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I. J. Arnquist

Publications and source records attributed to I. J. Arnquist.

At least 19 recordsLinked to original sources

Demonstrating topological identification capabilities of the NEXT experiment at low pressure

The NEXT-100 detector is a high-pressure xenon time projection chamber utilising electroluminescence amplification for sub-1% FWHM energy resolution and topological discrimination, two key attributes required to achieve the NEXT programme's overarching goal of detecting neutrinoless double beta decay ($0 νββ$). The detector has completed its first physics run at the Laboratorio Subterráneo de Canfranc (LSC), with xenon at a pressure of $\sim$4 bar. In this paper we report on the first validation of NEXT-100's topological performance and present the first topological analysis conducted at low pressure within the detector programme. A Monte Carlo study characterising the effects of pressure on track topology is presented, with qualitative agreement observed in data. We then demonstrate the topological discrimination capabilities for $0νββ$-like events from $^{208}$Tl decays using a cut-based method considered the 'baseline' in NEXT's topological programme, upon which all future analyses will improve. The analysis described applies a set of selection cuts before implementing a background discrimination algorithm that yields a reported signal efficiency for double-electron tracks and background acceptance for single-electron tracks of 75.6 $\pm$ 1.9 (stat.) $^{+3.4}_{-4.1}$ (syst.) % and 14.7 $\pm$ 0.4 (stat.) $^{+0.7}_{-0.8}$ (syst.) %. These results demonstrate the excellent topological discrimination capabilities of the NEXT-100 detector in line with NEXT-White, which achieved a signal efficiency and background acceptance of 71.6 $\pm$ 1.5 (stat.) $\pm$ 0.3 (syst.) % and 20.6 $\pm$ 0.4 (stat.) $\pm$ 0.3 (syst.) % respectively.

hep-ex

Characterization of CRYO ASIC for charge readout in the nEXO experiment

nEXO is a proposed next-generation experiment searching for the neutrinoless double beta decay of $^{136}$Xe using a tonne-scale liquid xenon (LXe) time projection chamber (TPC). To image the ionization signals from events in the liquid xenon, the detector will employ metallized fused-silica charge collection tiles instrumented with cryogenic application-specific integrated circuits (ASICs), referred to as CRYO ASIC, which are designed to operate directly in LXe to minimize input capacitance and pick-up noise. Here we present the performance of the CRYO ASIC mounted on an auxiliary printed circuit board and evaluated both in a cryogenic environmental chamber and in a dedicated LXe test stand. We demonstrate that the ASICs achieve the desired performance at liquid xenon temperatures, showing a gain stability better than 0.2% over 24-hour operation and reliable in-situ calibration using an on-chip pulser. In the LXe test stand, we show that boiling caused by the chip heat dissipation can be mitigated by operating the system above ~0.1 MPa. The in-LXe noise measured agrees with simulation, which indicates it the $150~e^-$ design requirement can be satisfied. These results establish CRYO ASIC as a viable low-noise in-LXe charge readout solution for nEXO.

physics.ins-det

Detection of scintillation light in noble gases with wavelength-shifting optical fibers

Wavelength-shifting (WLS) techniques enable particle detectors based on noble gases, whose scintillation light is predominantly emitted in the vacuum-ultraviolet. We investigate WLS fibers coated with tetraphenyl butadiene (TPB) for scintillation light detection in gaseous xenon and argon at pressures up to 8.5 bar, motivated by future high-pressure xenon time-projection chambers of the NEXT program. Two detector configurations are studied: an elongated high-pressure vessel with four PTFE panels equipped with WLS fibers read by temperature-stabilized SiPMs, and a compact box-shaped detector operated at 1 bar Xe with WLS fibers read out by PMTs. Both operate with continuous gas purification. The detector response is characterized using cosmic muons and alpha particles from a $^{241}$Am source. With the SiPM setup, we measure a light collection efficiency (LCE) of ${1.18 \pm 0.01~\mathrm{(sta.)}~^{+0.07}_{-0.09}~\mathrm{(sys.)}~\%}$ for xenon and ${1.07 \pm 0.01~\mathrm{(sta.)}~^{+0.06}_{-0.08}~\mathrm{(sys.)}~\%}$ for argon. With PMT readout, we measure a LCE of ${0.45 \pm 0.01~\mathrm{(sta.)} \pm 0.05~\mathrm{(sys.)}~\%}$ in xenon, in agreement with the SiPM result once photon detection efficiency is accounted for. Average scintillation waveforms in xenon and argon are studied to assess the time structure of the emitted light. Cosmic-muon measurements yield a mean energy required to produce a scintillation photon $45\pm7~\mathrm{(sta.)}~^{+4}_{-5}~\mathrm{(sys.)}~\mathrm{eV}$ at 1.5 bar, in agreement with the literature. The results demonstrate that TPB-coated WLS fiber systems can reliably detect scintillation light in high-pressure gaseous noble detectors, with a LCE representing an upper limit for realistic large-scale TPCs, where additional photon losses from materials and fiber attenuation are expected.

