arXiv subjects

S. M. Kazakov

Publications and source records attributed to S. M. Kazakov.

At least 37 records · Page 2Linked to original sources

arXiv2005

NMR and dc-susceptibility studies of NaVGe2O6

We report the results of measurements of the dc magnetic susceptibility chi(T) and of the 23Na nuclear magnetic resonance (NMR) response of NaVGe2O6, a material in which the V ions form a network of interacting one-dimensional spin S=1 chains. The experiments were made at temperatures between 2.5 and 300 K. The chi(T) data suggest that the formation of the expected low-temperature Haldane phase is intercepted by an antiferromagnetic phase transition at 18 K. The transition is also reflected in the 23Na NMR spectra and the corresponding spin-lattice relaxation rate 1/T1(T). In the ordered phase, 1/T1(T) decreases by orders of magnitude with decreasing temperature, indicating the formation of a gap of the order of 12 K in the magnetic excitation spectrum.

cond-mat.other↗

arXiv2005

The two colors of MgB2

We present the anisotropic optical conductivity of MgB$_{2}$ between 0.1 and 3.7 eV at room temperature obtained on single crystals of different purity by the spectroscopic ellipsometry and reflectance measurements. The bare (unscreened) plasma frequency $ω_{p}$ is almost isotropic and equal to 6.3 eV, which contrasts some earlier reports of a very small value of $ω_{p}$. The data suggests that the $σ$-bands are characterized by a stronger electron-phonon coupling $λ_ {tr}$ but smaller impurity scattering $γ_{imp}$, compared to the $π$-bands. The optical response along the boron planes is marked by an intense interband transition at 2.6 eV, due to which the reflectivity plasma edges along the a- and c-axes are shifted with respect to each other. As a result, the sample spectacularly changes color from a blueish-silver to the yellow as the polarization is rotated from the in-plane direction towards the c-axis. The optical spectra are in good agreement with the published {\it ab initio} calculations. The remaining discrepancies can be explained by the relative shift of $σ$-bands and $π$-bands by about 0.2 eV compared to the theoretical band structure, in agreement with the de Haas-van Alphen experiments. The widths of the Drude and the interband peaks are both very sensitive to the sample purity.

cond-mat.supr-con↗

arXiv2005

de Haas-van Alphen effect investigation of the electronic structure of Al substituted MgB_2

We report a de Haas-van Alphen (dHvA) study of the electronic structure of Al doped crystals of MgB$_2$. We have measured crystals with $\sim 7.5$% Al which have a $T_c$ of 33.6 K, ($\sim 14$% lower than pure MgB$_2$). dHvA frequencies for the $σ$ tube orbits in the doped samples are lower than in pure MgB$_2$, implying a $16\pm2%$ reduction in the number of holes in this sheet of Fermi surface. The mass of the quasiparticles on the larger $σ$ orbit is lighter than the pure case indicating a reduction in electron-phonon coupling constant $λ$. These observations are compared with band structure calculations, and found to be in excellent agreement.

cond-mat.supr-con↗

arXiv2005

Superconducting vortex profile from fixed point measurements The Lazy Fisherman tunnelling microscopy method

We introduce a mode of operation for studying the vortex phase in superconductors using scanning tunnelling microscopy (STM). While in the conventional STM method, the tip is scanned over a sample in which a fixed vortex pattern is prepared, in our "Lazy Fisherman" method the STM tip is kept fixed at a selected location while the vortices are being moved by varying the applied magnetic field. By continuously acquiring the local tunnelling conductance spectra, dI/dV(V), we detect the changes in the local density of states under the tip due to the vortex motion. With no need for scanning, the method permits one to extend the study of vortices to samples in which scanning is difficult or even impossible due to surface nonuniformity and allows one to study vortex dynamics. Using a statistical analysis of the spectra, we reconstruct the single vortex zero bias conductance profile. We apply the method to the c-axis face of an MgB$_2$ single crystal sample and obtain a vortex profile with a coherence length, xi of 57+-2 nm.

