-muscles

The control of strain in two-dimensional materials opens exciting perspectives for the engineering of their electronic properties. While this expectation has been validated by artificial-lattice studies, it remains elusive in the case of atomic lattices. Remarkable results were obtained on nanobubbles and nano-wrinkles, or using scanning probes; microscale strain devices were implemented exploiting deformable substrates or external loads. These devices lack, however, the flexibility required to fully control and investigate arbitrary strain profiles. Here, we demonstrate a novel approach making it possible to induce strain in graphene using polymeric micrometric artificial muscles (MAMs) that contract in a controllable and reversible way under an electronic stimulus. Our method exploits the mechanical response of poly-methyl-methacrylate (PMMA) to electron-beam irradiation. Inhomogeneous anisotropic strain and out-of-plane deformation are demonstrated and studied by Raman, scanning-electron and atomic-force microscopy. These can all be easily combined with the present device architecture. The flexibility of the present method opens new opportunities for the investigation of strain and nanomechanics in two-dimensional materials.

cond-mat.mes-hall↗

Defect Line Terahertz Quantum Cascade Laser

We present terahertz quantum cascade lasers operating at a defect mode of a photonic crystal bandgap. This class of devices exhibits single mode emission and low threshold current compared to standard metal-metal lasers. The mode selectivity is an intrinsic property of the chosen fabrication design. The lower lasing threshold effect, already reported in photonic crystal quantum cascade lasers, is further enhanced in the ultra-flat-dispersion defect line. The presented results pave the way for integrated circuitry operating in the terahertz regime and have important applications in the field of quantum cascade lasers, spectroscopy and microcavity lasers.

physics.optics↗

Anisotropic straining of graphene using micropatterned SiN membranes

We use micro-Raman spectroscopy to study strain profiles in graphene monolayers suspended over SiN membranes micropatterned with holes of non-circular geometry. We show that a uniform differential pressure load $ΔP$ over elliptical regions of free-standing graphene yields measurable deviations from hydrostatic strain conventionally observed in radially-symmetric microbubbles. The top hydrostatic strain $\bar{\varepsilon}$ we observe is estimated to be $\approx0.7\%$ for $ΔP = 1\,{\rm bar}$ in graphene clamped to elliptical SiN holes with axis $40$ and $20\,{\rm μm}$. In the same configuration, we report a $G_\pm$ splitting of $10\,{\rm cm^{-1}}$ which is in good agreement with the calculated anisotropy $Δ\varepsilon \approx 0.6\%$ for our device geometry. Our results are consistent with the most recent reports on the Grüneisen parameters. Perspectives for the achievement of arbitrary strain configurations by designing suitable SiN holes and boundary clamping conditions are discussed.

cond-mat.mtrl-sci↗

Mid-Infrared intersubband polaritons in dispersive metal-insulator-metal resonators

We demonstrate room-temperature strong-coupling between a mid-infrared ($λ$=9.9 $μ$m) intersubband transition and the fundamental cavity mode of a metal-insulator-metal resonator. Patterning of the resonator surface enables surface-coupling of the radiation and introduces an energy dispersion which can be probed with angle-resolved reflectivity. In particular, the polaritonic dispersion presents an accessible energy minimum at k=0 where - potentially - polaritons can accumulate. We also show that it is possible to maximize the coupling of photons into the polaritonic states and - simultaneously - to engineer the position of the minimum Rabi splitting at a desired value of the in-plane wavevector. This can be precisely accomplished via a simple post-processing technique. The results are confirmed using the temporal coupled mode theory formalism and their significance in the context of the concept of strong critical coupling is highlighted.