physics.ins-det

Radon-induced backgrounds in the NEXT-100 experiment

The NEXT-100 detector at the LSC aims at the first competitive search for the \bbnonu decay using a high-pressure \Xe{136} electroluminescent time projection chamber. The first low-background run of NEXT-100 at 3.95 bar has been devoted to the measurement of the radon-induced backgrounds impacting this search. The contributions from both the internal and external airborne radon have been evaluated. The internal \Rn{222} activity is found to be (0.95$\pm$0.04(stat)$\pm$0.09(sys)) Bq/m$^3$, while no traces of \Rn{220} have been observed. Most of the \Rn{222} progeny plate-out on the surface of the cathode of the detector, leading to a rate of Rn-induced \Bi{214} of (0.97$\pm$0.05(stat)$\pm$0.10(sys)) Hz for visible energies above 400 keV. The corresponding background index in the \bbnonu region of interest is evaluated as (7.3$\pm$1.5(stat)$\pm$0.8(sys))$\times10^{-4}$ counts/(keV$\cdot$kg$\cdot$yr) after selection of the fully contained events. This background index is reduced to $\sim$4$\times10^{-5}$ counts/(keV$\cdot$kg$\cdot$yr) by applying a topological selection requiring only one double-electron-like track in the events. This value is one order of magnitude below the total radiogenic background expectation in NEXT-100. By analyzing the correlation of the airborne radon activity and the measured rate of events in NEXT-100, it is concluded that the detector operates in a virtually radon-free environment thanks to the radon abatement system of the LSC.

hep-ex

Novel High-Radiopurity Doped Amorphous Silicon Resistors for Low-Background Detectors

We present the results of a study of lightly doped amorphous silicon used as a resistive medium for high-radiopurity resistors in nuclear and particle physics research instrumentation. Prototypes are produced for a Time Projection Chamber design for the nEXO neutrinoless double-beta decay search experiment that meet requirements for ultra-high radiopurity, good mechanical, cryogenic and high voltage performance, as well as useful vacuum ultraviolet (VUV) reflectivity. Further study is warranted to refine production methods and to confirm that the technology used here is useful for more general applications.

physics.ins-det

Electroluminescence Yield Measurements in Xenon Gas with the NEXT-DEMO++ Detector

The NEXT-DEMO++ detector, a high-pressure xenon gas time projection chamber serving as a prototype for the NEXT-100 experiment, was used to measure the electroluminescence (EL) yield as a function of reduced electric field ($E/p$) across pressures from 2.0 to 9.4 bar, utilizing the 41.5 keV de-excitation peak of $^{83m}$Kr. These measurements were made to examine the pressure dependence of the slope of the reduced EL yield $Y/p$, which has shown inconsistencies in the literature. The reduced yield was fitted with a linear model, revealing a modest ($\sim$5%) change in slope, beginning around 5 bar and increasing with pressure up to 9.4 bar.

physics.ins-det

The nEXO Radioassay Program

Material radioactivity compilations, such as the one presented here, are important enablers of science. They are useful for the selection of radiopure materials used in the design and construction of low-energy rare-event search experiments. They allow researchers developing such experiments to save time on material studies and avoid costly duplication of effort. The data presented here were generated in support of the planned nEXO double-beta decay search. This work contains among the most restrictive constraints on the natural radioactivity content of materials of general interest to the low-radioactivity community, found in any tabulation of this kind. In this study, various techniques were employed; they are described here.

physics.ins-det

Design of a high voltage delivery system for noble liquid time projection chambers