cond-mat.supr-con↗

arXiv2005

Temperature dependent anisotropy of the penetration depth and coherence length in MgB$_2

We report measurements of the temperature dependent anisotropies ($γ_λ$ and $γ_ξ$) of both the London penetration depth $λ$ and the upper critical field of MgB$_2$. Data for $γ_λ=λ_c/λ_a$ was obtained from measurements of $λ_{a}$ and $λ_c$ on a single crystal sample using a tunnel diode oscillator technique. $γ_ξ=H_{c2}^{\parallel c}/H_{c2}^{\bot c}$ was deduced from field dependent specific heat measurements on the same sample. $γ_λ$ and $γ_ξ$ have opposite temperature dependencies, but close to $T_c$ tend to a common value ($γ_λ\simeq γ_ξ=1.75\pm0.05$). These results are in good agreement with theories accounting for the two gap nature of MgB$_2$

cond-mat.supr-con↗

arXiv2005

Evidence for a smooth superconductor to normal state transition for nonzero applied magnetic field in RbOs2O6

The effect of the magnetic field on the critical behavior of RbOs2O6 is investigated. We present and analyze magnetization data, revealing remarkable consistency with a magnetic field induced finye size effect. It is traced back that at temperatures Tp(H) smaller than Tc the correlation length cannot grow beyond the limiting length scale set by the magnetic field. Thus, for nonzero H the transition from the superconducting to the normal state turns out to be smooth and the apropriately scaled magnetization data fall on a single curve.

cond-mat.supr-con↗

arXiv2005

Intrinsic thermodynamic properties of the pyrochlore superconductor RbOs2O6 extracted by condensation energy analysis

We develop a general procedure for the analysis of bulk thermodynamic data of a superconductor for samples containing a metallic non-superconducting second phase. The method is based on the condensation energy and it allows the extraction of the intrinsic properties of a superconductor even for non-ideal samples. Applying this procedure to the recently discovered geometrically frustrated beta-pyrochlore superconductor RbOs2O6 (Tc = 6.4 K) yields a Sommerfeld coefficient as high as 79 mu J/g/K^2 (44 mJ/mol_f.u./K^2). RbOs2O6 is inferred to be a strong type-II superconductor (kappa(Tc) = 23) in the intermediate-coupling regime similar to niobium (lambda_ep \approx 1). From the upper critical field mu_0 H_c2 \approx 6 T at 0 K, we estimate a Ginzburg-Landau coherence length xi \approx 74 AA. The condensation energy is 860 mu J/g (483 mJ/mol_f.u.) resulting in 1/(8 pi) (gamma_1 Tc^2)/DeltaU_1 \approx 0.15, a value well in the range of conventional phonon-mediated superconductors. The superconducting electronic specific heat indicates conventional s-wave pairing. The experimental Sommerfeld coefficient of 44 mJ/mol_f.u./K^2 is about 4 times larger than the one found in band structure calculations. Together with the electron-phonon coupling constant lambda_ep \approx 1 this leaves an additional lambda_add \approx 2.4 for enhancement due to other mechanisms.

cond-mat.supr-con↗

arXiv2004

Study of pressure effect on the magnetic penetration depth in MgB$_2$

A study of the pressure effect on the magnetic penetration depth $λ$ in polycrystalline MgB$_{2}$ was performed by measuring the temperature dependence of the magnetization under an applied pressure of 0.15 and 1.13 GPa. We found that $λ^{-2}$ at low temperature is only slightly affected by pressure [$\frac{Δλ^{-2}}{λ^{-2}} = 1.5(9)%$], in contrast to cuprate superconductors, where, in the same range of pressure, a very large effect on $λ^{-2}$ was found. Theoretical estimates indicate that most of the pressure effect on $λ^{-2}$ in MgB$_2$ arises from the electron-phonon interaction.

