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B. J. van Wees

Publications and source records attributed to B. J. van Wees.

At least 55 records · Page 3Linked to original sources

Temperature dependent transport characteristics of graphene/n-Si diodes

Realizing an optimal Schottky interface of graphene on Si is challenging, as the electrical transport strongly depends on the graphene quality and the fabrication processes. Such interfaces are of increasing research interest for integration in diverse electronic devices as they are thermally and chemically stable in all environments, unlike standard metal/semiconductor interfaces. We fabricate such interfaces with n-type Si at ambient conditions and find their electrical characteristics to be highly rectifying, with minimal reverse leakage current ($<$10$^{-10}$ A) and rectification of more than $10^6$. We extract Schottky barrier height of 0.69 eV for the exfoliated graphene and 0.83 eV for the CVD graphene devices at room temperature. The temperature dependent electrical characteristics suggest the influence of inhomogeneities at the graphene/n-Si interface. A quantitative analysis of the inhomogeneity in Schottky barrier heights is presented using the potential fluctuation model proposed by Werner and Güttler.

cond-mat.mes-hall↗

Spin transport in graphene nanostructures

Graphene is an interesting material for spintronics, showing long spin relaxation lengths even at room temperature. For future spintronic devices it is important to understand the behavior of the spins and the limitations for spin transport in structures where the dimensions are smaller than the spin relaxation length. However, the study of spin injection and transport in graphene nanostructures is highly unexplored. Here we study the spin injection and relaxation in nanostructured graphene with dimensions smaller than the spin relaxation length. For graphene nanoislands, where the edge length to area ratio is much higher than for standard devices, we show that enhanced spin-flip processes at the edges do not seem to play a major role in the spin relaxation. On the other hand, contact induced spin relaxation has a much more dramatic effect for these low dimensional structures. By studying the nonlocal spin transport through a graphene quantum dot we observe that the obtained values for spin relaxation are dominated by the connecting graphene islands and not by the quantum dot itself. Using a simple model we argue that future nonlocal Hanle precession measurements can obtain a more significant value for the spin relaxation time for the quantum dot by using high spin polarization contacts in combination with low tunneling rates.

cond-mat.mes-hall↗

Simultaneous detection of the spin-Hall magnetoresistance and the spin-Seebeck effect in Platinum and Tantalum on Yttrium Iron Garnet

The spin-Seebeck effect (SSE) in platinum (Pt) and tantalum (Ta) on yttrium iron garnet (YIG) has been investigated by both externally heating the sample (using an on-chip Pt heater on top of the device) as well as by current-induced heating. For SSE measurements, external heating is the most common method to obtain clear signals. Here we show that also by current-induced heating it is possible to directly observe the SSE, separate from the also present spin-Hall magnetoresistance (SMR) signal, by using a lock-in detection technique. Using this measurement technique, the presence of additional 2nd order signals at low applied magnetic fields and high heating currents is revealed. These signals are caused by current-induced magnetic fields (Oersted fields) generated by the used AC-current, resulting in dynamic SMR signals.

cond-mat.mes-hall↗

Observation of anomalous Hanle spin precession lineshapes resulting from interaction with localized states

It has been shown recently that in spin precession experiments, the interaction of spins with localized states can change the response to a magnetic field, leading to a modified, effective spin relaxation time and precession frequency. Here, we show that also the shape of the Hanle curve can change, so that it cannot be fitted with the solutions of the conventional Bloch equation. We present experimental data that shows such an effect arising at low temperatures in epitaxial graphene on silicon carbide with localized states in the carbon buffer layer. We compare the strength of the effect between materials with different growth methods, epitaxial growth by sublimation and by chemical vapor deposition. The presented analysis gives information about the density of localized states and their coupling to the graphene states, which is inaccessible by charge transport measurements and can be applied to any spin transport channel that is coupled to localized states.

cond-mat.mes-hall↗

Controlling spin relaxation in hexagonal BN-encapsulated graphene with a transverse electric field

