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H. L. Stormer

Publications and source records attributed to H. L. Stormer.

At least 19 recordsLinked to original sources

Interaction-induced shift of the cyclotron resonance of graphene using infrared spectroscopy

We report a study of the cyclotron resonance (CR) transitions to and from the unusual $n=0$ Landau level (LL) in monolayer graphene. Unexpectedly, we find the CR transition energy exhibits large (up to 10%) and non-monotonic shifts as a function of the LL filling factor, with the energy being largest at half-filling of the $n=0$ level. The magnitude of these shifts, and their magnetic field dependence, suggests that an interaction-enhanced energy gap opens in the $n=0$ level at high magnetic fields. Such interaction effects normally have limited impact on the CR due to Kohn's theorem [W. Kohn, Phys. Rev. {\bf 123}, 1242 (1961)], which does not apply in graphene as a consequence of the underlying linear band structure.

cond-mat.mes-hall

Dirac charge dynamics in graphene by infrared spectroscopy

A remarkable manifestation of the quantum character of electrons in matter is offered by graphene, a single atomic layer of graphite. Unlike conventional solids where electrons are described with the Schrodinger equation, electronic excitations in graphene are governed by the Dirac Hamiltonian. Some of the intriguing electronic properties of graphene, such as massless Dirac quasiparticles with linear energy-momentum dispersion, have been confirmed by recent observations. Here we report an infrared (IR) spectromicroscopy study of charge dynamics in graphene integrated in gated devices. Our measurements verify the expected characteristics of graphene and, owing to the previously unattainable accuracy of IR experiments, also uncover significant departures of the quasiparticle dynamics from predictions made for Dirac fermions in idealized, free standing graphene. Several observations, including a marked deviation of the energy bands from the simple linear dispersion, point to the relevance of many body interactions to the rather exotic electromagnetic response in graphene.

cond-mat.mes-hall

Band structure asymmetry of bilayer graphene revealed by infrared spectroscopy

We report on infrared spectroscopy of bilayer graphene integrated in gated structures. We observed a significant asymmetry in the optical conductivity upon electrostatic doping of electrons and holes. We show that this finding arises from a marked asymmetry between the valence and conduction bands, which is mainly due to the inequivalence of the two sublattices within the graphene layer. From the conductivity data, the energy difference of the two sublattices is determined.

cond-mat.mes-hall

Ultrahigh electron mobility in suspended graphene

We have achieved mobilities in excess of 200,000 cm^2/Vs at electron densities of ~2*10^11 cm^-2 by suspending single layer graphene. Suspension ~150 nm above a Si/SiO_2 gate electrode and electrical contacts to the graphene was achieved by a combination of electron beam lithography and etching. The specimens were cleaned in situ by employing current-induced heating, directly resulting in a significant improvement of electrical transport. Concomitant with large mobility enhancement, the widths of the characteristic Dirac peaks are reduced by a factor of 10 compared to traditional, non-suspended devices. This advance should allow for accessing the intrinsic transport properties of graphene.

cond-mat.mes-hall

Temperature dependent transport in suspended graphene

The resistivity of ultra-clean suspended graphene is strongly temperature dependent for 5K 0.5*10^11 cm^-2, the resistivity increases with increasing T and is linear above 50K, suggesting carrier scattering from acoustic phonons. At T=240K the mobility is ~120,000 cm^2/Vs, higher than in any known semiconductor. At the charge neutral point we observe a non-universal conductivity that decreases with decreasing T, consistent with a density inhomogeneity <10^8 cm^-2.

cond-mat.mes-hall

Cyclotron resonance in bilayer graphene

We present the first measurements of cyclotron resonance of electrons and holes in bilayer graphene. In magnetic fields up to B = 18 T we observe four distinct intraband transitions in both the conduction and valence bands. The transition energies are roughly linear in B between the lowest Landau levels, whereas they follow \sqrt{B} for the higher transitions. This highly unusual behavior represents a change from a parabolic to a linear energy dispersion. The density of states derived from our data generally agrees with the existing lowest order tight binding calculation for bilayer graphene. However in comparing data to theory, a single set of fitting parameters fails to describe the experimental results.

cond-mat.mes-hall

Experimental studies of the fractional quantum Hall effect in the first excited Landau level