cond-mat.supr-con↗

arXiv2004

Study of the magnetic penetration depth in RbOs_2O_6

Measurements of the magnetic field penetration depth λin the pyrochlore superconductor RbOs_2O_6 (T_c\simeq6.3 K) were carried out by means of the muon-spin-rotation (\muSR) technique. At low temperatures λ^{-2}(T) saturates and becomes constant below T\simeq 0.2T_c, in agreement with what is expected for weak-coupled s-wave BCS superconductors. The value of λat T=0 was found to be in the range of 250 nm to 300 nm. \muSR and equilibrium magnetization measurements both reveal that at low temperatures $λ$ is almost (at the level of 10%) independent of the applied magnetic field. This result suggests that the superconducting energy gap in RbOs_2O_6 is isotropic.

cond-mat.supr-con↗

arXiv2004

Influence of carbon substitution on the heat transport in single crystalline MgB2

We report data on the thermal conductivity κ(T,H) in the basal plane of hexagonal single-crystalline and superconducting Mg(B_{1-x}C_x)_2 (x= 0.03, 0.06) at temperatures between 0.5 and 50 K, and in external magnetic fields H between 0 and 50 kOe. The substitution of carbon for boron leads to a considerable reduction of the electronic heat transport, while the phonon thermal conductivity seems to be much less sensitive to impurities. The introduction of carbon enhances mostly the intraband scattering in the σ-band. In contrast to the previously observed anomalous behavior of pure MgB$_2$, the Wiedemann-Franz law is valid for Mg(B_0.94 C_0.06)_2 at low temperatures.

cond-mat.supr-con↗

arXiv2004

Al substitution in MgB2 crystals: influence on superconducting and structural properties

Single crystals of Mg1-xAlxB2 have been grown at a pressure of 30 kbar using the cubic anvil technique. Precipitation free crystals with x < 0.1 were obtained as a result of optimization of already developed MgB2 crystal growth procedure. Systematic decrease of the c-axis lattice constant with increasing Al content, when the a-axis lattice constant is practically unchanged, was observed. Variation of the critical temperature on Al content in Mg1-xAlxB2 crystals was found to be slightly different than that one observed for polycrystalline samples since, even a very small substitution of 1-2% of Al leads to the decrease of Tc by about 2-3 K. X-ray and high resolution transmission electron microscopy investigations indicate on the appearance of second precipitation phase in the crystals with x > 0.1. This is in a form of non-superconducting MgAlB4 domains in the structure of superconducting Mg1-xAlxB2 matrix. Resistivity and magnetic investigations show the slight increase of the upper critical field, Hc2, for H//c for the samples with small x, significant reduction of the Hc2 anisotropy at lower temperatures, and decrease of the residual resistance ratio value for Al substituted samples as compared to those of unsubstituted crystals. Superconducting gaps variation as a function of Al content, investigated with point contact spectroscopy for the series of the crystals with Tc in the range from 20 to 37 K, does not indicate on the merging of the gaps with decreasing Tc down to 20 K. It may be related to an appearance of the precipitation phase in the Mg1-xAlxB2 structure.

cond-mat.supr-con↗

arXiv2004

Evidence for Single-gap Superconductivity in Mg(B_{1-x}C_x)_2 Single Crystals with x=0.132 from Point-Contact Spectroscopy

We report the results of the first directional point-contact measurements in Mg(B_{1-x}C_{x})_2 single crystals with 0.047 <= x <= 0.132. The two-gap superconductivity typical of MgB_2 persists up to x=0.105. In this region, the values of the gaps Delta_{sigma} and Delta_{pi} were determined by fitting the Andreev-reflection conductance curves with a two-band Blonder-Tinkham-Klapwijk (BTK) model, and confirmed by the single-band BTK fit of the sigma- and pi-band conductances, separated by means of a magnetic field. At x=0.132, when T_{c}=19 K, we clearly observed for the first time the merging of the two gaps into one of amplitude Delta~3 meV.