We experimentally study the electronic spin transport in hBN encapsulated single layer graphene nonlocal spin valves. The use of top and bottom gates allows us to control the carrier density and the electric field independently. The spin relaxation times in our devices range up to 2 ns with spin relaxation lengths exceeding 12 $μ$m even at room temperature. We obtain that the ratio of the spin relaxation time for spins pointing out-of-plane to spins in-plane is $τ_{\bot} / τ_{||} \approx$ 0.75 for zero applied perpendicular electric field. By tuning the electric field this anisotropy changes to $\approx$0.65 at 0.7 V/nm, in agreement with an electric field tunable in-plane Rashba spin-orbit coupling.

cond-mat.mes-hall↗

Verification of the Thomson-Onsager reciprocity relation for spin caloritronics

We investigate the Thomson-Onsager relation between the spin-dependent Seebeck and spin-dependent Peltier effect. To maintain identical device and measurement conditions we measure both effects in a single Ni$_{80}$Fe$_{20}$/Cu/Ni$_{80}$Fe$_{20}$ nanopillar spin valve device subjected to either an electrical or a thermal bias. In the low bias regime, we observe similar spin signals as well as background responses, as required by the Onsager reciprocity relation. However, at large biases, deviation from reciprocity occurs due to dominant nonlinear contribution of the temperature dependent transport coefficients. By systematic modeling of these nonlinear thermoelectric effects and measuring higher order thermoelectric responses for different applied biases, we identify the transition between the two regimes as the point at which Joule heating start to dominate over Peltier heating. Our results signify the importance of local equilibrium for the validity of this phenomenological reciprocity relation.

cond-mat.mes-hall↗

Comparison between thermal and current driven spin-transfer torque in nanopillar metallic spin valves

We investigate the relation between thermal spin-transfer torque (TSTT) and the spin-dependent Seebeck effect (SDSE), which produces a spin current when a temperature gradient is applied across a metallic ferromagnet, in nanopillar metallic spin valves. Comparing its angular dependence (aSDSE) with the angle dependent magnetoresistance (aMR) measurements on the same device, we are able to verify that a small spin heat accumulation builds up in our devices. From the SDSE measurement and the observed current driven STT switching current of 0.8 mA in our spin valve devices, it was estimated that a temperature difference of 230 K is needed to produce an equal amount of TSTT. Experiments specifically focused on investigating TSTT show a response that is dominated by overall heating of the magnetic layer. Comparing it to the current driven STT experiments we estimate that only ~10% of the response is due to TSTT. This leads us to conclude that switching dominated by TSTT requires a direct coupling to a perfect heat sink to minimize the effect of overall heating. Nevertheless the combined effect of heating, STT and TSTT could prove useful for inducing magnetization switching when further investigated and optimized.

cond-mat.mes-hall↗

Spin dependent quantum interference in non-local graphene spin valves

Spin dependent electron transport measurements on graphene are of high importance to explore possible spintronic applications. Up to date all spin transport experiments on graphene were done in a semi-classical regime, disregarding quantum transport properties such as phase coherence and interference. Here we show that in a quantum coherent graphene nanostructure the non-local voltage is strongly modulated. Using non-local measurements, we separate the signal in spin dependent and spin independent contributions. We show that the spin dependent contribution is about two orders of magnitude larger than the spin independent one, when corrected for the finite polarization of the electrodes. The non-local spin signal is not only strongly modulated but also changes polarity as a function of the applied gate voltage. By locally tuning the carrier density in the constriction we show that the constriction plays a major role in this effect and indicates that it can act as a spin filter device. Our results show the potential of quantum coherent graphene nanostructures for the use in future spintronic devices.

cond-mat.mes-hall↗

Absence of hyperfine effects in $^{13}$C-graphene spin valve devices

The carbon isotope $^{13}$C, in contrast to $^{12}$C, possesses a nuclear magnetic moment and can induce electron spin dephasing in graphene. This effect is usually neglected due to the low abundance of $^{13}$C in natural carbon allotropes ($\sim$1 %). Chemical vapor deposition (CVD) allows for artificial synthesis of graphene solely from a $^{13}$C precursor, potentially amplifying the influence of the nuclear magnetic moments. In this work we study the effect of hyperfine interactions in pure $^{13}$C-graphene on its spin transport properties. Using Hanle precession measurements we determine the spin relaxation time and observe a weak increase of $τ_{s}$ with doping and a weak change of $τ_{s}$ with temperature, as in natural graphene. For comparison we study spin transport in pure $^{12}$C-graphene, also synthesized by CVD, and observe similar spin relaxation properties. As the signatures of hyperfine effects can be better resolved in oblique spin-valve and Hanle configurations, we use finite-element modeling to emulate oblique signals in the presence of a hyperfine magnetic field for typical graphene properties. Unlike in the case of GaAs, hyperfine interactions with $^{13}$C nuclei influence electron spin transport only very weakly, even for a fully polarized nuclear system. Also, in the measurements of the oblique spin-valve and Hanle effects no hyperfine features could be resolved. This work experimentally confirms the weak character of hyperfine interactions and the negligible role of $^{13}$C atoms in the spin dephasing processes in graphene.