We present a spectrum of experimental data on the fractional quantum Hall effect (FQHE) states in the first excited Landau level, obtained in an ultrahigh mobility two-dimensional electron system (2DES) and at very low temperatures and report the following results: For the even-denominator FQHE states, the sample dependence of the nu=5/2 state clearly shows that disorder plays an important role in determining the energy gap at nu=5/2. For the developing nu=19/8 FQHE state the temperature dependence of the Rxx minimum implies an energy gap of ~5mK.The energy gaps of the odd-denominator FQHE states at nu=7/3 and 8/3 also increase with decreasing disorder, similar to the gap at 5/2 state. Unexpectedly and contrary to earlier data on lower mobility samples, in this ultra-high quality specimen, the nu=13/5 state is missing, while its particle-hole conjugate state, the nu=12/5 state, is a fully developed FQHE state. We speculate that this disappearance might indicate a spin polarization of the nu=13/5 state. Finally, the temperature dependence is studied for the two-reentrant integer quantum Hall states around nu=5/2 and is found to show a very narrow temperature range for the transition from quantized to classical value.

cond-mat.mes-hall

The Nature of Quantum Hall States near the Charge Neutral Dirac Point in Graphene

We investigate the quantum Hall (QH) states near the charge neutral Dirac point of a high mobility graphene sample in high magnetic fields. We find that the QH states at filling factors $ν=\pm1$ depend only on the perpendicular component of the field with respect to the graphene plane, indicating them to be not spin-related. A non-linear magnetic field dependence of the activation energy gap at filling factor $ν=1$ suggests a many-body origin. We therefore propose that the $ν=0$ and $\pm1$ states arise from the lifting of the spin and sub-lattice degeneracy of the $n=0$ LL, respectively.

cond-mat.mes-hall

Measurement of Scattering Rate and Minimum Conductivity in Graphene

The conductivity of graphene samples with various levels of disorder is investigated for a set of specimens with mobility in the range of $1-20\times10^3$ cm$^2$/V sec. Comparing the experimental data with the theoretical transport calculations based on charged impurity scattering, we estimate that the impurity concentration in the samples varies from $2-15\times 10^{11}$ cm$^{-2}$. In the low carrier density limit, the conductivity exhibits values in the range of $2-12e^2/h$, which can be related to the residual density induced by the inhomogeneous charge distribution in the samples. The shape of the conductivity curves indicates that high mobility samples contain some short range disorder whereas low mobility samples are dominated by long range scatterers.

cond-mat.mes-hall

Infrared spectroscopy of Landau levels in graphene

We report infrared studies of the Landau level (LL) transitions in single layer graphene. Our specimens are density tunable and show \textit{in situ} half-integer quantum Hall plateaus. Infrared transmission is measured in magnetic fields up to B=18 T at selected LL fillings. Resonances between hole LLs and electron LLs, as well as resonances between hole and electron LLs are resolved. Their transition energies are proportional to $\sqrt{B}$ and the deduced band velocity is $\tilde{c}\approx1.1\times10^6$ m/s. The lack of precise scaling between different LL transitions indicates considerable contributions of many-particle effects to the infrared transition energies.

cond-mat.mes-hall

Room-Temperature Quantum Hall Effect in Graphene

The quantum Hall effect (QHE), one example of a quantum phenomenon that occur on a truly macroscopic scale, has been attracting intense interest since its discovery in 1980 and has helped elucidate many important aspects of quantum physics. It has also led to the establishment of a new metrological standard, the resistance quantum. Disappointingly, however, the QHE could only have been observed at liquid-helium temperatures. Here, we show that in graphene - a single atomic layer of carbon - the QHE can reliably be measured even at room temperature, which is not only surprising and inspirational but also promises QHE resistance standards becoming available to a broader community, outside a few national institutions.

cond-mat.mes-hall

Disorder mediated splitting of the cyclotron resonance in two-dimensional electron systems

We perform a direct study of the magnitude of the anomalous splitting in the cyclotron resonance (CR) of a two-dimensional electron system (2DES) as a function of sample disorder. In a series of AlGaAs/GaAs quantum wells, identical except for a range of carbon doping in the well, we find the CR splitting to vanish at high sample mobilities but to increase dramatically with increasing impurity density and electron scattering rates. This observation lends strong support to the conjecture that the non-zero wavevector, roton-like minimum in the dispersion of 2D magnetoplasmons comes into resonance with the CR, with the two modes being coupled via disorder.