Noble liquid time projection chambers (TPCs) are a leading technology in the detection of ionizing radiation, particularly in applications such as accelerator neutrino physics, dark matter detection, and neutrinoless double beta decay. This paper addresses the design considerations for implementing stable high voltage (HV) systems within large noble liquid TPCs, with a focus on the nEXO experiment. Utilizing insights from prior HV research and experimental investigations, we outline factors influencing HV stability and discuss design choices to improve stability and prevent electrical discharges. A novel HV delivery system concept is presented, tailored for the nEXO TPC, which incorporates these design considerations while also meeting the stringent radiopurity requirements of the nEXO neutrinoless double beta decay search. These design considerations and their specific implementation towards a HV delivery system offer guidance to future experiments applying high voltage in noble liquid environments.

physics.ins-det

Enhanced sensitivity to trace $^{238}$U impurity of sapphire via coincidence neutron activation analysis

Sapphire has mechanical and electrical properties that are advantageous for the construction of internal components of radiation detectors such as time projection chambers and bolometers. However, it has proved difficult to assess its $\rm ^{232}Th$ and $\rm ^{238}U$ content down to the picogram per gram level. This work reports an experimental verification of a computational study that demonstrates $γγ$ coincidence counting, coupled with neutron activation analysis (NAA), can reach ppt sensitivities. Combining results from $γγ$ coincidence counting with those of earlier single-$γ$ counting based NAA shows that a sample of Saint Gobain sapphire has $\rm ^{232}Th$ and $\rm ^{238}U$ concentrations of $<0.26$ ppt and $<2.3$ ppt, respectively; the best constraints on the radiopurity of sapphire.

nucl-ex

Demonstration of Sub-Percent Energy Resolution in the NEXT-100 Detector

NEXT-100 is a high-pressure xenon time projection chamber with electroluminescent amplification, designed to operate with up to approximately 70.5 kg at 13.5 bar. It is the most recent detector developed by the NEXT collaboration to search for the neutrinoless double-beta decay ($ββ0ν$) of Xe-136. The NEXT gas TPC technology offers the best energy resolution near the Q-value of the decay ($Q_{ββ}$ = 2458 keV) among xenon detectors, which is set by design to be <1% FWHM. We report here the high-energy calibration of the detector using a Th-228 source, demonstrating linear response and an energy resolution of $(0.90 \pm 0.02)$% FWHM at the Tl-208 photopeak (2615 keV). This performance extrapolates to a resolution at the double-beta decay end-point of $R(Q_{ββ})$ = $(0.93 \pm 0.02)$% FWHM, confirming the detector's capability for precision energy measurement in the search for $ββ0ν$.

physics.ins-det

First results of the NEXT-100 detector using $^{83m}$Kr decays

The NEXT collaboration is investigating the double beta decay of $^{136}$Xe using high-pressure gas electroluminescent time projection chambers, which provide excellent energy resolution together with a robust topological signature. Operating at the Laboratorio Subterráneo de Canfranc (LSC) and building on the success of the NEXT-White detector, the NEXT-100 apparatus began commissioning in May 2024 and started operation with xenon at a pressure of 4 bar in October 2024. We report here the first results obtained with NEXT-100 using low-energy calibration data from $^{83m}$Kr decays, which allow mapping of the detector response in the active volume and monitoring of its stability over time. After homogenizing the light response, we achieve an energy resolution of 4.37% FWHM at 41.5 keV for $^{83m}$Kr point-like energy deposits contained in a radius of 425 mm. In a fiducial region representing the operating conditions of NEXT-100 at 10 bar we obtain an improved energy resolution of 4.16% FWHM. These results are in good agreement with that obtained in NEXT-White, and an $E^{-1/2}$ extrapolation to $Q_{ββ}$ yields an energy resolution close to 0.5% FWHM, well below the 1% FWHM design target.

hep-ex

The NEXT-100 Detector

The NEXT collaboration is dedicated to the study of double beta decays of $^{136}$Xe using a high-pressure gas electroluminescent time projection chamber. This advanced technology combines exceptional energy resolution ($\leq 1\%$ FWHM at the $Q_{ββ}$ value of the neutrinoless double beta decay) and powerful topological event discrimination. Building on the achievements of the NEXT-White detector, the NEXT-100 detector started taking data at the Laboratorio Subterráneo de Canfranc (LSC) in May of 2024. Designed to operate with xenon gas at 13.5 bar, NEXT-100 consists of a time projection chamber where the energy and the spatial pattern of the ionising particles in the detector are precisely retrieved using two sensor planes (one with photo-multiplier tubes and the other with silicon photo-multipliers). The detector has been operating at stable conditions using argon and xenon gases at $\sim$4 bar and drift fields of 74 V/cm and 118 V/cm, respectively. Alpha decays from the $^{222}$Rn chain have been used to test and monitor the stability of the detector, showing a constant electron lifetime in the drift volume. In this paper, in addition to reporting the results of the commissioning run, we provide a detailed description of the NEXT-100 detector, describe its assembly, and present the current estimation of the radiopurity budget.