cond-mat.mes-hall↗

Coherent perfect absorption in photonic structures

The ability to drive a system with an external input is a fundamental aspect of light-matter interaction. The coherent perfect absorption (CPA) phenomenon extends to the general multibeam interference phenomenology the well known critical coupling concepts. This interferometric control of absorption can be employed to reach full delivery of optical energy to nanoscale systems such as plasmonic nanoparticles, and multi-port interference can be used to enhance the absorption of a nanoscale device when it is embedded in a strongly scattering system, with potential applications to nanoscale sensing. Here we review the two-port CPA in reference to photonic structures which can resonantly couple to the external fields. A revised two-port theory of CPA is illustrated, which relies on the Scattering Matrix formalism and is valid for all linear two-port systems with reciprocity. Through a semiclassical approach, treating two-port critical coupling conditions in a non-perturbative regime, it is demonstrated that the strong coupling regime and the critical coupling condition can indeed coexist; in this situation, termed strong critical coupling, all the incoming energy is converted into polaritons. Experimental results are presented, which clearly display the elliptical trace of absorption as function of input unbalance in a thin metallo-dielectric metamaterial, and verify polaritonic CPA in an intersubband-polariton photonic-crystal membrane resonator. Concluding remarks discuss the future perspectives of CPA with photonic structures.

physics.optics↗

Photonic bands and defect modes in metallo-dielectric photonic crystal slabs

Photonic components based on structured metallic elements show great potential for device applications where field enhancement and confinement of the radiation on a subwavelength scale is required. In this paper we report a detailed study of a prototypical metallo-dielectric photonic structure, where features well known in the world of dielectric photonic crystals, like band gaps and defect modes, are exported to the metallic counterpart, with interesting applications to infrared science and technology, as for instance in quantum well infrared photodetectors, narrow-band spectral filters, and tailorable thermal emitters.

physics.optics↗

Perfect energy-feeding into strongly coupled systems and interferometric control of polariton absorption

The ability to feed energy into a system, or - equivalently - to drive that system with an external input is a fundamental aspect of light-matter interaction. The key concept in many photonic applications is the "critical coupling" condition: at criticality, all the energy fed to the system via an input channel is dissipated within the system itself. Although this idea was crucial to enhance the efficiency of many devices, it was never considered in the context of systems operating in a non-perturbative regime. In this so-called strong coupling regime, the matter and light degrees of freedom are in fact mixed into dressed states, leading to new eigenstates called polaritons. Here we demonstrate that the strong coupling regime and the critical coupling condition can indeed coexist; in this situation, which we term strong critical coupling, all the incoming energy is converted into polaritons. A semiclassical theory - equivalently applicable to acoustics or mechanics - reveals that the strong critical coupling corresponds to a special curve in the phase diagram of the coupled light-matter oscillators. In the more general case of a system radiating via two scattering ports, the phenomenology displayed is that of coherent perfect absorption (CPA), which is then naturally understood and described in the framework of critical coupling. Most importantly, we experimentally verify polaritonic CPA in a semiconductor-based intersubband-polariton photonic-crystal membrane resonator. This result opens new avenues in the exploration of polariton physics, making it possible to control the pumping efficiency of a system almost independently of its Rabi energy, i.e., of the energy exchange rate between the electromagnetic field and the material transition.

quant-ph↗

Saturation and bistability of defect-mode intersubband polaritons

In this article we report about linear and nonlinear optical properties of intersubband cavity polariton samples, where the resonant photonic mode is a defect state in a metallo-dielectric photonic crystal slab. By tuning a single geometric parameter of the resonator, the cavity Q-factor can reach values as large as 85, with a consequent large cooperativity for the light-matter interaction. We show that a device featuring large cooperativity leads to sharp saturation, or even bistability, of the polariton states. This nonlinear dynamics occurs at the crossover between the weak and the strong coupling regimes, where the weak critical coupling concept plays a fundamental role.

cond-mat.mes-hall↗

Thermal noise and optomechanical features in the emission of a membrane-coupled compound cavity laser diode

We demonstrate the use of a compound optical cavity as linear displacement detector, by measuring the thermal motion of a silicon nitride suspended membrane acting as the external mirror of a near-infrared Littrow laser diode. Fluctuations in the laser optical power induced by the membrane vibrations are collected by a photodiode integrated within the laser, and then measured with a spectrum analyzer. The dynamics of the membrane driven by a piezoelectric actuator is investigated as a function of air pressure and actuator displacement in a homodyne configuration. The high Q-factor ($\sim 3.4\cdot 10^4$ at $8.3 \cdot 10^{-3}$ mbar) of the fundamental mechanical mode at $\sim 73$ kHz guarantees a detection sensitivity high enough for direct measurement of thermal motion at room temperature ($\sim 87$ pm RMS). The compound cavity system here introduced can be employed as a table-top, cost-effective linear displacement detector for cavity optomechanics. Furthermore, thanks to the strong optical nonlinearities of the laser compound cavity, these systems open new perspectives in the study of non-Markovian quantum properties at the mesoscale.