cond-mat.supr-con↗

arXiv2004

Evidence for s-wave superconductivity in the new beta-pyrochlore oxide RbOs2O6

We report the results of 87Rb NMR measurements on RbOs2O6, a new member of the family of the superconducting pyrochlore-type oxides with a critical temperature Tc = 6.4 K. In the normal state, the nuclear spin-lattice relaxation time T1 obeys the Korringa-type relation T1T = constant and the Knight shift is independent of temperature, indicating the absence of strong magnetic correlations. In the superconducting state, T1^{-1}(T) exhibits a tiny coherence enhancement just below Tc, and decreases exponentially with further decreasing temperatures. The value of the corresponding energy gap is close to that predicted by the conventional weak-coupling BCS theory. Our results indicate that RbOs2O6 is a conventional s-wave-type superconductor.

cond-mat.supr-con↗

arXiv2004

Synthesis of superconducting pyrochlore RbOs2O6

RbOs2O6, the third superconducting pyrochlore oxide (known so far), has been synthesized by encapsulation and by high pressure techniques. Suitable post chemical treatment of the as-prepared sample allowed us to eliminate the impurity phases. Bulk superconductivity with Tc=6.4 K was observed in magnetisation and specific heat measurements. The transition temperature of RbOs2O6 was found to be the same for both preparation methods. Structural investigations showed that Rb atoms occupy the 8b site in the pyrochlore lattice with a lattice parameter of 10.1137(1) A.

cond-mat.supr-con↗

arXiv2004

Anomaly in YBa2Cu4O8 charge distribution below Tc: a zero-field muSR study

Zero-field $μ$SR measurements in $^{63}$Cu isotope enriched and natural YBa$_2$Cu$_4$O$_8$ powders are presented. The temperature dependence of the $μ^+$ relaxation rate is characterized by a sizeable enhancement below T$_c$. The comparison of the asymmetry decay in the two samples reveals that the $μ^+$ relaxation is driven by nuclear dipole interaction from 300 K down to 4.2 K. It is argued that the increase in the relaxation below T$_c$ originates from a change in $μ^+$ site, possibly due to a modification in the charge distribution within CuO chains.

cond-mat.str-el↗

arXiv2004

A Point-Contact Study of the Superconducting Gaps in Al-Substituted and C-Substituted MgB_2 Single Crystals

We present the results of directional point-contact spectroscopy in state-of-the-art Mg_{1-x}Al_xB_2 and Mg(B_{1-y}C_{y})_2 single crystals produced at ETH, Zurich. Fitting the conductance curves of our point contacts, that always feature Andreev reflection structures, we obtained the doping dependence of the gap amplitudes. The results are discussed in comparison with other experimental findings and relevant theoretical predictions. We conclude that the physics of Al-substituted crystals at x > 0.09 might be governed by phase segregation, while C-substituted crystals unexpectedly show a doping-induced transition to single-gap superconductivity at y=0.132.

cond-mat.supr-con↗

arXiv2004

Anisotropy and internal field distribution of MgB2 in the mixed state at low temperatures

Magnetization and muon spin relaxation on MgB2 were measured as a function of field at 2 K. Both indicate an inverse-squared penetration depth strongly decreasing with increasing field H below about 1 T. Magnetization also suggests the anisotropy of the penetration depth to increase with increasing H, interpolating between a low Hc1 and a high Hc2 anisotropy. Torque vs angle measurements are in agreement with this finding, while also ruling out drastic differences between the mixed state anisotropies of the two basic length scales penetration depth and coherence length.

cond-mat.supr-con↗

arXiv2004

Damping of the de Haas-van Alphen oscillations in the superconducting state of MgB_2

The de Haas-van Alphen (dHvA) signal arising from orbits on the $π$ Fermi surface sheet of the two-gap superconductor MgB$_2$ has been observed in the vortex state below $H_{c2}$. An extra attenuation of the dHvA signal, beyond those effects described in the conventional Lifshitz-Kosevich expression, is seen due to the opening of the superconducting gap. Our data show that the $π$ band gap is still present up to $H_{c2}$. The data are compared to current theories of dHvA oscillations in the superconducting state which allow us to extract estimates for the evolution of the $π$ band gap with magnetic field. Contrary to results for other materials, we find that the most recent theories dramatically underestimate the damping in MgB$_2$.

cond-mat.supr-con↗