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arXiv · 2412.15591

Room-temperature nonlinear transport and microwave rectification in antiferromagnetic MnBi$_2$Te$_4$ films

Shanshan Liu·Rhonald Burgos·Enze Zhang·Naizhou Wang·Xiao-Bin Qiang·Chuanzhao Li·Qihan Zhang·Z. Z. Du·Rui Zheng·Jingsheng Chen·Qing-Hua Xu·Kai Leng·Weibo Gao·Faxian Xiu·Dimitrie Culcer·Kian Ping Loh
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Abstract

The discovery of the nonlinear Hall effect provides an avenue for studying the interplay among symmetry, topology, and phase transitions, with potential applications in signal doubling and high-frequency rectification. However, practical applications require devices fabricated on large area thin film as well as room-temperature operation. Here, we demonstrate robust room-temperature nonlinear transverse response and microwave rectification in MnBi$_2$Te$_4$ films grown by molecular beam epitaxy. We observe multiple sign-reversals in the nonlinear response by tuning the chemical potential. Through theoretical analysis, we identify skew scattering and side jump, arising from extrinsic spin-orbit scattering, as the main mechanisms underlying the observed nonlinear signals. Furthermore, we demonstrate radio frequency (RF) rectification in the range of 1-8 gigahertz at 300 K. These findings not only enhance our understanding of the relationship between nonlinear response and magnetism, but also expand the potential applications as energy harvesters and detectors in high-frequency scenarios.

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Shanshan Liu, Rhonald Burgos, Enze Zhang, Naizhou Wang, Xiao-Bin Qiang, Chuanzhao Li, Qihan Zhang, Z. Z. Du, Rui Zheng, Jingsheng Chen, Qing-Hua Xu, Kai Leng, Weibo Gao, Faxian Xiu, Dimitrie Culcer, Kian Ping Loh. 2024-12-20. Room-temperature nonlinear transport and microwave rectification in antiferromagnetic MnBi$_2$Te$_4$ films. https://doi.org/10.1038/s42005-024-01897-y

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