cond-mat.mes-hall↗

Universal lineshapes at the crossover between weak and strong critical coupling in Fano-resonant coupled oscillators

In this article we discuss a model describing key features concerning the lineshapes and the coherent absorption conditions in Fano-resonant dissipative coupled oscillators. The model treats on the same footing the weak and strong coupling regimes, and includes the critical coupling concept, which is of great relevance in numerous applications; in addition, the role of asymmetry is thoroughly analyzed. Due to the wide generality of the model, which can be adapted to various frameworks like nanophotonics, plasmonics, and optomechanics, we envisage that the analytical formulas presented here will be crucial to effectively design devices and to interpret experimental results.

physics.optics↗

Vertical coupling of laser glass microspheres to buried silicon nitride ellipses and waveguides

We demonstrate the integration of Nd3+ doped Barium-Titanium-Silicate microsphere lasers with a Silicon Nitride photonic platform. Devices with two different geometrical configurations for extracting the laser light to buried waveguides have been fabricated and characterized. The first configuration relies on a standard coupling scheme, where the microspheres are placed over strip waveguides. The second is based on a buried elliptical geometry whose working principle is that of an elliptical mirror. In the latter case, the input of a strip waveguide is placed on one focus of the ellipse, while a lasing microsphere is placed on top of the other focus. The fabricated elliptical geometry (ellipticity=0.9) presents a light collecting capacity that is 50% greater than that of the standard waveguide coupling configuration and could be further improved by increasing the ellipticity. Moreover, since the dimensions of the spheres are much smaller than those of the ellipses, surface planarization is not required. On the contrary, we show that the absence of a planarization step strongly damages the microsphere lasing performance in the standard configuration.

physics.optics↗

Linear and nonlinear capacitive coupling of electro-opto-mechanical photonic crystal cavities

We fabricate and characterize a microscale silicon electro-opto-mechanical system whose mechanical motion is coupled capacitively to an electrical circuit and optically via radiation pressure to a photonic crystal cavity. To achieve large electromechanical interaction strength, we implement an inverse shadow mask fabrication scheme which obtains capacitor gaps as small as 30 nm while maintaining a silicon surface quality necessary for minimizing optical loss. Using the sensitive optical read-out of the photonic crystal cavity, we characterize the linear and nonlinear capacitive coupling to the fundamental 63 MHz in-plane flexural motion of the structure, showing that the large electromechanical coupling in such devices may be suitable for realizing efficient microwave-to-optical signal conversion.

physics.optics↗

High performance bilayer-graphene Terahertz detectors

We report bilayer-graphene field effect transistors operating as THz broadband photodetectors based on plasma-waves excitation. By employing wide-gate geometries or buried gate configurations, we achieve a responsivity $\sim 1.2V/W (1.3 mA/W)$ and a noise equivalent power $\sim 2\times 10^{-9} W/Hz^{-1/2}$ in the 0.29-0.38 THz range, in photovoltage and photocurrent mode. The potential of this technology for scalability to higher frequencies and the development of flexible devices makes our approach competitive for a future generation of THz detection systems.

cond-mat.mes-hall↗

Photocurrent-based detection of Terahertz radiation in graphene

Graphene is a promising candidate for the development of detectors of Terahertz (THz) radiation. A well-known detection scheme due to Dyakonov and Shur exploits the confinement of plasma waves in a field-effect transistor (FET), whereby a dc photovoltage is generated in response to a THz field. This scheme has already been experimentally studied in a graphene FET [L. Vicarelli et al., Nature Mat. 11, 865 (2012)]. In the quest for devices with a better signal-to-noise ratio, we theoretically investigate a plasma-wave photodetector in which a dc photocurrent is generated in a graphene FET. The rectified current features a peculiar change of sign when the frequency of the incoming radiation matches an even multiple of the fundamental frequency of plasma waves in the FET channel. The noise equivalent power per unit bandwidth of our device is shown to be much smaller than that of a Dyakonov-Shur detector in a wide spectral range.

cond-mat.mes-hall↗