cond-mat.mes-hall↗

Transition between 1D and 0D spin transport studied by Hanle precession

The precession of electron spins in a perpendicular magnetic field, the so called Hanle effect, provides an unique insight into spin properties of a non-magnetic material. In practice, the spin signal is fitted to the analytic solution of the spin Bloch equation, which accounts for diffusion, relaxation and precession effects on spin. The analytic formula, however, is derived for an infinite length of the 1D spin channel. This is usually not satisfied in the real devices. The finite size of the channel length $l_{\text{dev}}$ leads to confinement of spins and increase of spin accumulation. Moreover, reflection of spins from the channel ends leads to spin interference, altering the characteristic precession lineshape. In this work we study the influence of finite $l_{\text{dev}}$ on the Hanle lineshape and show when it can lead to a two-fold discrepancy in the extracted spin coefficients. We propose the extension of the Hanle analytic formula to include the geometrical aspects of the real device and get an excellent agreement with a finite-element model of spin precession, where this geometry is explicitly set. We also demonstrate that in the limit of a channel length shorter than the spin relaxation length $λ_{s}$, the spin diffusion is negligible and a 0D spin transport description, with Lorentzian precession dependence applies. We provide a universal criterion for which transport description, 0D or 1D, to apply depending on the ratio $l_{\text{dev}}/λ_{s}$ and the corresponding accuracy of such a choice.

cond-mat.mes-hall↗

Fast pick up technique for high quality heterostructures of bilayer graphene and hexagonal boron nitride

We present a fast method to fabricate high quality heterostructure devices by picking up crystals of arbitrary sizes. Bilayer graphene is encapsulated with hexagonal boron nitride to demonstrate this approach, showing good electronic quality with mobilities ranging from 17 000 cm^2/V/s at room temperature to 49 000 cm^2/V/s at 4.2 K, and entering the quantum Hall regime below 0.5 T. This method provides a strong and useful tool for the fabrication of future high quality layered crystal devices.

cond-mat.mes-hall↗

Spin heat accumulation induced by tunneling from a ferromagnet

An electric current from a ferromagnet into a non-magnetic material can induce a spin-dependent electron temperature. Here it is shown that this spin heat accumulation, when created by tunneling from a ferromagnet, produces a non-negligible voltage signal that is comparable to that due to the coexisting electrical spin accumulation and can give a different Hanle spin precession signature. The effect is governed by the spin polarization of the Peltier coefficient of the tunnel contact, its Seebeck coefficient, and the spin heat resistance of the non-magnetic material, which is related to the electrical spin resistance by a spin-Wiedemann-Franz law. Moreover, spin heat injection is subject to a heat conductivity mismatch that is overcome if the tunnel interface has a sufficiently large resistance.

cond-mat.mes-hall↗

Observation of the spin Peltier effect

We report the observation of the spin Peltier effect (SPE) in the ferrimagnetic insulator Yttrium Iron Garnet (YIG), i.e. a heat current generated by a spin current flowing through a Platinum (Pt)|YIG interface. The effect can be explained by the spin torque that transforms the spin current in the Pt into a magnon current in the YIG. Via magnon-phonon interactions the magnetic fluctuations modulate the phonon temperature that is detected by a thermopile close to the interface. By finite-element modelling we verify the reciprocity between the spin Peltier and spin Seebeck effect. The observed strong coupling between thermal magnons and phonons in YIG is attractive for nanoscale cooling techniques.

cond-mat.mes-hall↗

Exchange magnetic field torques in YIG/Pt bilayers observed by the spin-Hall magnetoresistance