cond-mat.mes-hall

Single-Walled Carbon Nanotubes as Shadow Masks for Nanogap Fabrication

We describe a technique for fabricating nanometer-scale gaps in Pt wires on insulating substrates, using individual single-walled carbon nanotubes as shadow masks during metal deposition. More than 80% of the devices display current-voltage dependencies characteristic of direct electron tunneling. Fits to the current-voltage data yield gap widths in the 0.8-2.3 nm range for these devices, dimensions that are well suited for single-molecule transport measurements.

cond-mat.mes-hall

Landau Level Splitting in Graphene in High Magnetic Fields

The quantum Hall (QH) effect in two-dimensional (2D) electrons and holes in high quality graphene samples is studied in strong magnetic fields up to 45 T. QH plateaus at filling factors $ν=0,\pm 1,\pm 4$ are discovered at magnetic fields $B>$20 T, indicating the lifting of the four-fold degeneracy of the previously observed QH states at $ν=\pm(|n|+1/2)$, where $n$ is the Landau level index. In particular, the presence of the $ν=0, \pm 1$ QH plateaus indicates that the Landau level at the charge neutral Dirac point splits into four sublevels, lifting sublattice and spin degeneracy. The QH effect at $ν=\pm 4$ is investigated in tilted magnetic field and can be attributed to lifting of the spin-degeneracy of the $n=1$ Landau level.

cond-mat.mes-hall

Resistance scaling for Composite Fermions in the presence of a density gradient

The magnetoresistance, Rxx, at even-denominator fractional fillings, of an ultra high quality two-dimensional electron system at T ~ 35 mK is observed to be strictly linear in magnetic field, B. While at 35mK Rxx is dominated by the integer and fractional quantum Hall states, at T~1.2K an almost perfect linear relationship between Rxx vs B emerges over the whole magnetic field range except for spikes at the integer quantum Hall states. This linear Rxx cannot be understood within the Composite Fermion model, but can be explained through the existence of a density gradient in our sample.

cond-mat.mes-hall

Spin Susceptibility of a 2D Electron System in GaAs towards the Weak Interaction Region

We determine the spin susceptibility $χ$ in the weak interaction regime of a tunable, high quality, two-dimensional electron system in a GaAs/AlGaAs heterostructure. The band structure effects, modifying mass and g-factor, are carefully taken into accounts since they become appreciable for the large electron densities of the weak interaction regime. When properly normalized, $χ$ decreases monotonically from 3 to 1.1 with increasing density over our experimental range from 0.1 to $4\times10^{11} cm^{-2}$. In the high density limit, $χ$ tends correctly towards $χ\to 1$ and compare well with recent theory.

cond-mat.mes-hall

Quantization of the diagonal resistance: Density gradients and the empirical resistance rule in a 2D system

We have observed quantization of the diagonal resistance, R_xx, at the edges of several quantum Hall states. Each quantized R_xx value is close to the difference between the two adjacent Hall plateaus in the off-diagonal resistance, R_xy. Peaks in R_xx occur at different positions in positive and negative magnetic fields. Practically all R_xx features can be explained quantitatively by a ~1%/cm electron density gradient. Therefore, R_xx is determined by R_xy and unrelated to the diagonal resistivity rho_xx. Our findings throw an unexpected light on the empirical resistivity rule for 2D systems.

cond-mat.mes-hall

Acoustic phonon scattering in a low density, high mobility AlGaN/GaN field effect transistor

We report on the temperature dependence of the mobility, $μ$, of the two-dimensional electron gas in a variable density AlGaN/GaN field effect transistor, with carrier densities ranging from 0.4$\times10^{12}$ cm$^{-2}$ to 3.0$\times10^{12}$ cm$^{-2}$ and a peak mobility of 80,000 cm$^{2}$/Vs. Between 20 K and 50 K we observe a linear dependence $μ_{ac}^{-1} = α$T indicating that acoustic phonon scattering dominates the temperature dependence of the mobility, with $α$ being a monotonically increasing function of decreasing 2D electron density. This behavior is contrary to predictions of scattering in a degenerate electron gas, but consistent with calculations which account for thermal broadening and the temperature dependence of the electron screening. Our data imply a deformation potential D = 12-15 eV.

cond-mat.mtrl-sci