physics.ins-det

High Voltage Delivery and Distribution for the NEXT-100 Time Projection Chamber

A critical element in the realization of large liquid and gas time projection chambers (TPCs) is the delivery and distribution of high voltages into and around the detector. Such experiments require of order tens of kilovolts to enable electron drift over meter-scale distances. This paper describes the design and operation of the cathode feedthrough and high voltage distribution through the field cage of the NEXT-100 experiment, an underground TPC that will search for neutrinoless double beta decay $0νββ$. The feedthrough has been demonstrated to hold pressures up to 20~bar and sustain voltages as high as -65~kV, and the TPC is operating stably at its design high voltages. The system has been realized within the constraints of a stringent radiopurity budget and is now being used to execute a suite of sensitive double beta decay analyses.

physics.ins-det

Ultra-pure Nickel for Structural Components of Low-Radioactivity Instruments

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

nucl-ex

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 $μ$Bq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

physics.ins-det

Rare multi-nucleon decays with the full data sets of the Majorana Demonstrator

The Majorana Demonstrator was an ultra-low-background experiment designed for neutrinoless double-beta decay ($0νββ$) investigation in $^{76}$Ge. Located at the Sanford Underground Research Facility in Lead, South Dakota, the Demonstrator utilized modular high-purity Ge detector arrays within shielded vacuum cryostats, operating deep underground. The arrays, with a capacity of up to 40.4 kg (27.2 kg enriched to $\sim 88\%$ in $^{76}$Ge), have accumulated the full data set, totaling 64.5 kg yr of enriched active exposure and 27.4 kg yr of exposure for natural detectors. Our updated search improves previously explored three-nucleon decay modes in Ge isotopes, setting new partial lifetime limits of $1.83\times10^{26}$ years (90\% confidence level) for $^{76}$Ge($ppp$) $\rightarrow$ $^{73}$Cu e$^+π^+π^+$ and $^{76}$Ge($ppn$) $\rightarrow$ $^{73}$Zn e$^+π^+$. The partial lifetime limit for the fully inclusive tri-proton decay mode of $^{76}$Ge is found to be $2.1\times10^{25}$ yr. Furthermore, we have updated limits for corresponding multi-nucleon decays.

nucl-ex

Final Results of the MAJORANA DEMONSTRATOR's Search for Double-Beta Decay of $^{76}$Ge to Excited States of $^{76}$Se

$^{76}$Ge can $ββ$ decay into three possible excited states of $^{76}$Se, with the emission of two or, if the neutrino is Majorana, zero neutrinos. None of these six transitions have yet been observed. The MAJORANA DEMONSTRATOR was designed to study $ββ$ decay of $^{76}$Ge using a low background array of high purity germanium detectors. With 98.2 kg-y of isotopic exposure, the DEMONSTRATOR sets the strongest half-life limits to date for all six transition modes. For $2νββ$ to the $0^+_1$ state of $^{76}$Se, this search has begun to probe for the first time half-life values predicted using modern many-body nuclear theory techniques, setting a limit of $T_{1/2}>1.5\times10^{24}$ y (90% CL).

nucl-ex

Performance of an Optical TPC Geant4 Simulation with Opticks GPU-Accelerated Photon Propagation

We investigate the performance of Opticks, a NVIDIA OptiX API 7.5 GPU-accelerated photon propagation tool compared with a single-threaded Geant4 simulation. We compare the simulations using an improved model of the NEXT-CRAB-0 gaseous time projection chamber. Performance results suggest that Opticks improves simulation speeds by between 58.47+/-0.02 and 181.39+/-0.28 times relative to a CPU-only Geant4 simulation and these results vary between different types of GPU and CPU. A detailed comparison shows that the number of detected photons, along with their times and wavelengths, are in good agreement between Opticks and Geant4.

physics.ins-det