The effective field torque of an yttrium-iron-garnet film on the spin accumulation in an attached Pt film is measured by the spin-Hall magnetoresistance (SMR). As a result, the magnetization direction of a ferromagnetic insulating layer can be measured electrically. Experimental transverse and longitudinal resistances are well described by the theoretical model of SMR in terms of the direct and inverse spin-Hall effect, for different Pt thicknesses [3, 4, 8 and 35nm]. Adopting a spin-Hall angle of Pt $θ_{SH}=0.08$, we obtain the spin diffusion length of Pt ($λ=1.1\pm0.3$nm) as well as the real ($G_r=(7\pm3)\times10^{14}Ω^{-1}$m$^{-2}$) and imaginary part ($G_i=(5\pm3)\times10^{13}Ω^{-1}$m$^{-2}$) of the spin-mixing conductance and their ratio ($G_r/G_i=16\pm4$).

cond-mat.mes-hall↗

Spin-Hall Magnetoresistance in Platinum on Yttrium Iron Garnet: Dependence on platinum thickness and in-plane/out-of-plane magnetization

The occurrence of Spin-Hall Magnetoresistance (SMR) in platinum (Pt) on top of yttrium iron garnet (YIG) has been investigated, for both in-plane and out-of-plane applied magnetic fields and for different Pt thicknesses [3, 4, 8 and 35nm]. Our experiments show that the SMR signal directly depends on the in-plane and out-of-plane magnetization directions of the YIG. This confirms the theoretical description, where the SMR occurs due to the interplay of spin-orbit interaction in the Pt and spin-mixing at the YIG/Pt interface. Additionally, the sensitivity of the SMR and spin pumping signals on the YIG/Pt interface conditions is shown by comparing two different deposition techniques (e-beam evaporation and dc sputtering).

cond-mat.mes-hall↗

YIG thickness and frequency dependence of the spin-charge current conversion in YIG/Pt systems

We report the frequency dependence of the spin current emission in a hybrid ferrimagnetic insulator/normal metal system as function of the insulating layer thickness. The system is based on a yttrium iron garnet (YIG) film [0.2, 1, and 3 μm] grown by liquid-phase-epitaxy coupled with a spin current detector of platinum [6 nm]. A strong YIG thickness dependence of the efficiency of the spin pumping has been observed. The highest conversion factor ΔV/P_{abs} has been demonstrated for the thinner YIG (1.79 and 0.55 mV/mW^{-1} at 2.5 and 10 GHz, respectively) which presents an interest for the realisation of YIG-based devices. A strong YIG thickness dependence of the efficiency of the spin pumping has been also observed and we demonstrate the threshold frequency dependence of the three-magnon splitting process.

cond-mat.mtrl-sci↗

Fine structure of the lowest Landau level in suspended trilayer graphene

Magneto-transport experiments on ABC-stacked suspended trilayer graphene reveal a complete splitting of the twelve-fold degenerated lowest Landau level, and, in particular, the opening of an exchange-driven gap at the charge neutrality point. A quantitative analysis of distinctness of the quantum Hall plateaus as a function of field yields a hierarchy of the filling factors: ν=6, 4, and 0 are the most pronounced, followed by ν=3, and finally ν=1, 2 and 5. Apart from the appearance of a ν=4 state, which is probably caused by a layer asymmetry, this sequence is in agreement with Hund's rules for ABC-stacked trilayer graphene.

cond-mat.mes-hall↗

Comparison of hot-electron transmission in ferromagnetic Ni on epitaxial and polycrystalline Schottky interfaces

The hot-electron attenuation length in Ni is measured as a function of energy across two different Schottky interfaces viz. a polycrystalline Si(111)/Au and an epitaxial Si(111)/NiSi_2 interface using ballistic electron emission microscopy (BEEM). For similarly prepared Si(111) substrates and identical Ni thickness, the BEEM transmission is found to be lower for the polycrystalline interface than for the epitaxial interface. However, in both cases, the hot-electron attenuation length in Ni is found to be the same. This is elucidated by the temperature-independent inelastic scattering, transmission probabilities across the Schottky interface, and scattering at dissimilar interfaces.

cond-mat.mes-hall↗